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Lykourgos Bougas

Publications and source records attributed to Lykourgos Bougas.

At least 19 recordsLinked to original sources

Rapid parameter estimation of discrete decaying signals using autoencoder networks

In this work we demonstrate the use of neural networks for rapid extraction of signal parameters of discretely sampled signals. In particular, we use dense autoencoder networks to extract the parameters of interest from exponentially decaying signals and decaying oscillations. By using a three-stage training method and careful choice of the neural network size, we are able to retrieve the relevant signal parameters directly from the latent space of the autoencoder network at significantly improved rates compared to traditional algorithmic signal-analysis approaches. We show that the achievable precision and accuracy of this method of analysis is similar to conventional algorithm-based signal analysis methods, by demonstrating that the extracted signal parameters are approaching their fundamental parameter estimation limit as provided by the Cramér-Rao bound. Furthermore, we demonstrate that autoencoder networks are able to achieve signal analysis, and, hence, parameter extraction, at rates of 75 kHz, orders-of-magnitude faster than conventional techniques with similar precision. Finally, we explore the limitations of our approach, demonstrating that analysis rates of $>$200 kHz are feasible with further optimization of the transfer rate between the data-acquisition system and data-analysis system.

eess.SP↗

Chiral sensing with achiral anisotropic metasurfaces

Recently, we proposed a metasurface design for chiral sensing that (i) results in enhanced chiroptical signals by more than two orders of magnitude for ultrathin, subwavelength, chiral samples over a uniform and accessible area, (ii) allows for complete measurements of the total chirality (magnitude and sign of both its real and imaginary part), and (iii) offers the possibility for a crucial signal reversal (excitation with reversed polarization) that enables chirality measurements in an absolute manner, i.e., without the need for sample removal. Our design is based on the anisotropic response of the metasurface, rather than the superchirality of the generated near-fields, as in most contemporary nanophotonic-based chiral sensing approaches. Here, we derive analytically, and verify numerically, simple formulas that provide insight to the sensing mechanism and explain how anisotropic metasurfaces, in general, offer additional degrees of freedom with respect to their isotropic counterparts. We provide a detailed discussion of the key functionalities and benefits of our proposed design and we demonstrate practical measurement schemes for the unambiguous determination of an unknown chirality. Last, we provide the design principles towards broadband operation - from near-infrared to near-ultraviolet frequencies - opening the way for highly sensitive nanoscale chiroptical spectroscopy.

physics.optics↗

Rapid parameter determination of discrete damped sinusoidal oscillations

We present different computational approaches for the rapid extraction of the signal parameters of discretely sampled damped sinusoidal signals. We compare time- and frequency-domain-based computational approaches in terms of their accuracy and precision and computational time required in estimating the frequencies of such signals, and observe a general trade-off between precision and speed. Our motivation is precise and rapid analysis of damped sinusoidal signals as these become relevant in view of the recent experimental developments in cavity-enhanced polarimetry and ellipsometry, where the relevant time scales and frequencies are typically within the $\sim1-10\,μ$s and $\sim1-100$MHz ranges, respectively. In such experimental efforts, single-shot analysis with high accuracy and precision becomes important when developing experiments that study dynamical effects and/or when developing portable instrumentations. Our results suggest that online, running-fashion, microsecond-resolved analysis of polarimetric/ellipsometric measurements with fractional uncertainties at the $10^{-6}$ levels, is possible, and using a proof-of-principle experimental demonstration we show that using a frequency-based analysis approach we can monitor and analyze signals at kHz rates and accurately detect signal changes at microsecond time-scales.

physics.ins-det↗

Probing topological spin structures using light-polarization and magnetic microscopy

We present an imaging modality that enables detection of magnetic moments and their resulting stray magnetic fields. We use wide-field magnetic imaging that employs a diamond-based magnetometer and has combined magneto-optic detection (e.g. magneto-optic Kerr effect) capabilities. We employ such an instrument to image magnetic (stripe) domains in multilayered ferromagnetic structures.

cond-mat.mtrl-sci↗

Rapid online solid-state battery diagnostics with optically pumped magnetometers

Solid state battery technology is motivated by the desire to deliver flexible power storage in a safe and efficient manner. The increasingly widespread use of batteries from mass-production facilities highlights the need for a rapid and sensitive diagnostic for identifying battery defects. We demonstrate the use of atomic magnetometry to measure the magnetic fields around miniature solid-state battery cells. These fields encode information about battery manufacturing defects, state of charge, impurities, or can provide important insights into ageing processes. Compared with SQUID-based magnetometry, the availability of atomic magnetometers, however, highlights the possibility for a low-cost, portable, and flexible implementation of battery quality-control and characterization technology.

