arXiv subjects

Luke Caldwell

Publications and source records attributed to Luke Caldwell.

7 recordsLinked to original sources

arXiv2026

Near-deterministic loading of optical tweezer arrays via repulsive barricade potentials

Optical tweezers are a powerful tool for creating defect-free arrays of atoms and molecules, enabling advances in quantum simulation, computation, and precision metrology. However, the achievable array size is limited by the initial loading fraction, typically $50\,\%$ for atoms and $35\,\%$ for molecules. Here, we propose a general scheme for enabling multiple loading cycles by protecting trapped particles using a repulsive barrier. We show that collision-limited lifetimes of particles in protected tweezers can exceed one second, leading to filling fractions of over $80\%$ after four loading cycles. Combined with existing rearrangement techniques, this approach enables efficient unity filling of tweezer arrays and provides a scalable pathway towards larger quantum technology platforms.

physics.atom-ph↗

arXiv2023

Opportunities for Fundamental Physics Research with Radioactive Molecules

Molecules containing short-lived, radioactive nuclei are uniquely positioned to enable a wide range of scientific discoveries in the areas of fundamental symmetries, astrophysics, nuclear structure, and chemistry. Recent advances in the ability to create, cool, and control complex molecules down to the quantum level, along with recent and upcoming advances in radioactive species production at several facilities around the world, create a compelling opportunity to coordinate and combine these efforts to bring precision measurement and control to molecules containing extreme nuclei. In this manuscript, we review the scientific case for studying radioactive molecules, discuss recent atomic, molecular, nuclear, astrophysical, and chemical advances which provide the foundation for their study, describe the facilities where these species are and will be produced, and provide an outlook for the future of this nascent field.

nucl-ex↗

arXiv2022

A new bound on the electron's electric dipole moment

The Standard Model cannot explain the dominance of matter over anti-matter in our universe. This imbalance indicates undiscovered physics that violates combined CP symmetry. Many extensions to the Standard Model seek to explain the imbalance by predicting the existence of new particles. Vacuum fluctuations of the fields associated with these new particles can interact with known particles and make small modifications to their properties; for example, particles which violate CP symmetry will induce an electric dipole moment of the electron (eEDM). The size of the induced eEDM is dependent on the masses of the new particles and their coupling to the Standard Model. To date, no eEDM has been detected, but increasingly precise measurements probe new physics with higher masses and weaker couplings. Here we present the most precise measurement yet of the eEDM using electrons confined inside molecular ions, subjected to a huge intra-molecular electric field, and evolving coherently for up to 3 s. Our result is consistent with zero and improves on the previous best upper bound by a factor $\sim2.4$. Our sensitivity to $10^{-19}$ eV shifts in molecular ions provides constraints on broad classes of new physics above $10^{13}$ eV, well beyond the direct reach of the LHC or any other near- or medium-term particle collider.

physics.atom-ph↗

arXiv2022

Systematic and statistical uncertainty evaluation of the HfF$^+$ electron electric dipole moment experiment

We have completed a new precision measurement of the electron's electric dipole moment using trapped HfF$^+$ in rotating bias fields. We report on the accuracy evaluation of this measurement, describing the mechanisms behind our systematic shifts. Our systematic uncertainty is reduced by a factor of 30 compared to the first generation of this measurement. Our combined statistical and systematic accuracy is improved by a factor of 2 relative to any previous measurement.

physics.atom-ph↗

arXiv2022

Evidence of Two-Source King Plot Nonlinearity in Spectroscopic Search for New Boson

Optical precision spectroscopy of isotope shifts can be used to test for new forces beyond the Standard Model, and to determine basic properties of atomic nuclei. We measure isotope shifts on the highly forbidden ${}^2S_{1/2} \rightarrow {}^2F_{7/2}$ octupole transition of trapped $^{168,170,172,174,176}$Yb ions. When combined with previous measurements in Yb$^+$ and very recent measurements in Yb, the data reveal a King plot nonlinearity of up to 240$σ$. The trends exhibited by experimental data are explained by nuclear density functional theory calculations with the Fayans functional. We also find, with 4.3$σ$ confidence, that there is a second distinct source of nonlinearity, and discuss its possible origin.

physics.atom-ph↗

arXiv2022

Spectroscopy on the eEDM-sensitive states of ThF$^+$

An excellent candidate molecule for the measurement of the electron's electric dipole moment (eEDM) is thorium monofluoride (ThF$^+$) because the eEDM-sensitive state, $^3Δ_1$, is the electronic ground state, and thus is immune to decoherence from spontaneous decay. We perform spectroscopy on $X\,^3Δ_1$ to extract three spectroscopic constants crucial to the eEDM experiment: the hyperfine coupling constant, the molecular frame electric dipole moment, and the magnetic $g$-factor. To understand the impact of thermal blackbody radiation on the vibrational ground state, we study the lifetime of the first excited vibrational manifold of $X\,^3Δ_1$. We perform ab initio calculations, compare them to our results, and discuss prospects for using ThF$^+$ in a new eEDM experiment at JILA.

physics.atom-ph↗

arXiv2018

Ultracold molecules for quantum simulation: rotational coherences in CaF and RbCs

We explore the uses of ultracold molecules as a platform for future experiments in the field of quantum simulation, focusing on two molecular species, $^{40}$Ca$^{19}$F and $^{87}$Rb$^{133}$Cs. We report the development of coherent quantum state control using microwave fields in both molecular species; this is a crucial ingredient for many quantum simulation applications. We demonstrate proof-of-principle Ramsey interferometry measurements with fringe spacings of $\sim 1~\rm kHz$ and investigate the dephasing time of a superposition of $N=0$ and $N=1$ rotational states when the molecules are confined. For both molecules, we show that a judicious choice of molecular hyperfine states minimises the impact of spatially varying transition-frequency shifts across the trap. For magnetically trapped $^{40}$Ca$^{19}$F we use a magnetically insensitive transition and observe a coherence time of 0.61(3) ms. For optically trapped $^{87}$Rb$^{133}$Cs we exploit an avoided crossing in the AC Stark shift and observe a maximum coherence time of 0.75(6) ms.

cond-mat.quant-gas↗