arXiv subjects

M. B. Salamon

Publications and source records attributed to M. B. Salamon.

At least 37 records · Page 2Linked to original sources

arXiv2005

Anomalous Paramagnetic Effects in the Mixed State of LuNi2B2C

Anomalous paramagnetic effects in dc magnetization were observed in the mixed state of LuNi2B2C, unlike any reported previously. It appears as a kink-like feature for H > 30 kOe and becomes more prominent with increasing field. A specific heat jump at the corresponding temperature suggests that the anomaly is due to a true bulk transition. A magnetic flux transition from a square to an hexagonal lattice is consistent with the anomaly.

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arXiv2004

Evolution of superconducting order in Pr(Os$_{1-x}$Ru$_{x}$)$_{4}$Sb$_{12}$

We report measurements of the magnetic penetration depth $λ$ in single crystals of Pr(Os$_{1-x}$Ru$_{x}$)$_{4}$Sb$_{12}$ down to 0.1 K. Both $λ$ and superfluid density $ρ_{s}$ exhibit an exponential behavior for the $x$$\geq$0.4 samples, going from weak ($x$=0.4,0.6), to moderate, coupling ($x$=0.8). For the $x$$\leq$0.2 samples, both $λ$ and $ρ_{s}$ vary as $T^{2}$ at low temperatures, but $ρ_{s}$ is s-wave-like at intermediate to high temperatures. Our data are consistent with a three-phase scenario, where a fully-gapped phase at $T_{c1}$ undergoes two transitions: first to an unconventional phase at $T_{c2}$$\lesssim$$T_{c1}$, then to a nodal low-$T$ phase at $T_{c3}$$<$$T_{c2}$, for small values of $x$.

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arXiv2004

Study on Unconventional Superconductors via Angle-resolved Specific Heat

The gap function in unconventional superconductors may vanish at points or lines in momentum space, permitting electronic excitations, termed nodal quasiparticles, to exist at temperatures well below the superconducting transition. In the vortex phase, the presence of nodal quasiparticles should be directly observable through the variation of the heat capacity with the angle between a magnetic field and the location of the zeroes of the gap. The heat capacity of candidate non-magnetic unconventional superconductors Lu(Y)Ni2B2C were found to exhibit fourfold oscillations with field angle, the first such observation. The observed angular variations are in quantitative agreement with theory, confirming that quasiparticles are created via Doppler shifts at nodes along <100>. Anomalous disorder effects have been also observed in the field-angle dependent heat capacity C_{p}(α). In a slightly disordered sample, anomalous secondary minima along <110> appeared for μ_{0}H > 1 T, leading to an eightfold pattern. The coexistence of an anisotropic superconducting gap and nonlocal effects is shown to drive the anomalous behavior. These results demonstrate that field-angle-dependent heat capacity can be a powerful tool in probing the momentum-space gap structure in unconventional superconductors such as high T_{c} cuprates, heavy fermions, borocarbides, etc.

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arXiv2004

Lamellar phase separation and dynamic competition in La0.23Ca0.77MnO3

We report the coexistence of lamellar charge-ordered (CO) and charge-disordered (CD) domains, and their dynamical behavior, in La0.23Ca0.77MnO3. Using high resolution transmission electron microscopy (TEM), we show that below Tcd~170K a CD-monoclinic phase forms within the established CO-orthorhombic matrix. The CD phase has a sheet-like morphology, perpendicular to the q vector of the CO superlattice (a axis of the Pnma structure). For temperatures between 64K and 130K, both the TEM and resistivity experiments show a dynamic competition between the two phases: at constant T, the CD phase slowly advances over the CO one. This slow dynamics appears to be linked to the magnetic transitions occurring in this compound, suggesting important magnetoelastic effects.