physics.app-ph↗

Action potentials induce biomagnetic fields in Venus flytrap plants

Upon stimulation, plants elicit electrical signals that can travel within a cellular network analogous to the animal nervous system. It is well-known that in the human brain, voltage changes in certain regions result from concerted electrical activity which, in the form of action potentials (APs), travels within nerve-cell arrays. Electrophysiological techniques like electroencephalography, magnetoencephalography, and magnetic resonance imaging are used to record this activity and to diagnose disorders. In the plant kingdom, two types of electrical signals are observed: all-or-nothing APs of similar amplitudes to those seen in humans and animals, and slow-wave potentials of smaller amplitudes. Sharp APs appear restricted to unique plant species like the "sensitive plant", Mimosa pudica, and the carnivorous Venus flytrap, Dionaea muscipula. Here we ask the question, is electrical activity in the Venus flytrap accompanied by distinct magnetic signals? Using atomic optically pumped magnetometers, biomagnetism in AP-firing traps of the carnivorous plant was recorded. APs were induced by heat stimulation, and the thermal properties of ion channels underlying the AP were studied. The measured magnetic signals exhibit similar temporal behavior and shape to the fast de- and repolarization AP phases. Our findings pave the way to understanding the molecular basis of biomagnetism, which might be used to improve magnetometer-based noninvasive diagnostics of plant stress and disease.

physics.bio-ph↗

Photoluminescence at the ground state level anticrossing of the nitrogen-vacancy center in diamond

The nitrogen-vacancy center (NV center) in diamond at magnetic fields corresponding to the ground state level anticrossing (GSLAC) region gives rise to rich photoluminescence (PL) signals due to the vanishing energy gap between the electron spin states, which enables to have an effect on the NV center's luminescence for a broad variety of environmental couplings. In this article we report on the GSLAC photoluminescence signature of NV ensembles in different spin environments at various external fields. We investigate the effects of transverse electric and magnetic fields, P1 centers, NV centers, and the $^{13}$C nuclear spins, each of which gives rise to a unique PL signature at the GSLAC. The comprehensive analysis of the couplings and related optical signal at the GSLAC provides a solid ground for advancing various microwave-free applications at the GSLAC, including but not limited to magnetometry, spectroscopy, dynamic nuclear polarization (DNP), and nuclear magnetic resonance (NMR) detection. We demonstrate that not only the most abundant $^{14}$NV center but the $^{15}$NV can also be utilized in such applications and that nuclear spins coupled to P1 centers can be polarized directly by the NV center at the GSLAC, through a giant effective nuclear $g$-factor arising from the NV center-P1 center-nuclear spin coupling. We report on new alternative for measuring defect concentration in the vicinity of NV centers and on the optical signatures of interacting, mutually aligned NV centers.

cond-mat.mes-hall↗

Continuous-Wave Cavity Ring-Down Polarimetry

We present a new cavity-based polarimetric scheme for highly sensitive and time-resolved measurements of birefringence and dichroism, linear and circular, that employs rapidly-pulsed single-frequency CW laser sources and extends current cavity-based spectropolarimetric techniques. We demonstrate how the use of a CW laser source allows for gains in spectral resolution, signal intensity and data acquisition rate compared to traditional pulsed-based cavity ring-down polarimetry (CRDP). We discuss a particular CW-CRDP modality that is different from intensity-based cavity-enhanced polarimetric schemes as it relies on the determination of the polarization-rotation frequency during a ring-down event generated by large intracavity polarization anisotropies. We present the principles of CW-CRDP and validate the applicability of this technique for measurement of the non-resonant Faraday effect in solid SiO$_2$ and CeF$_3$ and gaseous butane. We give a general analysis of the fundamental sensitivity limits for CRDP techniques and show how the presented frequency-based methodology alleviates the requirement for high finesse cavities to achieve high polarimetric sensitivities, and, thus, allows for the extension of cavity-based polarimetric schemes into different spectral regimes but most importantly renders the CW-CRDP methodology particularly suitable for robust portable polarimetric instrumentations.

