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M. B. Plenio

Publications and source records attributed to M. B. Plenio.

At least 37 records · Page 2Linked to original sources

Sharp reversals of steady-state nuclear polarisation as a tool for quantum sensing

The polarisation dynamics of nuclear spins weakly coupled to an NV center is highly sensitive to the parameters of the microwave control and the nuclear Larmor frequency. What is commonly regarded as a challenge, we propose here as a resource for quantum sensing. By varying a single experimental parameter in a suitable set-up, i.e., the Rabi frequency of a continual microwave driving or the nuclear Larmor frequency, we predict periodic reversals of the steady-state polarisation of the nuclear spin. Crucially, interference between the transverse and longitudinal dipolar interaction of electron and nuclear spins results in remarkably sharp steady-state polarisation reversals of nuclear spins within only a few tens of Hz change in the nuclear Larmor frequency. Our method is particularly robust against imperfections such as decoherence of the electron spin and the frequency resolution of the sensor is not limited by the coherence time $T_2$ of the electron sensor.

quant-ph↗

Soft Quantum Control for Highly Selective Interactions among Joint Quantum Systems

We propose a quantum control scheme aimed at interacting systems that gives rise to highly selective coupling among their near-to-resonance constituents. Our protocol implements temporal control of the interaction strength, switching it on and off again adiabatically. This soft temporal modulation significantly suppresses off-resonant contributions in the interactions. Among the applications of our method we show that it allows us to perform an efficient rotating-wave approximation in a wide parameter regime, the elimination of side peaks in quantum sensing experiments, and selective high-fidelity entanglement gates on nuclear spins with close frequencies. We apply our theory to nitrogen-vacancy centers in diamond and demonstrate the possibility for the detection of weak electron-nuclear coupling under the presence of strong perturbations.

quant-ph↗

Pulsed Dynamical Decoupling for Fast and Robust Two-Qubit Gates on Trapped Ions

We propose a pulsed dynamical decoupling protocol as the generator of tunable, fast, and robust quantum phase gates between two microwave-driven trapped ion hyperfine qubits. The protocol consists of sequences of $π$-pulses acting on ions that are oriented along an externally applied magnetic field gradient. In contrast to existing approaches, in our design the two vibrational modes of the ion chain cooperate under the influence of the external microwave driving to achieve significantly increased gate speeds. Our scheme is robust against the dominant noise sources, which are errors on the magnetic field and microwave pulse intensities, as well as motional heating, predicting two-qubit gates with fidelities above $99.9\%$ in tens of microseconds.

quant-ph↗

Proposal for Quantum Simulation via All-Optically Generated Tensor Network States

We devise an all-optical scheme for the generation of entangled multimode photonic states encoded in temporal modes of light. The scheme employs a nonlinear down-conversion process in an optical loop to generate one- and higher-dimensional tensor network states of light. We illustrate the principle with the generation of two different classes of entangled tensor network states and report on a variational algorithm to simulate the ground-state physics of many-body systems. We demonstrate that state-of-the-art optical devices are capable of determining the ground-state properties of the spin-1/2 Heisenberg model. Finally, implementations of the scheme are demonstrated to be robust against realistic losses and mode mismatch.

quant-ph↗

A resource theory of superposition

The superposition principle lies at the heart of many non-classical properties of quantum mechanics. Motivated by this, we introduce a rigorous resource theory framework for the quantification of superposition of a finite number of linear independent states. This theory is a generalization of resource theories of coherence. We determine the general structure of operations which do not create superposition, find an elementary connection to unambiguous state discrimination, and propose several general quantitative superposition measures. We show that several main results from resource theories of coherence still hold in our more general setting. Of special importance are two results about the free completion of trace decreasing operations and the free probabilistic transformation between pure states that are also valid for the special case of coherence.

quant-ph↗

Sensing phase-transitions via nitrogen-vacancy centers in diamond

Ultra-thin layers of liquids on a surface behave differently from bulk liquids due to liquid-surface interactions. Some examples are significant changes in diffusion properties and the temperature at which the liquid-solid phase transition takes place. Indeed, molecular dynamics simulations suggest that thin layers of water on a diamond surface may remain solid even well above room temperature. However, because of the small volumes that are involved, it is exceedingly difficult to examine these phenomena experimentally with current technologies. In this context, shallow NV centers promise a highly sensitive tool for the investigation of magnetic signals emanating from liquids and solids that are deposited on the surface of a diamond. Moreover, NV centers are non-invasive sensors with extraordinary performance even at room-temperature. To that end, we present here a theoretical work, complemented with numerical evidence based on bosonization techniques, that predicts the measurable signal from a single NV center when interacting with large spin baths in different configurations. We therefore propose single NV centers as sensors capable to resolve structural water features at the nanoscale and even sensitive to phase transitions.

