arXiv subjects

Lunyong Zhang

Publications and source records attributed to Lunyong Zhang.

13 recordsLinked to original sources

arXiv2023

Giant magnetocaloric effect and hysteresis loss in Mn$_x$Fe$_{2-x}$P$_{0.5}$Si$_{0.5}$ ($x$ = 0.7-1.2) microwires at ambient temperatures

Magnetocaloric microwires are very promising for energy-efficient magnetic refrigeration in micro electromechanical systems (MEMS) and nano electromechanical systems (NEMS). Creating microwires that exhibit large magnetocaloric effects around room temperature represents an important but challenging task. Here, we report a tunable giant magnetocaloric effect around room temperature in Mn$_x$Fe$_{2-x}$P$_{0.5}$Si$_{0.5}$ ($x$ = 0.7-1.2) microwires by utilizing a melt-extraction technique paired with thermal treatment and chemical engineering. The isothermal magnetic entropy change DeltaSiso and Curie temperature (TC) can be tuned by adjusting the Mn/Fe ratio. The TC varies from 351 to 190 K as x increases from 0.8 to 1.2. Among the compositions investigated, the x = 0.9 sample shows the largest value of DeltaSiso = 18.3 J kg$^{-1}$ K$^{-1}$ for a field change of 5 T around 300 K. After subtracting magnetic hysteresis loss, a large refrigerant capacity of ~284.6 J kg$^{-1}$ is achieved. Our study paves a new pathway for the design of novel magnetocaloric microwires for active magnetic refrigeration at ambient temperatures.

physics.app-ph↗

arXiv2023

Topological Magnetoresistance of Magnetic Skyrmionic Bubbles

Magnetic skyrmions offer promising prospects for constructing future energy-efficient and high-density information technology, leading to extensive explorations of new skyrmionic materials recently. The topological Hall effect has been widely adopted as a distinctive marker of skyrmion emergence. Alternately, here we propose a novel signature of skyrmion state by quantitatively investigating the magnetoresistance (MR) induced by skyrmionic bubbles in CeMn2Ge2. An intriguing finding was revealed: the anomalous MR measured at different temperatures can be normalized into a single curve, regardless of sample thickness. This behavior can be accurately reproduced by the recent chiral spin textures MR model. Further analysis of the MR anomaly allowed us to quantitatively examine the effective magnetic fields of various scattering channels. Remarkably, the analyses, combined with the Lorentz transmission electronic microscopy results, indicate that the in-plane scattering channel with triplet exchange interactions predominantly governs the magnetotransport in the Bloch-type skyrmionic bubble state. Our results not only provide insights into the quantum correction on MR induced by skyrmionic bubble phase, but also present an electrical probing method for studying chiral spin texture formation, evolution and their topological properties, which opens up exciting possibilities for identifying new skyrmionic materials and advancing the methodology for studying chiral spin textures.

cond-mat.mtrl-sci↗

arXiv2021

A perspective magnetic bed comprising Gd alloy multi-microwires for energy-efficient magnetic refrigeration

We have designed a new magnetic bed structure with desirable table-like magnetocaloric effect (MCE) by using three kinds of soft ferromagnetic Gd-Al-Co microwire arrays with different Curie temperatures ($T_C$). The $T_C$ interval of these three wires is ~10 K and the designed new structure named Sample A. This sample shows a smooth table-like magnetic entropy change ($ΔS_M$) at high applied field change ($μ_0 ΔH=5 T$) ranging from ~92 K to ~107 K. The maximum entropy change ($-ΔS_M^{\rm max}$) and refrigerant capacity (RC) for Sample A at $μ_0 ΔH=5 T$ are calculated to be ~9.42 Jkg$^{-1}$K$^{-1}$ and ~676 Jkg$^{-1}$. The calculated curves of $-ΔS_M(T)$ and the corresponding experimental data match well with each other, suggesting that the desirable magnetocaloric properties of the microwire arrays can be designed. Simulation shows that the RC values of the designed systems increase when increasing the interval of $T_C$. The table-like MCE and the enhanced heat-transfer efficiency due to the enhanced surface areas of the microwires make this newly designed magnetic bed very promising for use in energy-efficient magnetic refrigerators.

