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Loren Pfeiffer

Publications and source records attributed to Loren Pfeiffer.

At least 37 records · Page 2Linked to original sources

Correlated double-electron additions at the edge of a two-dimensional electronic system

We create laterally large and low disorder quantum well based quantum dots to study single electron additions to two dimensional electron systems (2DES). Electrons tunnel into these dots across an AlGaAs tunnel barrier from a single $n+$ electrode. Using single-electron capacitance spectroscopy in a dilution refrigerator, we identify capacitance peaks for the addition of the first electron to a dot and record subsequent peaks in the addition spectrum up to occupancies of thousands of electrons. Here, we report two remarkable phenomena that occur in the filling factor range $ν=2$ to $ν=5$ while selectively probing electron additions to the edge states of the dot: (1) Coulomb blockade peaks arise from the entrance of two electrons rather than one; (2) at and near filling factor 5/2 and at fixed gate voltage, these double-height peaks appear uniformly with a periodicity of $h/2e$. At other filling factors in the range $ν=2$ to $ν=5$, the mean periodicity for the twice-height electron peaks remains $h/2e$, but the twice-height peaks are instead further bunched into pairs of double-height peaks, with pairs spaced $h/e$ apart. The unusual two-electron Coulomb blockade peaks suggest a novel pair tunneling effect that involves electron correlations that arise in the quantum dot, with spectra at $ν=5/2$ identical to those previously only seen in superconducting dots.

cond-mat.mes-hall↗

A Microscopic Lattice for Two-dimensional Dipolar Excitons

We report a two-dimensional artificial lattice for dipolar excitons confined in a GaAs double quantum well. Exploring the regime of large fillings per lattice site, we verify that the lattice depth competes with the magnitude of excitons repulsive dipolar interactions to control the degree of localisation in the lattice potential. Moreover, we show that dipolar excitons radiate a narrow-band photoluminescence, with a spectral width of a few hundreds of micro-eV at 340 mK, in both localised and delocalised regimes. This makes our device suitable for explorations of dipolar excitons quasi-condensation in a periodic potential.

cond-mat.mes-hall↗

Quasi-condensation of bilayer excitons in a periodic potential

We study two-dimensional excitons confined in a lattice potential, for high fillings of the lattice sites. We show that a quasi-condensate is possibly formed for small values of the lattice depth, but for larger ones the critical phase-space density for quasi-condensation rapidly exceeds our experimental reach, due to the increase of the excitons effective mass. On the other hand, in the regime of a deep lattice potential where excitons are strongly localised at the lattice sites, we show that an array of phase-independent quasi-condensates, different from a Mott insulating phase, is realised.

cond-mat.quant-gas↗

Demonstration of dipolar-induced enhancement of parametric effects in polariton waveguides

Exciton-polaritons are hybrid light-matter excitations arising from the non-perturbative coupling of a photonic mode and an excitonic resonance. Behaving as interacting photons, they show optical third-order nonlinearities providing effects such as optical parametric oscillation or amplification. It has been suggested that polariton-polariton interactions can be greatly enhanced by inducing aligned electric dipoles in their excitonic part. However direct evidence of a true particle-particle interaction, such as superfluidity or parametric scattering is still missing. In this work, we demonstrate that dipolar interactions can be used to enhance parametric effects such as self-phase modulation in waveguide polaritons. By quantifying these optical nonlinearities we provide a reliable experimental measurement of the direct dipolar enhancement of polariton-polariton interactions.

physics.optics↗

Demonstration of a Tunable Antenna-Coupled Intersubband Terahertz (TACIT) Mixer

A fast, voltage-tunable terahertz mixer based on the intersubband transition of a high-mobility 2-dimensional electron gas (2DEG) has been fabricated from a single 40 nm GaAs-AlGaAs square quantum well heterostructure. The device is called a Tunable Antenna-Coupled Intersubband Terahertz (TACIT) mixer, and shows tunability of the detection frequency from 2.52 THz to 3.11 THz with small (< 1 V) top gate and back gate voltage biases. Mixing at 2.52 THz has been observed at 60 K with a -3dB intermediate frequency (IF) bandwidth exceeding 6 GHz.