quant-ph↗

Arbitrary Nuclear Spin Gates in Diamond Mediated by a NV-center Electron Spin

We propose a protocol that achieves arbitrary N-qubit interactions between nuclear spins and that can measure directly nuclear many-body correlators by appropriately making the nuclear spins interact with a nitrogen vacancy (NV) center electron spin. The method takes advantage of recently introduced dynamical decoupling techniques and demonstrates that action on the electron spin is sufficient to fully exploit nuclear spins as robust quantum registers. Our protocol is general, being applicable to other nuclear spin based platforms with electronic spin defects acting as mediators as the case of silicon carbide.

quant-ph↗

Towards hyperpolarization of oil molecules via nitrogen-vacancy centers in diamond

Efficient polarization of organic molecules is of extraordinary relevance when performing nuclear magnetic resonance (NMR) and imaging. Commercially available routes to dynamical nuclear polarization (DNP) work at extremely low-temperatures, thus bringing the molecules out of their ambient thermal conditions and relying on the solidification of organic samples. In this work we investigate polarization transfer from optically-pumped nitrogen vacancy centers in diamond to external molecules at room temperature. This polarization transfer is described by both an extensive analytical analysis and numerical simulations based on spin bath bosonization and is supported by experimental data in excellent agreement. These results set the route to hyperpolarization of diffusive molecules in different scenarios and consequently, due to increased signal, to high-resolution NMR.

quant-ph↗

Proposal for enhanced resolution in nanoscale NMR: quantum sensing with pulses of finite duration

The nitrogen vacancy (NV) color center in diamond is an enormously important platform for the development of quantum sensors, including for single spin and single molecule NMR. Detection of weak single-spin signals is greatly enhanced by repeated sequences of microwave pulses; in these dynamical decoupling (DD) techniques, the key control parameters swept in the experiment are the time intervals, $τ$, between pulses. Here we show that, in fact, the pulse duration offers a powerful additional control parameter. While previously, a non-negligible pulse-width has been considered simply a source of experimental error, here we elucidate the underlying quantum dynamics: we identify a landscape of quantum-state crossings which are usually closed (inactive) but may be controllably activated (opened) by adjusting the pulse-width from zero. We identify these crossings with recently observed but unexpected dips (so called spurious dips) seen in the quantum coherence of the NV spin. With this new understanding, both the position and strength of these sharp features may be accurately controlled; they co-exist with the usual broader coherence dips of short-duration microwave pulses, but their sharpness allows for higher resolution spectroscopy with quantum diamond sensors, or their analogues.

quant-ph↗

Steady state preparation of long-lived nuclear spin singlet pair at room temperature

The coherent high-fidelity generation of nuclear spins in long-lived singlet states which may find application as quantum memory or sensor represents a considerable experimental challenge. Here we propose a dissipative scheme that achieves the preparation of pairs of nuclear spins in long-lived singlet states by a protocol that combines the interaction between the nuclei and a periodically reset electron spin of an NV center with local rf-control of the nuclear spins. The final state of this protocol is independent of the initial preparation of the nuclei, is robust to external field fluctuations and can be operated at room temperature. We show that a high fidelity singlet pair of a 13C dimer in a nuclear bath in diamond can be generated under realistic experimental conditions.

quant-ph↗

Dissipatively stabilized quantum sensor based on indirect nuclear-nuclear interactions

We propose to use a dissipatively engineered nitrogen vacancy (NV) center as a mediator of interaction between two nuclear spins that are protected from decoherence and relaxation of the NV. Under ambient conditions this scheme achieves highly selective high-fidelity quantum gates between nuclear spins in a quantum register even at large NV-nuclear distances. Importantly, this method allows for the use of nuclear spins as a sensor rather than a memory, while the NV spin acts as an ancillary system for the initialization and read out of the sensor. The immunity to the decoherence and relaxation of the NV center leads to a tunable sharp frequency filter while allowing at the same time the continuous collection of the signal to achieve simultaneously high spectral selectivity and high signal-to-noise ratio (SNR).

quant-ph↗

Efficient tomography of a quantum many-body system

Quantum state tomography (QST) is the gold standard technique for obtaining an estimate for the state of small quantum systems in the laboratory. Its application to systems with more than a few constituents (e.g. particles) soon becomes impractical as the effort required grows exponentially in the number of constituents. Developing more efficient techniques is particularly pressing as precisely-controllable quantum systems that are well beyond the reach of QST are emerging in laboratories. Motivated by this, there is a considerable ongoing effort to develop new characterisation tools for quantum many-body systems. Here we demonstrate Matrix Product State (MPS) tomography, which is theoretically proven to allow the states of a broad class of quantum systems to be accurately estimated with an effort that increases efficiently with constituent number. We first prove that this broad class includes the out-of-equilbrium states produced by 1D systems with finite-range interactions, up to any fixed point in time. We then use the technique to reconstruct the dynamical state of a trapped-ion quantum simulator comprising up to 14 entangled spins (qubits): a size far beyond the reach of QST. Our results reveal the dynamical growth of entanglement and description complexity as correlations spread out during a quench: a necessary condition for future beyond-classical performance. MPS tomography should find widespread use to study large quantum many-body systems and to benchmark and verify quantum simulators and computers.