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arXiv2004

Specific Heat Study of the Magnetic Superconductor HoNi2B2C

The complex magnetic transitions and superconductivity of HoNi2B2C were studied via the dependence of the heat capacity on temperature and in-plane field angle. We provide an extended, comprehensive magnetic phase diagram for B // [100] and B // [110] based on the thermodynamic measurements. Three magnetic transitions and the superconducting transition were clearly observed. The 5.2 K transition (T_{N}) shows a hysteresis with temperature, indicating the first order nature of the transition at B=0 T. The 6 K transition (T_{M}), namely the onset of the long-range ordering, displays a dramatic in-plane anisotropy: T_{M} increases with increasing magnetic field for B // [100] while it decreases with increasing field for B // [110]. The anomalous anisotropy in T_{M} indicates that the transition is related to the a-axis spiral structure. The 5.5 K transition (T^{*}) shows similar behavior to the 5.2 K transition, i.e., a small in-plane anisotropy and scaling with Ising model. This last transition is ascribed to the change from a^{*} dominant phase to c^{*} dominant phase.

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arXiv2004

Evidence for the Coexistence of Anisotropic Superconducting Gap and Nonlocal Effects in the Non-magnetic Superconductor LuNi2B2C

A study of the dependence of the heat capacity Cp(alpha) on field angle in LuNi2B2C reveals an anomalous disorder effect. For pure samples, Cp(alpha) exhibits a fourfold variation as the field H < Hc2 is rotated in the [001] plane, with minima along <100> (alpha = 0). A slightly disordered sample, however, develops anomalous secondary minima along <110> for H > 1 T, leading to an 8-fold pattern. The anomalous pattern is discussed in terms of coexisting superconducting gap anisotropy and non-local effects.

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arXiv2004

Berry's phase contribution to the anomalous Hall effect of gadolinium

When conduction electrons are forced to follow the local spin texture, the resulting Berry phase can induce an anomalous Hall effect (AHE). In gadolinium, as in double-exchange magnets, the exchange interaction is mediated by the conduction electrons and the AHE may therefore resemble that of chromium dioxide and other metallic double-exchange ferromagnets. The Hall resistivity, magnetoresistance, and magnetization of single crystal gadolinium were measured in fields up to 30 T. Measurements between 2 K and 400 K are consistent with previously reported data. A scaling analysis for the Hall resistivity as a function of the magnetization suggests the presence of a Berry's-phase contribution to the anomalous Hall effect.

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arXiv2004

Probing the superconducting gap symmetry of PrRu$_{4}$Sb$_{12}$: A comparison with PrOs$_{4}$Sb$_{12}$

We report measurements of the magnetic penetration depth $λ$ in single crystals of PrRu$_{4}$Sb$_{12}$ down to 0.1 K. Both $λ$ and superfluid density $ρ_{s}$ exhibit an exponential behavior for $T$ $<$ 0.5$T_{c}$, with parameters $Δ$(0)/\textit{k}$_{B}$\textit{T}$_{c}$ = 1.9 and $λ(0)$ = 2900 Å. The value of $Δ$(0) is consistent with the specific-heat jump value of $ΔC/γT_{c}$ = 1.87 measured elsewhere, while the value of $λ(0)$ is consistent with the measured value of the electronic heat-capacity coefficient $γ$. Our data are consistent with PrRu$_{4}$Sb$_{12}$ being a moderate-coupling, fully-gapped superconductor. We suggest experiments to study how the nature of the superconducting state evolves with increasing Ru substitution for Os.

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arXiv2003

Direct Observation of Nodal Quasiparticles in an Unconventional Superconductor: Field-angle Dependent Heat Capacity of YNi2B2C

Field-angle dependent heat capacity of the non-magnetic borocarbide superconductor YNi2B2C reveals a clear fourfold oscillation, the first observation of its kind. The observed angular variations were analyzed as a function of magnetic field angle, field intensity and temperature to provide its origin. The quantitative agreement between experiment and theory strongly suggests that we are directly observing nodal quasiparticles generated along <100> by the Doppler effect. The results demonstrate that field-angle heat capacity can be a powerful tool in probing the momentum-space gap structure in unconventional superconductors such as high Tc cuprates, heavy fermion superconductors, etc.

