arXiv subjects

Luca Vannucci

Publications and source records attributed to Luca Vannucci.

At least 19 recordsLinked to original sources

arXiv2025

Theory of single-photon emission from neutral and charged excitons in a polarization-selective cavity

Single-photon sources based on neutral or charged excitons in a semiconductor quantum dot are attractive resources for photonic quantum computers and simulators. To obtain indistinguishable photons, the source is pumped on resonance with polarized laser pulses, and the output is collected in orthogonal polarization. However, for sources featuring vertical emission of light, 50% of the emitted photons are unavoidably lost in this way. Here, we theoretically study the quantum dynamics of an exciton embedded in an asymmetric vertical cavity that favors emission in a specific polarization. We identify the configuration for optimal state initialization and demonstrate a path toward near-unity polarized efficiency. We also derive simple analytical formulas for the photon output in each polarization as a function of the Purcell-enhanced emission rates, which shed light on the physical mechanism behind our results.

cond-mat.mes-hall↗

arXiv2025

Exciton and biexciton preparation via coherent swing-up excitation in a GaAs quantum dot embedded in micropillar cavity

Coherent control of quantum emitters is essential for scalable quantum photonic technologies. The recently proposed swing-up of quantum emitter (SUPER) scheme allows efficient and coherent preparation of single photons via off-resonant, red-detuned laser pulses, simplifying laser suppression and enhancing photon collection. We present a systematic study of SUPER excitation applied to a single GaAs quantum dot in a low-Q micropillar cavity. We perform a comparison of the key figures of merit against the well-established two-photon excitation (TPE). Despite requiring higher excitation powers, SUPER achieves near-unity population inversion of the exciton state ($\sim$95%) and high single-photon purity ($g^{(2)}=0.03$) comparable to that under TPE, while also exhibiting a shortened decay time ($\sim$200 ps) reducing the time jitter in the exciton population. A polarization-resolved analysis reveals that when both excitation and collection are aligned with one of the exciton dipoles, SUPER results in polarized single-photon emission, exceeding the resonant TPE saturation by a factor of 1.45. Under optimized excitation conditions, we also observe biexciton preparation via a distinct SUPER resonance, confirmed by the appearance of the biexciton emission line, constituting the first experimental demonstration of biexciton preparation using SUPER. These findings are in good agreement with a proposed four-level theoretical model that incorporates the biexciton state. We also report that a slight misalignment of laser polarization induces an additional SUPER resonance that selectively populates the orthogonal exciton dipole, without altering the nominal excitation polarization. This unexpected behavior reveals a new degree of freedom for coherent state preparation. Our findings establish the SUPER scheme as a versatile tool for state-selective exciton and biexciton control.

physics.optics↗

arXiv2025

Photonic "hourglass" design beyond the standard bulk model of phonon decoherence

We study the impact of mechanical vibrations on the performance of the photonic "hourglass" structure, which is predicted to emit single photons on-demand with near-unity efficiency and indistinguishability. Previous investigations neglected the impact of vibrational modes inherent to this quasi-1D geometry, relying instead on a three-dimensional bulk assumption for the phonon modes. However, it has been shown that phonon decoherence has a much stronger impact in 1D structures as compared with bulk media. Here, we surprisingly demonstrate the robustness of the photonic hourglass design, achieving close-to-unity indistinguishability even by incorporating a detailed description of the vibrational modes. We explain this unexpected result in terms of the large Purcell enhancement of the hourglass single-photon source, which eliminates the negative effect of phonons. Our findings highlight the key role of high-Q optical cavities in mitigating the detrimental effect of phonon decoherence, even for structures of reduced dimensionality.

quant-ph↗

arXiv2024

One-dimensional photonic wire as a single-photon source: Implications of cavity QED to a phonon bath of reduced dimensionality

While the semiconductor quantum dot placed in a solid-state material allows for deterministic emission of single photons, the photon indistinguishability is strongly influenced by the intrinsic coupling to lattice vibrations, phonons, of the solid-state environment. This work investigates the phonon-induced decoherence for a quantum dot placed in the one-dimensional system of a homogeneous cylindrical nanowire. Such a structure supports multiple longitudinal phonon branches, and we consider both a linear and a quadratic coupling of the emitter to these modes. Under a polaron approach, we initially derive an analytical expression for the 1D pure dephasing rate, which leads to a reduced pure dephasing rate compared with bulk. By implementing these results into a full cavity quantum electrodynamic model, we demonstrate that multimode coupling is necessary to correctly predict the indistinguishability in a 1D system, which may otherwise be significantly underestimated.

