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Lou Kondic

Publications and source records attributed to Lou Kondic.

At least 55 records · Page 3Linked to original sources

Stability of thin fluid films characterised by a complex form of structural/effective disjoining pressure

We discuss instabilities of fluid films of nanoscale thickness, with a particular focus on films where the destabilising mechanism allows for linear instability, metastability, and absolute stability. Our study is motivated by nematic liquid crystal films; however we note that similar instability mechanisms, and forms of the effective disjoining pressure, appear in other contexts, such as the well-studied problem of polymeric films on two-layered substrates. The analysis is carried out within the framework of the long-wave approximation, which leads to a fourth order nonlinear partial different equation for the film thickness. Within the considered formulation, the nematic character of the film leads to an additional contribution to the disjoining pressure, changing its functional form. This effective disjoining pressure is characterised by the presence of a local maximum for non-vanishing film thickness. Such a form leads to complicated instability evolution that we study by analytical means, including application of marginal stability criteria, and by extensive numerical simulations that help us develop a better understanding of instability evolution in the nonlinear regime. This combination of analytical and computational techniques allows us to reach novel understanding of relevant instability mechanisms, and of their influence on transient and fully developed fluid film morphologies.

cond-mat.soft↗

Evolution of force networks in dense granular matter close to jamming

When dense granular systems are exposed to external forcing, they evolve on the time scale that is typically related to the externally imposed one (shear or compression rate, for example). This evolution could be characterized by observing temporal evolution of contact networks. However, it is not immediately clear whether the force networks, defined on contact networks by considering force interactions between the particles, evolve on a similar time scale. To analyze the evolution of these networks, we carry out discrete element simulations of a system of soft frictional disks exposed to compression that leads to jamming. By using the tools of computational topology, we show that close to jamming transition, the force networks evolve on the time scale which is much faster than the externally imposed one. The presentation will discuss the factors that determine this fast time scale.

cond-mat.soft↗

Direct numerical simulation of variable surface tension flows using a Volume-of-Fluid method

We develop a general methodology for the inclusion of variable surface tension into a Volume-of-Fluid based Navier-Stokes solver. This new numerical model provides a robust and accurate method for computing the surface gradients directly by finding the tangent directions on the interface using height functions. The implementation is applicable to both temperature and concentration dependent surface tension, along with the setups involving a large jump in the temperature between the fluid and its surrounding, as well as the situations where the concentration should be strictly confined to the fluid domain, such as the mixing of fluids with different surface tension coefficients. We demonstrate the applicability of our method to thermocapillary migration of bubbles and coalescence of drops characterized by different surface tension.

physics.flu-dyn↗

Granular Impact: A Grain-scale Approach

This work summarizes a series of studies on two-dimensional granular impact, where an intruding object strikes a granular material at high speed. Many previous studies on granular impact have used a macroscopic force law, which is dominated by an inertial drag term proportional to the intruder velocity squared. The primary focus here is on the microscopic force response of the granular material, and how the grain-scale effects give rise to this inertial drag term. We show that the inertial drag arises from intermittent collisions with force-chain-like structures. We construct a simple collisional model to explain the inertial drag, as well as off-axis instability and rotations. Finally, we show how the granular response changes when the intruder speed approaches $d/t_c$, leading to a failure of the inertial drag description in this regime. Here, $d$ is the mean particle diameter and $t_c$ the characteristic momentum-transfer time between two grains.

cond-mat.soft↗

Interfacial Dynamics of Thin Viscoelastic Films and Drops

We present a computational investigation of thin viscoelastic films and drops on a solid substrate subject to the van der Waals interaction force, in two spatial dimensions. The governing equations are obtained within a long-wave approximation of the Navier-Stokes equations with Jeffreys model for viscoelastic stresses. We investigate the effects of viscoelasticity, Newtonian viscosity, and the substrate slippage on the dynamics of thin viscoelastic films. We also study the effects of viscoelasticity on drops that spread or recede on a prewetted substrate. For dewetting films, the numerical results show the presence of multiple secondary droplets for higher values of elasticity, consistently with experimental findings. For drops, we find that elastic effects lead to deviations from the Cox-Voinov law for partially wetting fluids. In general, elastic effects enhance spreading, and suppress retraction, compared to Newtonian ones.

