arXiv subjects

Lu Guo

Publications and source records attributed to Lu Guo.

At least 37 records · Page 2Linked to original sources

arXiv2022

Microscopic study on fusion reactions $^{40,48}\mathrm{Ca}+{}^{78}\mathrm{Ni}$ and the effect of tensor force

We provide a microscopic description of the fusion reactions between $^{40,48}$Ca and $^{78}$Ni. The internuclear potentials are obtained using the density-constrained (DC) time-dependent Hartree-Fock (TDHF) approach and fusion cross sections are calculated via the incoming wave boundary condition method. By performing DC-TDHF calculations at several selected incident energies, the internuclear potentials for both systems are obtained and the energy-dependence of fusion barrier are revealed. The influence of tensor force on internuclear potentials of $^{48}\mathrm{Ca}+{}^{78}\mathrm{Ni}$ is more obvious than those of $^{40}\mathrm{Ca}+{}^{78}\mathrm{Ni}$. By comparing the calculated fusion cross sections between $^{40}\mathrm{Ca}+{}^{78}\mathrm{Ni}$ and $^{48}\mathrm{Ca}+{}^{78}\mathrm{Ni}$, an interesting enhancement of sub-barrier fusion cross sections for the former system is found, which can be explained by the narrow width of internuclear potential for $^{40}\mathrm{Ca}+{}^{78}\mathrm{Ni}$ while the barrier heights and positions are very close to each other. The tensor force suppresses the sub-barrier fusion cross sections of both two systems.

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arXiv2022

Effects of the tensor force on low-energy heavy-ion fusion reactions: A mini review

In recent several years, the tensor force, one of the most important components of the nucleon-nucleon force, has been implemented in time-dependent density functional theories and it has been found to influence many aspects of low-energy heavy-ion reactions, such as dissipation dynamics, sub-barrier fusions, low-lying vibration states of colliding partners. Especially, the effects of tensor force on fusion reactions have been investigated from the internuclear potential to fusion cross sections systematically. In this work we present a mini review on the recent progresses on this topic. Considering the recent progress of low-energy reaction theories, we will also mention more possible effects of the tensor force on reaction dynamics.

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arXiv2022

Microscopic study of the compound nucleus formation in cold-fusion reactions

The understanding of the fusion probability is of particular importance to reveal the mechanism of producing superheavy elements. We present a microscopic study of the compound nucleus formation by combining time-dependent density functional theory, coupled-channels approach, and dynamical diffusion models. The fusion probability and compound nucleus formation cross sections for cold-fusion reactions $^{48}$Ca+$^{208}$Pb, $^{50}$Ti+$^{208}$Pb, and $^{54}$Cr+$^{208}$Pb are investigated and it is found that the deduced capture barriers, capture cross sections for these reactions are consistent with experimental data. Above the capture barrier, our calculations reproduce the measured fusion probability reasonably well. Our studies demonstrate that the restrictions from the microscopic dynamic theory improve the predictive power of the coupled-channels and diffusion calculations.

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arXiv2020

Route to in situ synthesis of epitaxial Pr2Ir2O7 thin films guided by thermodynamic calculations

In situ growth of pyrochlore iridate thin films has been a long-standing challenge due to the low reactivity of Ir at low temperatures and the vaporization of volatile gas species such as IrO3(g) and IrO2(g) at high temperatures and high oxygen partial pressures. To address this challenge, we combine thermodynamic analysis of the Pr-Ir-O2 system with experimental results from the conventional physical vapor deposition (PVD) technique of co-sputtering. Our results indicate that only high growth temperatures yield films with crystallinity sufficient for utilizing and tailoring the desired topological electronic properties. Thermodynamic calculations indicate that high deposition temperatures and high partial pressures of gas species O2(g) and IrO3(g), are required to stabilize Pr2Ir2O7. We further find that the gas species partial pressure requirements are beyond that achievable by any conventional PVD technique. We experimentally show that conventional PVD growth parameters produce exclusively Pr3IrO7, which conclusion we reproduce with theoretical calculations. Our findings provide solid evidence that in situ synthesis of Pr2Ir2O7 thin films is fettered by the inability to grow with oxygen partial pressure on the order of 10 Torr, a limitation inherent to the PVD process. Thus, we suggest high-pressure techniques, in particular chemical vapor deposition (CVD), as a route to synthesis of Pr2Ir2O7, as this can support thin film deposition under the high pressure needed for in situ stabilization of Pr2Ir2O7.

