arXiv subjects

Ludvik Martinu

Publications and source records attributed to Ludvik Martinu.

5 recordsLinked to original sources

arXiv2025

Field-enhancement and nonlocal effects in epsilon-near-zero photonic gap antennas

In recent years, the large electric field enhancement and tight spatial confinement supported by the so-called epsilon near-zero (ENZ) mode has attracted significant attention for the realization of efficient nonlinear optical devices. Here, we experimentally demonstrate ENZ photonic gap antennas (PGAs), which consist of a dielectric pillar within which a thin slab of indium tin oxide (ITO) material is embedded. In ENZ PGAs, hybrid dielectric-ENZ modes emerge from strong coupling between the dielectric antenna modes and the ENZ bulk plasmon resonance. These hybrid modes efficiently couple to free space and allow for large enhancements of the incident electric field over nearly an octave bandwidth, without the stringent lateral nanofabrication requirements of conventional plasmonic or dielectric nanoantennas. To understand the modal features, we probe the linear response of single ENZ PGAs with dark field scattering and interpret the results in terms of a simple coupled oscillator framework. Third harmonic generation (THG) is used to probe the ITO local fields and large enhancements are observed in the THG efficiency over a broad spectral range. Surprisingly, sharp peaks emerge on top of the nonlinear response, which were not predicted by full wave calculations. These peaks are attributed to the ENZ material's nonlocal response, which once included using a hydrodynamic model for the ITO permittivity improves the agreement of our calculations for both the linear and nonlinear response. This proof of concept demonstrates the potential of ENZ PGAs, which we have previously shown can support electric field enhancements of up to 100--200X, and the importance of including nonlocal effects when describing the response of thin ENZ layers. Importantly, inclusion of the ITO nonlocality leads to increases in the predicted field enhancement, as compared to the local calculation.

physics.optics↗

arXiv2022

Broadband field-enhancement in epsilon-near-zero photonic gap antennas

In recent years, the large electric field enhancement and tight spatial confinement supported by the so-called epsilon-near-zero (ENZ) mode have attracted significant attention for the realization of efficient nonlinear optical devices. Here, we experimentally demonstrate a new type of antenna, termed an ENZ photonic gap antenna (PGA), which consists of a dielectric pillar within which a thin slab of indium tin oxide (ITO) material is embedded. In ENZ PGAs, hybrid dielectric-ENZ modes emerge from strong coupling between the dielectric antenna modes and the ENZ bulk plasmon resonance. These hybrid modes efficiently couple to free space and allow for large enhancements of the incident electric field over nearly an octave bandwidth, without the stringent lateral nanofabrication requirements required by conventional plasmonic or dielectric nanoantennas. The linear response of single ENZ PGAs is probed using dark field scattering and interpreted using a simple coupled oscillator framework. Third harmonic generation is used to probe the field enhancement and large enhancements are observed in the THG efficiency over a broad spectral range. This proof of concept demonstrates the potential of ENZ PGAs, which we have previously shown can support electric field enhancements of up to 100--200X, which is comparable with those of the best plasmonic antennas.

physics.optics↗

arXiv2018

Interacting polariton fluids in a monolayer of tungsten disulfide

Atomically thin transition metal dichalcogenides (TMDs) possess a number of properties that make them attractive for realizing room-temperature polariton devices. An ideal platform for manipulating polariton fluids within monolayer TMDs is that of Bloch surface waves, which confine the electric field to a small volume near the surface of a dielectric mirror. Here we demonstrate that monolayer tungsten disulfide ($\text{WS}_2$) can sustain Bloch surface wave polaritons (BSWPs) with a Rabi splitting of 43 meV and propagation constants reaching 33 $μ$m. In addition, we evidence strong polariton-polariton nonlinearities within BSWPs, which manifest themselves as a reversible blueshift of the lower polariton resonance by up to 12.9$\pm$0.5 meV. Such nonlinearities are at the heart of polariton devices and have not yet been demonstrated in TMD polaritons. As a proof of concept, we use the nonlinearity to implement a nonlinear polariton source. Our results demonstrate that BSWPs using TMDs can support long-range propagation combined with strong nonlinearities, enabling potential applications in integrated optical processing and polaritonic circuits.

cond-mat.quant-gas↗

arXiv2001

Structural properties of silicon dioxide thin films densified by medium-energy particles

Classical molecular-dynamics simulations have been carried out to investigate densification mechanisms in silicon dioxide thin films deposited on an amorphous silica surface, according to a simplified ion-beam assisted deposition (IBAD) scenario. We compare the structures resulting from the deposition of near-thermal (1 eV) SiO$_{2}$ particles to those obtained with increasing fraction of 30 eV SiO$_{2}$ particles. Our results show that there is an energy interval - between 12 and 15 eV per condensing SiO$_2$ unit on average - for which the growth leads to a dense, low-stress amorphous structure, in satisfactory agreement with the results of low-energy ion-beam experiments. We also find that the crossover between low- and high-density films is associated with a tensile to compressive stress transition, and a simultaneous healing of structural defects of the {\em a-}SiO$_2$ network, namely three- and four-fold rings. It is observed, finally, that densification proceeds through significant changes at intermediate length scales (4--10 Å), leaving essentially unchanged the ``building blocks'' of the network, viz. the Si(O$_{1/2}$)$_{4}$ tetrahedra. This latter result is in qualitative agreement with the mechanism proposed to explain the irreversible densification of amorphous silica recovered from high pressures ($\sim$ 15--20 GPa).

cond-mat.mtrl-sci↗

arXiv1998

A simple method for the determination of slowly varying refractive index profiles from in situ spectrophotometric measurements

Reliable control of the deposition process of optical films and coatings frequently requires monitoring of the refractive index profile throughout the layer. In the present work a simple in situ approach is proposed which uses a WKBJ matrix representation of the optical transfer function of a single thin film on a substrate. Mathematical expressions are developed which represent the minima and maxima envelopes of the curves transmittance-vs-time and reflectance-vs-time. The refractive index and extinction coefficient depth profiles of different films are calculated from simulated spectra as well as from experimental data obtained during PECVD of silicon-compound films. Variation of the deposition rate with time is also evaluated from the position of the spectra extrema as a function of time. The physical and mathematical limitations of the method are discussed.

physics.optics↗