arXiv subjects

Lorenzo Dominici

Publications and source records attributed to Lorenzo Dominici.

At least 19 recordsLinked to original sources

arXiv2026

Direct Spatiotemporal Imaging of Charge Carrier Dynamics in Operative Semiconductor Devices

Understanding charge carrier dynamics within electronic devices is crucial, as it governs both the internal evolution of signals and the externally measurable current. Yet, direct imaging of these dynamics remains elusive: existing approaches are often indirect or inherently perturbative. Here, we introduce Carrier Dynamics by Pockels Imaging (CDPI), a sensitive, quantitative, and non-invasive method that enables direct access to internal charge dynamics. By probing the local electric field, CDPI visualizes photogenerated electron clouds in real space while simultaneously correlating their evolution with both conduction and displacement currents, thereby establishing a unified picture of carrier transport. The technique provides direct insight into fundamental mechanisms \textemdash including drift, diffusion, carrier-carrier interactions, trapping and detrapping \textemdash as well as the spatiotemporal evolution of carrier cloud morphology. Demonstrated in CdTe radiation detectors with micrometre-scale spatial resolution and nanosecond temporal resolution, CDPI is broadly applicable to systems exhibiting appreciable electro-optic responses. Beyond conventional semiconductors, the approach extends to organic, perovskite, and two-dimensional optoelectronic materials, offering a new paradigm for directly linking internal carrier dynamics to device-level functionality.

physics.optics↗

arXiv2026

Electric-Field Mapping of Optically Perturbed CdTe Radiation Detectors

In radiation detectors, the spatial distribution of the electric field plays a fundamental role in their operation. Access to this field distribution is of strategic importance, especially when investigating the perturbing effects induced by incident radiation. For example, one dangerous effect that prevents their proper operation is the accumulation of internal space charge. Here, we probe the two-dimensional electric field in a Schottky CdTe detector using the Pockels effect and report on its local perturbation after exposure to an optical beam at the anode electrode. Our electro-optical imaging setup, together with a custom processing routine, allows the extraction of the electric-field vector maps and their dynamics during a voltage bias-optical exposure sequence. The results are in agreement with numerical simulations, allowing us to confirm a two-level model based on a dominant deep level. Such a simple model is indeed able to fully account for both the temporal and spatial dynamics of the perturbed electric field. This approach thus allows a deeper understanding of the main mechanisms affecting the non-equilibrium electric-field distribution in CdTe Schottky detectors, such as those leading to polarization. In the future, it could also be used to predict and improve the performance of planar or electrode-segmented detectors.

physics.optics↗

arXiv2026

Pulse, polarization and topology shaping of polariton fuids

Here we present different approaches to ultrafast pulse and polarization shaping, based on a ``quantum fluid'' platform of polaritons. Indeed we exploit the normal modes of two dimensional polariton fluids made of strong coupled quantum well excitons and microcavity photons, by rooting different polarization and topological states into their sub-picosecond Rabi oscillations. Coherent control of two resonant excitation pulses allows us to prepare the desired state of the polariton, taking benefit from its four-component features given by the combination of the two normal modes with the two degrees of polarization. An ultrafast imaging based on the digital off-axis holography technique is implemented to study the polariton complex wavefunction with time and space resolution. We show in order coherent control of the polariton state on the Bloch sphere, an ultrafast polarization sweeping of the Poincaré sphere, and the dynamical twist of full Poincaré states such as the skyrmion on the sphere itself. Finally, we realize a new kind of ultrafast swirling vortices by adding the angular momentum degree of freedom to the two-pulse scheme. These oscillating topology states are characterized by one or more inner phase singularities tubes which spirals around the axis of propagation. The mechanism is devised in the splitting of the vortex into the upper and lower polaritons, resulting in an oscillatory exchange of energy and angular momentum and in the emitted time and space structured photonic packets.

cond-mat.other↗

arXiv2025

Fully Integrated Perovskite Polaritonic Circuits with Tunable Lasing and Nonlinear Amplification

Photonic integrated circuits are emerging as a key technology for compact and energy-efficient optical information processing. Yet, their practical implementation remains limited by the intrinsically weak optical nonlinearities of conventional materials, which demand high power and large footprints to achieve significant nonlinear responses. Exciton-polaritons, hybrid light-matter excitations of semiconducting materials, offer a promising solution by combining strong optical nonlinearities with the high speed and large scalability typical of photonic devices. However, despite their potential, working on-chip polaritonic elements demonstrating room temperature coherent lasing, controllable nonlinear propagation, or amplification have remained elusive. Here we demonstrate a fully integrated perovskite polaritonic circuit that overcomes these limitations. Using a single-step microfluidic lithographic technique, we realize waveguide circuits with integrated gratings that simultaneously act as couplers and mirrors, forming in-plane Fabry-Pérot cavities. These structures support robust in-plane polariton lasing between gratings, yielding coherent emission along the waveguide. Furthermore, we observe clear signatures of strong nonlinear self-phase modulation and, for the first time, optical amplification of guided polaritons at room temperature. Our simple, scalable platform opens the way to low-power, highly nonlinear optical circuits for integrated photonics and neuromorphic architectures operating at room temperature.

