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Lukas Janssen

Publications and source records attributed to Lukas Janssen.

At least 37 records · Page 2Linked to original sources

Spin vestigial orders in extended Heisenberg-Kitaev models near hidden SU(2) points: Application to Na$_2$Co$_2$TeO$_6$

The honeycomb magnet Na$_2$Co$_2$TeO$_6$ has recently been argued to realize an approximate hidden SU(2) symmetry that can be understood by means of a duality transformation. Using large-scale classical Monte Carlo simulations, we study the finite-temperature phase diagram of the pertinent Heisenberg-Kitaev-$Γ$-$Γ'$ model near the hidden-SU(2)-symmetric point, in the presence of a six-spin ring exchange perturbation. At low temperatures, the model features collinear single-$\mathbf{q}$ zigzag and noncollinear triple-$\mathbf{q}$ ground states, depending on the sign of the ring exchange coupling. We show that in the vicinity of the hidden-SU(2)-symmetric point, the magnetic long-range orders melt in two stages. The corresponding finite-temperature transitions are continuous and fall into 2D Ising and 2D Potts universality classes, respectively. The two fluctuation-induced phases at intermediate temperatures spontaneously break spin rotational and lattice translational symmetries, respectively, but both leave time reversal symmetry intact. They are characterized by finite expectation values of a real, symmetric, traceless, second-rank tensor, and are naturally understood as vestigial orders of the underlying magnetic states. We identify these vestigial orders as $\mathbb{Z}_3$ spin nematic and $\mathbb{Z}_4$ spin current density wave phases, respectively. For increasing ring exchange perturbations, the width of the vestigial phases decreases, eventually giving rise to a direct first-order transition from the magnetically-ordered phase to the disordered paramagnet. We propose the $\mathbb{Z}_4$ spin current density wave phase, which is the vestigial phase of the primary triple-$\mathbf q$ magnetic order, as a natural candidate for the paramagnetic 2D long-range-ordered state observed in Na$_2$Co$_2$TeO$_6$ in a small window above the antiferromagnetic ordering temperature.

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The Nordic-walking mechanism and its explanation of deconfined pseudocriticality from Wess-Zumino-Witten theory

The understanding of phenomena falling outside the Ginzburg-Landau paradigm of phase transitions represents a key challenge in condensed matter physics. A famous class of examples is constituted by the putative deconfined quantum critical points between two symmetry-broken phases in layered quantum magnets, such as pressurised SrCu$_2$(BO$_3$)$_2$. Experiments find a weak first-order transition, which simulations of relevant microscopic models can reproduce. The origin of this behaviour has been a matter of considerable debate for several years. In this work, we demonstrate that the nature of the deconfined quantum critical point can be best understood in terms of a novel dynamical mechanism, termed Nordic walking. Nordic walking denotes a renormalisation group flow arising from a beta function that is flat over a range of couplings. This gives rise to a logarithmic flow that is faster than the well-known walking behaviour, associated with the annihilation and complexification of fixed points, but still significantly slower than the generic running of couplings. The Nordic-walking mechanism can thus explain weak first-order transitions, but may also play a role in high-energy physics, where it could solve hierarchy problems. We analyse the Wess-Zumino-Witten field theory pertinent to deconfined quantum critical points with a topological term in 2+1 dimensions. To this end, we construct an advanced functional renormalisation group approach based on higher-order regulators. We thereby calculate the beta function directly in 2+1 dimensions and provide evidence for Nordic walking.

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Triple-q order in Na$_2$Co$_2$TeO$_6$ from proximity to hidden-SU(2)-symmetric point

In extended Heisenberg-Kitaev-Gamma-type spin models, hidden-SU(2)-symmetric points are isolated points in parameter space that can be mapped to pure Heisenberg models via nontrivial duality transformations. Such points generically feature quantum degeneracy between conventional single-q and exotic multi-q states. We argue that recent single-crystal inelastic neutron scattering data place the honeycomb magnet Na$_2$Co$_2$TeO$_6$ in proximity to such a hidden-SU(2)-symmetric point. The low-temperature order is identified as a triple-q state arising from the Néel antiferromagnet with staggered magnetization in the out-of-plane direction via a 4-sublattice duality transformation. This state naturally explains various distinctive features of the magnetic excitation spectrum, including its surprisingly high symmetry and the dispersive low-energy and flat high-energy bands. Our result demonstrates the importance of bond-dependent exchange interactions in cobaltates, and illustrates the intriguing magnetic behavior resulting from them.

