arXiv subjects

Loren N. Pfeiffer

Publications and source records attributed to Loren N. Pfeiffer.

At least 37 records · Page 2Linked to original sources

arXiv2025

Collective neutral excitations as sensitive probe for the quality of 2D charge carrier systems in ultra-pure GaAs quantum wells

Ultra-clean low-dimensional interacting charge carrier systems are the basis to explore correlated states and phases. We report the observation of very narrow collective intersubband excitations (ISBE) of 2D electron systems (2DESs) with ultra-high mobilities in high quality GaAs quantum well structures. These findings from resonant inelastic light scattering (RILS) experiments are used as tools for exploration of links between transport mobility and collective electron behavior in 2DES of high perfection. We find that the linewidths of collective ISBE modes can be very narrow with values smaller than 80μeV. Comparison of ISBE measurements from several high-mobility samples exhibits a variation in linewidth of more than a factor of two. There is, however, a surprising lack of direct correlation between ISBE linewidth with mobility in the range 15x10^6 cm^2/Vs<μ<24x10^6 cm^2/Vs. ISBE by RILS are discussed as a sensitive probe to characterize the interacting electron systems for fractional quantum Hall effect (FQHE) studies.

cond-mat.mes-hall↗

arXiv2024

Design and Fabrication of Robust Hybrid Photonic Crystal Cavities

Heterogeneously integrated hybrid photonic crystal cavities enable strong light-matter interactions with solid-state, optically addressable quantum memories. A key challenge to realizing high quality factor (Q) hybrid photonic crystals is the reduced index contrast on the substrate compared to suspended devices in air. This challenge is particularly acute for color centers in diamond because of diamond's high refractive index, which leads to increased scattering loss into the substrate. Here we develop a design methodology for hybrid photonic crystals utilizing a detailed understanding of substrate-mediated loss, which incorporates sensitivity to fabrication errors as a critical parameter. Using this methodology we design robust, high-Q, GaAs-on-diamond photonic crystal cavities, and by optimizing our fabrication procedure we experimentally realize cavities with Q approaching 30,000 at a resonance wavelength of 955 nm.

physics.optics↗

arXiv2024

Targeted Polariton Flow Through Tailored Photonic Defects

In non-Hermitian open quantum systems, such as polariton condensates, local tailoring of gains and losses opens up an interesting possibility to realize functional optical elements. Here, we demonstrate that deliberately introducing losses via a photonic defect, realized by reducing the quality factor of a DBR mirror locally within an ultrahigh-quality microcavity, may be utilized to create directed polariton currents towards the defect. We discuss the role of polariton-polariton interactions in the process and how to tailor the effective decay time of a polariton condensate via coupling to the defect. Our results highlight the far-reaching potential of non-Hermitian physics in polaritonics.

cond-mat.mes-hall↗

arXiv2024

Reconfigurable quantum fluid molecules of bound states in the continuum

Topological bound states in the continuum are confined wave-mechanical objects that offer advantageous ways to enhance light-matter interactions in compact photonic devices. In particular, their large quality factor in the strong-coupling regime has recently enabled the demonstration of Bose-Einstein condensation of bound-state-in-the-continuum polaritons. Here, we show that condensation into a negative-mass bound state in the continuum exhibits interaction-induced state confinement, opening opportunities for optically reprogrammable molecular arrays of quantum fluids of light. We exploit this optical trapping mechanism to demonstrate that such molecular complexes show hybridization with macroscopic modes with unusual topological charge multiplicity. Additionally, we demonstrate the scalability of our technique by constructing extended mono- and diatomic chains of bound-state-in-the-continuum polariton fluids that display non-Hermitian band formation and the opening of a minigap. Our findings offer insights into large-scale, reprogrammable, driven, dissipative many-body systems in the strong-coupling regime.

physics.optics↗

arXiv2024

Emerging supersolidity from a polariton condensate in a photonic crystal waveguide

A supersolid is a counter-intuitive phase of matter where its constituent particles are arranged into a crystalline structure, yet they are free to flow without friction. This requires the particles to share a global macroscopic phase while being able to reduce their total energy by spontaneous, spatial self-organisation. This exotic state of matter has been achieved in different systems using Bose-Einstein condensates coupled to cavities, possessing spin-orbit coupling, or dipolar interactions. Here we provide experimental evidence of a new implementation of the supersolid phase in a novel non-equilibrium context based on exciton-polaritons condensed in a topologically non-trivial, bound-in-the-continuum state with exceptionally low losses. We measure the density modulation of the polaritonic state indicating the breaking of translational symmetry with a remarkable precision of a few parts in a thousand. Direct access to the phase of the wavefunction allows us to additionally measure the local coherence of the superfluid component. We demonstrate the potential of our synthetic photonic material to host phonon dynamics and a multimode excitation spectrum.

