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M. A. Tanatar

Publications and source records attributed to M. A. Tanatar.

At least 127 records · Page 7Linked to original sources

Magneto-optical study of Ba(Fe$_{1-x}$T$_{x}$)$_2$As$_2$ (T=Co, Ni) single crystals irradiated with heavy-ions

Optimally doped single crystals of Ba(Fe$_{1-x}$T$_x$)$_2$As$_2$ (T=Co, Ni) were irradiated with 1.4 GeV $^{208}$Pb$^{56+}$ ions at fluences corresponding to matching fields of $B_ϕ=0.1, 0.5, 1$ and 2 T. Magneto-optical imaging has been used to map the distribution of the magnetic induction in the irradiated samples. The imaging is complemented by the magnetization measurements. The results show a substantial enhancement of the apparent critical current densities as revealed by the much larger Bean penetration fields and an increase of the hysteretic magnetization. However, the effect depends on the compound, temperature and applied magnetic field. In \FeCo crystals, at 15 K and low fields, the enhancement appears to scale with the irradiation dose at a rate of about 0.27 MA$\cdot$cm$^{-2}$T$^{-1}$, whereas in \FeNi crystals, higher irradiation doses are less effective. Our results suggest that moderate irradiation with heavy ions is a an effective way to \emph{homogeneously} enhance the current-currying capabilities of pnictide superconductors.

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London penetration depth and superfluid density in single crystals of Fe(Te,Se) and Fe(Te,S) superconductors

The in-plane London penetration depth, $λ(T)$, was measured in single crystals of the iron-chalcogenide superconductors Fe$_{1.03}$(Te$_{0.63}$Se$_{0.37}$) and Fe$_{1.06}$(Te$_{0.88}$S$_{0.14}$) by using a radio-frequency tunnel diode resonator. As is also the case for the iron-pnictides, these iron-chalcogenides exhibit a nearly quadratic temperature variation of $λ(T)$ at low temperatures. The absolute value of the penetration depth in the $T \to 0$ limit was determined for Fe$_{1.03}$(Te$_{0.63}$Se$_{0.37})$ by using an Al coating technique, giving $λ(0)\approx560 \pm 20$ nm. The superfluid density $ρ_s(T)=λ^2(0)/λ^2(T)$ was fitted with a self-consistent two-gap $γ-$model. While two different gaps are needed to describe the full-range temperature variation of $ρ_s(T)$, a non-exponential behavior at low temperatures requires additional factors, such as scattering and/or significant gap anisotropy.

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London penetration depth and strong pair-breaking in iron-based superconductors

The low temperature variation of the London penetration depth for a number of iron-pnictide and iron-chalcogenide superconductors is nearly quadratic, $Δλ(T) = βT^n$ with $n\approx 2$. The coefficient in this dependence shows a robust scaling, $β\propto 1/T_c^3$ across different families of these materials. We associate the scaling with a strong pair-breaking. The same mechanism have recently been suggested to explain the scalings of the specific heat jump, $ΔC \propto T_c^3$, and of the slopes of the upper critical field, $dH_{c2}/dT\propto T_c$ in these materials. This suggests that thermodynamic and electromagnetic properties of the iron-based superconductors can be described within a strong pair-breaking scenario.

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Three-dimensional nodal superconducting gap in single crystals Ba(Fe$_{1-x}$Ni$_x$)$_2$As$_2$

The London penetration depth, $λ$, is directly related to the density, $n_{s}$, of the Cooper pairs ($λ^{2}\propto 1/n_{s}$) and its variation with temperature provides valuable insight into the pairing mechanism. Here we study the evolution with doping of the temperature dependence of the in-plane ($λ_{ab}$) and out-of-plane ($λ_{c}$) penetration depths in single crystals of electron-doped Ba(Fe$_{1-x}$Ni$_x$)$_2$As$_2$. As is the case for other pnictides, $λ(T) \sim T^n$ over the whole doping range and this behavior extends down to at least $T=T_c/100$, setting a very small upper limit on the gap minimum. Furthermore, in the overdoped regime: 1) the exponent $n$ becomes substantially smaller than 2, which is incompatible with the models that explain power-law behavior to be due to scattering; 2) the exponent $n$ becomes anisotropic, with $λ_{c}(T)$ showing a clear $T$-linear behavior over a large temperature interval. These findings suggest that in the overdoped regime the superconducting gap in iron-based pnictide superconductors develops nodal structure, which unlike in the cuprates, cannot be understood within a two-dimensional picture.