physics.optics↗

arXiv2025

Low-power multi-mode fiber projector overcomes shallow neural networks classifiers

In the domain of disordered photonics, the characterization of optically opaque materials for light manipulation and imaging is a primary aim. Among various complex devices, multi-mode optical fibers stand out as cost-effective and easy-to-handle tools, making them attractive for several tasks. In this context, we cast these fibers into random hardware projectors, transforming an input dataset into a higher dimensional speckled image set. The goal of our study is to demonstrate that using such randomized data for classification by training a single logistic regression layer improves accuracy compared to training on direct raw images. Interestingly, we found that the classification accuracy achieved is higher than that obtained with the standard transmission matrix model, a widely accepted tool for describing light transmission through disordered devices. We conjecture that the reason for such improved performance could be due to the fact that the hardware classifier operates in a flatter region of the loss landscape when trained on fiber data, which aligns with the current theory of deep neural networks. These findings suggest that the class of random projections operated by multi-mode fibers generalize better to previously unseen data, positioning them as promising tools for optically-assisted neural networks. With this study, in fact, we want to contribute to advancing the knowledge and practical utilization of these versatile instruments, which may play a significant role in shaping the future of neuromorphic machine learning.

physics.optics↗

arXiv2023

Coupled quantum vortex kinematics and Berry curvature in real space

The Berry curvature provides a powerful tool to unify several branches of science through their geometrical aspect: topology, energy bands, spin and vector fields. While quantum defects -- phase vortices and skyrmions -- have been in the spotlight, as rotational entities in condensates, superfluids and optics, their dynamics in multi-component fields remain little explored. Here we use two-component microcavity polaritons to imprint a dynamical pseudospin texture in the form of a double full Bloch beam, a conformal continuous vortex beyond unitary skyrmions. The Berry curvature plays a key role to link various quantum spaces available to describe such textures. It explains for instance the ultrafast spiraling in real space of two singular vortex cores, providing in particular a simple expression -- also involving the complex Rabi frequency -- for their intricate velocity. Such Berry connections open new perspectives for understanding and controlling highly-structured quantum objects, including strongly asymmetric cases or even higher multi-component fields.

physics.optics↗

arXiv2022

Topologically driven Rabi-oscillating interference dislocation

Quantum vortices are the quantized version of classical vortices. Their center is a phase singularity or vortex core around which the flow of particles as a whole circulates and is typical in superfluids, condensates and optical fields. However, the exploration of the motion of the phase singularities in coherently-coupled systems is still underway. We theoretically analyze the propagation of an interference dislocation in the regime of strong coupling between light and matter, with strong mass imbalance, corresponding to the case of microcavity exciton-polaritons. To this end, we utilize combinations of vortex and tightly focused Gaussian beams, which are introduced through resonant pulsed pumping. We show that a dislocation originates from self-interference fringes, due to the non-parabolic dispersion of polaritons combined with moving Rabi-oscillating vortices. The morphology of singularities is analyzed in the Poincaré space for the pseudospin associated to the polariton states. The resulting beam carries orbital angular momentum with decaying oscillations due to the loss of overlap between the normal modes of the polariton system.

cond-mat.quant-gas↗

arXiv2022

Optical Writing and Electro-Optic Imaging of Reversible Space Charges in Semi-Insulating CdTe Diodes

Deep levels control the space charge in electrically compensated semi-insulating materials. They limit the performance of radiation detectors but their interaction with free carriers can be favorably exploited in these devices to manipulate the spatial distribution of the electric field by optical beams. By using semi-insulating CdTe diodes as a case study, our results show that optical doping functionalities are achieved. As such, a highly stable, flux-dependent, reversible and spatially localized space charge is induced by a line-shaped optical beam focused on the cathode contact area. Real-time non-invasive imaging of the electric field is obtained through the Pockels effect. A simple and convenient method to retrieve the two-dimensional electric field components is presented. Numerical simulations involving just one deep level responsible for the electrical compensation confirm the experimental findings and help to identify the underlying mechanism and critical parameters enabling the optical writing functionalities.

physics.optics↗

arXiv2021

Single-step transmission matrix retrieval for fast imaging through multi-mode fibers