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arXiv2003

Probing the superconducting gap symmetry of PrOs$_{4}$Sb$_{12}$: A penetration depth study

We report measurements of the magnetic penetration depth $λ$ in single crystals of PrOs$_{4}$Sb$_{12}$ down to $\sim$0.1 K using a tunnel-diode based, self-inductive technique at 21 MHz, with the ac field applied along the \textit{a}, \textit{b} and \textit{c} directions. In all three field orientations the penetration depth and superfluid density $ρ_{s}$ tend to follow a power law, $λ\sim \mathit{T}^{2}, ρ_{s} \sim \mathit{T}% ^{2}$ at low temperatures. $ρ_{s}$ for various gap functions have been calculated, and data is best fit by the $^{3}$He A-phase-like gap with multidomains, each having two point nodes along a cube axis, and parameter $Δ_{0}$(0)/\textit{k}$_{B}$\textit{T}$_{c}$ = 2.6. This suggests that PrOs$_{4}$Sb$_{12}$ is a strong-coupling superconductor with two point nodes on the Fermi surface. We also confirm the observation of the double transitions at 1.75 K and 1.85 K seen in other measurements.

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arXiv2003

Griffiths singularities and magnetoresistive manganites

The large, so-called colossal, magnetoresistivity of doped manganese oxides based on LaMnO3 has attracted considerable attention, but only one unusual feature of the ferromagnetic transition in these compounds. We examine in this paper the progression of magnetic and thermodynamic behavior as the transition temperature is made to vary from 360 K to 218 K by changing the divalent dopant. Single crystals of La_{0.7}Sr_{0.3}MnO3, as is well known, show modest magnetoresistivity and conventional critical behavior. La$_{0.7}$Pb$_{0.3}$ Mn$O_3$, and to an even greater extent, La$_{0.7}$Ca$_{0.3}$MnO$_3$, have unusual magnetic properties extending more than 100 K above the transition. We treat the properties of the latter samples in the context of a Griffiths phase in which the transition temperature is depressed from its maximum value T_{G} by random bond-angle bending.

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arXiv2002

Fluctuation Study of the Specific Heat of MgB2

The specific heat of polycrystalline Mg$^{11}$B$_{2}$ has been measured with high resolution ac calorimetry from 5 to 45 K at constant magnetic fields. The excess specific heat above T$_{c}$ is discussed in terms of Gaussian fluctuations and suggests that Mg$^{11}$B$_{2}$ is a bulk superconductor with Ginzburg-Landau coherence length $ξ_{0}=26$ Å. The transition-width broadening in field is treated in terms of lowest-Landau-level (LLL) fluctuations. That analysis requires that $ξ_{0}=20$ Å. The underestimate of the coherence length in field, along with deviations from 3D LLL predictions, suggest that there is an influence from the anisotropy of B$_{c2}$ between the c-axis and the a-b plane.

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arXiv2002

Anomalous Hall Effect of Calcium-doped Lanthanum Cobaltite Films

The Hall resistivity, magnetoresistance, and magnetization of La_{1-x}Ca_{x}CoO_{3} epitaxial films with x between 0.25 and 0.4 grown on lanthanum aluminate were measured in fields up to 7 T. The x=1/3 film, shows a reentrant metal insulator transition. Below 100 K, the x=1/3 and 0.4 films have significant coercivity which increases with decreasing temperature. At low temperature the Hall resistivity remains large and essentially field independent in these films, except for a sign change at the coercive field that is more abrupt than the switching of the magnetization. A unique magnetoresistance behavior accompanies this effect. These results are discussed in terms of a percolation picture and the mixed spin state model for this system. We propose that the low-temperature Hall effect is caused by spin-polarized carriers scattering off of orbital disorder in the spin-ordered clusters.

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arXiv2002

Non-Locality and Strong Coupling in the Heavy Fermion Superconductor CeCoIn$_{5}$: A Penetration Depth Study

We report measurements of the magnetic penetration depth $λ$ in single crystals of CeCoIn$_{5}$ down to $\sim$0.14 K using a tunnel-diode based, self-inductive technique at 28 MHz. While the in-plane penetration depth tends to follow a power law, $λ_{//} \sim {\it T}^{3/2}$, the data are better described as a crossover between linear ({\it T} $\gg $ ${\it T}^\ast $) and quadratic ({\it T} $\ll {\it T}^\ast $) behavior, with ${\it T}^\ast $ the crossover temperature in the strong-coupling limit. The {\it c}-axis penetration depth $λ_{\perp} $ is linear in {\it T}, providing evidence that CeCoIn$_{5}$ is a {\it d}-wave superconductor with line nodes along the {\it c}-axis. The different temperature dependences of $λ_{//} $ and $λ_{\perp} $ rule out impurity effects as the source of ${\it T}^{\ast} $.