cond-mat.mtrl-sci↗

arXiv2019

Spontaneous Hall Effect enhanced by local Ir moments in epitaxial Pr$_2$Ir$_2$O$_7$ thin films

Rare earth pyrochlore Iridates (RE2Ir2O7) consist of two interpenetrating cation sublattices, the RE with highly-frustrated magnetic moments, and the Iridium with extended conduction orbitals significantly mixed by spin-orbit interactions. The coexistence and coupling of these two sublattices create a landscape for discovery and manipulation of quantum phenomena such as the topological Hall effect, massless conduction bands, and quantum criticality. Thin films allow extended control of the material system via symmetry-lowering effects such as strain. While bulk Pr2Ir2O7 shows a spontaneous hysteretic Hall effect below 1.5K, we observe the effect at elevated temperatures up to 15K in epitaxial thin films on (111) YSZ substrates synthesized via solid phase epitaxy. Similar to the bulk, the lack of observable long-range magnetic order in the thin films points to a topological origin. We use synchrotron-based element-specific x-ray diffraction (XRD) and x-ray magnetic circular dichroism (XMCD) to compare powders and thin films to attribute the spontaneous Hall effect in the films to localization of the Ir moments. We link the thin film Ir local moments to lattice distortions absent in the bulk-like powders. We conclude that the elevated-temperature spontaneous Hall effect is caused by the topological effect originating either from the Ir or Pr sublattice, with interaction strength enhanced by the Ir local moments. This spontaneous Hall effect with weak net moment highlights the effect of vanishingly small lattice distortions as a means to discover topological phenomena in metallic frustrated magnetic materials.

cond-mat.mtrl-sci↗

arXiv2019

Influence of the tensor interaction on heavy-ion fusion cross sections

[Background] While the tensor interaction has been shown to significantly affect the nuclear structure of exotic nuclei, its influence on nuclear reactions has only recently been investigated. The primary reason for this neglect is the fact that most studies of nuclear dynamics do not include the tensor force at all in their models. Indeed, only a few Skyrme parametrizations consider the tensor interaction in parameter determination. With modern research facilities extending our ability to probe exotic nuclei, a correct description of nuclear dynamics and heavy-ion fusion is vital to both supporting and leading experimental efforts. [Method] Fusion cross sections are calculated using ion-ion potentials generated by the fully microscopic density-constrained time-dependent Hartree-Fock (DC-TDHF) method with the complete Skyrme tensor interaction. [Results] For light nuclei, the tensor force only slightly changes the sub-barrier fusion cross sections at very low energies. Heavier nuclei, however, begin to exhibit a substantial hindrance effect in the sub-barrier region. This effect is strongest in spin-unsaturated systems, though can manifest in other configurations as well. Static, ground state deformation effects of the tensor force can also affect cross sections by shifting the fusion barrier. [Conclusions] The tensor interaction has a measurable effect on the fusion cross sections of nuclei spanning the nuclear chart. The effect comes from both static effects present in the ground state and dynamic processes arising from the time evolution of the system. This motivates the development of a modern Skyrme parameter set that includes all time-odd and tensor terms and that studies moving forward should include the tensor force to ensure a more robust and complete description of nuclei.

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arXiv2019

Microscopic studies of production cross sections in multinucleon transfer reaction $^{58}$Ni+$^{124}$Sn

\item[Background] Multinucleon transfer reaction at low-energy collisions is considered to be a promising method for the production of new exotic nuclei, which are difficult to be produced by other methods. The theoretical studies are required to provide reliable predictions for the experiments and promote the understanding of the microscopic mechanism in multinucleon transfer reactions. \item[Purpose] We provide a predictive approach for production cross sections, and testify how and to what extent the microscopic approach works well in multinucleon transfer reaction. \item[Methods] We employ the approach TDHF+GEMINI, which combines the microscopic time-dependent Hartree-Fock (TDHF) with the state-of-art statistical model GEMINI++, to take into account both the multinucleon transfer dynamics and the secondary deexcitation process. The properties of primary products in multinucleon transfer process, such as transfer probabilities and primary cross sections, are extracted from TDHF dynamics by using the particle-number projection method. Production cross sections for secondary products are evaluated by using the statistical model GEMINI++. \item[Results] We investigate the influence of colliding energies and deformation orientations of target and projectile nuclei on multinucleon transfer dynamics in the reaction $^{58}$Ni+$^{124}$Sn...... \item[Conclusions] The microscopic approach TDHF+GEMINI reasonably reproduces the experimental data at energies close to the Coulomb barrier and well accounts for the multinucleon transfer mechanism. The present studies clearly reveal the applicability of TDHF+GEMINI method in multinucleon transfer reactions, which thus deserves as a promising tool to predict the properties of new reactions.