cond-mat.mes-hall↗

arXiv2024

SUPER excitation of quantum emitters is a multi-photon process

The swing-up of quantum emitter population (SUPER) scheme allows to populate the excited state of a quantum emitter with near-unity fidelity using two red-detuned laser pulses. Its off-resonant, yet fully coherent nature has attracted significant interest in quantum photonics as a valuable tool for preparing single-photon sources in their excited state on demand, while simultaneously ensuring straightforward spectral filtering of the laser. However, the physical understanding of this mechanism in terms of energy exchange between the electromagnetic field and the emitter is still lacking. Here, we present a fully quantized model of the swing-up excitation and demonstrate that it is in fact a multi-photon process, where one of the modes loses two or more photons while the other gains at least one. Our findings provide an unexpected physical interpretation of the SUPER scheme and unveil a new non-linear interaction between single emitters and multiple field modes.

quant-ph↗

arXiv2024

Single-photon emitters in WSe$_2$: Critical role of phonons on excitation schemes and indistinguishability

Within optical quantum information processing, single-photon sources based on a two-level system in a semiconductor material allow for on-demand generation of single photons. To initiate the spontaneous emission process, it is necessary to efficiently populate the excited state. However, reconciling the requirement for on-demand excitation with both high efficiency and high photon indistinguishability remains a challenge due to the presence of charge noise and phonon-induced decoherence in the solid-state environment. Here, we propose a method for reconstructing the phonon spectral density experienced by WSe$_{2}$ quantum emitters in the emission process. Using the reconstructed phonon spectral density, we analyze the performance of the resonant, phonon-assisted, and Swing-UP of the quantum EmitteR population (SUPER) swing-up excitation schemes. Under resonant excitation, we obtain an exciton preparation fidelity limited to $\sim$0.80 by the strong phonon coupling, which improves to 0.96 for the SUPER scheme (or 0.89, depending on the type of emitter considered). Under near-resonant phonon-assisted excitation, we observe near-unity excitation fidelity up to 0.976 (0.997). Additionally, we demonstrate that, assuming the suppression of the phonon sidebands, residual dephasing mechanisms such as charge/spin fluctuations are the dominating decoherence mechanisms undermining the photon indistinguishability.

quant-ph↗

arXiv2024

High-purity and stable single-photon emission in bilayer WSe$_2$ via phonon-assisted excitation

The excitation scheme is essential for single-photon sources, as it governs exciton preparation, decay dynamics, and the spectral diffusion of emitted photons. While phonon-assisted excitation has shown promise in other quantum emitter platforms, its proper implementation and systematic comparison with alternative excitation schemes have not yet been demonstrated in transition metal dichalcogenide (TMD) quantum emitters. Here, we investigate the impact of various optical excitation strategies on the single-photon emission properties of bilayer WSe$_2$ quantum emitters. Based on our theoretical predictions for the exciton preparation fidelity, we compare excitation via the longitudinal acoustic and breathing phonon modes to conventional above-band and near-resonance excitations. Under acoustic phonon-assisted excitation, we achieve narrow single-photon emission with a reduced spectral diffusion of 0.0129 nm, a 1.8-fold improvement over above-band excitation. Additionally, excitation through breathing-phonon mode yields a high purity of $ 0.947\pm 0.079\,$ and reduces the decay time by over an order of magnitude, reaching $(1.33 \pm 0.04)\,$ns. Our comprehensive study demonstrates the crucial role of phonon-assisted excitation in optimizing the performance of WSe$_2$-based quantum emitters, providing valuable insights for the development of single-photon sources for quantum photonics applications.

quant-ph↗

arXiv2024

Tailoring Polarization in WSe$_2$ Quantum Emitters through Deterministic Strain Engineering

Quantum emitters in transition metal dichalcogenides (TMDs) have recently emerged as a promising platform for generating single photons for optical quantum information processing. In this work, we present an approach for deterministically controlling the polarization of fabricated quantum emitters in a tungsten diselenide (WSe$_2$) monolayer. We employ novel nanopillar geometries with long and sharp tips to induce a controlled directional strain in the monolayer, and we report on fabricated WSe$_2$ emitters producing single photons with a high degree of polarization $(99\pm 4 \%)$ and high purity ($g^{(2)}(0) = 0.030 \pm 0.025$). Our work paves the way for the deterministic integration of TMD-based quantum emitters for future photonic quantum technologies.