physics.app-ph↗

arXiv2021

Evolution of topological defects at two sequential phase transitions of Nd2SrFe2O7

How topological defects, unavoidable at symmetry-breaking phase transitions in a wide range of systems, evolve through consecutive phase transitions with different broken symmetries remains unexplored. Nd2SrFe2O7, a bilayer ferrite, exhibits two intriguing structural phase transitions and dense networks of the so-called type-II Z8 structural vortices at room temperature, so it is an ideal system to explore the topological defect evolution. From our extensive experimental investigation, we demonstrate that the cooling rate at the second-order transition (1290oC) plays a decisive role in determining the vortex density at room temperature, following the universal Kibble-Zurek mechanism. In addition, we discovered a transformation between topologically-distinct vortices (Z8 to Z4 vortices) at the first-order transition (550oC), which conserves the number of vortex cores. Remarkably, the Z4 vortices consist of two phases with an identical symmetry but two distinct magnitudes of an order parameter. Furthermore, when lattice distortion is enhanced by chemical doping, a new type of topological defects emerges: loop domain walls with orthorhombic distortions in the tetragonal background, resulting in unique pseudo-orthorhombic twins. Our findings open a new avenue to explore the evolution of topological defects through multiple phase transitions.

cond-mat.other↗

arXiv2020

Magnetic phase transitions and spin density distribution in the molecular multiferroic GaV$_4$S$_8$ system

We have carried out neutron diffraction and small angle neutron scattering measurements on a high quality single crystal of the cubic lacunar spinel multiferroic, GaV$_4$S$_8$, as a function of magnetic field and temperature to determine the magnetic properties for the single electron that is located on the tetrahedrally coordinated V$_4$ molecular unit. Our results are in good agreement with the structural transition at 44 K from cubic to rhombohedral symmetry where the system becomes a robust ferroelectric, while long range magnetic order develops below 13 K in the form of an incommensurate cycloidal magnetic structure, which can transform into a Néel-type skyrmion phase in a modest applied magnetic field. Below 5.9(3) K, the crystal enters a ferromagnetic phase, and we find the magnetic order parameter indicates a long range ordered ground state with an ordered moment of 0.23(1) $μ_\mathrm{B}$ per V ion. Both polarized and unpolarized neutron data in the ferroelectric-paramagnetic phase have been measured to determine the magnetic form factor. The data are consistent with a model of the single spin being uniformly distributed across the V$_4$ molecular unit, rather than residing on the single apical V ion, in substantial agreement with the results of first-principles theory. In the magnetically ordered state, polarized neutron measurements are important since both the cycloidal and ferromagnetic order parameters are clearly coupled to the ferroelectricity, causing the structural peaks to be temperature and field dependent. For the ferromagnetic ground state, the spins are locked along the $[1,1,1]$ direction by a surprisingly large anisotropy.

cond-mat.str-el↗

arXiv2019

Origin of Ising magnetism in Ca3Co2O6 unveiled by orbital imaging

The one-dimensional cobaltate Ca3Co2O6 is an intriguing material having an unconventional magnetic structure, displaying quantum tunneling phenomena in its magnetization. Using a newly developed experimental method, s-core-level non-resonant inelastic x-ray scattering (s-NIXS), we were able to image the atomic Co 3d orbital that is responsible for the Ising magnetism in this system. We show that we can directly observe that it is the complex d2 orbital occupied by the sixth electron at the high-spin Co-trig{3+} (d6) sites that generates this behavior. This is extremely rare in the research field of transition metal compounds, and is only made possible by the delicately balanced prismatic trigonal coordination. The ability to directly relate the orbital occupation with the local crystal structure is essential to model the magnetic properties of this system.