physics.ins-det↗

Acousto-electric study of microwave-induced current domains

Surface Acoustic Waves (SAW) have been utilized to investigate the properties of a two-dimensional electron system, subjected to a perpendicular magnetic field and monochromatic microwave radiation, in the regime where the so-called microwave-induced zero-resistance states form. Contrary to conventional magneto-transport in Hall bar and van der Pauw geometries, the collimated SAW beam probes only the bulk of the electronic system exposed to this wave. Clear signatures appear in the SAW propagation velocity corroborating that neither contacts, nor sample edges are a root source for their emergence. By virtue of the directional nature of this probing method and with the assistance of theoretical modelling, we were also able to demonstrate that the SAW response depends on the angle between its propagation vector and the orientation of domains which spontaneously form when zero-resistance is observed in transport. This confirms in unprecedented manner the formation of an inhomogeneous phase under these non-equilibrium conditions.

cond-mat.mes-hall↗

Josephson vortices in a long Josephson junction formed by phase twist in a polariton superfluid

Quantum fluids of light are an emerging platform for energy efficient signal processing, ultra-sensitive interferometry and quantum simulators at elevated temperatures. Here we demonstrate the optical control of the topological excitations induced in a large polariton condensate, realising the bosonic analog of a long Josephson junction and reporting the first observation of bosonic Josephson vortices. When a phase difference is imposed at the boundaries of the condensate, two extended regions become separated by a sharp $π$-slippage of the phase and a solitonic depletion of the density, forming an insulating barrier with a suppressed order parameter. The superfluid behavior, that is a smooth phase gradient across the system instead of the sharp phase jump, is recovered at higher polariton densities and it is mediated by the nucleation of Josephson vortices within the barrier. Our results contribute to the understanding of dissipation and stability of elementary excitations in macroscopic quantum systems.

cond-mat.quant-gas↗

Optical Frequency Combs from High-Order Sideband Generation

We report on the generation of frequency combs from the recently-discovered phenomenon of high-order sideband generation (HSG). A near-band gap continuous-wave (cw) laser with frequency $f_\text{NIR}$ was transmitted through an epitaxial layer containing GaAs/AlGaAs quantum wells that were driven by quasi-cw in-plane electric fields $F_\text{THz}$ between 4 and 50 kV/cm oscillating at frequencies $f_\text{THz}$ between 240 and 640 GHz. Frequency combs with teeth at $f_\text{sideband}=f_\text{NIR}+nf_\text{THz}$ ($n$ even) were produced, with maximum reported $n>120$, corresponding to a maximum comb span $>80$ THz. Comb spectra with the identical product $f_\text{THz}\times F_\text{THz}$ were found to have similar spans and shapes in most cases, as expected from the picture of HSG as a scattering-limited electron-hole recollision phenomenon. The HSG combs were used to measure the frequency and linewidth of our THz source as a demonstration of potential applications.

physics.optics↗

Fully guided electrically-controlled exciton polaritons

We demonstrate two types of waveguide structures which optically confine exciton- polaritons in two dimensions and act as polaritonic channels. We show a strong optical confinement in an etched rectangular waveguide, that significantly increases the propa- gation distance of the polaritons and allow to direct them in curved trajectories. Also, we show low-loss optical guiding over a record-high of hundreds of microns which is com- bined seamlessly with electrical control of the polaritons, in a strip waveguide formed by electrically conductive and optically transparent strips deposited on top of a planar waveguide. Both structures are scalable and easy to fabricate and offer new possibilities for designing complex polaritonic devices.

