arXiv subjects

Louk Rademaker

Publications and source records attributed to Louk Rademaker.

At least 55 records · Page 3Linked to original sources

arXiv2019

Charge Smoothening and Band Flattening due to Hartree corrections in Twisted Bilayer Graphene

Doping twisted bilayer graphene away from charge neutrality leads to an enormous buildup of charge inhomogeneities within each Moiré unit cell. Here we show, using unbiased real-space self-consistent Hartree calculations on a relaxed lattice, that Coulomb interactions smoothen this charge imbalance by changing the occupation of earlier identified `ring' orbitals in the AB/BA region and `center' orbitals at the AA region. For hole doping, this implies an increase of the energy of the states at the ${\bf Γ}$ point, leading to a further flattening of the flat bands and a pinning of the Van Hove singularity at the Fermi level. The charge smoothening will affect the subtle competition between different possible correlated phases.

cond-mat.str-el↗

arXiv2019

Construction of Many-Body Eigenstates with Displacement Transformations

Many-body eigenstates beyond the gaussian approximation can be constructed in terms of local integrals of motion (IOM), although their actual computation has been until now a daunting task. We present a new practical computation of IOMS based on displacement transformations. It represents a general and systematic way to extend Hartree-Fock and configuration interaction theories to higher order. Our method combines minimization of energy and energy variance of a reference state with exact diagonalization. We show that our implementation is able to perform ground state calculations with high precision for relatively large systems. Since it keeps track of the IMO's forming a reference state, our method is particularly efficient dealing with excited states, both in accuracy and the number of different states that can be constructed.

quant-ph↗

arXiv2018

Charge-transfer insulation in twisted bilayer graphene

We studied the real space structure of states in twisted bilayer graphene at the `magic angle' $θ= 1.08^\circ$. The flat bands close to charge neutrality are composed of a mix of `ring' and `center' orbitals around the AA stacking region. An effective model with localized orbitals is constructed, which necessarily includes more than just the four flat bands. Long-range Coulomb interaction causes a charge-transfer at half-filling of the flat bands from the `center' to the `ring' orbitals. Consequently, the Mott phase is a featureless spin-singlet paramagnet. We estimate the effective Heisenberg coupling that favors the singlet coupling to be $J = 3.3$ K, consistent with experimental values. The superconducting state depends on the nature of the dopants: hole-doping yields $p+ip$-wave whereas electron-doping yields $d+id$-wave pairing symmetry.

cond-mat.str-el↗

arXiv2018

Suppressed Density of States in Self-Generated Coulomb Glasses

We investigate the structure of metastable states in self-generated Coulomb glasses. In dramatic contrast to disordered electron glasses, we find that these states lack marginal stability. Such absence of marginal stability is reflected by the suppression of the single-particle density of states into an exponentially soft gap of the form $g(ε) \sim e^{-V / ξ|ε|}$. To analytically explain this behavior, we extend the stability criterion of Efros and Shklovskii to incorporate local charge correlations, in qualitative agreement with our numerical findings. Our work suggests the existence of a new class of self-generated glasses dominated by strong geometric frustration.

cond-mat.stat-mech↗

arXiv2017

Quantum Thermalization and the Expansion of Atomic Clouds

The ultimate consequence of quantum many-body physics is that even the air we breathe is governed by strictly unitary time evolution. The reason that we perceive it nonetheless as a completely classical high temperature gas is due to the incapacity of our measurement machines to keep track of the dense many-body entanglement of the gas molecules. The question thus arises whether there are instances where the quantum time evolution of a macroscopic system is qualitatively different from the equivalent classical system? Here we study this question through the expansion of noninteracting atomic clouds. While in many cases the full quantum dynamics is indeed indistinguishable from classical ballistic motion, we do find a notable exception. The subtle quantum correlations in a Bose gas approaching the condensation temperature appear to affect the expansion of the cloud, as if the system has turned into a diffusive collision-full classical system.

cond-mat.quant-gas↗

arXiv2017

Phonon linewidth due to electron-phonon interactions with strong forward scattering in FeSe thin films on oxide substrates

The discovery of an enhanced superconducting transition temperature $T_c$ in monolayers of FeSe grown on several oxide substrates has opened a new route to high-$T_c$ superconductivity through interface engineering. One proposal for the origin of the observed enhancement is an electron-phonon (e-ph) interaction across the interface that peaked at small momentum transfers. In this paper, we examine the implications of such a coupling on the phononic properties of the system. We show that a strong forward scattering leads to a sizable broadening of phonon lineshape, which may result in charge instabilities at long-wavelengths. However, we further find that the inclusion of Coulombic screening significantly reduces the phonon broadening. Our results show that one might not expect anomalously broad phonon linewidths in the FeSe interface systems, despite the fact that the e-ph interaction has a strong peak in the forward scattering (small $q$) direction.

