SearcharxivSearch

arXiv subjects

Louis Martin-Monier

Publications and source records attributed to Louis Martin-Monier.

10 recordsLinked to original sources

Nanophotonic control of spatial information in scintillation detectors

X-rays enable non-invasive imaging across medicine, security, materials science, and beyond, yet modern systems remain constrained by the need to resolve finer structures at lower radiation dose. Scintillators are the dominant materials for detecting X-rays, but face a longstanding compromise: thick scintillators absorb X-rays effectively, whereas optical photons generated throughout their volume spread before detection, degrading spatial information. Existing scintillator architectures largely try to preserve resolution by physically confining light using pixels, columnar crystals, or microstructured channels. Here, we show that high-resolution detection does not require the volumetric confinement of scintillation light. A metalens integrated directly with a bulk scintillator uses nanophotonic wavefront control to preferentially transfer high-spatial-frequency information from volumetrically generated scintillation light to the detector, while retaining the X-ray absorption of a thick scintillator. We experimentally recover fine spatial detail in X-ray images of inorganic and biological specimens. In a detector geometry relevant to computed tomography (CT), the experimentally validated model predicts a fivefold reduction in required X-ray dose and a 25-fold increase in resolution bandwidth relative to a state-of-the-art pixelated scintillator. These results establish wavefront engineering as a route to separating efficient X-ray absorption from optical image formation, with the potential for substantially higher-resolution, lower-dose CT.

physics.optics

Dosimetric characterization of a nanophotonic scintillator and applications to real-time in-vivo total body irradiation dosimetry

Purpose: Recent advances in metasurface photonics and manufacturing have enabled a nanophotonic surface coating to be applied to conventional scintillators, which has been shown to significantly improve light yield. However, the dosimetric properties of such coatings has not been established. We performed the first dosimetric characterization of a nanophotonic scintillator and explored clinical application to real-time in-vivo total body irradiation (TBI) dosimetry. Methods: A 4.5x1.5 cm cerium-doped yttrium aluminum garnet (YAG:Ce) scintillator, half patterned with the nanophotonic structure, half left unpatterned, enabled direct comparison between conventional and nanophotonic surfaces. The scintillator was placed in a 3D-printed light-tight box with an off-axis CMOS camera and irradiated with a clinical linear accelerator. Absolute dosimetry was done with dose-calibrated radiochromic film. For TBI, the scintillator was positioned on an anthropomorphic phantom in a TBI booth, with signal measured by both CMOS and consumer-grade phone cameras under different room lighting conditions. Results: The nanophotonic scintillator showed a 4.1x increase in signal and a 3.7x increase in contrast-to-noise ratio versus the conventional scintillator. Both scintillators exhibited dose-rate independence and linear dose response, with modest energy dependence. For TBI, the nanophotonic scintillator produced a clearly detectable signal with both CMOS and phone cameras, whereas the conventional scintillator signal was undetectable. Conclusions: Nanophotonic structures significantly enhance light output of conventional scintillators without impacting their dosimetric properties. Nanophotonic scintillators may enable real-time in-vivo TBI dosimetry. Future work should investigate this technology for improved dosimetry equipment and X-ray imaging detectors.

physics.med-ph

Wavefront Engineering for Scintillation-Based Imaging

Recent research in nanophotonics for scintillation-based imaging has demonstrated promising improvements in scintillator performance. In parallel, advances in nanophotonics have enabled wavefront control through metasurfaces, a capability that has transformed fields such as microscopy by allowing tailored control of optical propagation. This naturally raises the following question, which we address in this perspective: can wavefront-control strategies be leveraged to improve scintillation-based imaging? To answer this question, we explore nanophotonic- and metasurface-enabled wavefront control in scintillators to mitigate image blurring arising from their intrinsically diffuse light emission. While depth-of-field extension in scintillation faces fundamental limitations absent in microscopy, this approach reveals promising avenues, including stacked scintillators, selective spatial-frequency enhancement, and X-ray energy-dependent imaging. These results clarify the key distinctions in adapting wavefront engineering to scintillation and its potential to enable tailored detection strategies.