physics.flu-dyn↗

Instability of nanometric fluid films on a thermally conductive substrate

We consider thin fluid films placed on thermally conductive substrates and exposed to time-dependent spatially uniform heat source. The evolution of the films is considered within the long-wave framework in the regime such that both fluid/substrate interaction, modeled via disjoining pressure, and Marangoni forces, are relevant. We analyze the problem by the means of linear stability analysis as well as by time-dependent nonlinear simulations. The main finding is that when self-consistent computation of the temperature field is performed, a complex interplay of different instability mechanisms results. This includes either monotonous or oscillatory dynamics of the free surface. In particular, we find that the oscillatory behavior is absent if the film temperature is assumed to be slaved to the current value of the film thickness. The results are discussed within the context of liquid metal films, but are of relevance to dynamics of any thin film involving variable temperature of the free surface, such that the temperature and the film interface itself evolve on comparable time scales.

cond-mat.soft↗

Steady Flow Dynamics during Granular Impact

We study experimentally and computationally the dynamics of granular flow during impacts, where intruders strike a collection of disks from above. In the regime where granular force dynamics are much more rapid than the intruder motion, we find that the particle flow near the intruder is proportional to the instantaneous intruder speed; it is essentially constant when normalized by that speed. The granular flow is nearly divergence-free and remains in balance with the intruder, despite the latter's rapid deceleration. Simulations indicate that this observation is insensitive to grain properties, which can be explained by the separation of time scales between intergrain force dynamics and intruder dynamics. Assuming there is a comparable separation of time scales, we expect our results are applicable to a broad class of dynamic or transient granular flows. Our results suggest that descriptions of static-in-time granular flows might be extended or modified to describe these dynamic flows. Additionally, we find that accurate grain-grain interactions are not necessary to correctly capture the granular flow in this regime.

cond-mat.soft↗

Scaling Properties of Force Networks for Compressed Particulate Systems

We consider, computationally and experimentally, the scaling properties of force networks in the systems of circular particles exposed to compression in two spatial dimensions. The simulations consider polydisperse and monodisperse particles, both frictional and frictionless, and in experiments we use monodisperse and bidisperse particles. While for some of the considered systems we observe consistent scaling exponents describing the behavior of the force networks, we find that this behavior is it not universal. In particular, monodisperse frictionless systems that partially crystallize under compression, show scaling properties that are significantly different compared to the other considered systems. The findings of non-universality are confirmed by explicitly computing fractal dimension for the considered systems. The results of physical experiments are consistent with the results obtained in simulations of frictional particles.

physics.comp-ph↗

A volume of fluid method for simulating fluid/fluid interfaces in contact with solid boundaries

In this paper, we present a novel approach to model the fluid/solid interaction forces in a direct solver of the Navier-Stokes equations based on the volume of fluid interface tracking method. The key ingredient of the model is the explicit inclusion of the fluid/solid interaction forces into the governing equations. We show that the interaction forces lead to a partial wetting condition and in particular to a natural definition of the equilibrium contact angle. We present two numerical methods to discretize the interaction forces that enter the model; these two approaches differ in complexity and convergence. To validate the computational framework, we consider the application of these models to simulate two-dimensional drops at equilibrium, as well as drop spreading. We demonstrate that the model, by including the underlying physics, captures contact line dynamics for arbitrary contact angles. More generally, the approach permits novel means to study contact lines, as well as a diverse range of phenomena that previously could not be addressed in direct simulations.