physics.optics↗

arXiv2023

Enhancing the efficiency of quantum-dot-based single-photon source designs by suppressing background emission using concentric rings

In this paper, we theoretically demonstrate that a few-period circular Bragg reflector consisting of concentric rings placed around an infinite nanowire with an embedded quantum dot can increase the fraction of radiative emission into the fundamental $\mathrm{HE}_{11}$ mode ($\beta=\Gamma_{\rm HE_{11}}/\Gamma_{\rm Total}$) up to 0.999 due to enhanced suppression of the emission into radiation modes caused by a photonic bandgap effect. We then apply this strategy in the practically relevant case of the finite-sized single-photon source based on tapered nanowires and demonstrate that the collection efficiency can be improved. Additionally, we also show the beneficial effects of placing optimized rings around the micropillar single-photon source.

physics.optics↗

arXiv2023

Highly efficient and indistinguishable single-photon sources via phonon-decoupled two-color excitation

Single-photon sources with near-unity efficiency and indistinguishability play a major role in the development of quantum technologies. However, on-demand excitation of the emitter imposes substantial limitations to the source performance. Here, we show that coherent two-color pumping allows for population inversion arbitrarily close to unity in bulk quantum dots thanks to a decoupling effect between the emitter and its phonon bath. Driving a micropillar single-photon source with this scheme, we calculate very high photon emission into the cavity mode (0.95 photons per pulse) together with excellent indistinguishability (0.975) in a realistic configuration, thereby removing the limitations imposed by the excitation scheme on single-photon source engineering.

quant-ph↗

arXiv2023

Performance of the nanopost single-photon source: beyond the single-mode model

We present a detailed analysis of the physics governing the collection efficiency and the Purcell enhancement of the nanopost single-photon source. We show that a standard single-mode Fabry-Pérot model is insufficient to describe the device performance, which benefits significantly from scattering from the fundamental mode to radiation modes. We show how the scattering mechanism decouples the collection efficiency from the Purcell enhancement, such that maximum collection efficiency is obtained off-resonance. Finally, we discuss how this scattering mechanism can be beneficial for future single-photon source designs.

quant-ph↗

arXiv2022

Near-unity efficiency and photon indistinguishability for the "hourglass" single-photon source using suppression of background emission

An on-going challenge within scalable optical quantum information processing is to increase the collection efficiency $\varepsilon$ and the photon indistinguishability $η$ of the single-photon source towards unity. Within quantum dot-based sources, the prospect of increasing the product $\varepsilon η$ arbitrarily close to unity was recently questioned. In this work, we discuss the influence of the trade-off between efficiency and indistinguishability in the presence of phonon-induced decoherence, and we show that the photonic "hourglass" design allows for improving $\varepsilon η$ beyond the predicted maximum for the standard micropillar design subject to this trade-off. This circumvention of the trade-off is possible thanks to control of the spontaneous emission into background radiation modes, and our work highlights the importance of engineering of the background emission in future pursuits of near-unity performance of quantum dot single-photon sources.

quant-ph↗

arXiv2022

Near-unity efficiency in ridge waveguide-based, on-chip single-photon sources

We report a numerical design procedure for pursuing a near-unity coupling efficiency in quantum dot-cavity ridge waveguide single-photon sources by performing simulations with the finite element method. Our optimum design which is based on a 1D nanobeam cavity, achieves a high source efficiency $ε_{xy}$ of 97.7$\%$ for an isotropic in-plane dipole, together with a remarkable Purcell factor of 38.6. Such a good performance is mainly attributed to the high index contrast of GaAs/SiO$_2$ and a careful cavity design achieving constructive interference and low scattering losses. Furthermore, we analyze the bottleneck of the proposed platform, which is the mode mismatch between the cavity mode and the Bloch mode in the nanobeam. Accordingly, we present the optimization recipe of an arbitrarily high-efficiency on-chip single-photon source by implementing a taper section, whose high smoothness is beneficial to gradually overcoming the mode mismatch, and therefore leading to a higher Purcell factor and source efficiency. Finally, we see good robustness of the source properties in the taper-nanobeam system under the consideration of realistic fabrication imperfections on the hole variation.