physics.optics

Wide field-of-view and large depth-of-field metalenses

The ability to visualize both macroscopic and microscopic features over an extended field of view is essential for endoscopic imaging and other applications ranging from machine vision to microscopy. However, miniaturizing endoscopes introduces inherent trade-offs between size and optical performance, including field-of-view (FOV), depth-of-field (DOF), and resolution. These constraints limit the use of microendoscopes in clinical settings such as early cancer detection within narrow, hard-to-access anatomical regions, including the lung, ovaries, and pancreas. State-of-the-art microendoscopes typically rely on microlens assemblies that increase both cost and size. Their large f-numbers also hinder the collection of high-resolution information from live tissue. In this work, we present two compact metalens designs that provide wide FOV, extended DOF, and high resolution, enabled by custom-tailored point spread functions (PSFs). The devices achieve a full 172 degrees FOV, an extended DOF from 0.4 mm to beyond 300 mm, and a resolution of 30 line pairs per millimeter, all within a 1 mm x 1 mm x 0.2 mm footprint. A key advantage of our approach is the ability to transition seamlessly between low and high magnification without mechanical refocusing. Final images are reconstructed through backend deconvolution, highlighting the potential of hybrid imaging systems that integrate computational techniques with flat-optics components.

physics.optics

Wafer-scale conformal metasurface optics

Curved and conformal optics offer significant advantages by unlocking additional geometric degrees of freedom for optical design. These capabilities enable enhanced optical performance and are essential for meeting non-optical constraints, such as those imposed by ergonomics, aerodynamics, or wearability. However, existing fabrication techniques such as direct electron or laser beam writing on curved substrates, and soft-stamp-based transfer or nanoimprint lithography suffer from limitations in scalability, yield, geometry control, and alignment accuracy. Here, we present a scalable fabrication strategy for curved and conformal metasurface optics leveraging thermoforming, an industry-standard, high-throughput manufacturing process widely used for shaping thermoplastics. Our approach uniquely enables wafer-scale production of highly curved metasurface optics, achieving sub-millimeter radii of curvature and micron-level alignment precision. To guide the design and fabrication process, we developed a thermorheological model that accurately predicts and compensates for the large strains induced during thermoforming. This allows for precise control of metasurface geometry and preservation of optical function, yielding devices with diffraction-limited performance. As a demonstration, we implemented an artificial compound eye comprising freeform micro-metalens arrays. Compared to traditional micro-optical counterparts, the device exhibits an expanded field of view, reduced aberrations, and improved uniformity, highlighting the potential of thermoformed metasurfaces for next-generation optical systems.

physics.optics

Large-scale self-assembled nanophotonic scintillators for X-ray imaging

Scintillators are essential for converting X-ray energy into visible light in imaging technologies. Their widespread application in imaging technologies has been enabled by scalable, high-quality, and affordable manufacturing methods. Nanophotonic scintillators, which feature nanostructures at the scale of their emission wavelength, provide a promising approach to enhance emission properties like light yield, decay time, and directionality. However, scalable fabrication of such nanostructured scintillators has been a significant challenge, impeding their widespread adoption. Here, we present a scalable fabrication method for large-area nanophotonic scintillators based on the self-assembly of chalcogenide glass photonic crystals. This technique enables the production of nanophotonic scintillators over wafer-scale areas, achieving a six-fold enhancement in light yield compared to unpatterned scintillators. We demonstrate this approach using a conventional X-ray scintillator material, cerium-doped yttrium aluminum garnet (YAG:Ce). By analyzing the influence of surface nanofabrication disorder, we establish its effect on imaging performance and provide a route towards large-scale scintillation enhancements without decrease in spatial resolution. Finally, we demonstrate the practical applicability of our nanophotonic scintillators through X-ray imaging of biological and inorganic specimens. Our results indicate that this scalable fabrication technique could enable the industrial implementation of a new generation of nanophotonic-enhanced scintillators, with significant implications for advancements in medical imaging, security screening, and nondestructive testing.

