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Luca Razzari

Publications and source records attributed to Luca Razzari.

17 recordsLinked to original sources
arXiv2025

Polarization control via artificial optical nonlinearity in dielectric metasurfaces

Nonlinear optical phenomena are generally governed by geometry in matter systems, as they depend on the spatial arrangement of atoms within materials or molecules. Metasurfaces, through precisely designed geometries on a subwavelength scale, allow tailoring the optical response of a material far beyond its natural properties. Therefore, metasurfaces are highly appealing to enable the engineering of nonlinear optical interactions at an unprecedented level. Current studies on nonlinear metasurfaces predominantly focus on the phase control of the generated light. Nonetheless, investigating the tensorial nature of the nonlinearity of metasurfaces and its effect on the polarization of the generated light is critical to fully unlock a range of applications, such as nonlinear vector beam generation and nonlinear polarization imaging. Here, we study the artificial optical nonlinearity of a dielectric metasurface originating from its meta-atom symmetry and describe the third-order nonlinear behavior by considering the polarization degree of freedom. We establish an effective nonlinear medium model that serves as a design toolbox for developing amorphous silicon-based geometric metasurfaces with customizable features in third harmonic generation. We further extract quantitative values of the artificial nonlinear susceptibility tensor elements related to the investigated nonlinear process and geometry. The implemented functional devices demonstrate the versatility of dielectric metasurfaces in shaping the emitted light in terms of amplitude, phase, and polarization, for the precise engineering of novel nonlinear architectures targeting applications in nonlinear imaging and complex light generation.

physics.app-ph↗
arXiv2024

Enhanced Terahertz Spectroscopy of a Monolayer Transition Metal Dichalcogenide

Two-dimensional materials, including transition metal dichalcogenides, are attractive for a variety of applications in electronics as well as photonics and have recently been envisioned as an appealing platform for phonon polaritonics. However, their direct characterization in the terahertz spectral region, of interest for retrieving, e.g., their phonon response, represents a major challenge, due to the limited sensitivity of typical terahertz spectroscopic tools and the weak interaction of such long-wavelength radiation with sub-nanometer systems. In this work, by exploiting an ad-hoc engineered metallic surface enabling a ten-thousand-fold local absorption boost, we perform enhanced terahertz spectroscopy of a monolayer transition metal dichalcogenide (tungsten diselenide) and extract its dipole-active phonon resonance features. In addition, we use these data to obtain the monolayer effective permittivity around its phonon resonance. Via the direct terahertz characterization of the phonon response of such two-dimensional systems, this method opens the path to the rational design of phonon polariton devices exploiting monolayer transition metal dichalcogenides.

physics.optics↗
arXiv2022

Terahertz scanless hypertemporal imaging

Since its first demonstration in 1995, terahertz time-domain imaging has attracted an increasingly growing interest for its ability to reveal spectral fingerprints of materials, probe changes in refractive index and absorption, as well as detect the inner structure of complex objects via time-of-flight measurements. Practically, however, its widespread use has been hampered by the very long acquisition time typically required to spatially raster-scan the object and, for each spatial point, record the field in time via a delay line. Here, we address this fundamental bottleneck by implementing a scanless single-pixel imaging scheme, which sets the path for an unprecedented reduction of both system complexity and acquisition time. By properly exploiting natural wave diffraction, time-to-space encoding applied to terahertz point detection allows for an almost instantaneous capture of the terahertz waveforms, while multidimensional images are reconstructed via a computational approach. Our scheme is a promising solution for the development of next-generation fast and compact terahertz imagers perfectly suitable for high-repetition-rate laser sources.

physics.optics↗
arXiv2021

Analysis of external and internal disorder to understand band-like transport in n-type organic semiconductors

Charge transport in organic semiconductors is notoriously extremely sensitive to the presence of disorder, both internal and external (i.e. related to the interactions with the dielectric layer), especially for n-type materials. Internal dynamic disorder stems from large thermal fluctuations both in intermolecular transfer integrals and (molecular) site energies in weakly interacting van der Waals solids and sources transient localization of the charge carriers. The molecular vibrations that drive transient localization typically operate at low-frequency (< a-few-hundred cm-1), which renders it difficult to assess them experimentally. Hitherto, this has prevented the identification of clear molecular design rules to control and reduce dynamic disorder. In addition, the disorder can also be external, being controlled by the gate insulator dielectric properties. Here we report on a comprehensive study of charge transport in two closely related n-type molecular organic semiconductors using a combination of temperature-dependent inelastic neutron scattering and photoelectron spectroscopy corroborated by electrical measurements, theory and simulations. We provide unambiguous evidence that ad hoc molecular design enables to free the electron charge carriers from both internal and external disorder to ultimately reach band-like electron transport.