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Phonon thermal transport shaped by strong spin-phonon scattering in a Kitaev material Na$_2$Co$_2$TeO$_6$

The recent report of a half-quantized thermal Hall effect in the Kitaev material $α$-RuCl$_3$ has sparked a strong debate on whether it is generated by Majorana fermion edge currents or whether other more conventional mechanisms involving magnons or phonons are at its origin. A more direct evidence for Majorana fermions which could be expected to arise from a contribution to the longitudinal heat conductivity $κ_{xx}$ at $T\rightarrow0$ is elusive due to a very complex magnetic field dependence of $κ_{xx}$. Here, we report very low temperature (below 1~K) thermal conductivity ($κ$) of another candidate Kitaev material, Na$_2$Co$_2$TeO$_6$. The application of a magnetic field along different principal axes of the crystal reveals a strong directional-dependent magnetic-field ($\bf B$) impact on $κ$. We show that no evidence for mobile quasiparticles except phonons can be concluded at any field from 0~T to the field polarized state. In particular, severely scattered phonon transport is observed across the $B-T$ phase diagram, which is attributed to prominent magnetic fluctuations. Cascades of phase transitions are uncovered for all $\bf B$ directions by probing the strength of magnetic fluctuations via a precise record of $κ$($B$). Our results thus rule out recent proposals for itinerant magnetic excitations in Na$_2$Co$_2$TeO$_6$, and emphasise the importance of discriminating true spin liquid transport properties from scattered phonons in candidate materials.

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Magnetic quantum phase transition in a metallic Kondo heterostructure

We consider a two-dimensional quantum spin system described by a Heisenberg model that is embedded in a three-dimensional metal. The two systems couple via an antiferromagnetic Kondo interaction. In such a setup, the ground state generically remains metallic down to the lowest temperatures and allows us to study magnetic quantum phase transitions in metallic environments. From the symmetry point of view, translation symmetry is present in two out of three lattice directions such that crystal momentum is only partially conserved. Importantly, the construction provides a route to study, with negative-sign-free auxiliary-field quantum Monte Carlo methods, the physics of local moments in metallic environments. Our large-scale numerical simulations show that as a function of the Kondo coupling, the system has two metallic phases. In the limit of strong Kondo coupling, a paramagnetic heavy-fermion phase emerges. Here, the spin degree of freedom is screened by means of the formation of a composite quasiparticle that participates in the Luttinger count. At weak Kondo coupling, magnetic order is present. This phase is characterized by Landau-damped Goldstone modes. Furthermore, the aforementioned composite quasiparticle remains intact across the quantum phase transition.

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Gross-Neveu-Heisenberg criticality from $2+\boldsymbolε$ expansion

The Gross-Neveu-Heisenberg universality class describes a continuous quantum phase transition between a Dirac semimetal and an antiferromagnetic insulator. Such quantum critical points have originally been discussed in the context of Hubbard models on $π$-flux and honeycomb lattices, but more recently also in Bernal-stacked bilayer models, of potential relevance for bilayer graphene. Here, we demonstrate how the critical behavior of this fermionic universality class can be computed within an $ε$ expansion around the lower critical space-time dimension of two. This approach is complementary to the previously studied expansion around the upper critical dimension of four. The crucial technical novelty near the lower critical dimension is the presence of different four-fermion interaction channels at the critical point, which we take into account in a Fierz-complete way. By interpolating between the lower and upper critical dimensions, we obtain improved estimates for the critical exponents in 2+1 space-time dimensions. For the situation relevant to single-layer graphene, we find an unusually small leading-correction-to-scaling exponent, arising from the competition between different interaction channels. This suggests that corrections to scaling may need to be taken into account when comparing analytical estimates with numerical data from finite-size extrapolations.

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Marginal Fermi liquid at magnetic quantum criticality from dimensional confinement

Metallic quantum criticality is frequently discussed as a source for non-Fermi liquid behavior, but controlled theoretical treatments are scarce. Here we identify and study a novel magnetic quantum critical point in a two-dimensional antiferromagnet coupled to a three-dimensional environment of conduction electrons. Using sign-problem-free quantum Monte Carlo simulations and an effective field-theory analysis, we demonstrate that the quantum critical point is characterized by marginal Fermi liquid behavior. In particular, we compute the electrical resistivity for transport across the magnetic layer, which is shown to display a linear temperature dependence at criticality. Experimental realizations in Kondo heterostructures are discussed.