Recovering the transmission matrix of a disordered medium is a challenging problem in disordered photonics. Usually, its reconstruction relies on a complex inversion that aims at connecting a fully-controlled input to the deterministic interference of the light field scrambled by the device. At the moment, iterative phase-retrieval protocols provide the fastest reconstructing frameworks, converging in a few tens of iterations. Exploiting the knowledge of speckle correlations, we construct a new phase retrieval algorithm that reduces the computational cost to a single iteration. Besides being faster, our method is effective also using less measurements than state-of-the-art protocols. Thanks to reducing computation time by one order of magnitude, our result can be groundbreaking for real-time optical operations in medical imaging.

physics.comp-ph↗

arXiv2021

Shaping the topology of light with a moving Rabi-oscillating vortex

Quantum vortices are the analogue of classical vortices in optics, Bose-Einstein condensates, superfluids and superconductors, where they provide the elementary mode of rotation and orbital angular momentum. While they mediate important pair interactions and phase transitions in nonlinear fluids, their linear dynamics is useful for the shaping of complex light, as well as for topological entities in multi-component systems, such as full Bloch beams. Here, setting a quantum vortex into directional motion in an open-dissipative fluid of microcavity polaritons, we observe the self-splitting of the packet, leading to the trembling movement of its center of mass, whereas the vortex core undergoes ultrafast spiraling along diverging and converging circles, in a sub-picosecond precessing fashion. This singular dynamics is accompanied by vortex-antivortex pairs creation and annihilation, and a periodically changing topological charge. The spiraling and branching mechanics represent a direct manifestation of the underlying Bloch pseudospin space, whose mapping is shown to be rotating and splitting itself. Its reshaping is due to three simultaneous drives along the distinct directions of momentum and complex frequency, by means of the differential group velocities, Rabi frequency and dissipation rates, which are natural assets in coupled fields such as polaritons. This state, displaying linear momentum dressed with oscillating angular momentum, confirms the richness of multi-component and open quantum fluids and their innate potentiality to implement sophisticated and dynamical topological textures of light.

physics.optics↗

arXiv2021

Dynamics of a vortex lattice in an expanding polariton quantum fluid

If a quantum fluid is driven with enough angular momentum, at equilibrium the ground state of the system is given by a lattice of quantised vortices whose density is prescribed by the quantization of circulation. We report on the first experimental study of the Feynman-Onsager relation in a non-equilibrium polariton fluid, free to expand and rotate. Upon initially imprinting a lattice of vortices in the quantum fluid, we track the vortex core positions on picosecond time scales. We observe an accelerated stretching of the lattice and an outward bending of the linear trajectories of the vortices, due to the repulsive polariton interactions. Access to the full density and phase fields allows us to detect a small deviation from the Feynman-Onsager rule in terms of a transverse velocity component, due to the density gradient of the fluid envelope acting on the vortex lattice.

cond-mat.quant-gas↗

arXiv2021

Macroscopic Two-Dimensional Polariton Condensates

We report a record-size, two-dimensional polariton condensate of a fraction of a millimeter radius free from the presence of an exciton reservoir. This macroscopically occupied state is formed by the ballistically expanding polariton flow that relaxes and condenses over a large area outside of the excitation spot. The density of this trap-free condensate is < 1 polariton/μm^2, reducing the phase noise induced by the interaction energy. Moreover, the backflow effect, recently predicted for the nonparabolic polariton dispersion, is observed here for the first time in the fast-expanding wave packet.

cond-mat.quant-gas↗

arXiv2021

Full-Bloch beams and ultrafast Rabi-rotating vortices

Strongly-coupled quantum fields, such as multi-component atomic condensates, optical fields and polaritons, are remarkable systems where the simple dynamics of coupled oscillators can meet the intricate phenomenology of quantum fluids. When the coupling between the components is coherent, not only the particles number, but also their phase texture that maps the linear and angular momentum, can be exchanged. Here, on a system of exciton-polaritons, we have realized a so-called full-Bloch beam: a configuration in which all superpositions of the upper and the lower polariton -- all quantum states of the associated Hilbert space -- are simultaneously present at different points of the physical space, evolving in time according to Rabi-oscillatory dynamics. As a result, the light emitted by the cavity displays a peculiar dynamics of spiraling vortices endowed with oscillating linear and angular momentum and exhibiting ultrafast motion of their cores with striking accelerations to arbitrary speeds. This remarkable vortex motion is shown to result from distortions of the trajectories by a homeomorphic mapping between the Rabi rotation of the full wavefunction on the Bloch sphere and Apollonian circles in the real space where the observation is made. Such full-Bloch beams offer new prospects at a fundamental level regarding their topological properties or in the interpretation of quantum mechanics, and the Rabi-rotating vortices they yield should lead to interesting applications such as ultrafast optical tweezers.

cond-mat.quant-gas↗

arXiv2020

Demonstration of dipolar-induced enhancement of parametric effects in polariton waveguides