cond-mat.supr-con↗

arXiv2016

Many-body localization and delocalization from the perspective of Integrals of Motion

We study many-body localization (MBL) and delocalization from the perspective of integrals of motion (IOMs). MBL can be understood phenomenologically through the existence of macroscopically many localized IOMs. However, IOMs exist for all many-body systems, and non-localized IOMs determine properties on the ergodic side of the MBL transition too. Here we explore their properties using our method of displacement transformations. We show how different quantities can be calculated using the IOMs as an expansion in the number of operators. For all values of disorder the typical IOMs are localized, suggesting the importance of rare fluctuations in understanding the delocalization transition.

cond-mat.str-el↗

arXiv2016

Universality and critical behavior of the dynamical Mott transition in a system with long-range interactions

We study numerically the voltage-induced breakdown of a Mott insulating phase in a system of charged classical particles with long-range interactions. At half-filling on a square lattice this system exhibits Mott localization in the form of a checkerboard pattern. We find universal scaling behavior of the current at the dynamic Mott insulator-metal transition and calculate scaling exponents corresponding to the transition. Our results are in agreement, up to a difference in universality class, with recent experimental evidence of dynamic Mott transition in a system of interacting superconducting vortices.

cond-mat.str-el↗

arXiv2016

Avoiding Stripe Order: Emergence of the Supercooled Electron Liquid

In the absence of disorder, electrons can display glassy behavior through supercooling the liquid state, avoiding the solidification into a charge ordered state. Such supercooled electron liquids are experimentally found in organic $θ$-$MM'$ compounds. We present theoretical results that qualitatively capture the experimental findings. At intermediate temperatures, the conducting state crosses over into a weakly insulating pseudogap phase. The stripe order phase transition is first order, so that the liquid phase is metastable below $T_s$. In the supercooled liquid phase the resistivity increases further and the density of states at the Fermi level is suppressed, indicating kinetic arrest and the formation of a glassy state. Our results are obtained using classical Extended Dynamical Mean Field Theory.

cond-mat.str-el↗

arXiv2015

Explicit Local Integrals of Motion for the Many-Body Localized State

Recently, it has been suggested that the Many-Body Localized phase can be characterized by local integrals of motion. Here we introduce a Hilbert space preserving renormalization scheme that iteratively finds such integrals of motion exactly. Our method is based on the consecutive action of a similarity transformation using displacement operators. We show, as a proof of principle, localization and the delocalization transition in interacting fermion chains with random onsite potentials. Our scheme of consecutive displacement transformations can be used to study Many Body Localization in any dimension, as well as disorder-free Hamiltonians.

cond-mat.str-el↗

arXiv2015

Enhanced superconductivity due to forward scattering in FeSe thin films on SrTiO3 substrates

We study the consequences of an electron-phonon ($e$-$ph$) interaction that is strongly peaked in the forward scattering ($\mathbf{q} = 0$) direction in a two-dimensional superconductor using Migdal-Eliashberg theory. We find that strong forward scattering results in an enhanced $T_c$ that is linearly proportional to the strength of the dimensionless $e$-$ph$ coupling constant $λ_m$ in the weak coupling limit. This interaction also produces distinct replica bands in the single-particle spectral function, similar to those observed in recent angle-resolved photoemission experiments on FeSe monolayers on SrTiO$_3$ and BaTiO$_3$ substrates. By comparing our model to photoemission experiments, we infer an $e$-$ph$ coupling strength that can provide a significant portion of the observed high $T_c$ in these systems.

cond-mat.supr-con↗

arXiv2015

The Tower of States and the Entanglement Spectrum in a Coplanar Antiferromagnet

We extend the analytical arguments of Metlitski and Grover (arXiv:1112.5166) to compute the entanglement spectrum and entanglement entropy of coplanar antiferromagnets with $SO(3)$ order parameter symmetry. The low-energy states in the entanglement spectrum exhibit the tower of states structure, as is expected for systems that undergo spontaneous symmetry breaking. Our results are consistent with numerical results on the triangular and Kagomé lattice.

cond-mat.str-el↗

arXiv2015

Impurity Bound States and Greens Function Zeroes as Local Signatures of Topology

We show that the local in-gap Greens function of a band insulator $\mathbf{G}_0 (ε,\mathbf{k}_{\parallel},\mathbf{r}_{\perp}=0)$, with $\mathbf{r}_\perp$ the position perpendicular to a codimension-1 or -2 impurity, reveals the topological nature of the phase. For a topological insulator, the eigenvalues of this Greens function attain zeros in the gap, whereas for a trivial insulator the eigenvalues remain nonzero. This topological classification is related to the existence of in-gap bound states along codimension-1 and -2 impurities. Whereas codimension-1 impurities can be viewed as 'soft edges', the result for codimension-2 impurities is nontrivial and allows for a direct experimental measurement of the topological nature of 2d insulators.

