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M. Avrigeanu

Publications and source records attributed to M. Avrigeanu.

At least 19 recordsLinked to original sources

Long-standing problem: The nuclear level density angular-momentum dependence and isomeric data assessment

Recent 91,92,93Tc activation for deuterons incident on natMo has become a challenge for the nuclear level density (NLD) angular-momentum dependence. Actually, replacement of the moment of inertia rigid-body value Ir by half of it, within a given NLD parameter set, demands a change of the rest of NLD parameters significantly beyond their fitted limits. The corresponding uncertainty of calculated cross sections versus the NLD parameter accuracy is also higher, while use of either the same or distinct compound-nucleus and preequilibrium emission spin distributions becomes significant at higher incident energies. Nevertheless, the current way to describe experimental isomeric cross sections by using at most half of Ir values provides agreement of the measured and calculated data at the price of less and less correct NLDs. The moment of inertia relevance for the NLD correctness also emphasizes the value of a direct method to endorse it. Further measurements of average resonance spacings of s-wave neutrons and protons, corresponding to different spins of the same nucleus, are therefore highly demanded.

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Modeling of Deuteron Induced Reactions on Molybdenum at Low Energies

The activities of the EUROfusion consortium on the development of high quality nuclear data for fusion applications include evaluations of deuteron induced reactions and related data libraries for needs of the DEMO fusion power plant and IFMIF-DONES neutron--source nuclear analyses. Molybdenum is one of the major constituents of the reference stainless steels used in critical components of these projects. While the TENDL deuteron data library was the current reference used by EUROfusion, need of its further improvement has already been pointed out. The weak binding energy of the deuteron is responsible for the high complexity of its interaction with nuclei, involving also a variety of reactions initiated by the nucleons following the deuteron breakup. Their analysis completed that of the deuteron interactions with Mo and its stable isotopes, from elastic scattering to pre-equilibrium and compound--nucleus reactions, up to 50 MeV. A particular attention has been paid to the breakup, stripping, and pick-up direct interactions which amount to around half of the deuteron total--reaction cross section. The due account of most experimental data has validated the present approach, highlighted some prevalent features, and emphasized weak points and consequently the need for modeling/evaluation upgrade.

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Deuteron-induced reactions on manganese at low energies

The scarce data systematics and complexity of deuteron interactions demand the update of both the experimental database and theoretical frame of deuteron activation cross sections. Various reactions induced by neutrons and protons following the deuteron breakup (BU) should be also taken into account. On the other hand, deuteron reaction cross sections recommended recently for high-priority elements are still based on data fit without predictive power. Purpose: Accurate new measurements of low-energy deuteron-induced reaction cross sections for monoisotopic (55Mn) natural manganese target enhance the related database as well as the opportunity of an unitary and consistent account of the related reaction mechanisms. Method: Activation cross sections of 54,56Mn, and 51Cr nuclei by deuterons on $^{55}$Mn were measured at energies <20 MeV by the stacked-foil technique and high resolution gamma spectrometry at the U-120M cyclotron of CANAM, NPI CAS. Then all available data for deuterons on 55Mn up to 50 MeV are analyzed paying particular attention to BU and direct reaction (DR) mechanisms. Results: Newly measured activation cross sections strengthen the deuteron database at low energies, at once with a consistent account for the first time of all available data. Conclusions: Due account of deuteron-induced reactions on 55Mn, including particularly the new experimental data at low energies, is provided by a suitable BU and DR assessment.