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Intrinsic pinning on structural domains in underdoped single crystals of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$

Critical current density was studied in single crystals of Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ for the values of $x$ spanning the entire doping phase diagram. A noticeable enhancement was found for slightly underdoped crystals with the peak at $x = 0.058$. Using a combination of polarized-light imaging, x-ray diffraction and magnetic measurements we associate this behavior with the intrinsic pinning on structural domains in the orthorhombic phase. Domain walls extend throughout the sample thickness in the direction of vortices and act as extended pinning centers. With the increasing $x$ domain structure becomes more intertwined and fine due to a decrease of the orthorhombic distortion. This results in the energy landscape with maze-like spatial modulations favorable for pinning. This finding shows that iron-based pnictide superconductors, characterized by high values of the transition temperature, high upper critical fields, and low anisotropy may intrinsically have relatively high critical current densities.

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Quasiparticle Heat Transport in Ba$_{1-x}$K$_x$Fe$_2$As$_2$: Evidence for a k-dependent Superconducting Gap without Nodes

The thermal conductivity $κ$ of the iron-arsenide superconductor Ba$_{1-x}$K$_x$Fe$_2$As$_2$ ($T_c \simeq$ 30 K) was measured in single crystals at temperatures down to $T \simeq 50$ mK ($\simeq T_c$/600) and in magnetic fields up to $H = 15$ T ($\simeq H_{c2}$/4). A negligible residual linear term in $κ/T$ as $T \to 0$ shows that there are no zero-energy quasiparticles in the superconducting state. This rules out the existence of line and in-plane point nodes in the superconducting gap, imposing strong constraints on the symmetry of the order parameter. It excludes d-wave symmetry, drawing a clear distinction between these superconductors and the high-$T_c$ cuprates. However, the fact that a magnetic field much smaller than $H_{c2}$ can induce a residual linear term indicates that the gap must be very small on part of the Fermi surface, whether from strong anisotropy or band dependence, or both.

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Direct imaging of the structural domains in iron pnictides AFe2As2 (A = Ca, Sr, Ba)

The parent compounds of recently discovered iron-arsenide superconductors, $A$Fe$_2$As$_2$ with alkaline earth $A$=Ca, Sr, Ba, undergo simultaneous structural and magnetic phase transitions at a temperature $T_{SM}$. Using a combination of polarized light microscopy and spatially resolved high-energy synchrotron X-ray diffraction we show that the orthorhombic distortion leads to the formation of 45$^o$-type structural domains in all parent compounds. Domains penetrate through the sample thickness in the $c$- direction and are not affected by crystal defects such as growth terraces. The domains form regular stripe patterns in the plane with a characteristic dimension of 10 to 50 $μm$. The direction of the stripes is fixed with respect to the tetragonal (100) and (010) directions but can change by 90$^o$ on thermal cycling through the transition. This domain pattern may have profound implications for intrinsic disorder and anisotropy of iron arsenides.

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Non-exponential London penetration depth in RFeAsO$_{0.9}$F$_{0.1}$ (R=La,Nd) single crystals

The superconducting penetration depth, $λ(T)$, has been measured in RFeAsO$_{0.9}$F$_{0.1}$ (R=La,Nd) single crystals (R-1111). In Nd-1111, we find an upturn in $λ(T)$ upon cooling and attribute it to the paramagnetism of the Nd ions, similar to the case of the electron-doped cuprate Nd-Ce-Cu-O. After the correction for paramagnetism, the London penetration depth variation is found to follow a power-law behavior, $Δλ_L(T)\propto T^{2}$ at low temperatures. The same $T^2$ variation of $λ(T)$ was found in non-magnetic La-1111 crystals. Analysis of the superfluid density and of penetration depth anisotropy over the full temperature range is consistent with two-gap superconductivity. Based on this and on our previous work, we conclude that both the RFeAsO (1111) and BaFe$_2$As$_2$ (122) families of pnictide superconductors exhibit unconventional two-gap superconductivity.

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Resistivity Anisotropy of $AE$Fe$_2$As$_2$ ($AE$ =Ca, Sr, Ba): direct versus Montgomery technique measurements

The anisotropy of electrical resistivity was measured in parent compounds of the iron-arsenic high temperature superconductors, AEFe2As2 with Alkali Earth elements AE=Ca,Sr, Ba. Measurements were performed using both the Montgomery technique and direct resistivity measurements on samples cut along principal crystallographic directions. The anisotropy ratio γ_ρ=ρ_c/ρ_a is well below 10 for all compounds in the whole temperature range studied (4 to 300 K), in notable contrast to previous reports. The anisotropy at room temperature increases from about 2 in Ca, to about 4 in Sr and Ba. In all compounds the resistivity ratio decreases on cooling through the structural/antiferromagnetic transition temperature T_{SM}, with the change mainly coming from stronger variation in ρ_a as compared with ρ_c. This suggests that the transitions stronger affect the two-dimensional parts of the Fermi surface. We compare our experimental observations with band structure calculations, and find similar trend in the evolution of anisotropy with the size of AE ion. Our results show that the electronic structure of the iron pnictides has large contribution from three-dimensional areas of the Fermi surface.

