arXiv subjects

Luis S. Froufe-Pérez

Publications and source records attributed to Luis S. Froufe-Pérez.

17 recordsLinked to original sources

arXiv2026

Strong suppression of the photonic density of states in three-dimensional disordered silicon networks

Photonic bandgaps can open not only in crystalline dielectric materials but also in amorphous structures. Self-uniform amorphous gyroid networks have been proposed as promising disordered photonic architectures. Motivated by numerical studies, we combine direct laser-writing lithography with advanced materials processing to fabricate these structures from high-refractive-index silicon. Spectroscopic measurements at mid-infrared wavelengths reveal pronounced transmission minima. To investigate the formation of photonic band gaps in amorphous structures, we develop polarization-resolved transmission spectroscopy that separates ballistic and multiply scattered contributions, enabling direct identification of the underlying transport regimes. We observe a strong suppression of diffuse transmission, providing direct experimental evidence for a breakdown of conventional diffuse transport associated with a strongly reduced photonic density of states. Together with large-scale numerical simulations, our results establish the presence of a deep photonic pseudogap in an amorphous three-dimensional dielectric material and open new opportunities for observing disorder-induced localization phenomena, including Anderson localization of light.

physics.optics↗

arXiv2025

Tuning pair interactions in colloidal systems using random light fields

We propose a method to tune interactions between absorptionless colloidal particle pairs. This is achieved via optimization of the spectral energy density of a homogeneous random optical field. Several standard and more exotic interaction potentials, as well as their negative counterparts, are shown to be successfully tuned. We show that the effective dimensionality of the space of potential functions that can be created by this means can reach up to several tens.

cond-mat.soft↗

arXiv2025

Pure many-body interactions in colloidal systems by artificial random light fields

We propose a method to generate pure many-body interactions in colloidal systems by using optical forces induced by random optical fields with an optimized spectral energy density. To assess the feasibility in general settings, we develop a simple model for Lorentzian electric and magnetic dipole response. An optimization procedure is then introduced to design the spectral energy density of the random field that minimizes pair interactions at constant electromagnetic energy density. We conclude that, under rather general circumstances, it is possible to effectively cancel pair interactions within a range of distance. Hence a colloid can be driven to interact exclusively through many-body interactions

cond-mat.soft↗

arXiv2023

Light in correlated disordered media

The optics of correlated disordered media is a fascinating research topic emerging at the interface between the physics of waves in complex media and nanophotonics. Inspired by photonic structures in nature and enabled by advances in nanofabrication processes, recent investigations have unveiled how the design of structural correlations down to the subwavelength scale could be exploited to control the scattering, transport and localization of light in matter. From optical transparency to superdiffusive light transport to photonic gaps, the optics of correlated disordered media challenges our physical intuition and offers new perspectives for applications. This article reviews the theoretical foundations, state-of-the-art experimental techniques and major achievements in the study of light interaction with correlated disorder, covering a wide range of systems -- from short-range correlated photonic liquids, to Lévy glasses containing fractal heterogeneities, to hyperuniform disordered photonic materials. The mechanisms underlying light scattering and transport phenomena are elucidated on the basis of rigorous theoretical arguments. We overview the exciting ongoing research on mesoscopic phenomena, such as transport phase transitions and speckle statistics, and the current development of disorder engineering for applications such as light-energy management and visual appearance design. Special efforts are finally made to identify the main theoretical and experimental challenges to address in the near future.

physics.optics↗

arXiv2023

Efficient structural color from pigment-loaded nanostructures

Color can originate from wavelength-dependence in the absorption of pigments or the scattering of nanostructures. While synthetic colors are dominated by the former, vivid structural colors found in nature have inspired much research on the latter. However, many of the most vibrant colors in nature involve the interactions of structure and pigment. Here, we demonstrate that pigment can be exploited to efficiently create bright structural color at wavelengths outside its absorption band. We created pigment-enhanced Bragg reflectors by sequentially spin-coating layers of poly-vinyl alcohol (PVA) and polystyrene (PS) loaded with $β$-carotene (BC). With only 10 double layers, we acheived a peak reflectance over $0.8$ at 550 nm and normal incidence. A pigment-free multilayer made of the same materials would require 25 double layers to achieve the same reflectance. Further, pigment loading suppressed the Bragg reflector's characteristic iridescence. Using numerical simulations, we further show that similar pigment loadings could significantly expand the gamut of non-iridescent colors addressable by photonic glasses.