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Role of consistent parameter sets in an assessment of the alpha-particle optical potential below the Coulomb barrier

Background: Further studies of high-precision measurements of alpha-induced reaction data below the Coulomb barrier have still raised questions about the alpha-particle optical model potential (OMP) within various mass ranges, i.e. for 64Zn, 108Cd, 113,115In, 121,123Sb, and 191,193Ir target nuclei. Purpose: The accuracy as well as eventual uncertainties and/or systematic errors of using a previous optical potential are much better considered by analysis of such accurate data. Method: Statistical model (SM) calculations of the (alpha,x) reaction cross sections have been carried out using model parameters which were previously obtained by analyzing independent data, particularly gamma-ray strength functions, and taking into account their uncertainties and questions of extrapolation for nuclei without similar data. Results: Consistent description of the recent alpha-induced reaction data is provided by the above-mentioned optical potential with no empirical rescaling factors of either its own parameters or the gamma and/or nucleon widths. Effects of still uncertain SM parameters on calculated alpha-induced reaction cross sections and conclusions on the alpha-OMP can be now discussed due to unprecedented precision of the new data. Conclusions: The alpha-particle optical potential has been confirmed at incident energies below the Coulomb barrier using statistical-model parameters validated through a former analysis of independent data.

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Consistent account of deuteron-induced reactions on Cr up to 60 MeV

Purpose: Accurate new measurements of low-energy deuteron-induced reaction cross sections for natural Cr target can enhance the related database and the opportunity for an unitary and consistent account of the involved reaction mechanisms. Methods: The activation cross sections of $^{51,52,54}$Mn, $^{51}$Cr, and $^{48}$V nuclei for deuterons incident on natural Cr at energies up to 20 MeV, were measured by the stacked-foil technique and high resolution gamma spectrometry using U-120M cyclotron of the Center of Accelerators and Nuclear Analytical Methods (CANAM) of the Nuclear Physics Institute of the Czech Academy of Sciences (NPI CAS). They as well as formerly available data for deuteron interactions with Cr isotopes up to 60 MeV are the object of an extended analysis of all processes from elastic scattering until the evaporation from fully equilibrated compound system, but with a particular attention given to the BU and DR mechanisms. Results: The new measured activation excitation functions proved essential for the enrichment of the deuteron database, while the theoretical analysis of all available data strengthens for the first time their consistent account provided that (i) a suitable BU and DR assessment is completed by (ii) the assumption of PE and CN contributions corrected for decrease of the total-reaction cross section due to the leakage of the initial deuteron flux towards BU and DR processes. Conclusions: The suitable description of nuclear mechanisms involved within deuteron-induced reactions on chromium, taking into account especially the BU and DR direct processes, is validated by an overall agreement of the calculated and measured cross sections including particularly the new experimental data at low energies.

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Consistent optical potential for incident and emitted low-energy $α$ particles. II. $α$-emission in fast-neutron induced reactions on Zr isotopes

Background: Challenging questions of the $α$-particle optical-model potential (OMP) are still pointed out by recent high-precision measurements of $α$-induced reaction data below the Coulomb barrier. Moreover, the reliability of a previous OMP for $α$-particles on nuclei within the mass number range 45$\leq$$A$$\leq$209 has been recently proved for emitted $α$ particles as well, but only in the case of proton-induced reactions on Zn isotopes [Phys. Rev. C {\bf 91}, 064611 (2015), Paper I]. Purpose: Analysis of most recent $(α,γ)$ reaction data for Ge and Zr isotopes, which provides an additional validation of the above-mentioned potential, is related to a further account of $α$-particle emission in neutron-induced reactions on Zr isotopes, at the same time with a suitable description of all competitive processes. Methods: A consistent parameter set, established or validated by independent analysis of recent various data, particularly $γ$-ray strength functions, have been involved within model calculation of the $(α,γ)$ as well as $(n,α)$ reaction cross sections. The latter are part of the whole analysis of the neutron activation of Zr isotopes, in order to avoid any error compensation or latent ambiguity. Results: The aforesaid potential provides a consistent description of recent $α$-induced reaction data with no empirical rescaling factors of the $γ$ and/or nucleon widths. On the other hand, its use leads to underestimated predictions of the pre-equilibrium emission and statistical models for the $(n,α)$ reaction cross sections. Conclusions: An optical potential with a volume imaginary component seems to be needed to describe the low-energy $α$-particle evaporation, while only surface absorption occurs in $α$-induced reactions at similar energies.