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Non-exponential London penetration depth in Ba$_{1-}$K$_{x}$Fe$_{2}$As$_{2}$ single crystals

We have studied the in- and out-of-plane magnetic penetration depths in the hole- doped iron based superconductor Ba$_{1-x}$K$_{x}$Fe$_{2}$As$_{2}$ ($T_{c}\approx$ 30K). The study was performed on single crystals grown from different fluxes and we find that the results are nearly the same. The in-plane London penetration depth $λ_{ab}$ does not show exponential saturation at low temperature, as would be expected from a fully gapped superconductor. Instead, $λ_{ab}(T)$ shows a power-law behavior, $λ\propto T^{n}$ ($n\approx 2$), down to $T\approx 0.02 T_{c}$, similar to the electron doped Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$. The penetration depth anisotropy $γ_λ=λ_{c}(T)/λ_{ab}(T)$ increases upon cooling, opposite to the trend observed in the anisotropy of the upper critical field, $γ_ξ=H_{c2}^{\perp c}(0)/H_{c2}^{\parallel c}(0)$. These are universal characteristics of both the electron and hole doped 122 systems, suggesting unconventional superconductivity. The behavior of the in-plane superfluid density $ρ_{ab}(T)$ is discussed in light of existing theoretical models proposed for the iron pnictides superconductors.

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Universal heat transport in a heavy-fermion superconductor

The symmetry of the order parameter is the defining property of a superconductor and a strong clue to its pairing mechanism. While d-wave symmetry is firmly established in high-Tc superconductors, in no heavy-fermion superconductor is the symmetry known definitively. One way to elucidate the order parameter is to locate the symmetry-imposed nodes in the energy gap by measuring the heat carried by the zero-energy quasiparticles associated with those nodes as a function of direction. As verified in high-Tc superconductors a line of nodes yields universal heat transport independent of impurity scattering. Here we show that heat conduction in the heavy-fermion superconductor CeIrIn5 is also universal, but only for a current perpendicular to the tetragonal axis of its crystal structure, not parallel to it. This uniaxial anisotropy is strong evidence for a line of nodes in the basal plane, which is inconsistent with the d-wave symmetry proposed for the isostructural superconductor CeCoIn5. Different symmetries in the two materials would explain why the phase diagram of these heavy-fermion compounds consists of two separate superconducting domes.

cond-mat.str-el↗

Doping dependent Irreversible Magnetic Properties of Ba(Fe1-xCox)2As2 Single Crystals

We discuss the irreversible magnetic properties of self-flux grown Ba(Fe1-xCox)2As2 single crystals for a wide range of concentrations covering the whole phase diagram from the underdoped to the overdoped regime, x=0.038, 0.047, 0.058, 0.071, 0.074, 0.10, 0.106 and 0.118. Samples were characterized by a magneto-optical method and show excellent spatial uniformity of the superconducting state. The overall behavior closely follows classical Bean model of the critical state. The field-dependent magnetization exhibits second peak at a temperature and doping - dependent magnetic field, Hp. The evolution of this fishtail feature with doping is discussed. Magnetic relaxation is time-logarithmic and unusually fast. Similar to cuprates, there is an apparent crossover from collective elastic to plastic flux creep above Hp. At high fields, the field dependence of the relaxation rate becomes doping independent. We discuss our results in the framework of the weak collective pinning and show that vortex physics in iron-based pnictide crystals is much closer to high-Tc cuprates than to conventional s-wave (including MgB2) superconductors.

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Anisotropic London Penetration Depth and Superfluid Density in Single Crystals of Iron-based Pnictide Superconductors

In- and out-of-plane magnetic penetration depths were measured in three iron-based pnictide superconducting systems. All studied samples of both 122 systems show a robust power-law behavior, $λ(T) T^n$, with the sample-dependent exponent n=2-2.5, which is indicative of unconventional pairing. This scenario could be possible either through scattering in a $s_{\pm }$ state or due to nodes in the superconducting gap. In the Nd-1111 system, the interpretation of data may be obscured by the magnetism of rare-earth ions. The overall anisotropy of the pnictide superconductors is small. The 1111 system is about two times more anisotropic than the 122 system. Our data and analysis suggest that the iron-based pnictides are complex superconductors in which a multiband three-dimensional electronic structure and strong magnetic fluctuations play important roles.