physics.optics

Unravelling and circumventing failure mechanisms in chalcogenide optical phase change materials

Chalcogenide optical phase change materials (PCMs) have garnered significant interest for their growing applications in programmable photonics, optical analog computing, active metasurfaces, and beyond. Limited endurance or cycling lifetime is however increasingly becoming a bottleneck toward their practical deployment for these applications. To address this issue, we performed a systematic study elucidating the cycling failure mechanisms of Ge$_2$Sb$_2$Se$_4$Te (GSST), a common optical PCM tailored for infrared photonic applications, in an electrothermal switching configuration commensurate with their applications in on-chip photonic devices. We further propose a set of design rules building on insights into the failure mechanisms, and successfully implemented them to boost the endurance of the GSST device to over 67,000 cycles.

physics.optics

Second harmonic generation from Chalcogenide metasurfaces via mode coupling engineering

Dielectric metasurfaces have shown prominent applications in nonlinear optics due to strong field enhancement and low dissipation losses at the nanoscale. Chalcogenide glasses are one of the promising materials for the observation of nonlinear effects due to their high intrinsic nonlinearities. Here, we demonstrate, experimentally and theoretically, that significant second harmonic generation can be obtained within amorphous chalcogenide based metasurfaces by relying on the coupling between lattice and particle resonances. We further show that the high quality factor resonance at the origin of the second harmonic generation can be tuned over a wide wavelength range using a simple and versatile fabrication approach. The measured second harmonic intensity is orders of magnitude higher than that from a deposited chalcogenide film, and more than three orders of magnitude higher than conventional plasmonic and Silicon-based structures. Fabricated via a simple and scalable technique, these all-dielectric architectures are ideal candidates for the design of flat non-linear optical components on flexible substrates.

physics.optics

Prediction of Self-Assembled Dewetted Nanostructures for Photonics Applications via a Continuum Mechanics Framework

When a liquid film lies on a non-wettable substrate, the configuration is unstable and the film then retracts from a solid substrate to form droplets. This phenomenon, known as dewetting, commonly leads to undesirable morphological changes. Nevertheless, recent works have demonstrated the possibility to harness dewetting by employing templated substrates with a degree of precision on par with advanced lithographic processes for high-performance nanophotonic applications. Since resonant behavior is highly sensitive to geometrical changes, predicting quantitatively dewetting dynamics is of high interest. In this work, we develop a continuum model that predicts the evolution of a thin film on a patterned substrate, from the initial reflow to the nucleation and growth of holes. We provide an operative framework based on macroscopic measurements to model the intermolecular interactions at the origin of the dewetting process, involving length scales that span from sub-nanometer to micron range. A comparison of experimental and simulated results shows that the model can accurately predict the final distributions, thereby offering novel predictive tools to tailor the optical response of dewetted nanostructures.

physics.flu-dyn

Novel design strategies for modulating conductive stretchable system response based on periodic assemblies

Soft electronics have recently gathered considerable interest thanks to their bio-mechanical compatibility. An important feature of such deformable conductors is their electrical response to strain. While development of stretchable materials with high gauge factors has attracted considerable attention, there is a growing need for stretchable conductors whose response to deformation can be accurately engineered to provide arbitrary resistance-strain relationships. The rare studies addressing this issue have focused on deterministic geometries of single rigid materials, limiting the scope of such strategies. Herein, we introduce the novel concept of periodic stretchable patterns combining multiple conductive materials to produce tailored responses. Using shortest-path algorithms, we establish a computationally efficient selection method to obtain required resistance-strain relationship. Using this algorithm, we identify and experimentally demonstrate constant resistance-strain responses up to 50% elongation using a single micro-textured material. Finally, we demonstrate counter-intuitive sinusoidal responses by integrating three materials, with interesting applications in sensing and soft robotics.

cond-mat.soft