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arXiv2018

The influence of tensor force on the microscopic heavy-ion interaction potential

Background: The tensor interaction is known to play an important role in the nuclear structure studies of exotic nuclei. However, most microscopic studies of low-energy nuclear reactions neglect the tensor force, resulting in a lack of knowledge concerning the effect of the tensor force on HIC...... Purpose: The theoretical study of the influence of the tensor force on heavy-ion interaction potentials is required to further our understanding of the microscopic mechanisms entailed in fusion dynamics. Method: The full Skyrme tensor force is implemented into the static Hartree-Fock and dynamic density-constrained time-dependent Hartree-Fock (DC-TDHF) theory to calculate both static (frozen density) and dynamic microscopic interaction potentials for reactions involving exotic and stable nuclei. Results: The static potentials are found to be systematically higher than the dynamical results, which are attributed to the microscopic dynamical effects included in TDHF. We also show that the dynamical potential barriers vary more significantly by the inclusion of tensor force than the static barriers. The influence of isoscalar and isovector tensor terms is also investigated with the TIJ set of forces. For light systems, the tensor force is found to have an imperceptible effect on the nucleus-nucleus potential. However, for medium and heavy spin-unsaturated reactions, the potentials may change from a fraction of an MeV to almost 2 MeV by the inclusion of tensor force, indicating a strong impact of the tensor force on sub-barrier fusion. Conclusions: The tensor force could indeed play a large role in the fusion of nuclei, with spin-unsaturated systems seeing a systematic increase in ion-ion barrier height and width. This fusion hindrance is partly due to static, ground state effects from the inclusion of the tensor force, though additional hindrance appears when studying nuclear dynamics.

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arXiv2018

Isotopic trends of quasifission and fusion-fission in the reactions $^{48}$Ca+$^{239,244}$Pu

Background: Quasifission and fusion-fission are primary mechanisms to prevent the production of superheavy elements. The recent experimental measurements reveal that the fusion-evaporation cross section in the $3n$ reaction channel of $^{48}$Ca+$^{239}$Pu is 50 times lower than using $^{244}$Pu as target nucleus. However, the precise mechanisms of this remarkable isotopic dependence are not well understood. Purpose: To understand the experimental observation of the rapid decrease of stability of superheavy nuclei as the neutron number decreases, the theoretical studies of quasifission and fusion-fission in connection with experimental production for $Z$=114 flerovium isotopes are required to investigate the possible differences in reaction mechanisms induced by these two targets. Methods: We propose an approach called TDHF+HIVAP to take into account both the evolution of dinuclear system and the deexcitation of compound nucleus, which combines the microscopic time-dependent Hartree-Fock (TDHF) method for the fusion and quasifission dynamics with the statistical evaporation model HIVAP for fusion-fission dynamics. Results: ......The quantum shell effect displays a crucial role in both the quasifission and the fusion-fission processes. The quasifission is considerably reduced and the survival probability is enhanced around one order of magnitude in the reaction using $^{244}$Pu target as compared to the $^{239}$Pu case. Conclusions: The studies by using TDHF+HIVAP method well account for the experimental observations and the present method clearly shows its applicability in the reaction mechanisms of quasifission and fusion-fission dynamics. The experimental and theoretical results encourage the use of neutron-rich targets for the production of new superheavy elements.