cond-mat.mes-hall↗

arXiv2024

Quantum coherence of a long-lifetime exciton-polariton condensate

In recent years, quantum information science has made significant progress, leading to a multitude of quantum protocols for the most diverse applications. States carrying resources such as quantum coherence are a key component for these protocols. In this study, we optimize the quantum coherence of a nonresonantly excited exciton-polariton condensate of long living polaritons by minimizing the condensate's interaction with the surrounding reservoir of excitons and free carriers. By combining experimental phase space data with a displaced thermal state model, we observe how quantum coherence builds up as the system is driven above the condensation threshold. Our findings demonstrate that a spatial separation between the condensate and the reservoir enhances the state's maximum quantum coherence directly beyond the threshold. These insights pave the way for integrating polariton systems into hybrid quantum devices and advancing applications in quantum technologies.

cond-mat.mes-hall↗

arXiv2024

Bose-Einstein condensation of polaritons at room temperature in a GaAs/AlGaAs structure

We report the canonical properties of Bose-Einstein condensation of polaritons, seen previously in many low-temperature experiments, at room temperature in a GaAs/AlGaAs structure. These effects include a nonlinear energy shift of the polaritons, showing that they are not non-interacting photons, and dramatic line narrowing due to coherence, giving coherent emission with spectral width of 0.24 meV at room temperature with no external stabilization. This opens up the possibility of room temperature nonlinear optical devices based on polariton condensation.

cond-mat.quant-gas↗

arXiv2024

Narrow-linewidth exciton-polariton laser

Exciton-polariton laser is a promising source of coherent light for low-energy applications due to its low-threshold operation. However, a detailed experimental study of its spectral purity, which directly affects its coherence properties is still missing. Here}, we present a high-resolution spectroscopic investigation of the energy and linewidth of an exciton-polariton laser in the single-mode regime, which derives its coherent emission from an optically pumped and confined exciton-polariton condensate. We report an ultra-narrow linewidth of 56~MHz or 0.24~$μ$eV, corresponding to a coherence time of 5.7~ns. The narrow linewidth is consistently achieved by using an exciton-polariton condensate with a high photonic content confined in an optically induced trap. Contrary to previous studies, we show that the excitonic reservoir created by the pump and responsible for creating the trap does not strongly affect the emission linewidth as long as the condensate is trapped and the pump power is well above the condensation (lasing) threshold. \red{The long coherence time of the exciton-polariton system uncovered here opens up opportunities for manipulating its macroscopic quantum state, which is essential for applications in classical and quantum computing.

physics.optics↗

arXiv2024

Measurement of exciton fraction of microcavity exciton-polaritons using transfer-matrix modeling

We present a careful calibration of the exciton fraction of polaritons in high-$Q$ ($\sim 300,000$), long-lifetime ($\sim 300$ ps), GaAs/AlGaAs microcavities.This is a crucial parameter for many-body theories which include the polariton-polariton interactions.It is much harder to establish this number in high-$Q$ structures compared to low-$Q$ structures, because the upper polariton is nearly invisible in high-$Q$ cavities.We present a combination of photoluminescence, photoluminescence excitation, and reflectivity measurements to highly constrain the fit model, and compare the results of this model to the results from low-$Q$ structures.We present a fitted curve of exciton fraction as a function of the lower polariton energy for multiple samples which have been used in prior experiments.

cond-mat.mes-hall↗

arXiv2024

Coherence measurements of polaritons in thermal equilibrium reveal a power law for two-dimensional condensates

We have created a spatially homogeneous polariton condensate in thermal equilibrium, up to very high condensate fraction. Under these conditions, we have measured the coherence as a function of momentum, and determined the total coherent fraction of this boson system from very low density up to density well above the condensation transition. These measurements reveal a consistent power law for the coherent fraction as a function of the total density over nearly three orders of its magnitude. The same power law is seen in numerical simulations solving the two-dimensional Gross-Pitaevskii equation for the equilibrium coherence. This power law has not been predicted by prior analytical theories.