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Role of the direct processes in low-energy deuteron interactions

An extended analysis of the key role of direct interactions, i.e., breakup, stripping and pick-up processes, has been carried out for deuteron-induced reactions. Particular comments concern the deuteron breakup which is the dominant mechanism involved in surrogate reactions on heavy nuclei, around the Coulomb barrier.

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Additive empirical parametrization and microscopic study of the deuteron breakup

Comparative assessment of the total breakup proton-emission cross sections measured for 56 MeV deuteron interaction with target nuclei from $^{12}$C to $^{209}$Bi, with an empirical parametrization and recently calculated microscopic neutron-removal cross sections has been done at the same time with similar data measured at 15, 25.5, 70, and 80 MeV. Comparable mass dependances of the elastic-breakup (EB) cross sections provided by the empirical parametrization and the microscopic results have been also found at the deuteron energy of 56 MeV, while the assessment of absolute-values variance up to a factor of two has been not possible due to the lack of EB measurements at energies higher than 25.5 MeV. While the similarities represent an additional validation of the microscopic calculations, the cross-section difference should be considered within the objectives of further measurements.

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Comment on "Solution of the $α$-Potential Mystery in the $γ$ Process and Its Impact on the Nd/Sm Ratio in Meteorites"

A competition of the low-energy Coulomb excitation (CE) with the compound nucleus (CN) formation in $α$-induced reactions below the Coulomb barrier has been assumed by Rauscher [Phys. Rev. Lett. 111, 061104 (2013)] in order to use the same optical model (OM) potential for description of the latter and the alpha-particle emission as well. In this Comment we show that the corresponding partial waves and integration radii provide evidence for the distinct account of the CE cross section and OM total-reaction cross section.

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Analysis of uncertainties in alpha-particle optical-potential assessment below the Coulomb barrier

Background: Recent high-precision measurements of alpha-induced reaction data below the Coulomb barrier have pointed out questions of the alpha-particle optical-model potential (OMP) which are yet open within various mass ranges. Purpose: The applicability of a previous optical potential and eventual uncertainties and/or systematic errors of the OMP assessment at low energies can be further considered on this basis. Method: Nuclear model parameters based on the analysis of recent independent data, particularly gamma-ray strength functions, have been involved within statistical model calculation of the (alpha,x) reaction cross sections. Results: The above-mentioned potential provides a consistent description of the recent alpha-induced reaction data with no empirical rescaling factors of the and/or nucleon widths. Conclusions: A suitable assessment of alpha-particle optical potential below the Coulomb barrier should involve the statistical-model parameters beyond this potential on the basis of a former analysis of independent data.

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Further explorations of the alpha-particle optical model potential at low energies for the mass range A=45-209

The recent high-precision measurements of alpha-particle induced reaction data below the Coulomb barrier (B) make possible the understanding of limits and possible improvement of a previous optical model potential (OMP) for alpha-particles on nuclei within the mass number range 45 130. Moreover, underestimation of reaction cross sections for well-deformed nuclei is removed by using ~7% larger radius for the surface imaginary part of this spherical OMP. Improved input parameters based on recent independent data, particularly gamma-ray strength functions, but no empirical rescaling factor of the gamma and/or neutron widths have been involved within statistical model calculation of the corresponding (alpha,x) reaction cross sections.

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Does deuteron-induced fission on actinide nuclei prevails over the breakup at low incident energies?

An analysis of the $^{231}$Pa$(d,3n)$$^{230}$U reaction excitation function at energies around the Coulomb barrier has taken into account the pre-equilibrium and compound-nucleus cross sections corrected for the deuteron-breakup decrease of the total reaction cross section, as well as the inelastic breakup enhancement. The analysis reveals the dominance of the deuteron breakup mechanism unlike a former assessment in this respect of the deuteron-induced fission process.