cond-mat.mes-hall↗

Attractive dipolar coupling between stacked exciton fluids

The interaction between aligned dipoles is long-ranged and highly anisotropic: it changes from repulsive to attractive depending on the relative positions of the dipoles. We report on the observation of the attractive component of the dipolar coupling between excitonic dipoles in stacked semiconductor bilayers. We show that the presence of a dipolar exciton fluid in one bilayer modifies the spatial distribution and increases the binding energy of excitonic dipoles in a vertically remote layer. The binding energy changes are explained by a many-body polaron model describing the deformation of the exciton cloud due to its interaction with a remote dipolar exciton. The results open the way for the observation of theoretically predicted new and exotic collective phases, the realization of interacting dipolar lattices in semiconductor systems as well as for engineering and sensing their collective excitations.

cond-mat.quant-gas↗

Strongly interacting dipolar-polaritons

Exciton-polaritons are mutually interacting quantum hybridizations of confined photons and electronic excitations. Here we demonstrate a system of optically guided, electrically polarized exciton-polaritons ('dipolaritons') that displays up to 200-fold enhancement of the polariton-polariton interaction strength compared to unpolarized polaritons. The magnitude of the dipolar interaction enhancement can be turned on and off and be easily tuned over a very wide range by varying the applied polarizing electric-field. The very large interaction strengths and the very long propagation distances of these fully-guided dipolaritons open up new opportunities for realizing complex quantum circuitry and quantum simulators, as well as topological states based on exciton-polaritons, for which the interactions between polaritons need to be large and spatially or temporally controlled. The results also raise fundamental questions on the origin of such large enhancements.

cond-mat.mes-hall↗

Interaction between stimulated current injection and polariton condensate

In this paper, we see a strong effect of the injected current on the light emission from the polariton condensate in an n-i-n structure, when we monitor the luminescence intensity under applied bias at various pump powers. We present here three thresholds for nonlinear increase of the intensity. We show that small changes of the incoherent injected current lead to stimulated enhancement of the coherent light emission from free carriers. We conclude that the polariton condensate-current system is a highly nonlinear electro-optical system.

cond-mat.mes-hall↗

Dynamical birefringence: Electron-hole recollisions as probes of Berry curvature

The direct measurement of Berry phases is still a great challenge in condensed matter systems. The bottleneck has been the ability to adiabatically drive an electron coherently across a large portion of the Brillouin zone in a solid where the scattering is strong and complicated. We break through this bottleneck and show that high-order sideband generation (HSG) in semiconductors is intimately affected by Berry phases. Electron-hole recollisions and HSG occur when a near-band gap laser beam excites a semiconductor that is driven by sufficiently strong terahertz (THz)-frequency electric fields. We carried out experimental and theoretical studies of HSG from three GaAs/AlGaAs quantum wells. The observed HSG spectra contain sidebands up to the 90th order, to our knowledge the highest-order optical nonlinearity observed in solids. The highest-order sidebands are associated with electron-hole pairs driven coherently across roughly 10% of the Brillouin zone around the Γpoint. The principal experimental claim is a dynamical birefringence: the sidebands, when the order is high enough (> 20), are usually stronger when the exciting near-infrared (NIR) and the THz electric fields are polarized perpendicular than parallel; the sideband intensities depend on the angles between the THz field and the crystal axes in samples with sufficiently weak quenched disorder; and the sidebands exhibit significant ellipticity that increases with increasing sideband order, despite nearly linear excitation and driving fields. We explain dynamical birefringence by generalizing the three-step model for high order harmonic generation. The hole accumulates Berry phases due to variation of its internal state as the quasi-momentum changes under the THz field. Dynamical birefringence arises from quantum interference between time-reversed pairs of electron-hole recollision pathways.