cond-mat.soft↗

arXiv2023

Bandgap fluctuations and robustness in two-dimensional hyperuniform dielectric materials

We numerically study the statistical fluctuations of photonic band gaps in ensembles of stealthy hyperuniform disordered patterns. We find that at low stealthiness, where correlations are weak, band gaps of different system realizations appear over a wide frequency range, are narrow, and generally do not overlap. Interestingly, above a critical value of stealthiness $χ\gtrsim 0.35$, the bandgaps become large and overlap significantly from realization to realization, while a second gap appears. These observations extend our understanding of photonic bandgaps in disordered systems and provide information on the robustness of gaps in practical applications.

physics.class-ph↗

arXiv2022

Light transport through amorphous photonic materials with localization and bandgap regimes

We propose a framework that unifies the description of light transport in three-dimensional amorphous dielectric materials that exhibit both localization and a photonic bandgap. To this end, we argue that coherent reflection near and in the bandgap attenuates the generation of diffuse or localized photons. Using the self-consistent theory of localization and considering the density of states of photons, we can quantitatively describe all transport regimes: Transparency, light diffusion, localization, and bandgap. Comparing the model with numerical data on optical transport in hyperuniform dielectric networks confirms our findings.

physics.optics↗

arXiv2020

Experimental Tuning of Transport Regimes in Hyperuniform Disordered Photonic Materials

We present wave transport experiments in hyperuniform disordered arrays of cylinders with high dielectric permittivity. Using microwaves, we show that the same material can display transparency, photon diffusion, Anderson localization, or a full band gap, depending on the frequency $ν$ of the electromagnetic wave. Interestingly, we find a second weaker band gap, which appears to be related to the second peak of the structure factor. Our results emphasize the importance of spatial correlations on different length scales for the formation of photonic band gaps.

cond-mat.dis-nn↗

arXiv2020

Transition from Light Diffusion to Localization in Three-Dimensional Amorphous Dielectric Networks near the Band Edge

Localization of light is the photon analog of electron localization in disordered lattices for whose discovery Anderson received the Nobel prize in 1977. The question about its existence in open three-dimensional materials has eluded an experimental and full theoretical verification for decades. Here we study numerically electromagnetic vector wave transmittance through realistic digital representations of hyperuniform dielectric networks, a new class of highly correlated but disordered photonic band gap materials. We identify the evanescent decay of the transmitted power in the gap and diffusive transport far from the gap. Near the gap, we find that transport sets off diffusive but, with increasing slab thickness, crosses over gradually to a faster decay, signaling localization. We show that we can describe the transition to localization at the mobility edge using the self-consistent theory of localization based on the concept of a position-dependent diffusion coefficient.

physics.optics↗

arXiv2017

Transport Phase Diagram and Anderson Localization in Hyperuniform Disordered Photonic Materials

Hyperuniform disordered photonic materials (HDPM) are spatially correlated dielectric structures with unconventional optical properties. They can be transparent to long-wavelength radiation while at the same time have isotropic band gaps in another frequency range. This phenomenon raises fundamental questions concerning photon transport through disordered media. While optical transparency is robust against recurrent multiple scattering, little is known about other transport regimes like diffusive multiple scattering or Anderson localization. Here we investigate band gaps, and we report Anderson localization in two-dimensional stealthy HDPM using numerical simulations of the density of states and optical transport statistics. To establish a unified view, we propose a transport phase diagram. Our results show that, depending only on the degree of correlation, a dielectric material can transition from localization behavior to a bandgap crossing an intermediate regime dominated by tunneling between weakly coupled states.

physics.optics↗

arXiv2016

The Role of Short-Range Order and Hyperuniformity in the Formation of Band Gaps in Disordered Photonic Materials

We study photonic band gap formation in two-dimensional high refractive index disordered materials where the dielectric structure is derived from packing disks in real and reciprocal space. Numerical calculations of the photonic density of states demonstrate the presence of a band gap for all polarizations in both cases. We find that the band gap width is controlled by the increase in positional correlation inducing short-range order and hyperuniformity concurrently. Our findings suggest that the optimization of short-range order, in particular the tailoring of Bragg scattering at the isotropic Brillouin zone, are of key importance for designing disordered PBG materials.

