arXiv subjects

Lucia Hackermueller

Publications and source records attributed to Lucia Hackermueller.

10 recordsLinked to original sources

arXiv2025

Exploiting complex 3D-printed surface structures for portable quantum technologies

Portable quantum technologies require robust, lightweight apparatus with superior performance. For techniques dependent upon high-vacuum environments, such as atom interferometers and atomic clocks, 3D-printing enables new avenues to tailor in-vacuum gas propagation dynamics. We demonstrate intricate, fine-scale surface patterning of 3D-printed vacuum components to increase the rate at which gas particles collide with the surface. By applying a non-evaporable getter coating for use as a surface pump, we show that the patterned surface pumps gas particles 3.8 times faster than an equivalent flat areas. These patterns can be directly integrated into additively manufactured components, enabling application in close proximity to key experimental regions and contributing to overall mass-reduction. We develop numerical simulations that show good agreement with this result and predict up to a ten-fold increase in pumping rate, for realistic surface structures. Our work has direct applications in enabling passively-pumped portable quantum technologies, but also establishes 3D-printing as a powerful technique for the creation of optimized surface patterning to provide enhanced control over high-vacuum gas dynamics for a broad range of applications.

quant-ph↗

arXiv2023

Detecting Dark Domain Walls

Light scalar fields, with double well potentials and direct matter couplings, undergo density driven phase transitions, leading to the formation of domain walls. Such theories could explain dark energy, dark matter or source the nanoHz gravitational-wave background. We describe an experiment that could be used to detect such domain walls in a laboratory experiment, solving for the scalar field profile, and showing how the domain wall affects the motion of a test particle. We find that, in currently unconstrained regions of parameter space, the domain walls leave detectable signatures.

gr-qc↗

arXiv2019

Cold atoms in micromachined waveguides: a new platform for atom-photon interaction

Hybrid quantum devices, incorporating both atoms and photons, can exploit the benefits of both to enable scalable architectures for quantum computing and quantum communication, as well as chip-scale sensors and single-photon sources. Production of such devices depends on the development of an interface between their atomic and photonic components. This should be compact, robust and compatible with existing technologies from both fields. Here we demonstrate such an interface. Cold cesium atoms are trapped inside a transverse, 30 $\mu$m diameter through-hole in an optical fiber, created via laser micromachining. When the guided light is on resonance with the cesium $D_2$ line, up to 87% of it is absorbed by the atoms. The corresponding optical depth per unit length is 700 cm$^{-1}$, higher than any reported for a comparable system. This is important for miniaturisation and scalability. The technique can be equally effective in optical waveguide chips and other existing photonic systems, providing a new platform for fundamental research.

physics.atom-ph↗

arXiv2008

A Kapitza-Dirac-Talbot-Lau interferometer for highly polarizable molecules

Research on matter waves is a thriving field of quantum physics and has recently stimulated many investigations with electrons, neutrons, atoms, Bose-condensed ensembles, cold clusters and hot molecules. Coherence experiments with complex objects are of interest for exploring the transition to classical physics, for measuring molecular properties and they have even been proposed for testing new models of space-time. For matter-wave experiments with complex molecules, the strongly dispersive effect of the interaction between the diffracted molecule and the grating wall is a major challenge because it imposes enormous constraints on the velocity selection of the molecular beam. We here describe the first experimental realization of a new interferometer that solves this problem by combining the advantages of a Talbot-Lau setup with the benefits of an optical phase grating and we show quantum interference with new large molecules.

quant-ph↗

arXiv2007

Optical polarizabilities of large molecules measured in near-field interferometry

We discuss a novel application of matter wave interferometry to characterize the scalar optical polarizability of molecules at 532 nm. The interferometer presented here consists of two material absorptive gratings and one central optical phase grating. The interaction of the molecules with the standing light wave is determined by the optical dipole force and is therefore directly dependent on the molecular polarizability at the wavelength of the diffracting laser light. By comparing the observed matter-wave interference contrast with a theoretical model for several intensities of the standing light wave and molecular velocities we can infer the polarizability in this first proof-of-principle experiment for the fullerenes C60 and C70 and we find a good agreement with literature values.

quant-ph↗

arXiv2005

Influence of molecular temperature on the coherence of fullerenes in a near-field interferometer

We study C70 fullerene matter waves in a Talbot-Lau interferometer as a function of their temperature. While the ideal fringe visibility is observed at moderate molecular temperatures, we find a gradual degradation of the interference contrast if the molecules are heated before entering the interferometer. A method is developed to assess the distribution of the micro-canonical temperatures of the molecules in free flight. This way the heating-dependent reduction of interference contrast can be compared with the predictions of quantum theory. We find that the observed loss of coherence agrees quantitatively with the expected decoherence rate due to the thermal radiation emitted by the hot molecules.

quant-ph↗

arXiv2004

Decoherence of matter waves by thermal emission of radiation

Emergent quantum technologies have led to increasing interest in decoherence - the processes that limit the appearance of quantum effects and turn them into classical phenomena. One important cause of decoherence is the interaction of a quantum system with its environment, which 'entangles' the two and distributes the quantum coherence over so many degrees of freedom as to render it unobservable. Decoherence theory has been complemented by experiments using matter waves coupled to external photons or molecules, and by investigations using coherent photon states, trapped ions and electron interferometers. Large molecules are particularly suitable for the investigation of the quantum-classical transition because they can store much energy in numerous internal degrees of freedom; the internal energy can be converted into thermal radiation and thus induce decoherence. Here we report matter wave interferometer experiments in which C70 molecules lose their quantum behaviour by thermal emission of radiation. We find good quantitative agreement between our experimental observations and microscopic decoherence theory. Decoherence by emission of thermal radiation is a general mechanism that should be relevant to all macroscopic bodies.

quant-ph↗

arXiv2003

The wave nature of biomolecules and fluorofullerenes

We demonstrate quantum interference for tetraphenylporphyrin, the first biomolecule exhibiting wave nature, and for the fluorofullerene C60F48 using a near-field Talbot-Lau interferometer. For the porphyrins, which are distinguished by their low symmetry and their abundant occurence in organic systems, we find the theoretically expected maximal interference contrast and its expected dependence on the de Broglie wavelength. For C60F48 the observed fringe visibility is below the expected value, but the high contrast still provides good evidence for the quantum character of the observed fringe pattern. The fluorofullerenes therefore set the new mark in complexity and mass (1632 amu) for de Broglie wave experiments, exceeding the previous mass record by a factor of two.

quant-ph↗

arXiv2003

Decoherence in a Talbot Lau interferometer: the influence of molecular scattering

We study the interference of C70 fullerenes in a Talbot-Lau interferometer with a large separation between the diffraction gratings. This permits the observation of recurrences of the interference contrast both as a function of the de Broglie wavelength and in dependence of the interaction with background gases. We observe an exponential decrease of the fringe visibility with increasing background pressure and find good quantitative agreement with the predictions of decoherence theory. From this we extrapolate the limits of matter wave interferometry and conclude that the influence of collisional decoherence may be well under control in future experiments with proteins and even larger objects.

quant-ph↗

arXiv2003

Collisional decoherence observed in matter wave interferometry

We study the loss of spatial coherence in the extended wave function of fullerenes due to collisions with background gases. From the gradual suppression of quantum interference with increasing gas pressure we are able to support quantitatively both the predictions of decoherence theory and our picture of the interaction process. We thus explore the practical limits of matter wave interferometry at finite gas pressures and estimate the required experimental vacuum conditions for interferometry with even larger objects.

quant-ph↗