physics.chem-ph↗

Absolute chiral sensing in dielectric metasurfaces with signal reversals

Sensing molecular chirality at the nanoscale has been a long-standing challenge due to the inherently weak nature of chiroptical signals, and nanophotonic approaches have proven fruitful in accessing these signals. However, in most cases, absolute chiral sensing of the total chiral refractive index has not been possible, while the strong inherent signals from the nanostructures themselves obscure the weak chiroptical signals. Here, we propose a dielectric metamaterial system that overcomes these limitations and allows for absolute measurements of the total chirality, and the possibility for a crucial signal reversal that enables chirality measurements without the need for sample removal. As proof of principle, we demonstrate signal-enhancements by a factor of 200 for ultrathin, sub-wavelength, chiral samples over a uniform and accessible area.

physics.app-ph↗

Noncovalent force spectroscopy using wide-field optical and diamond-based magnetic imaging

A realization of the force-induced remnant magnetization spectroscopy (FIRMS) technique of specific biomolecular binding is presented where detection is accomplished with wide-field optical and diamond-based magnetometry using an ensemble of nitrogen-vacancy (NV) color centers. The technique may be adapted for massively parallel screening of arrays of nanoscale samples.

physics.ins-det↗

A surface plasmon platform for angle-resolved chiral sensing

Chiral sensitive techniques have been used to probe the fundamental symmetries of the universe, study biomolecular structures, and even develop safe drugs. As chiral signals are inherently weak and often suppressed by large backgrounds, different techniques have been proposed to overcome the limitations of traditionally used chiral polarimetry. Here, we propose an angle-resolved chiral surface plasmon resonance (CHISPR) scheme that can detect the absolute chirality (handedness and magnitude) of a chiral sample and is sensitive to both the real and imaginary part of a chiral sample's refractive index. We present analytical results and numerical simulations of CHISPR measurements, predicting signals in the mdeg range for chiral samples of <100nm thickness at visible wavelengths. Moreover, we present a theoretical analysis that clarifies how our far-field measurements elucidate the underlying physics. This CHISPR protocol does not require elaborate fabrication and has the advantage of being directly implementable on existing surface plasmon resonance instrumentation.

physics.app-ph↗

Variable single-axis magnetic-field generator using permanent magnets

We present a design for producing precisely adjustable and alternating single-axis magnetic fields based on nested Halbach dipole pairs consisting of permanent magnets only. Our design allows for three dimensional optical and mechanical access to a region with strong adjustable dipolar fields, is compatible with systems operating under vacuum, and does not effectively dissipate heat under normal operational conditions. We present a theoretical analysis of the properties and capabilities of our design, and construct a proof-of-concept prototype. Using our prototype, we demonstrate fields of up to several kilogauss with field homogeneities of better than 5%, which are harmonically modulated at frequencies of $\sim$1Hz with a power consumption of approximately 1W. Moreover, we discuss how our design can be modified to generate adjustable quadrupolar magnetic fields with gradients as large as 9.5T/m in a region of optical and mechanical access. Our design is scalable and can be constructed to be suitable for table-top experiments, as in the case of polarimetric and magnetometric setups that require strong alternating magnetic fields, but also for large scale applications such as generators.

physics.ins-det↗

Infrared laser magnetometry with a NV doped diamond intracavity etalon

We propose an hybrid laser system consisting of a semiconductor external cavity laser associated to an intra-cavity diamond etalon doped with nitrogen-vacancy color centers. We consider laser emission tuned to the infrared absorption line that is enhanced under the magnetic field dependent nitrogen-vacancy electron spin resonance and show that this architecture leads to a compact solid-state magnetometer that can be operated at room-temperature. The sensitivity to the magnetic field limited by the photon shot-noise of the output laser beam is estimated to be around $250~\mathrm{fT/\sqrt{Hz}}$. Unlike usual NV center infrared magnetometry, this method would not require an external frequency stabilized laser. Since the proposed system relies on the competition between the laser threshold and an intracavity absorption, such laser-based optical sensor could be easily adapted to a broad variety of physical systems.

physics.optics↗

Eddy-current imaging with nitrogen-vacancy centers in diamond

We demonstrate microwave-free eddy-current imaging using nitrogen-vacancy centers in diamond. By detecting the eddy-current induced magnetic field of conductive samples, we can distinguish between different materials and shapes and identify structural defects. Our technique allows for the discrimination of different materials according to their conductivity. The sensitivity of the measurements is calculated as 8$\times 10 ^{5}$\,S/m\,$\sqrt[]{\textrm{Hz}}$ at 3.5\,MHz, for a cylindrical sample with radius $r_0$\,=\,1\,mm and height $h$\,=\,0.1\,mm (volume $\sim$\,0.3\,mm$^3$), at a distance of 0.5\,mm. In comparison with existing technologies, the diamond-based device exhibits a superior bandwidth and spatial resolution. In particular, we demonstrate a flat frequency response from DC to 3.5 MHz and a spatial resolution of 348\,$\pm$\,2\,$μ$m.