physics.optics↗

arXiv2015

High-quality photonic crystals with a nearly complete band gap obtained by direct inversion of woodpile templates with titanium dioxide

Photonic crystal materials are based on a periodic modulation of the dielectric constant on length scales comparable to the wavelength of light. These materials can exhibit photonic band gaps; frequency regions for which the propagation of electromagnetic radiation is forbidden due to the depletion of the density of states. In order to exhibit a full band gap, 3D PCs must present a threshold refractive index contrast that depends on the crystal structure. In the case of the so-called woodpile photonic crystals this threshold is comparably low, approximately 1.9 for the direct structure. Therefore direct or inverted woodpiles made of high refractive index materials like silicon, germanium or titanium dioxide are sought after. Here we show that, by combining multiphoton lithography and atomic layer deposition, we can achieve a direct inversion of polymer templates into TiO$_{2}$ based photonic crystals. The obtained structures show remarkable optical properties in the near-infrared region with almost perfect specular reflectance, a transmission dip close to the detection limit and a Bragg length comparable to the lattice constant.

physics.optics↗

arXiv2011

Probing statistical properties of Anderson localization with quantum emitters

Wave propagation in disordered media can be strongly modified by multiple scattering and wave interference. Ultimately the so-called Anderson-localized regime is reached when the waves become strongly confined in space. So far, Anderson localization of light has been probed in transmission experiments by measuring the intensity of an external light source after propagation through a disordered medium. However, discriminating between Anderson localization and losses in these experiments remains a major challenge. Here we present an alternative approach where we use quantum emitters embedded in disordered photonic crystal waveguides as light sources. Anderson-localized modes are efficiently excited and the analysis of the photoluminescence spectra allows to explore their statistical properties paving a way for controlling Anderson localization in disordered photonic crystals.

quant-ph↗

arXiv2010

Optical amplification enhancement in photonic crystals

Improving and controlling the efficiency of a gain medium is one of the most challenging problems of laser research. By measuring the gain length in an opal based photonic crystal doped with laser dye, we demonstrate that optical amplification is more than twenty-fold enhanced along the Gamma-K symmetry directions of the face centered cubic photonic crystal. These results are theoretically explained by directional variations of the density of states, providing a quantitative connection between density of the states and light amplification.

physics.optics↗

arXiv2009

Towards a random laser with cold atoms

Atoms can scatter light and they can also amplify it by stimulated emission. From this simple starting point, we examine the possibility of realizing a random laser in a cloud of laser-cooled atoms. The answer is not obvious as both processes (elastic scattering and stimulated emission) seem to exclude one another: pumping atoms to make them behave as amplifier reduces drastically their scattering cross-section. However, we show that even the simplest atom model allows the efficient combination of gain and scattering. Moreover, supplementary degrees of freedom that atoms offer allow the use of several gain mechanisms, depending on the pumping scheme. We thus first study these different gain mechanisms and show experimentally that they can induce (standard) lasing. We then present how the constraint of combining scattering and gain can be quantified, which leads to an evaluation of the random laser threshold. The results are promising and we draw some prospects for a practical realization of a random laser with cold atoms.

physics.atom-ph↗

arXiv2009

Threshold of a Random Laser with Cold Atoms

We address the problem of achieving an optical random laser with a cloud of cold atoms, in which gain and scattering are provided by the same atoms. The lasing threshold can be defined using the on-resonance optical thickness b0 as a single critical parameter. We predict the threshold quantitatively, as well as power and frequency of the emitted light, using two different light transport models and the atomic polarizability of a strongly-pumped two-level atom. We find a critical b0 on the order of 300, which is within reach of state-of-the-art cold-atom experiments. Interestingly, we find that random lasing can already occur in a regime of relatively low scattering.

physics.atom-ph↗

arXiv2008

Density of states governs light scattering in photonic crystals

We describe a smooth transition from (fully ordered) photonic crystal to (fully disordered) photonic glass that enables us to make an accurate measurement of the scattering mean free path in nanostructured media and, in turn, establishes the dominant role of the density of states. We have found one order of magnitude chromatic variation in the scattering mean free path in photonic crystals for just $\sim 3%$ shift around the band-gap ($\sim 27$ nm in wavelength).

physics.optics↗