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Nematic Quantum Criticality in Dirac Systems

We investigate nematic quantum phase transitions in two different Dirac fermion models. The models feature twofold and fourfold, respectively, lattice rotational symmetries that are spontaneously broken in the ordered phase. Using negative-sign-free quantum Monte Carlo simulations and an $ε$-expansion renormalization group analysis, we show that both models exhibit continuous phase transitions. In contrast to generic Gross-Neveu dynamical mass generation, the quantum critical regime is characterized by large velocity anisotropies, with fixed-point values being approached very slowly. Hence both experimental and numerical investigations will not be representative of the infrared fixed point, but of a crossover regime characterized by drifting exponents.

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Metallic and Deconfined Quantum Criticality in Dirac Systems

Motivated by the physics of spin-orbital liquids, we study a model of interacting Dirac fermions on a bilayer honeycomb lattice at half filling, featuring an explicit global SO(3)$\times$U(1) symmetry. Using large-scale auxiliary-field quantum Monte Carlo (QMC) simulations, we locate two zero-temperature phase transitions as function of increasing interaction strength. First, we observe a continuous transition from the weakly-interacting semimetal to a different semimetallic phase in which the SO(3) symmetry is spontaneously broken and where two out of three Dirac cones acquire a mass gap. The associated quantum critical point can be understood in terms of a Gross-Neveu-SO(3) theory. Second, we subsequently observe a transition towards an insulating phase in which the SO(3) symmetry is restored and the U(1) symmetry is spontaneously broken. While strongly first order at the mean-field level, the QMC data is consistent with a direct and continuous transition. It is thus a candidate for a new type of deconfined quantum critical point that features gapless fermionic degrees of freedom.

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Phase diagrams of SO($N$) Majorana-Hubbard models: Dimerization, internal symmetry breaking, and fluctuation-induced first-order transitions

We study the zero-temperature phase diagrams of Majorana-Hubbard models with SO($N$) symmetry on two-dimensional honeycomb and $π$-flux square lattices, using mean-field and renormalization group approaches. The models can be understood as real counterparts of the SU($N$) Hubbard-Heisenberg models, and may be realized in Abrikosov vortex phases of topological superconductors, or in fractionalized phases of strongly-frustrated spin-orbital magnets. In the weakly-interacting limit, the models feature stable and fully symmetric Majorana semimetal phases. Increasing the interaction strength beyond a finite threshold for large $N$, we find a direct transition towards dimerized phases, which can be understood as staggered valence bond solid orders, in which part of the lattice symmetry is spontaneously broken and the Majorana fermions acquire a mass gap. For small to intermediate $N$, on the other hand, phases with spontaneously broken SO($N$) symmetry, which can be understood as generalized Néel antiferromagnets, may be stabilized. These antiferromagnetic phases feature fully gapped fermion spectra for even $N$, but gapless Majorana modes for odd $N$. While the transitions between Majorana semimetal and dimerized phases are strongly first order, the transitions between Majorana semimetal and antiferromagnetic phases are continuous for small $N \leq 3$ and weakly first order for intermediate $N \geq 4$. The weakly-first-order nature of the latter transitions arises from fixed-point annihilation in the corresponding effective field theory, which contains a real symmetric tensorial order parameter coupled to the gapless Majorana degrees of freedom, realizing interesting examples of fluctuation-induced first-order transitions.

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Nesting instability of gapless U(1) spin liquids with spinon Fermi pockets in two dimensions

Quantum spin liquids are exotic states of matter that may be realized in frustrated quantum magnets and feature fractionalized excitations and emergent gauge fields. Here, we consider a gapless U(1) spin liquid with spinon Fermi pockets in two spatial dimensions. Such a state appears to be the most promising candidate to describe the exotic field-induced behavior observed in numerical simulations of the antiferromagnetic Kitaev honeycomb model. A similar such state may also be responsible for the recently-reported quantum oscillations of the thermal conductivity in the field-induced quantum paramagnetic phase of $α$-RuCl$_3$. We consider the regime close to a Lifshitz transition, at which the spinon Fermi pockets shrink to small circles around high-symmetry points in the Brillouin zone. By employing renormalization group and mean-field arguments, we demonstrate that interactions lead to a gap opening in the spinon spectrum at low temperatures, which can be understood as a nesting instability of the spinon Fermi surface. This leads to proliferation of monopole operators of the emergent U(1) gauge field and confinement of spinons. While signatures of fractionalization may be observable at finite temperatures, the gapless U(1) spin liquid state with nested spinon Fermi pockets is ultimately unstable at low temperatures towards a conventional long-range-ordered ground state, such as a valence bond solid. Implications for Kitaev materials in external magnetic fields are discussed.