physics.optics↗

arXiv2022

Design and fabrication of ridge waveguide-based nanobeam cavities for on-chip single-photon sources

We report on the design of nanohole/nanobeam cavities in ridge waveguides for on-chip, quantum-dot-based single-photon generation. Our design overcomes limitations of a low-refractive-index-contrast material platform in terms of emitter-mode coupling efficiency and yields an outcoupling efficiency of 0.73 to the output ridge waveguide. Importantly, this high coupling efficiency is combined with broadband operation of 9 nm full-width half-maximum. We provide an explicit design procedure for identifying the optimum geometrical parameters according to the developed design. Besides, we fabricate and optically characterize a proof-of-concept waveguide structure. The results of the microphotoluminescence measurements provide evidence for cavity-enhanced spontaneous emission from the quantum dot, thus supporting the potential of our design for on-chip single-photon sources applications.

physics.optics↗

arXiv2020

Anisotropic properties of monolayer 2D materials: an overview from the C2DB database

We analyze the occurrence of in-plane anisotropy in the electronic, magnetic, elastic and transport properties of more than one thousand 2D materials from the C2DB database. We identify hundreds of anisotropic materials and classify them according to their point group symmetry and degree of anisotropy. A statistical analysis reveals that a lower point group symmetry and a larger amount of different elements in the structure favour all types of anisotropies, which could be relevant for future materials design approaches. Besides, we identify novel compounds, predicted to be easily exfoliable from a parent bulk compound, with anisotropies that largely outscore those of already known 2D materials. Our findings provide a comprehensive reference for future studies of anisotropic response in atomically-thin crystals and point to new previously unexplored materials for the next generation of anisotropic 2D devices.

cond-mat.mtrl-sci↗

arXiv2020

Conductance of quantum spin Hall edge states from first principles: the critical role of magnetic impurities and inter-edge scattering

The outstanding transport properties expected at the edge of two-dimensional time-reversal invariant topological insulators have proven to be challenging to realize experimentally, and have so far only been demonstrated in very short devices. In search for an explanation to this puzzling observation, we here report a full first-principles calculation of topologically protected transport at the edge of novel quantum spin Hall insulators - specifically, Bismuth and Antimony halides - based on the non-equilibrium Green's functions formalism. Our calculations unravel two different scattering mechanisms that may affect two-dimensional topological insulators, namely time-reversal symmetry breaking at vacancy defects and inter-edge scattering mediated by multiple co-operating impurities, possibly non-magnetic. We discuss their drastic consequences for typical non-local transport measurements as well as strategies to mitigate their negative impact. Finally, we provide an instructive comparison of the transport properties of topologically protected edge states to those of the trivial edge states in MoS$_2$ ribbons. Although we focus on a few specific cases (in terms of materials and defect types) our results should be representative for the general case and thus have significance beyond the systems studied here.

cond-mat.mes-hall↗

arXiv2018

Hong-Ou-Mandel heat noise in the quantum Hall regime

We investigate heat current fluctuations induced by a periodic train of Lorentzian-shaped pulses, carrying an integer number of electronic charges, in a Hong-Ou-Mandel interferometer implemented in a quantum Hall bar in the Laughlin sequence. We demonstrate that the noise in this collisional experiment cannot be reproduced in a setup with a single drive, in contrast to what is observed in the charge noise case. Nevertheless, the simultaneous collision of two identical levitons always leads to a total suppression even for the Hong-Ou-Mandel heat noise at all filling factors, despite the presence of emergent anyonic quasi-particle excitations in the fractional regime. Interestingly, the strong correlations characterizing the fractional phase are responsible for a remarkable oscillating pattern in the HOM heat noise, which is completely absent in the integer case. These oscillations can be related to the recently predicted crystallization of levitons in the fractional quantum Hall regime.

cond-mat.mes-hall↗

arXiv2018

Crystallization of Levitons in the fractional quantum Hall regime

Using a periodic train of Lorentzian voltage pulses, which generates soliton-like electronic excitations called Levitons, we investigate the charge density backscattered off a quantum point contact in the fractional quantum Hall regime. We find a regular pattern of peaks and valleys, reminiscent of analogous self-organization recently observed for optical solitons in non-linear environments. This crystallization phenomenon is confirmed by additional side dips in the Hong-Ou-Mandel noise, a feature that can be observed in nowadays electron quantum optics experiments.

cond-mat.mes-hall↗