cond-mat.mes-hall↗

arXiv2015

Glassy dynamics in geometrically frustrated Coulomb liquids without disorder

We show that introducing long-range Coulomb interactions immediately lifts the massive ground state degeneracy induced by geometric frustration for electrons on quarter-filled triangular lattices in the classical limit. Important consequences include the stabilization of a stripe-ordered crystalline (global) ground state, but also the emergence of very many low-lying metastable states with amorphous "stripe-glass" spatial structures. Melting of the stripe order thus leads to a frustrated Coulomb liquid at intermediate temperatures, showing remarkably slow (viscous) dynamics, with very long relaxation times growing in Arrhenius fashion upon cooling, as typical of strong glass formers. On shorter time scales, the system falls out of equilibrium and displays the aging phenomena characteristic of supercooled liquids above the glass transition. Our results show remarkable similarity with the recent observations of charge-glass behavior in ultra-clean triangular organic materials of the $θ$-(BEDT-TTF)$_2$ family.

cond-mat.str-el↗

arXiv2014

How bilayer excitons can greatly enhance thermoelectric efficiency

Currently, one of the major nanotechnological challenges is to design thermoelectric devices that have a high figure of merit. To that end, we propose to use bilayer excitons. Bilayer exciton systems are shown to have an improved thermopower and an enhanced electric counterflow and thermal conductivity, with respect to regular semiconductor-based thermoelectrics. Here we present a roadmap towards experimental realization of a bilayer exciton thermocouple. A bilayer exciton heterostructures of $p$- and $n$-doped Bi$_2$Te$_3$ can have a figure of merit $zT \sim 60$. Another material suggestion is to make a bilayer out of electron-doped SrTiO$_3$ and hole-doped Ca$_3$Co$_4$O$_9$.

cond-mat.mtrl-sci↗

arXiv2013

Determinant quantum Monte Carlo study of exciton condensation in the bilayer Hubbard model

We studied the possibility of exciton condensation in a strongly correlated bilayer extended Hubbard model using Determinant Quantum Monte Carlo. To model both the onsite repulsion U and the interlayer interaction V we introduced a novel update scheme extending the standard Sherman-Morrison update. We observe that the sign problem increases dramatically with the inclusion of the interlayer interaction V, which prohibits at this stage a unequivocal conclusion regarding the presence of exciton condensation. However, enhancement of the interlayer tunneling results suggest that the strongest exciton condensation tendency lies around 10-20 % p/n-doping. Magnetic properties and conductivity turn out to be relatively independent of the interlayer interaction.

cond-mat.str-el↗

arXiv2013

Exciton condensation in strongly correlated electron bilayers

We studied the possibility of exciton condensation in Mott insulating bilayers. In these strongly correlated systems an exciton is the bound state of a double occupied and empty site. In the strong coupling limit the exciton acts as a hard-core boson. Its physics are captured by the exciton t-J model, containing an effective XXZ model describing the exciton dynamics only. Using numerical simulations and analytical mean field theory we constructed the ground state phase diagram. Three homogeneous phases can be distinguished: the antiferromagnet, the exciton checkerboard crystal and the exciton superfluid. For most model parameters, however, we predict macroscopic phase separation between these phases. The exciton superfluid exists only for large exciton hopping energy. Additionally we studied the collective modes and susceptibilities of the three phases. In the superfluid phase we find the striking feature that the bandwidth of the spin-triplet excitations, potentially detectable by resonant inelastic x-ray scattering (RIXS), is proportional to the superfluid density. The superfluid phase mode is visible in the charge susceptibility, measurable by RIXS or electron energy loss spectroscopy (EELS).

cond-mat.str-el↗

arXiv2013

Influence of long-range interactions on charge ordering phenomena on a square lattice

Usually complex charge ordering phenomena arise due to competing interactions. We have studied how such ordered patterns emerge from the frustration of a long-ranged interaction on a lattice. Using the lattice gas model on a square lattice with fixed particle density, we have identified several interesting phases; such as a generalization of Wigner crystals at low particle densities and stripe phases at densities in between rho = 1/3 and rho = 1/2. These stripes act as domain walls in the checkerboard phase present at half-filling. The phases are characterised at zero temperatures using numerical simulations, and mean field theory is used to construct a finite temperature phase diagram.

cond-mat.stat-mech↗