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Lorant Zs. Szabo

Publications and source records attributed to Lorant Zs. Szabo.

3 recordsLinked to original sources

Ultrashort laser pulse driven currents in conductors: physical mechanisms and time scales

The response of conduction band electrons to a local, pulse-like external excitation is investigated. The charge density wave packets that emerge as a consequence of the excitation leave the interaction region with a speed close to the initial state's band velocity, but there are also oscillations with essentially the same frequency as that of the laser field. As a good estimation, the excitation can also be considered as a localized, time-dependent ponderomotive potential, leading to slowly varying current oscillations. The role of all these effects are investigated for different electron energies, carrier frequencies and sizes of the interaction area.

quant-ph↗

Improved emission of SiV diamond color centers embedded into concave plasmonic core-shell nanoresonators

Configuration of three different concave silver core-shell nanoresonators was numerically optimized to enhance the excitation and emission of embedded silicon vacancy (SiV) diamond color centers simultaneously. According to the tradeoff between the radiative rate enhancement and quantum efficiency (QE) conditional optimization was performed to ensure ~2-3-4 and 5-fold apparent cQE enhancement of SiV color centers with ~10% intrinsic QE. The enhancement spectra, as well as the near-field and charge distribution were inspected to uncover the physics underlying behind the optical responses. The conditionally optimized coupled systems were qualified by the product of the radiative rate enhancements at the excitation and emission, which is nominated as Px factor. The optimized spherical core-shell nanoresonator containing a centralized emitter is capable of enhancing considerably the emission via bonding dipolar resonance. The Px factor is 529-fold with 49.7% cQE at the emission. Decentralization of the emitter leads to appearance of higher order multipolar modes, which is not advantageous caused by their nonradiative nature. Transversal and longitudinal dipolar resonances of the optimized ellipsoidal core-shell resonator were tuned to the excitation and emission, respectively. The simultaneous enhancements result in 6.2x10^5 Px factor with 50.6% cQE at the emission. Rod-shaped concave core-shell nanoresonators exploit similarly transversal and longitudinal dipolar resonances, moreover they enhance the fluorescence more significantly due to their antenna-like geometry. Px factor of 8.34x10^5 enhancement is achievable while the cQE is 50.3% at the emission. The enhancement can result in 2.03x10^6-fold Px factor, when the criterion regarding the minimum QE is set to 20%.

physics.optics↗

Enhancing diamond color center fluorescence via optimized plasmonic nanorod configuration

A novel numerical methodology has been developed, which makes possible to optimize arbitrary emitting dipole and plasmonic nano-resonator configuration with an arbitrary objective function. By selecting quantum efficiency as the objective function that has to be maximized at preselected Purcell factor criteria, optimization of plasmonic nanorod based configurations has been realized to enhance fluorescence of NV and SiV color centers in diamond. Gold and silver nanorod based configurations have been optimized to enhance excitation and emission separately, as well as both processes simultaneously, and the underlying nanophotonical phenomena have been inspected comparatively. It has been shown that considerable excitation enhancement is achieved by silver nanorods, while nanorods made of both metals are appropriate to enhance emission. More significant improvement can be achieved via silver nanorods at both wavelengths of both color centers. It has been proven that theoretical limits originating from metal dielectric properties can be approached by simultaneous optimization, which results in configurations determined by preferences corresponding to the emission. Larger emission enhancement is achieved via both metals in case of SiV center compared to the NV center. Gold and silver nanorod based configurations making possible to improve SiV centers quantum efficiency by factors of 1.18 and 5.25 are proposed, which have potential applications in quantum information processing.

physics.optics↗