quant-ph↗

Decoherence enhances performance of quantum walks applied to graph isomorphism testing

Computational advantages gained by quantum algorithms rely largely on the coherence of quantum devices and are generally compromised by decoherence. As an exception, we present a quantum algorithm for graph isomorphism testing whose performance is optimal when operating in the partially coherent regime, as opposed to the extremes of fully coherent or classical regimes. The algorithm builds on continuous-time quantum stochastic walks (QSWs) on graphs and the algorithmic performance is quantified by the distinguishing power (DIP) between non-isomorphic graphs. The QSW explores the entire graph and acquires information about the underlying structure, which is extracted by monitoring stochastic jumps across an auxiliary edge. The resulting counting statistics of stochastic jumps is used to identify the spectrum of the dynamical generator of the QSW, serving as a novel graph invariant, based on which non-isomorphic graphs are distinguished. We provide specific examples of non-isomorphic graphs that are only distinguishable by QSWs in the presence of decoherence.

quant-ph↗

Transport enhancement from incoherent coupling between one-dimensional quantum conductors

We study the non-equilibrium transport properties of a highly anisotropic two-dimensional lattice of spin-1/2 particles governed by a Heisenberg XXZ Hamiltonian. The anisotropy of the lattice allows us to approximate the system at finite temperature as an array of incoherently coupled one-dimensional chains. We show that in the regime of strong intrachain interactions, the weak interchain coupling considerably boosts spin transport in the driven system. Interestingly, we show that this enhancement increases with the length of the chains, which is related to superdiffusive spin transport. We describe the mechanism behind this effect, compare it to a similar phenomenon in single chains induced by dephasing, and explain why the former is much stronger.

cond-mat.str-el↗

Hot entanglement in a simple dynamical model

How mixed can one component of a bi-partite system be initially and still become entangled through interaction with a thermalized partner? We address this question here. In particular, we consider the question of how mixed a two-level system and a field mode may be such that free entanglement arises in the course of the time evolution according to a Jaynes-Cummings type interaction. We investigate the situation for which the two-level system is initially in mixed state taken from a one-parameter set, whereas the field has been prepared in an arbitrary thermal state. Depending on the particular choice for the initial state and the initial temperature of the quantised field mode, three cases can be distinguished: (i) free entanglement will be created immediately, (ii) free entanglement will be generated, but only at a later time different from zero, (iii) the partial transpose of the joint state remains positive at all times. It will be demonstrated that increasing the initial temperature of the field mode may cause the joint state to become distillable during the time evolution, in contrast to a non-distillable state at lower initial temperatures. We further assess the generated entanglement quantitatively, by evaluating the logarithmic negativity numerically, and by providing an analytical upper bound.

quant-ph↗

Pulse-phase control for spectral disambiguation in quantum sensing protocols

We present a method to identify spurious signals generated by finite-width pulses in quantum sensing experiments and apply it to recently proposed dynamical decoupling sequences for accurate spectral interpretation. We first study the origin of these fake resonances and quantify their behavior in a situation that involves the measurement of a classical magnetic field. Here we show that a change of the initial phase of the sensor or, equivalently, of the decoupling pulses leads to oscillations in the spurious signal intensity while the real resonances remain intact. Finally we extend our results to the quantum regime for the unambiguous detection of remote nuclear spins by utilization of a nitrogen vacancy sensor in diamond.

quant-ph↗

Noise-resilient Quantum Computing with a Nitrogen-Vacancy Center and Nuclear Spins

Selective control of qubits in a quantum register for the purposes of quantum information processing represents a critical challenge for dense spin ensembles in solid state systems. Here we present a protocol that achieves a complete set of selective single and two-qubit gates on nuclear spins in such an ensemble in diamond facilitated by a nearby NV center. The protocol suppresses internuclear interactions as well as unwanted coupling between the NV center and other spins of the ensemble to achieve quantum gate fidelities well exceeding 99% . Notably, our method can be applied to weakly coupled, distant, spins and therefore represents a scalable procedure that exploits the exceptional properties of nuclear spins in diamond as robust quantum memories.

quant-ph↗

Coherent control of quantum systems as a resource theory

Control at the interface between the classical and the quantum world is fundamental in quantum physics. In particular, how classical control is enhanced by coherence effects is an important question both from a theoretical as well as from a technological point of view. In this work, we establish a resource theory describing this setting and explore relations to the theory of coherence, entanglement and information processing. Specifically, for the coherent control of quantum systems the relevant resources of entanglement and coherence are found to be equivalent and closely related to a measure of discord. The results are then applied to the DQC1 protocol and the precision of the final measurement is expressed in terms of the available resources.

quant-ph↗