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Anisotropy of the Optimally-Doped Iron Pnictide Superconductor Ba(Fe0.926Co0.074)2As2

Anisotropies of electrical resistivity, upper critical field, London penetration depth and critical currents have been measured in single crystals of the optimally doped iron pnictide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$, $x$=0.074 and $T_c \sim$23 K. The normal state resistivity anisotropy was obtained by employing both the Montgomery technique and direct measurements on samples cut along principal crystallographic directions. The ratio $γ_ρ = ρ_c /ρ_a$ is about 4$\pm$1 just above $T_c$ and becomes half of that at room temperature. The anisotropy of the upper critical field, $γ_{H} = H_{c2,ab} /H_{c2,c} $, as determined from specific heat measurements close to $T_c$, is in the range of 2.1 to 2.6, depending on the criterion used. A comparable low anisotropy of the London penetration depth, $γ_λ=λ_{c}/λ_{ab}$, was recorded from TDR measurements and found to persist deep into the superconducting state. An anisotropy of comparable magnitude was also found in the critical currents, $γ_j=j_{c,ab}/j_{c,c}$, as determined from both direct transport measurements ($\sim$1.5) and from the analysis of the magnetization data ($\sim$3). Overall, our results show that iron pnictide superconductors manifest anisotropies consistent with essentially three-dimensional intermetallic compound and bear little resemblance to cuprates.

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The London penetration depth in single crystals of Ba(Fe_{1-x}Co_x)_2As_2 at various doping levels

The London penetration depth $λ(T)$ has been measured in single crystals of Ba(Fe$_{1-x}$Co$_{x}$)$_{2}$As$_{2}$ using the tunnel diode resonator technique. The measured doping levels of $x=$~0.038, 0.047, 0.058, 0.074 and 0.10 range from underdoped to overdoped concentrations. The measurements have shown that the density of carriers participating in superconductivity decreases sharply in the underdoped regime, but the penetration depth as a function of temperature exhibits a robust power law, $Δλ(T)\sim T^{n}$, for all measured dopings, with $n$ between 2 and 2.5. We discuss the implications of these results and possible interpretations of such robust behavior.

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Unconventional London penetration depth in Ba(Fe0.93Co0.07)2As2 single crystals

The London penetration depth, $λ(T)$, has been measured in several single crystals of Ba(Fe$_{0.93}$Co$_{0.07}$)$_2$As$_2$. Thermodynamic, electromagnetic, and structural characterization measurements confirm that these crystals are of excellent quality. The observed low temperature variation of $λ(T)$ follows a power-law, $Δλ(T) \sim T^n$ with $n=2.4 \pm 0.1$, indicating the existence of normal quasiparticles down to at least $0.02T_c$. This is in contrast to recent penetration depth measurements on single crystals of NdFeAsO$_{1-x}$F$_x$ and SmFeAsO$_{1-x}$F$_x$, which indicate an anisotropic but nodeless gap. We propose that a more three-dimensional character in the electronic structure of Ba(Fe$_{0.93}$Co$_{0.07}$)$_2$As$_2$ may lead to an anisotropic $s-$wave gap with point nodes that would explain the observed $λ(T)$.

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Vortex phase diagram of Ba(Fe0.93Co0.07)2As2 single crystals

Detailed measurements of the global and local electromagnetic properties of Ba(Fe$_{0.93}$Co$_{0.07}$)$_{2}$As$_{2}$ single crystals are reported. Analysis of the irreversible magnetic response provides strong evidence for similar vortex physics in this Fe-based pnictide superconductor to the high-$T_{c}$ cuprates, such as Y-Ba-Cu-O or Nd-Ce-Cu-O. In particular, we have found a nonmonotonic "fishtail" magnetization in $M(H,T=const)$ loops and its signature is also present in $M(H=const,T)$ scans. The supercurrent density is evaluated by using several techniques, including direct transport measurements. At 5 K we estimate its value to be a moderate $j \approx 2.6 \pm 0.2 \times 10^5$ A/cm$^2$. Analysis of the magnetic relaxation is consistent with the collective pinning and creep models (weak pinning and fast creep) and suggests a crossover from the collective to the plastic creep regime in fields exceeding the value corresponding to the maximum in fishtail magnetization.

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