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arXiv2018

The Role of Tensor Force in Heavy-Ion Fusion Dynamics

The tensor force is implemented into the time-dependent Hartree-Fock (TDHF) theory so that both exotic and stable collision partners, as well as their dynamics in heavy-ion fusion, can be described microscopically. The role of tensor force on fusion dynamics is systematically investigated for $^{40}\mathrm{Ca}+\mathrm{^{40}Ca}$, $^{40}\mathrm{Ca}+\mathrm{^{48}Ca}$, $^{48}\mathrm{Ca}+\mathrm{^{48}Ca}$, $^{48}\mathrm{Ca}+\mathrm{^{56}Ni}$, and $^{56}\mathrm{Ni}+\mathrm{^{56}Ni}$ reactions which vary by the total number of spin-unsaturated magic numbers in target and projectile. A notable effect on fusion barriers and cross sections is observed by the inclusion of tensor force. The origin of this effect is analyzed. The influence of isoscalar and isovector tensor terms is investigated with the T$IJ$ forces. These effects of tensor force in fusion dynamics are essentially attributed to the shift of low-lying vibration states of colliding partners and nucleon transfer in the asymmetric reactions. Our calculations of above-barrier fusion cross sections also show that tensor force does not significantly affect the dynamical dissipation at near-barrier energies.

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arXiv2016

New neutron-rich isotope production in $^{154}$Sm+$^{160}$Gd

Deep inelastic scattering in $^{154}$Sm+$^{160}$Gd at energies above the Bass barrier is for the first time investigated with two different microscopic dynamics approaches: improved quantum molecular dynamics (ImQMD) model and time dependent Hartree-Fock (TDHF) theory. No fusion is observed from both models. The capture pocket disappears for this reaction due to strong Coulomb repulsion and the contact time of the di-nuclear system formed in head-on collisions is about 700 fm/c at an incident energy of 440 MeV. The isotope distribution of fragments in the deep inelastic scattering process is predicted with the simulations of the latest ImQMD-v2.2 model together with a statistical code (GEMINI) for describing the secondary decay of fragments. More than 40 extremely neutron-rich unmeasured nuclei with $58 \le Z\le 76$ are observed and the production cross sections are at the order of ${\rm μb}$ to mb. The multi-nucleon transfer reaction of Sm+Gd could be an alternative way to synthesize new neutron-rich lanthanides which are difficult to be produced with traditional fusion reactions or fission of actinides.

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arXiv2014

Effect of tensor force on dissipation dynamics in time-dependent Hartree-Fock theory

The role of tensor force on the collision dynamics of $^{16}$O+$^{16}$O is investigated in the framework of a fully three-dimensional time-dependent Hartree-Fock theory. The calculations are performed with modern Skyrme energy functional plus tensor terms. Particular attention is given on the analysis of dissipation dynamics in heavy-ion collisions. The energy dissipation is found to decrease as an initial bombarding energy increases in deep-inelastic collisions for all the Skyrme parameter sets studied here because of the competition between the collective motion and the single-particle degrees of freedom. We reveal that the tensor forces may either enhance or reduce the energy dissipation depending on the different parameter sets. The fusion cross section without tensor force overestimates the experimental value by about 25\%, while the calculation with tensor force T11 has good agreement with experimental cross section.

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arXiv2014

Dissipation dynamics and spin-orbit force in time-dependent Hartree-Fock theory

We investigate the one-body dissipation dynamics in heavy-ion collisions of $^{16}{\rm O}$+$^{16}{\rm O}$ using a fully three-dimensional time-dependent Hartree-Fock (TDHF) theory with the modern Skyrme energy functional and without any symmetry restrictions. The energy dissipation is revealed to decrease in deep-inelastic collisions of the light systems as the bombarding energy increases owing to the competition between collective motion and single-particle degrees of freedom. The role of spin-orbit force is given particular emphasis in deep-inelastic collisions. The spin-orbit force causes a significant enhancement of the dissipation. The time-even coupling of spin-orbit force plays a dominant role at low energies, while the influence of time-odd terms is notable at high energies. About 40-65\% of the total dissipation depending on the different parameter sets is predicted to arise from the spin-orbit force. The theoretical fusion cross section has a reasonably good agreement with the experimental data, considering that no free parameters are adjusted to reaction dynamics in the TDHF approach.