cond-mat.str-el↗

arXiv2019

Polar and phase domain walls with conducting interfacial states in a Weyl semimetal MoTe2

Much of the dramatic growth in research on topological materials has focused on topologically protected surface states. While the domain walls of topological materials such as Weyl semimetals with broken inversion or time-reversal symmetry can provide a hunting ground for exploring topological interfacial states, such investigations have received little attention to date. Here, utilizing in-situ cryogenic transmission electron microscopy combined with first-principles calculations, we discover intriguing domain-wall structures in MoTe2, both between polar variants of the low-temperature(T) Weyl phase, and between this and the high-T high-order topological phase. We demonstrate how polar domain walls can be manipulated with electron beams and show that phase domain walls tend to form superlattice-like structures along the c axis. Scanning tunneling microscopy indicates a possible signature of a conducting hinge state at phase domain walls. Our results open avenues for investigating topological interfacial states and unveiling multifunctional aspects of domain walls in topological materials.

cond-mat.mtrl-sci↗

arXiv2017

Temperature-Driven Topological Transition in 1T'-MoTe2

The topology of Weyl semimetals requires the existence of unique surface states. Surface states have been visualized in spectroscopy measurements, but their connection to the topological character of the material remains largely unexplored. 1T'-MoTe2, presents a unique opportunity to study this connection. This material undergoes a phase transition at 240K that changes the structure from orthorhombic (putative Weyl semimetal) to monoclinic (trivial metal), while largely maintaining its bulk electronic structure. Here we show from temperature-dependent quasiparticle interference measurements that this structural transition also acts as a topological switch for surface states in 1T'-MoTe2. At low temperature, we observe strong quasiparticle scattering, consistent with theoretical predictions and photoemission measurements for the surface states in this material. In contrast, measurements performed at room temperature show the complete absence of the scattering wavevectors associated with the trivial surface states. These distinct quasiparticle scattering behaviors show that 1T'-MoTe2 is ideal for separating topological and trivial electronic phenomena via temperature dependent measurements.

cond-mat.mtrl-sci↗

arXiv2017

Quasiparticle Interference of Surface States in Type-II Weyl Semimetal WTe$_2$

Topological Weyl semimetal (TWS) is a metal, where low energy excitations behave like Weyl fermions of high-energy physics. It was recently shown that due to the lower symmetry of condensed matter systems, they can realize two distinct types of Weyl fermions. The type-I Weyl fermion in a metal is formed by a linear crossing of two bands at a point in the crystalline momentum space - Brillouin zone (BZ). The second type TWSs host type-II Weyl points appearing at the touching points of electron and hole pockets, which is a result of tilted linear dispersion. The type-II TWS was predicted to exist in several compounds, including WTe$_2$. Several ARPES studies of WTe$_2$ were reported so far, having contradictory conclusions on the topological nature of observed Fermi arcs. In this work, we report the results of spectroscopic imaging with a scanning tunneling microscope and first principle calculations, establishing a clear quasiparticle interference features of the surface states of WTe$_2$. Our work provides a strong evidence for surface state scattering. Although the surface Fermi arcs are clearly observed, it is still difficult to prove the existence of predicted Type-II Weyl points in the bulk.

cond-mat.str-el↗

arXiv2017

Review of Spin Orbit Coupled Semimetal SrIrO3 in thin film form

Spin orbit coupling provides a mechanism to lock the momentum of electron to its spin degree, recent years was revealed to be essential in arousing many novel physical behaviors. SrIrO3 is a typical metallic member of the strong spin orbit coupling iridate family. Its orthorhombic phase was confirmed as a particular spin orbit coupling assistant electron correlated semimetal with small electron and hole pockets, and was supposed to host versatile topological phases, with prospect of opening a new topological matter field based on oxides. The existing experiments have demonstrated that orthorhombic SrIrO3 can be easily synthesized at two dimensional scale films under the substrate lattice constraint, and the films display Fermi-liquid behavior in high temperature and generally two dimensional weak localization resulted metal insulator transition. The properties of orthorhombic SrIrO3 film are sensitive to the rotation and tilting angle, as well as the interlayer coupling of the IrO6 octahedras, consequently can be tuned through substrate strain engineering and size scale. For example, the film was approached a state similar to Sr2IrO4 at the ultrathin limit to several unit cell, becoming a canted antiferromagnetic semiconductor/insulator. The existing knowledges suggest urgent demands of researches on the superlattices constructed with orthorhombic SrIrO3, for further understanding the evolution mechanism of the electron structure, and so the relevant magnetic state and topological phases in the orthorhombic SrIrO3 and its family.