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Isomeric cross sections of fast-neutron induced reactions on $^{197}$Au

Recent accurate data obtained for the isomeric cross section of the $^{197}$Au$(n,2n)$ reaction provide a valuable opportunity to consider the question of the effective moment of inertia of the nucleus within a local consistent model analysis of all available reaction data for the $^{197}$Au target nucleus. Thus, a definite proof of a moment of inertia equal to that of the rigid--body has been obtained for $^{196}$Au nucleus while an inference of the half rigid--body value is suggested for the $^{194}$Ir nucleus. The usefulness of further measurements at incident energies up to $\ge$40 MeV has also been proved.

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Low and medium energy deuteron-ind ced reactions on $^{63,65}$Cu nuclei

The activation cross sections of (d,p), (d,2n), (d,3n), and (d,2p) reactions on 63,65Cu were measured in the energy range from 4 to 20 MeV using the stacked-foils technique. Then, following the available elastic-scattering data analysis that provided the optical potential for reaction cross sections calculations, an increased effort has been devoted to the breakup mechanism, the direct reaction stripping, and the pre-equilibrium and compound-nucleus cross section calculations, corrected for the breakup and stripping decrease of the total reaction cross section. The overall agreement between the measured and calculated deuteron activation cross sections proves the correctness of the nuclear mechanisms account, next to the simultaneous analysis of the elastic-scattering and reaction data.

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Comment on 'Excitation function for the radionuclide 46Sc produced in the irradiation of 45Sc with deuterons and 6He'

We show that the model analysis of new measured (d,p), (d,t), (6He,5He), and (6He,4He) reaction cross sections at incident energies around the Coulomb barrier (J. Phys. G: Nucl. Part. Phys. 38 (2011) 035106) led to results that are not consistent with similar calculated and evaluated data. On the other hand, it should be corrected by taking into account the direct processes.

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High precision $^{89}$Y($α$,$α$)$^{89}$Y scattering at low energies

Elastic scattering cross sections of the $^{89}$Y($α$,$α$)$^{89}$Y reaction have been measured at energies E$_{c.m.}$ = 15.51 and 18.63 MeV. The high precision data for the semi-magic $N = 50$ nucleus $^{89}$Y are used to derive a local potential and to evaluate the predictions of global and regional $α$-nucleus potentials. The variation of the elastic alpha scattering cross sections along the $N = 50$ isotonic chain is investigated by a study of the ratios of angular distributions for $^{89}$Y($α$,$α$)$^{89}$Y and $^{92}$Mo($α$,$α$)$^{92}$Mo at E$_{c.m.} \approx$ 15.51 and 18.63 MeV. This ratio is a very sensitive probe at energies close to the Coulomb barrier, where scattering data alone is usually not enough to characterize the different potentials. Furthermore, $α$-cluster states in $^{93}$Nb = $^{89}$Y $\otimes$ $α$ are investigated.

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Analysis of alpha-induced reactions on $^{151}$Eu below the Coulomb barrier

Novel measurements of $(α,γ)$ and $(α$,n) reaction cross sections on the target nucleus $^{151}$Eu, close to the reaction thresholds, support the setting up of recent parameters of the $α$-particle optical model potential below the Coulomb barrier. A better understanding of the $α$-particle optical potential at these energies leads to a statistical model analysis of additional partial cross sections that were formerly measured but not considered within the model analysis. On this basis we have tentatively assigned a modified $J^π$=9$^-$ spin and parity to the 22.7-h isomer in $^{154}$Tb.

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Alpha-particle optical potential proofs at astrophysically relevant energies

$(α,γ)$ and $(α$,n) reaction cross sections recently measured close to the reaction thresholds are rather well described by a previously developed regional optical potential. Thus, particular features of the $α$-particle optical potential at energies below the Coulomb barrier, besides parameters describing $α$-particle elastic scattering at higher energies are confirmed. Additional limitations of similar statistical model calculations for minor reaction channels are shown to be most likely due to an overlooked process or critical values of statistical model parameters around closed nuclear shells.

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