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Gross-Neveu-Heisenberg criticality from competing nematic and antiferromagnetic orders in bilayer graphene

We study the phase diagram of an effective model of competing nematic and antiferromagnetic orders of interacting electrons on the Bernal-stacked honeycomb bilayer, as relevant for bilayer graphene. In the noninteracting limit, the model features a semimetallic ground state with quadratic band touching points at the Fermi level. Taking the effects of short-range interactions into account, we demonstrate the existence of an extended region in the mean-field phase diagram characterized by coexisting nematic and antiferromagnetic orders. By means of a renormalization group approach, we reveal that the quantum phase transition from nematic to coexistent nematic-antiferromagnetic orders is continuous and characterized by emergent Lorentz symmetry. It falls into the $(2+1)$-dimensional relativistic Gross-Neveu-Heisenberg quantum universality class, which has recently been much investigated in the context of interacting Dirac systems in two spatial dimensions. The coexistence-to-antiferromagnetic transition, by contrast, turns out to be weakly first order as a consequence of the absence of continuous spatial rotational symmetry on the honeycomb bilayer. Implications for experiments in bilayer graphene are discussed.

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Fractionalized quantum criticality in spin-orbital liquids from field theory beyond the leading order

Two-dimensional spin-orbital magnets with strong exchange frustration have recently been predicted to facilitate the realization of a quantum critical point in the Gross-Neveu-SO(3) universality class. In contrast to previously known Gross-Neveu-type universality classes, this quantum critical point separates a Dirac semimetal and a long-range-ordered phase, in which the fermion spectrum is only partially gapped out. Here, we characterize the quantum critical behavior of the Gross-Neveu-SO(3) universality class by employing three complementary field-theoretical techniques beyond their leading orders. We compute the correlation-length exponent $ν$, the order-parameter anomalous dimension $η_ϕ$, and the fermion anomalous dimension $η_ψ$ using a three-loop $ε$ expansion around the upper critical space-time dimension of four, a second-order large-$N$ expansion (with the fermion anomalous dimension obtained even at the third order), as well as a functional renormalization group approach in the improved local potential approximation. For the physically relevant case of $N=3$ flavors of two-component Dirac fermions in 2+1 space-time dimensions, we obtain the estimates $1/ν= 1.03(15)$, $η_ϕ= 0.42(7)$, and $η_ψ= 0.180(10)$ from averaging over the results of the different techniques, with the displayed uncertainty representing the degree of consistency among the three methods.

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Field-induced intermediate ordered phase and anisotropic interlayer interactions in $α$-RuCl$_3$

In $α$-RuCl$_3$, an external magnetic field applied within the honeycomb plane can induce a transition from a magnetically ordered state to a disordered state that is potentially related to the Kitaev quantum spin liquid. In zero field, single crystals with minimal stacking faults display a low-temperature state with in-plane zigzag antiferromagnetic order and a three-layer periodicity in the direction perpendicular to the honeycomb planes. Here, we present angle-dependent magnetization, ac susceptibility, and thermal transport data that demonstrate the presence of an additional intermediate-field ordered state at fields below the transition to the disordered phase. Neutron diffraction results show that the magnetic structure in this phase is characterized by a six-layer periodicity in the direction perpendicular to the honeycomb planes. Theoretically, the intermediate ordered phase can be accounted for by including spin-anisotropic couplings between the layers in a three-dimensional spin model. Together, this demonstrates the importance of interlayer exchange interactions in $α$-RuCl$_3$.