cond-mat.mtrl-sci↗

Full Momentum and Energy Resolved Spectral Function of a 2D Electronic System

The single-particle spectral function measures the density of electronic states (DOS) in a material as a function of both momentum and energy, providing central insights into phenomena such as superconductivity and Mott insulators. While scanning tunneling microscopy (STM) and other tunneling methods have provided partial spectral information, until now only angle-resolved photoemission spectroscopy (ARPES) has permitted a comprehensive determination of the spectral function of materials in both momentum and energy. However, ARPES operates only on electronic systems at the material surface and cannot work in the presence of applied magnetic fields. Here, we demonstrate a new method for determining the full momentum and energy resolved electronic spectral function of a two-dimensional (2D) electronic system embedded in a semiconductor. In contrast with ARPES, the technique remains operational in the presence of large externally applied magnetic fields and functions for electronic systems with zero electrical conductivity or with zero electron density. It provides a direct high-resolution and high-fidelity probe of the dispersion and dynamics of the interacting 2D electron system. By ensuring the system of interest remains under equilibrium conditions, we uncover delicate signatures of many-body effects involving electron-phonon interactions, plasmons, polarons, and a novel phonon analog of the vacuum Rabi splitting in atomic systems.

cond-mat.mes-hall↗

Time-resolved two-photon excitation of long-lifetime polaritons

Recent studies of two-photon excitation of exciton-polaritons in microcavities have considered the possibility of an allowed absorption process into the $2p$-state of the excitons which participate in the polariton effect. Here we report time-resolved measurements of two-photon excitation directly into the lower polariton states invoking the $1s$ state of the excitons. Although this process is forbidden by symmetry for light at normal incidence, it is allowed at non-zero angle of incidence due to state mixing.

physics.optics↗

A dark incompressible dipolar liquid of excitons

The possible phases and the nano-scale particle correlations of two-dimensional interacting dipolar particles is a long-sought problem in many-body physics. Here we observe a spontaneous condensation of trapped two-dimensional dipolar excitons with internal spin degrees of freedom from an interacting gas into a high density, closely packed liquid state made mostly of dark dipoles. Another phase transition, into a bright, highly repulsive plasma is observed at even higher excitation powers. The dark liquid state is formed below a critical temperature $T_c \approx 4.8K$, and it is manifested by a clear spontaneous spatial condensation to a smaller and denser cloud, suggesting an attractive part to the interaction which goes beyond the purely repulsive dipole-dipole forces. Contributions from quantum mechanical fluctuations are expected to be significant in this strongly correlated, long living dark liquid. This is a new example of a two-dimensional atomic-like interacting dipolar quantum liquid, but where the coupling of light to its internal spin degrees of freedom plays a crucial role in the dynamical formation and the nature of resulting ground state.

cond-mat.quant-gas↗

Spin-Flipping Half Vortex in a Macroscopic Polariton Spinor Ring Condensate

We report the observation of vorticity in a macroscopic Bose-Einstein condensate of polaritons in a ring geometry. Because it is a spinor condensate, the elementary excitations are "half vortices" in which there is a phase rotation of $π$ in connection with a polarization vector rotation of $π$ around a closed path. This is clearly seen in the experimental observations of the polarization rotation around the ring. In the ring geometry, a new type of half vortex is allowed in which the handedness of the spin flips from one side of the ring to the other, in addition to the rotation of the linear polarization component; such a state is not allowed in a simply-connected geometry. Theoretical calculation of the energy of this state shows that when many-body interactions are taken into account, it is lower in energy than a simple half vortex. The direction of circulation of the flow around the ring fluctuates randomly between clockwise and counterclockwise from one shot to the next; this corresponds to spontaneous breaking of time-reversal symmetry in the system. These new, macroscopic polariton ring condensates allow for the possibility of direct control of the vorticity of the condensate.

cond-mat.quant-gas↗

Tunable Antenna Coupled Intersubband Terahertz Detector

We report on the development of a tunable antenna coupled intersubband terahertz (TACIT) detector based on GaAs/AlGaAs two dimensional electron gas. A successful device design and micro-fabrication process have been developed which maintain the high mobility (1.1x106 cm2/V-s at 10K) of a 2DEG channel in the presence of a highly conducting backgate. Gate voltage-controlled device resistance and direct THz sensing has been observed. The goal is to operate as a nearly quantum noise limited heterodyne sensor suitable for passively-cooled space platforms.

physics.ins-det↗