cond-mat.mtrl-sci↗

arXiv2016

Chiral Ordering Spin Associated Glass like State in SrRuO3SrIrO3 Superlattice

Heterostructure interface provides a powerful platform to observe rich emergent phenomena, such as interfacial superconductivity, nontrivial topological surface state. Here SrRuO3/SrIrO3 superlattices were epitaxially synthesized. The magnetic and electrical properties of these superlattices were characterized. Broad cusps in the zero field cooling magnetization curves and near stable residual magnetization below the broad cusps, as well as two steps magnetization hysteresis loops are observed. The magnetization relaxes following a modified Stretched function model indicating coexistence of spin glass and ferromagnetic ordering in the superlattices. Topological Hall effect was demonstrated at low temperature and weakened with the increase of SrIrO3 layer thickness. These results suggest that chiral ordering spin texture were generated at the interfaces due to the interfacial Dzyaloshinskii-Moriya (DM) interaction, which generates the spin glass behaviors. The present work demonstrates that SrIrO3 can effectively induce interface DM interactions in heterostructures, it would pave light on the new research directions of strong spin orbit interaction oxides, from the viewpoints of both basic science and prospective spintronics devices applications.

cond-mat.mtrl-sci↗

arXiv2014

Tunable Semimetallic State in Compressive-strained SrIrO3 Films Revealed by Transport Behaviors

Orthorhombic SrIrO3 is a typical spin-orbit-coupling correlated metal that shows diversified physical properties under the external stimuli. Here nonlinear Hall effect and weakly temperature-dependent resistance are observed in a SrIrO3 film epitaxially grown on SrTiO3 substrate. It infers that orthorhombic SrIrO3 is a semimetal oxide. However, linear Hall effect and insensitive-temperature-dependent resistance are observed in SrIrO3 films grown on (La,Sr)(Al,Ta)O3 (LSAT) substrates, suggesting a tunable semimetallic state due to band structure change in SrIrO3 films under different compressive strain. The mechanism of this evolution is explored in detail through strain-state analysis by reciprocal space mapping and electron diffraction, carrier density and mobility calculations, as well as electronic band structure evolution under compressive strain (predicted by tight-binding approximation). It might suggest that the strain-induced band shift leads to the semimetallic tuning in the SrIrO3 film grown on from SrTiO3 to LSAT substrates. Our findings illustrate the tunability of SrIrO3 properties and pave the way to induce novel physical states in SrIrO3 such as the proposed topological insulator state in heterostructures.

cond-mat.mtrl-sci↗

arXiv2013

Sensitively Temperature-Dependent Spin Orbit Coupling in SrIrO3 Thin Films

Spin orbit coupling plays a non-perturbation effect in many recently developed novel fields including topological insulators and spin-orbit assistant Mott insulators. In this paper, strongly temperature-dependent spin orbit coupling, revealed by weak anti-localization, is observed at low temperature in 5d strongly correlated compound, SrIrO3. As the temperature rising, increase rate of Rashba coefficient is nearly 30%-45%/K. The increase is nearly 100 times over that observed in semiconductor heterostructures. Microscopically, the large increase of Rashba coefficient is attributed to the significant evolution of effective Landé g factor on temperature, whose mechanism is discussed. Sensitively temperature-dependent spin orbit coupling in SrIrO3 might be applied in spintronic devices

cond-mat.mtrl-sci↗