cond-mat.quant-gas↗

arXiv2023

Critical fluctuations in a confined driven-dissipative quantum condensate

Phase fluctuations determine the low-energy properties of quantum condensates. However, at the condensation threshold, both density and phase fluctuations are relevant. While strong emphasis has been given to the investigation of phase fluctuations, which dominate the physics of the quantum system away from the critical point -- number fluctuations have been much less explored, even in thermal equilibrium. In this work, we report experimental observation and theoretical description of fluctuations in a circularly-confined non-equilibrium Bose-Einstein condensate of polaritons near the condensation threshold. We observe critical fluctuations, which combine the number fluctuations of a single-mode condensate state and competition between different states. The latter are analogous to mode hopping in photon lasers. Our theoretical analysis indicates that this phenomenon is of a quantum character, while classical noise of the pump is not sufficient to explain the experiments. The manifestation of a critical quantum state competition unlocks new possibilities for the study of condensate formation while linking to practical realizations in photonic lasers.

cond-mat.quant-gas↗

arXiv2023

Breaking a Bloch-wave interferometer: quasiparticle species-specific temperature-dependent nonequilibrium dephasing

Recently, high-order sideband polarimetry has been established as an experimental method that links the polarization of sidebands to an interference of Bloch wavefunctions. However, the robustness of sideband polarizations to increasing dephasing remains to be explored. Here, we investigate the dependence of high-order sideband generation in bulk gallium arsenide on dephasing by tuning temperature. We find that the intensities of the sidebands, but not their polarizations, depend strongly on temperature. Using our polarimetry method, we are able to isolate the contributions of electron-heavy hole (HH) and electron-light hole (LH) pairs to sideband intensities, and separately extract the nonequilibrium dephasing coefficients associated with the longitudinal optical (LO) phonons and acoustic (A) phonons for each species of electron-hole pair. We find that $Γ_{\text{HH},\text{A}} = 6.1 \pm 1.6$ $μ$eV/K, $Γ_{\text{LH},\text{A}} < 1.5$ $μ$eV/K, $Γ_{\text{HH},\text{LO}} = 14 \pm 3$ meV, and $Γ_{\text{LH},\text{LO}} = 30 \pm 3$ meV.

cond-mat.mes-hall↗

arXiv2023

Indium-Bond-And-Stop-Etch (IBASE) Technique for Dual-side Processing of Thin High-mobility GaAs/AlGaAs Epitaxial Layers

We present a reliable flip-chip technique for dual-side processing of thin (<1 micron) high-mobility GaAs/AlGaAs epitaxial layers. The technique allows the fabrication of small (micron-scale with standard UV photolithography) patterned back gates and dual-gate structures on the thin GaAs/AlGaAs films with good alignment accuracy using only frontside alignment. The technique preserves the high-mobility (>10^6 cm^2 /V-s at 2 K) and most (>95%) of the charge density of the 2-dimensional electron gas (2DEG) systems, and allows linear control of the charge density with small (< 1 V) electrostatic gate bias. Our technique is motivated by a novel THz quantum-well detector based on intersubband transitions in a single, wide GaAs/AlGaAs quantum well, in which a symmetric, well-aligned dual-gate structure (with a typical gate dimension of ~5 micron by 5 micron) is required for accurate and precise tuning of the THz detection frequency. Using our Indium-Bond-And-Stop-Etch (IBASE) technique, we realize such dual-gate structure on 660-nm thick GaAs/AlGaAs epitaxial layers that contain a modulation-doped, 40-nm wide, single square quantum well. By independently controlling the charge density and the DC electric field set between the gates, we demonstrate robust tuning of the intersubband absorption behavior of the 40-nm quantum well near 3.44 THz at 30 K.

physics.ins-det↗

arXiv2023

Dynamic Response of Wigner Crystals

The Wigner crystal, an ordered array of electrons, is one of the very first proposed many-body phases stabilized by the electron-electron interaction. This electron solid phase has been reported in ultra-clean two-dimensional electron systems at extremely low temperatures, where the Coulomb interaction dominants over the kinetic energy, disorder potential and thermal fluctuation. We closely examine this quantum phase with capacitance measurements where the device length-scale is comparable with the crystal's correlation length. The extraordinarily high performance of our technique makes it possible to quantitatively study the dynamic response of the Wigner crystal within the single crystal regime. Our result will greatly boost the study of this inscrutable electron solid.