quant-ph↗

Diamond magnetic microscopy of malarial hemozoin nanocrystals

Magnetic microscopy of malarial hemozoin nanocrystals was performed using optically detected magnetic resonance imaging of near-surface diamond nitrogen-vacancy centers. Hemozoin crystals were extracted from $Plasmodium$-$falciparum$-infected human blood cells and studied alongside synthetic hemozoin crystals. The stray magnetic fields produced by individual crystals were imaged at room temperature as a function of applied field up to 350 mT. More than 100 nanocrystals were analyzed, revealing the distribution of their magnetic properties. Most crystals ($96\%$) exhibit a linear dependence of stray field magnitude on applied field, confirming hemozoin's paramagnetic nature. A volume magnetic susceptibility $χ=3.4\times10^{-4}$ is inferred using a magnetostatic model informed by correlated scanning electron microscopy measurements of crystal dimensions. A small fraction of nanoparticles (4/82 for $Plasmodium$-produced and 1/41 for synthetic) exhibit a saturation behavior consistent with superparamagnetism. Translation of this platform to the study of living malaria-infected cells may shed new light on hemozoin formation dynamics and their interaction with antimalarial drugs.

cond-mat.mes-hall↗

Sawtooth wave adiabatic passage slowing of dysprosium

We report on sawtooth wave adiabatic passage (SWAP) slowing of bosonic and fermionic dysprosium isotopes by using a 136 kHz wide transition at 626 nm. A beam of precooled atoms is further decelerated in one dimension by the SWAP force and the amount of atoms at near zero velocity is measured. We demonstrate that the SWAP slowing can be twice as fast as in a conventional optical molasses operated on the same transition. In addition, we investigate the parameter range for which the SWAP force is efficiently usable in our set-up, and relate the results to the adiabaticity condition. Furthermore, we add losses to the hyperfine ground-state population of fermionic dysprosium during deceleration and observe more robust slowing with SWAP compared to slowing with the radiation pressure force.

physics.atom-ph↗

Widefield imaging of superconductor vortices with electron spins in diamond

Understanding the mechanisms behind high-$T_{c}$ Type-II superconductors (SC) is still an open task in condensed matter physics. One way to gain further insight into the microscopic mechanisms leading to superconductivity is to study the magnetic properties of the SC in detail, for example by studying the properties of vortices and their dynamics. In this work we describe a new method of wide-field imaging magnetometry using nitrogen-vacancy (NV) centers in diamond to image vortices in an yttrium barium copper oxide (YBCO) thin film. We demonstrate quantitative determination of the magnetic field strength of the vortex stray field, the observation of vortex patterns for different cooling fields and direct observation of vortex pinning in our disordered YBCO film. This method opens prospects for imaging of the magnetic-stray fields of vortices at frequencies from DC to several megahertz within a wide range of temperatures which allows for the study of both high-$T_{C}$ and low-$T_{C}$ SCs. The wide temperature range allowed by NV center magnetometry also makes our approach applicable for the study of phenomena like island superconductivity at elevated temperatures (e.g. in metal nano-clusters).

cond-mat.supr-con↗

Nondestructive in-line sub-picomolar detection of magnetic nanoparticles in flowing complex fluids

Over the last decades, the use of magnetic nanoparticles in research and commercial applications has increased dramatically. However, direct detection of trace quantities remains a challenge in terms of equipment cost, operating conditions and data acquisition times, especially in flowing conditions within complex media. Here we present the in-line, non-destructive detection of magnetic nanoparticles using high performance atomic magnetometers at ambient conditions in flowing media. We achieve sub-picomolar sensitivities measuring $\sim$30 nm ferromagnetic iron and cobalt nanoparticles that are suitable for biomedical and industrial applications, under flowing conditions in water and whole blood. Additionally, we demonstrate real-time surveillance of the magnetic separation of nanoparticles from water and whole blood. Overall our system has the merit of inline direct measurement of trace quantities of ferromagnetic nanoparticles with so far unreached sensitivities and could be applied in the biomedical field (diagnostics and therapeutics) but also in the industrial sector.

physics.app-ph↗