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arXiv2002

Skyrmion strings and the anomalous Hall effect in CrO$_2$

As in such 2D systems as the XY model, topological (or singularity point) defects are thought to play a crucial role in the phase transitions of 3D spin systems. In double exchange (DE) ferromagnets, the conduction electrons are strongly coupled with core spins through Hund's rule, and in the presence of non-trivial spin texture, acquire a Berry phase contribution to the anomalous Hall effect (AHE). We combine Hall and magnetization data on CrO$_2$ with a thermodynamical scaling hypothesis to confirm that the critical behavior of the topological-spin-defect density is consistent with that of the heat capacity. This analysis is the first experimental confirmation of the topological character of critical fluctuations.

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arXiv2002

Colossal Magnetoresistance is a Griffiths Singularity

It is now widely accepted that the magnetic transition in doped manganites that show large magnetoresistance is a type of percolation effect. This paper demonstrates that the transition should be viewed in the context of the Griffiths phase that arises when disorder suppresses a magnetic transition. This approach explains unusual aspects of susceptibility and heat capacity data from a single crystal of La$_{0.7}$Ca$_{0.3}$MnO$_{3}.$

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arXiv2000

Charge Transport in Manganites: Hopping Conduction, the Anomalous Hall Effect and Universal Scaling

The low-temperature Hall resistivity ρ_{xy} of La_{2/3}A_{1/3}MnO_3 single crystals (where A stands for Ca, Pb and Ca, or Sr) can be separated into Ordinary and Anomalous contributions, giving rise to Ordinary and Anomalous Hall effects, respectively. However, no such decomposition is possible near the Curie temperature which, in these systems, is close to metal-to-insulator transition. Rather, for all of these compounds and to a good approximation, the ρ_{xy} data at various temperatures and magnetic fields collapse (up to an overall scale), on to a single function of the reduced magnetization m=M/M_{sat}, the extremum of this function lying at m~0.4. A new mechanism for the Anomalous Hall Effect in the inelastic hopping regime, which reproduces these scaling curves, is identified. This mechanism, which is an extension of Holstein's model for the Ordinary Hall effect in the hopping regime, arises from the combined effects of the double-exchange-induced quantal phase in triads of Mn ions and spin-orbit interactions. We identify processes that lead to the Anomalous Hall Effect for localized carriers and, along the way, analyze issues of quantum interference in the presence of phonon-assisted hopping. Our results suggest that, near the ferromagnet-to-paramagnet transition, it is appropriate to describe transport in manganites in terms of carrier hopping between states that are localized due to combined effect of magnetic and non-magnetic disorder. We attribute the qualitative variations in resistivity characteristics across manganite compounds to the differing strengths of their carrier self-trapping, and conclude that both disorder-induced localization and self-trapping effects are important for transport.

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arXiv2000

Reentrant spin glass behavior in a layered manganite La1.2Sr1.8Mn2O7 single crystals

We report here a detailed study of AC/DC magnetization and longitudinal/transverse transport properties of La$_{1.2}$Sr$_{1.8}$Mn$_{2}$O$_{7}$ single crystals below $T_{c}$ = 121 K. We find that the resistivity upturn below 40 K is related to the reentrant spin glass phase at the same temperature, accompanied by additional anomalous Hall effects. The carrier concentration from the ordinary Hall effects remains constant during the transition and is close to the nominal doping level (0.4 holes/Mn). The spin glass behavior comes from the competition between ferromagnetic double exchange and antiferromagnetic superexchange interactions, which leads to phase separation, i.e. a mixture of ferromagnetic and antiferromagnetic clusters, representing the canted antiferromagnetic state.

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