Exciton-polaritons are hybrid light-matter excitations arising from the non-perturbative coupling of a photonic mode and an excitonic resonance. Behaving as interacting photons, they show optical third-order nonlinearities providing effects such as optical parametric oscillation or amplification. It has been suggested that polariton-polariton interactions can be greatly enhanced by inducing aligned electric dipoles in their excitonic part. However direct evidence of a true particle-particle interaction, such as superfluidity or parametric scattering is still missing. In this work, we demonstrate that dipolar interactions can be used to enhance parametric effects such as self-phase modulation in waveguide polaritons. By quantifying these optical nonlinearities we provide a reliable experimental measurement of the direct dipolar enhancement of polariton-polariton interactions.

physics.optics↗

arXiv2020

Temporal shaping and time varying orbital angular momentum of displaced vortices

The fundamental mode of rotation in quantum fluids is given by a vortex, whose quantized value yields the orbital angular momentum (OAM) per particle. If the vortex is displaced (off-centered) from the reference point for rotation, the angular momentum is reduced and becomes fractional. Such displaced vortices can further exhibit a peculiar dynamics in presence of confining potentials or couplings to other fields. We study analytically a number of 2D systems where displaced vortices exhibit a noteworthy dynamics, including time-varying self-sustained oscillation of the OAM, complex reshaping of their morphology with possible creation of vortex-antivortex pairs and peculiar trajectories for the vortex core with sequences of strong accelerations and decelerations which can even send the core to infinity and bring it back. Interestingly, these do not have to occur conjointly, with complex time dynamics of the vortex core and/or their wavepacket morphology possibly taking place without affecting the total OAM. Our results generalize to simple and fundamental systems a phenomenology recently reported with Rabi-coupled bosonic fields, showing their wider relevance and opening prospects for new types of control and structuring of the angular momentum of light and/or quantum fluids.

cond-mat.quant-gas↗

arXiv2020

Tuning the Berry curvature in 2D Perovskite

Topological physics and in particular its connection with artificial gauge fields is a forefront topic in different physical systems, ranging from cold atoms to photonics and more recently semiconductor dressed exciton-photon states, called polaritons. Engineering the energy dispersion of polaritons in microcavities through nanofabrication or exploiting the intrinsic material and cavity anisotropies has demonstrated many intriguing effects related to topology and emergent gauge fields. Here, we show that we can control the Berry curvature distribution of polariton bands in a strongly coupled organic-inorganic 2D perovskite single crystal. The spatial anisotropy of the perovskite crystal combined with photonic spin-orbit coupling make emerge two Hamilton's diabolical points in the dispersion. The application of an external magnetic field breaks time reversal symmetry thanks to the exciton Zeeman splitting. It splits the diabolical points degeneracy. The resulting bands show non-zero integral Berry curvature which we directly measure by state tomography. Crucially, we show that we can control the Berry curvature distribution in the band, the so-called band geometry, within the same microcavity.

physics.optics↗

arXiv2020

Observation of two thresholds leading to polariton condensation in 2D hybrid perovskites

Two dimensional (2D) perovskites are promising materials for photonic applications, given their outstanding nonlinear optical properties, ease of fabrication and versatility. In particular, exploiting their high oscillator strength, the crystalline form of 2D perovskites can be used as excitonic medium in optical microcavities, allowing for the study of their optical properties in the strong light-matter coupling regime. While polariton condensation has been observed in different materials at room temperature, here we observe for the first time two distinct threshold processes in a 2D perovskite, a material that has never shown spontaneous phase transition up to now. In particular, we demonstrate lasing from the bi-exciton state which contributes to populate the lower polariton branch and, at higher excitation powers, eventually leads to the formation of a polariton condensate. The emission linewidth narrowing and a spatial coherence over 50 x 50 um2 area are the smoking gun, the formation of a quantum coherent state in 2D hybrid perovskite. Our results not only show the formation of a polariton condensate in 2D perovskites but they are also crucial for the understanding of the physical mechanisms that leads to coherent phase transition in perovskite-based polariton microcavities.

physics.optics↗

arXiv2019

Directional Goldstone waves in polariton condensates close to equilibrium

Quantum fluids of light are realized in semiconductor microcavities by exciton-polaritons, solid-state quasi-particles with a light mass and sizeable interactions. Here, we use the microscopic analogue of oceanographic techniques to measure the excitation spectrum of a thermalised polariton condensate. Increasing the fluid density, we demonstrate the transition from a free-particle parabolic dispersion to a linear, sound-like Goldstone mode characteristic of superfluids at equilibrium. Notably, we show that excitations are created with a definite direction with respect to the condensate, analogous to how a sea breeze develops surface waves aligned with the wind. These results reveal the effect of asymmetric pumping on the collective excitations of a condensate. Furthermore, we measure the critical sound speed for polariton superfluids close to equilibrium.

cond-mat.quant-gas↗