cond-mat.mes-hall↗

arXiv2022

Enhanced thermalization of exciton-polaritons in optically generated potentials

Equilibrium Bose-Einstein condensation of exciton-polaritons, demonstrated with a long-lifetime microcavity [Phys. Rev. Lett. 118, 016602 (2017)], has proven that driven-dissipative systems can undergo thermodynamic phase transitions in the limit where the quasiparticle lifetime exceeds the thermalization time. Here, we identify the role of dimensionality and polariton interactions in determining the degree of thermalization in optically generated traps. To distinguish the effect of trapping from interactions and lifetimes, we measured the polariton distribution under four nonresonant Gaussian pumps in a square geometry and compared it with polariton distributions measured with each pump individually. We found that significant redistribution of polaritons arises by trapping and modification of the density of states. Surprisingly efficient polariton-polariton scattering below the condensation threshold is evidenced by the depletion of the inflection-point polaritons. Our work provides a deeper understanding of polariton distributions and their interactions under various geometries of optically generated potentials.

cond-mat.quant-gas↗

arXiv2022

Bogoliubov excitations of a polariton condensate in dynamical equilibrium with an incoherent reservoir

The classic Bogoliubov theory of weakly interacting Bose gases rests upon the assumption that nearly all the bosons condense into the lowest quantum state at sufficiently low temperatures. Here we develop a generalized version of Bogoliubov theory for the case of a driven-dissipative exciton-polariton condensate with a large incoherent uncondensed component, or excitonic reservoir. We argue that such a reservoir can consist of both excitonic high-momentum polaritons and optically dark superpositions of excitons across different optically active layers, such as multiple quantum wells in a microcavity. In particular, we predict interconversion between the dark and bright (light-coupled) excitonic states that can lead to a dynamical equilibrium between the condensate and reservoir populations. We show that the presence of the reservoir fundamentally modifies both the energy and the amplitudes of the Bogoliubov quasiparticle excitations due to the non-Galilean-invariant nature of polaritons. Our theoretical findings are supported by our experiment, where we directly detect the Bogoliubov excitation branches of an optically trapped polariton condensate in the high-density regime. By analyzing the measured occupations of the excitation branches, we extract the Bogoliubov amplitudes across a range of momenta and show that they agree with our generalized theory.

cond-mat.quant-gas↗

arXiv2022

Domain Textures in the Fractional Quantum Hall Effect

Impacts of domain textures on low-lying neutral excitations in the bulk of fractional quantum Hall effect (FQHE) systems are probed by resonant inelastic light scattering. We demonstrate that large domains of quantum fluids support long-wavelength neutral collective excitations with well-defined wave vector (momentum) dispersion that could be interpreted by theories for uniform phases. Access to dispersive low-lying neutral collective modes in large domains of FQHE fluids such as long wavelength magnetorotons at filling factor v=1/3 offer significant experimental access to strong electron correlation physics in the FQHE.

cond-mat.mes-hall↗

arXiv2021

Interaction Effects and Viscous Magneto-Transport in a Strongly Correlated 2D Hole System

Fermi liquid theory has been a foundation in understanding the electronic properties of materials. For weakly interacting two-dimensional (2D) electron or hole systems, electron-electron interactions are known to introduce quantum corrections to the Drude conductivity in the FL theory, giving rise to temperature dependent conductivity and magneto-resistance. Here we study the magneto-transport in a strongly interacting 2D hole system over a broad range of temperatures ($T$ = 0.09 to $>$1K) and densities $p=1.98-0.99\times10^{10}$ cm$^{-2}$ where the ratio between Coulomb energy and Fermi energy $r_s$ = 20 - 30. We show that while the system exhibits a negative parabolic magneto-resistance at low temperatures ($\lesssim$ 0.4K) characteristic of an interacting FL, the FL interaction corrections represent an insignificant fraction of the total conductivity. Surprisingly, a positive magneto-resistance emerges at high temperatures and grows with increasing temperature even in the regime $T \sim E_F$, close to the Fermi temperature. This unusual positive magneto-resistance at high temperatures is attributed to the collective viscous transport of 2D hole fluid in the hydrodynamic regime where holes scatter frequently with each other. These findings highlight the collective transport in a strongly interacting 2D system in the $r_s\gg 1$ regime and the hydrodynamic transport induced magneto-resistance opens up possibilities to new routes of magneto-resistance at high temperatures.

cond-mat.str-el↗