physics.flu-dyn↗

Nonlinear Force Propagation during Granular Impact

We experimentally study nonlinear force propagation into granular material during impact from an intruder, and we explain our observations in terms of the nonlinear grain-scale force relation. Using high-speed video and photoelastic particles, we determine the speed and spatial structure of the force response just after impact. We show that these quantities depend on a dimensionless parameter, $M'=t_c v_0/d$, where $v_0$ is the intruder speed at impact, $d$ is the particle diameter, and $t_c$ is the collision time for a pair of grains impacting at relative speed $v_0$. The experiments access a large range of $M'$ by using particles of three different materials. When $M' \ll 1$, force propagation is chain-like with a speed, $v_f$, satisfying $v_f \propto d/t_c$. For larger $M'$, the force response becomes spatially dense and the force propagation speed departs from $v_f\propto d/t_c$, corresponding to collective stiffening of a strongly compressed packing of grains.

cond-mat.soft↗

Evolution of Force Networks in Dense Particulate Media

We introduce novel sets of measures with the goal of describing dynamical properties of force networks in dense particulate systems. The presented approach is based on persistent homology and allows for extracting precise, quantitative measures that describe the evolution of geometric features of the interparticle forces, without necessarily considering the details related to individual contacts between particles. The networks considered emerge from discrete element simulations of two dimensional particulate systems consisting of compressible frictional circular disks. We quantify the evolution of the networks for slowly compressed systems undergoing jamming transition. The main findings include uncovering significant but localized changes of force networks for unjammed systems, global (system-wide) changes as the systems evolve through jamming, to be followed by significantly less dramatic evolution for the jammed states. We consider both connected components, related in loose sense to force chains, and loops, and find that both measures provide a significant insight into the evolution of force networks. In addition to normal, we consider also tangential forces between the particles and find that they evolve in the consistent manner. Consideration of both frictional and frictionless systems leads us to the conclusion that friction plays a significant role in determining the dynamical properties of the considered networks. We find that the proposed approach describes the considered networks in a precise yet tractable manner, allowing to identify novel features which could be difficult or impossible to describe using other approaches.

physics.data-an↗

Note on the hydrodynamic description of thin nematic films: strong anchoring model

We discuss the long-wave hydrodynamic model for a thin film of nematic liquid crystal in the limit of strong anchoring at the free surface and at the substrate. We rigorously clarify how the elastic energy enters the evolution equation for the film thickness in order to provide a solid basis for further investigation: several conflicting models exist in the literature that predict qualitatively different behaviour. We consolidate the various approaches and show that the long-wave model derived through an asymptotic expansion of the full nemato-hydrodynamic equations with consistent boundary conditions agrees with the model one obtains by employing a thermodynamically motivated gradient dynamics formulation based on an underlying free energy functional. As a result, we find that in the case of strong anchoring the elastic distortion energy is always stabilising. To support the discussion in the main part of the paper, an appendix gives the full derivation of the evolution equation for the film thickness via asymptotic expansion.

physics.flu-dyn↗

Modelling spreading dynamics of liquid crystals in three spatial dimensions

We study spreading dynamics of nematic liquid crystal droplets within the framework of the long-wave approximation. A fourth order nonlinear parabolic partial differential equation governing the free surface evolution is derived. The influence of elastic distortion energy and of imposed anchoring variations at the substrate are explored through linear stability analysis and scaling arguments, which yield useful insight and predictions for the behaviour of spreading droplets. This behaviour is captured by fully nonlinear time-dependent simulations of three dimensional droplets spreading in the presence of anchoring variations that model simple defects in the nematic orientation at the substrate.

physics.flu-dyn↗

Particle Scale Dynamics in Granular Impact

We perform an experimental study of granular impact, where intruders strike 2D beds of photoelastic disks from above. High-speed video captures the intruder dynamics and the local granular force response, allowing investigation of grain-scale mechanisms in this process. We observe rich acoustic behavior at the leading edge of the intruder, strongly fluctuating in space and time, and we show that this acoustic activity controls the intruder deceleration, including large force fluctuations at short time scales. The average intruder dynamics match previous studies using empirical force laws, suggesting a new microscopic picture, where acoustic energy is carried away and dissipated.