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Flux crystals, Majorana metals, and flat bands in exactly solvable spin-orbital liquids

Spin-orbital liquids are quantum disordered states in systems with entangled spin and orbital degrees of freedom. We study exactly solvable spin-orbital models in two dimensions with selected Heisenberg-, Kitaev-, and $Γ$-type interactions, as well as external magnetic fields. These models realize a variety of spin-orbital-liquid phases featuring dispersing Majorana fermions with Fermi surfaces, nodal Dirac or quadratic band touching points, or full gaps. In particular, we show that Zeeman magnetic fields can stabilize nontrivial flux patterns and induce metamagnetic transitions between states with different topological character. Solvable nearest-neighbor biquadratic spin-orbital perturbations can be tuned to stabilize zero-energy flat bands. We discuss in detail the examples of $\mathrm{SO}(2)$- and $\mathrm{SO}(3)$-symmetric spin-orbital models on the square and honeycomb lattices, and use group-theoretical arguments to generalize to $\mathrm{SO}(ν)$-symmetric models with arbitrary integer $ν> 1$. These results extend the list of exactly solvable models with spin-orbital-liquid ground states and highlight the intriguing general features of such exotic phases. Our models are thus excellent starting points for more realistic modellings of candidate materials.

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Antiferromagnetic critical point on graphene's honeycomb lattice: A functional renormalization group approach

Electrons on the half-filled honeycomb lattice are expected to undergo a direct continuous transition from the semimetallic into the antiferromagnetic insulating phase with increase of on-site Hubbard repulsion. We attempt to further quantify the critical behavior at this quantum phase transition by means of functional renormalization group (RG), within an effective Gross-Neveu-Yukawa theory for an SO(3) order parameter ("chiral Heisenberg universality class"). Our calculation yields an estimate of the critical exponents $ν\simeq 1.31$, $η_ϕ\simeq 1.01$, and $η_Ψ\simeq 0.08$, in reasonable agreement with the second-order expansion around the upper critical dimension. To test the validity of the present method we use the conventional Gross-Neveu-Yukawa theory with Z(2) order parameter ("chiral Ising universality class") as a benchmark system. We explicitly show that our functional RG approximation in the sharp-cutoff scheme becomes one-loop exact both near the upper as well as the lower critical dimension. Directly in 2+1 dimensions, our chiral-Ising results agree with the best available predictions from other methods within the single-digit percent range for $ν$ and $η_ϕ$ and the double-digit percent range for $η_Ψ$. While one would expect a similar performance of our approximation in the chiral Heisenberg universality class, discrepancies with the results of other calculations here are more significant. Discussion and summary of various approaches is presented.

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Fractionalized fermionic quantum criticality in spin-orbital Mott insulators

We study transitions between topological phases featuring emergent fractionalized excitations in two-dimensional models for Mott insulators with spin and orbital degrees of freedom. The models realize fermionic quantum critical points in fractionalized Gross-Neveu$^\ast$ universality classes in (2+1) dimensions. They are characterized by the same set of critical exponents as their ordinary Gross-Neveu counterparts, but feature a different energy spectrum, reflecting the nontrivial topology of the adjacent phases. We exemplify this in a square-lattice model, for which an exact mapping to a $t$-$V$ model of spinless fermions allows us to make use of large-scale numerical results, as well as in a honeycomb-lattice model, for which we employ $ε$-expansion and large-$N$ methods to estimate the critical behavior. Our results are potentially relevant for Mott insulators with $d^1$ electronic configurations and strong spin-orbit coupling, or for twisted bilayer structures of Kitaev materials.

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Microscopic models for Kitaev's sixteenfold way of anyon theories

In two dimensions, the topological order described by $\mathbb{Z}_2$ gauge theory coupled to free or weakly interacting fermions with a nonzero spectral Chern number $ν$ is classified by $ν\; \mathrm{mod}\; 16$ as predicted by Kitaev [Ann. Phys. 321, 2 (2006)]. Here we provide a systematic and complete construction of microscopic models realizing this so-called sixteenfold way of anyon theories. These models are defined by $Γ$ matrices satisfying the Clifford algebra, enjoy a global $\mathrm{SO}(ν)$ symmetry, and live on either square or honeycomb lattices depending on the parity of $ν$. We show that all these models are exactly solvable by using a Majorana representation and characterize the topological order by calculating the topological spin of an anyonic quasiparticle and the ground-state degeneracy. The possible relevance of the $ν=2$ and $ν=3$ models to materials with Kugel-Khomskii-type spin-orbital interactions is discussed.

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