cond-mat.mtrl-sci↗
arXiv2020

3D-Printed Photocathodes for Resonant, Terahertz-Field-Driven Ultrafast Electron Emission

Ultrashort photoemitted electron bunches can provide high electron currents within sub-picosecond timeframes, enabling time-resolved investigations of ultrafast physical processes with nanoscale resolution. Non-resonant conductive nanotips are typically employed to realize nanoscale photoelectron sources with high brightness. However, such emitters require complex non-scalable fabrication procedures featuring poor reproducibility. Planar resonant antennas fabricated via photolithography have been recently investigated, also because of their superior field enhancement properties. Nevertheless, the electron emission from these structures is parallel to the substrate plane, which limits their practical use as electron sources. In this work, we present an innovative out-of-plane, resonant nanoantenna design for field-driven photoemission enabled by high-resolution 3D printing. Numerical and experimental evidences demonstrate that gold-coated, terahertz resonant nanocones provide large local electric fields at their apex, automatically ensuring out-of-plane coherent electron emission and acceleration. We show that the resonant structures can be conveniently arranged in an array form, for a further significant electron extraction enhancement via a collective terahertz response. Remarkably, such collective behaviour can also be harvested to boost photoemission from an individual nano-source. Our approach opens the path for a new generation of photocathodes that can be reproducibly fabricated and designed at will, significantly relaxing the requirement for intense terahertz drivers.

physics.optics↗
arXiv2020

Nonlinear Mid-infrared Metasurface based on a Phase-Change Material

The mid-wave infrared (MWIR) spectral region (3-5 μm) is important to a vast variety of applications in imaging, sensing, spectroscopy, surgery, and optical communications. Efficient third-harmonic generation (THG), converting light from the MWIR range into the near-infrared, a region with mature optical detection and manipulation technologies, offers the opportunity to mitigate a commonly recognized limitation of current MWIR systems. In this work, we present the possibility of boosting THG in the MWIR through a metasurface design. Specifically, we demonstrate a 30-fold enhancement in a highly nonlinear phase change material Ge2Sb2Se4Te1 (GSST), by patterning arrays of subwavelength cylinders supporting a magnetic dipolar resonance. The unprecedented broadband transparency, large refractive index, and remarkably high nonlinear response, together with unique phase-change properties, make GSST-based metasurfaces an appealing solution for reconfigurable and ultra-compact nonlinear devices operating in the MWIR.

physics.optics↗
arXiv2019

Time-domain terahertz compressive imaging

We present an implementation of the single-pixel imaging approach into a terahertz (THz) time-domain spectroscopy (TDS) system. We demonstrate the indirect coherent reconstruction of THz temporal waveforms at each spatial position of an object, without the need of mechanical raster-scanning. First, we exploit such temporal information to realize (far-field) time-of-flight images. In addition, as a proof of concept, we apply a typical compressive sensing algorithm to demonstrate image reconstruction with less than 50% of the total required measurements. Finally, the access to frequency domain is also demonstrated by reconstructing spectral images of an object featuring an absorption line in the THz range. The combination of single-pixel imaging with compressive sensing algorithms allows to reduce both complexity and acquisition time of current THz-TDS imaging systems.

eess.IV↗
arXiv2019

Freeing electrons from extrinsic and intrinsic disorder yields band-like transport in n-type organic semiconductors

Charge transport in organic semiconductors is notoriously extremely sensitive to the presence of disorder, both intrinsic and extrinsic, especially for n-type materials. Intrinsic dynamic disorder stems from large thermal fluctuations both in intermolecular transfer integrals and (molecular) site energies in weakly interacting van der Waals solids and sources transient localization of the charge carriers. The molecular vibrations that drive transient localization typically operate at low-frequency (< a-few-hundred cm-1), which renders it difficult to assess them experimentally. Hitherto, this has prevented the identification of clear molecular design rules to control and reduce dynamic disorder. In addition, the disorder can also be extrinsic, being controlled by the gate insulator dielectric properties. Here we report on a comprehensive study of charge transport in two closely related n-type molecular organic semiconductors using a combination of temperature-dependent inelastic neutron scattering and photoelectron spectroscopy corroborated by electrical measurements, theory and simulations. We provide unambiguous evidence that ad hoc molecular design enables to free the electron charge carriers from both intrinsic and extrinsic disorder to ultimately reach band-like electron transport.