cond-mat.soft↗

Thin films flowing down inverted substrates: two dimensional flow

We consider free surface instabilities of films flowing on inverted substrates within the framework of lubrication approximation. We allow for the presence of fronts and related contact lines, and explore the role which they play in instability development. It is found that a contact line, modeled by a commonly used precursor film model, leads to free surface instabilities without any additional natural or excited perturbations. A single parameter D=(3Ca)^{1/3}\cotα$, where $Ca$ is the capillary number and $α$ is the inclination angle, is identified as a governing parameter in the problem. This parameter may be interpreted to reflect the combined effect of inclination angle, film thickness, Reynolds number and the fluid flux. Variation of $D$ leads to change of the wave-like properties of the instabilities, allowing us to observe traveling wave behavior, mixed waves, and the waves resembling solitary ones.

physics.flu-dyn↗

How do drops evaporate?

We consider evaporation of pure liquid drops on a thermally conductive substrate. Two evaporative models are considered: one that concentrates on the liquid phase in determining evaporative flux, and the other one that centers on the gas/vapor phase. A single governing equation for the evolution of drop thickness, including both models, is developed. Experiments are used to estimate relevant parameters. We show how the derived governing equation can be used to predict which evaporation model is appropriate under considered experimental conditions.

physics.flu-dyn↗

Stabilization of nonlinear velocity profiles in athermal systems undergoing planar shear flow

We perform molecular dynamics simulations of model granular systems undergoing boundary-driven planar shear flow in two spatial dimensions with the goal of developing a more complete understanding of how dense particulate systems respond to applied shear. In particular, we are interested in determining when these systems will possess linear velocity profiles and when they will develop highly localized velocity profiles in response to shear. In previous work on similar systems we showed that nonlinear velocity profiles form when the speed of the shearing boundary exceeds the speed of shear waves in the material. However, we find that nonlinear velocity profiles in these systems are unstable at very long times. The degree of nonlinearity slowly decreases in time; the velocity profiles become linear when the granular temperature and density profiles are uniform across the system at long times. We measure the time $t_l$ required for the velocity profiles to become linear and find that $t_l$ increases as a power-law with the speed of the shearing boundary and increases rapidly as the packing fraction approaches random close packing. We also performed simulations in which differences in the granular temperature across the system were maintained by vertically vibrating one of the boundaries during shear flow. We find that nonlinear velocity profiles form and are stable at long times if the difference in the granular temperature across the system exceeds a threshold value that is comparable to the glass transition temperature in an equilibrium system at the same average density. Finally, the sheared and vibrated systems form stable shear bands, or highly localized velocity profiles, when the applied shear stress is lowered below the yield stress of the static part of the system.

cond-mat.soft↗

On velocity profiles, stresses and Bagnold scaling of sheared granular system in zero gravity

We report the results of three-dimensional molecular dynamics simulations of sheared granular system in a Couette geometry.\cite{movies} The simulations use realistic boundary conditions that may be expected in physical experiments. For a range of boundary properties we report velocity and density profiles, as well as forces on the boundaries. In particular, we find that the results for the velocity profiles throughout the shearing cell depend strongly on the interaction of the system particles with the physical boundaries. Even frictional boundaries can allow for significant slippage of the particles, therefore, reducing the shear in the system. Next, we present shear rate dependence of stress, including mean force and force fluctuations, both for controlled volume, and for controlled stress configurations. We discuss the dependence of solid volume fraction on shear rate under the constant pressure condition, and Bagnold scaling in volume controlled experiments. In addition, we study the influence of oscillatory driving on the system properties.

cond-mat.soft↗