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Luciano Jacopo D'Onofrio

Publications and source records attributed to Luciano Jacopo D'Onofrio.

4 recordsLinked to original sources

Ultrafast laser-stimulated field emission from a metal: a non-equilibrium Green's functions approach

Ultrafast laser-assisted field emission from metallic nanotips is a promising route for generating coherent electron pulses. However, existing theoretical models often neglect many-body strong correlation effects in the emitter's electronic structure and its response to the optical field. In this work, we propose a theoretical framework based on the non-equilibrium Green's function formalism to simulate the out-of-equilibrium electron dynamics across a strongly driven matter-vacuum interface, in a one-dimensional model. Treating the tip-vacuum coupling perturbatively, we find that the interplay between strong-field emission and multi-photon emission regimes can be described in terms of a filtering of the emitter's local density of occupied states through field-dressed vacuum propagators. By including electron-electron interactions via the second-Born approximation, we show that correlation-induced modifications in the electronic structure are directly transferred to the far-field spectrum. Finally, by self-consistently solving the Dyson equation at the interface, we uncover a dynamic back-action regime driven by the optical field, characterized by a periodic polarization of the emitter, which reshapes the far-field spectrum. This shows that the non-equilibrium Green's functions approach provides a versatile framework for exploring and analyzing field emission of correlated electrons.

cond-mat.other↗

Spin selectivity induced by non-collinear spins in Rashba wires

We report a previously overlooked general mechanism to obtain highly efficient spin selectivity in conventional time-reversal symmetric one-dimensional systems without invoking phase decoherence. We reveal that Rashba quantum wires featuring non-collinear spin states at the Fermi level inherently possess spin-selective transport properties. We show that this spin noncollinearity can be systematically designed and engineered by introducing an additional pseudospin degree of freedom - such as valley, sublattice, or orbital angular momentum - into spin-orbit coupled systems. By applying this framework to multi-subband semiconducting quantum wires and oxide nanowires, we establish a generalized route toward quantum-coherent spin selectivity up to 10 %. Our findings offer practical design principles for spin-selective transport devices.

cond-mat.mes-hall↗

Robust spin splitting and fermiology in a layered altermagnet

Altermagnetism defies conventional classifications of collinear magnetic phases, standing apart from ferromagnetism and antiferromagnetism with its unique combination of spin-dependent symmetries, net-zero magnetization, and anomalous Hall transport. Although altermagnetic states have been realized experimentally, their integration into functional devices has been hindered by the structural rigidity and poor tunability of existing materials. First, through cobalt intercalation of the superconducting 2H-NbSe$_2$ polymorph, we induce and stabilize a robust altermagnetic phase and using both theory and experiment, we directly observe the lifting of Kramers degeneracy. Additionally, we present spectroscopic insight into a previously hinted low-temperature phase, and provide evidence of its electronic origin. While shedding light on overlooked aspects of altermagnetism, these findings open pathways to spin-based technologies and lay a foundation for advancing the emerging field of altertronics.

cond-mat.str-el↗

Field-driven attosecond photoinjection dynamics in semiconductors

The route towards manipulation of the optoelectronic properties of matter beyond the current limits of electronics starts from a comprehensive study of the ultrafast dynamics triggered by interaction with light. Among them, a fundamental role is played by charge photoinjection, a complex process that stems from the interplay of many different physical phenomena, which cannot be easily disentangled. Single- and multi-photon absorption, diabatic tunnelling, intra-band motion, and field-driven band dressing, all concur in determining the overall excited electron population, dictating the electro-optical properties of a material. Here we investigate ultrafast photoinjection in a prototypical semiconductor (monocrystalline germanium) by using attosecond transient reflection spectroscopy. The precise pump-field characterization ensured by a simultaneous attosecond streaking experiment, in tandem with a comprehensive theoretical approach, allowed us to disentangle the different physical phenomena unfolding at different positions in the reciprocal space and at different timing within the envelope of the pump pulse. Moreover, we found that intra-band phenomena hinder charge injection, in contrast to what was previously observed for resonant, direct band-gap semiconductors. Therefore, besides other known parameters as the central wavelength and peak intensity, our results indicate that the pulse temporal envelope and the local band structure probed by intra-band effects are of key importance to achieve an optimal control over the ultrafast carrier injection process and tailor the complex optical and electronic properties of a semiconductor on the few- to sub-femtosecond time scale.

physics.optics↗