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arXiv2013

Structural and Electronic Recovery Pathways of a Photoexcited Ultrathin VO2 Film

The structural and electronic recovery pathways of a photoexcited ultrathin VO2 film at nanosecond time scales have been studied using time-resolved x-ray diffraction and transient optical absorption techniques. The recovery pathways from the tetragonal metallic phase to the monoclinic insulating phase are highly dependent on the optical pump fluence. At pump fluences higher than the saturation fluence of 14.7 mJ/cm2, we observed a transient structural state with lattice parameter larger than that of the tetragonal phase, which is decoupled from the metal-to-insulator phase transition. Subsequently, the photoexcited VO2 film recovered to the ground state at characteristic times dependent upon the pump fluence, as a result of heat transport from the film to the substrate. We present a procedure to measure the time-resolved film temperature by correlating photoexcited and temperature-dependent x-ray diffraction measurements. A thermal transport model that incorporates changes of the thermal parameters across the phase transition reproduces the observed recovery dynamics. The optical excitation and fast recovery of ultrathin VO2 films provides a practical method to reversibly switch between the monoclinic insulating and tetragonal metallic state at nanosecond time scales.

cond-mat.str-el↗

arXiv2011

Microscopic Formulation of Interacting Boson Model for Rotational Nuclei

We propose a novel formulation of the Interacting Boson Model (IBM) for rotational nuclei with axially-symmetric strong deformation. The intrinsic structure represented by the potential energy surface (PES) of a given multi-nucleon system has a certain similarity to that of the corresponding multi-boson system. Based on this feature, one can derive an appropriate boson Hamiltonian as already reported. This prescription, however, has a major difficulty in rotational spectra of strongly deformed nuclei: the bosonic moment of inertia is significantly smaller than the corresponding nucleonic one. We present that this difficulty originates in the difference between the rotational response of a nucleon system and that of the corresponding boson system, and could arise even if the PESs of the two systems were identical. We further suggest that the problem can be cured by implementing $\hat{L} \cdot \hat{L}$ term into the IBM Hamiltonian, with coupling constant derived from the cranking approach of Skyrme mean-field models. The validity of the method is confirmed for rare-earth and actinoid nuclei, as their experimental rotational yrast bands are reproduced nicely.

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arXiv2008

Conservation Properties in the Time-Dependent Hartree Fock Theory

We discuss the conservation of angular momentum in nuclear time-dependent Hartree-Fock calculations for a numerical representation of wave functions and potentials on a three-dimensional cartesian grid. Free rotation of a deformed nucleus performs extremely well even for relatively coarse spatial grids. Heavy ion collisions produce a highly excited compound system associated with substantial nucleon emission. These emitted nucleons reach the bounds of the numerical box which leads to a decrease of angular momentum. We discuss strategies to distinguish the physically justified loss from numerical artifacts.

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arXiv2008

Triaxial nuclear models and the outer crust of nonaccreting cold neutron stars

The properties and composition of the outer crust of nonaccreting cold neutron stars are studied by applying the model of Baym, Pethick, and Sutherland (BPS) and taking into account for the first time triaxial deformations of nuclei. Two theoretical nuclear models, Hartree-Fock plus pairing in the BCS approximation (HF-BCS) with Skyrme SLy6 parametrization and Hartree-Fock-Bogolyubov (HFB) with Gogny D1S force, are used to calculate the nuclear masses. The two theoretical calculations are compared concerning their neutron drip line, binding energies, magic neutron numbers, and the sequence of nuclei in the outer crust of nonaccreting cold neutron stars, with special emphasis on the effect of triaxial deformations. The BPS model is extended by the higher-order corrections for the atomic binding, screening, exchange and zero-point energies. The influence of the higher-order corrections on the sequence of the outer crust is investigated.

astro-ph↗

arXiv2007

Triaxiality and shape coexistence in Germanium isotopes

The ground-state deformations of the Ge isotopes are investigated in the framework of Gogny-Hartree-Fock-Bogoliubov (HFB) and Skyrme Hartree-Fock plus pairing in the BCS approximation. Five different Skyrme parametrizations are used to explore the influence of different effective masses and spin-orbit models. There is generally good agreement for binding energies and deformations (total quadrupole moment, triaxiality) with experimental data where available (i.e., in the valley of stability). All calculations agree in predicting a strong tendency for triaxial shapes in the Ge isotopes with only a few exceptions due to neutron (sub-)shell closures. The frequent occurrence of energetically very close shape isomers indicates that the underlying deformation energy landscape is very soft. The general triaxial softness of the Ge isotopes is demonstrated in the fully triaxial potential energy surface. The differences between the forces play an increasing role with increasing neutron number. This concerns particularly the influence of the spin-orbit model, which has a visible effect on the trend of binding energies towards the drip line. Different effective mass plays an important role in predicting the quadrupole and triaxial deformations. The pairing strength only weakly affects binding energies and total quadrupole deformations, but considerably influences triaxiality.

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