cond-mat.mtrl-sci↗
arXiv2017

Towards On-Chip Integrated Optical Quantum Frequency Combs

Recent development in quantum photonics allowed to start the process of bringing photonic-quantum-based systems out of the lab into real world applications. As an example, devices for the exchange of a cryptographic key secured by the law of quantum mechanics are currently commercially available. In order to further boost this process, the next step is to migrate the results achieved by means of bulky and expensive setups to miniaturized and affordable devices. Integrated quantum photonics is exactly addressing this issue. In this paper we briefly review the most recent advancements in the generation of quantum states of light (at the core of quantum cryptography and computing) on chip. In particular, we focus on optical microcavities, as they can offer a solution to the issue of low efficiency (low number of photons generated) typical of the materials mostly used in integrated platforms. In addition, we show that specifically designed microcavities can also offer further advantages, such as compatibility with existing telecom standard (thus allowing to exploit the existing fiber network) and quantum memories (necessary in turns to extend the communication distance), as well as longitudinal multimode character. This last property (i.e. the increased dimensionality necessary for describing the quantum state of a photon) is achieved thanks to the generating multiple photon pairs on a frequency comb corresponding to the microcavity resonances. Further achievements include the possibility to fully exploit the polarization degree of freedom also for integrated devices. These results pave the way to the generation of integrated quantum frequency combs, that in turn may find application as quantum computing platform.

physics.optics↗
arXiv2017

First and second order all-optical integrating functions in a photonic integrated circuit

We demonstrate all-optical temporal integration of arbitrary optical waveforms with temporal features as short as ~1.9ps. By using a four-port micro-ring resonator based on CMOS compatible doped glass technology we perform the 1st- and 2nd-order cumulative time integral of optical signals over a bandwidth that exceeds 400GHz. This device has applications for a wide range of ultra-fast data processing and pulse shaping functions as well as in the field of optical computing for the real-time analysis of differential equations.

physics.optics↗
arXiv2014

Novel architecture for ultra-stable micro-ring resonator based optical frequency combs

We report a novel geometry for OPOs based on nonlinear microcavity resonators. This approach relies on a self-locked scheme that enables OPO emission without the need for thermal locking of the pump laser to the microcavity resonance. By exploiting a CMOS-compatible microring resonator, we achieve oscillation with a complete absence of shutting down, or self-terminating behavior, a very common occurrence in externally pumped OPOs. Further, this scheme consistently produces very wide bandwidth (>300nm, limited by our experimental set-up) combs that oscillate at a spacing of the FSR of the micro cavity resonance.

physics.optics↗
arXiv2014

Photonic Integrated Devices for Nonlinear Optics

We review our recent progresses on frequency conversion in integrated devices, focusing primarily on experiments based on strip-loaded and quantum-well intermixed AlGaAs waveguides, and on CMOS-compatible high-index doped silica glass waveguides. The former includes both second- and third-order interactions, demonstrating wavelength conversion by tunable difference-frequency generation over a bandwidth of more than nm, as well as broadband self-phase modulation and tunable four-wave mixing. The latter includes four-wave mixing using low-power continuous-wave light in microring resonators as well as hyper-parametric oscillation in a high quality factor resonator, towards the realization of an integrated multiple wavelength source with important applications for telecommunications, spectroscopy, and metrology.

physics.optics↗
arXiv2014

Hydex waveguides for nonlinear optics

We demonstrate a wide range of novel functions in integrated, CMOS compatible, devices. This platform has promise for telecommunications and on-chip WDM optical interconnects for computing.

physics.optics↗
arXiv2014

CMOS-compatible, multiplexed source of heralded photon pairs: towards integrated quantum combs

We report an integrated photon pair source based on a CMOS-compatible microring resonator that generates multiple, simultaneous, and independent photon pairs at different wavelengths in a frequency comb compatible with fiber communication wavelength division multiplexing channels (200 GHz channel separation) and with a linewidth that is compatible with quantum memories (110 MHz). It operates in a self-locked pump configuration, avoiding the need for active stabilization, making it extremely robust even at very low power levels.

quant-ph↗
arXiv2013

Nonlinear imaging and 3D-mapping of terahertz fields with Kerr media

We investigate the spatially and temporally resolved four-wave mixing of terahertz fields and optical pulses in large band-gap dielectrics, such as diamond. We show that it is possible to perform beam profiling and space-time resolved mapping of terahertz fields with sub-wavelength THz resolution by encoding the spatial information into an optical signal, which can then be recorded by a standard CCD camera.

physics.optics↗
arXiv2008

Polarization proximity effect in isolator crystal pairs

We experimentally studied the polarization dynamics (orientation and ellipticity) of near infrared light transmitted through magnetooptic Yttrium Iron Garnet crystal pairs using a modified balanced detection scheme. When the pair separation is in the sub-millimeter range, we observed a proximity effect in which the saturation field is reduced by up to 20%. 1D magnetostatic calculations suggest that the proximity effect originates from magnetostatic interactions between the dipole moments of the isolator crystals. This substantial reduction of the saturation field is potentially useful for the realization of low-power integrated magneto-optical devices.

cond-mat.mtrl-sci↗