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M. B. Silva Neto

Publications and source records attributed to M. B. Silva Neto.

At least 19 recordsLinked to original sources

Quantum-Critical, Spin-Fluctuation-driven Residual Resistivity and Emergent Universal Correlations in the Fermi-Liquid Regime of Heavy-Fermion Superconductors

We investigate correlations within the unconventional Fermi-liquid (FL) regime of quantum-critical (QC) heavy-fermion superconductors (HFSs) by tracking the pressure dependence of three quantities: the temperature-independent, SF-driven residual resistivity, $ρ^{ sf}_{0}(P)$; the FL scattering coefficient, $A(P)$; and the superconducting transition temperature, $T_c(P)$. The first two define the spin-fluctuation contribution to the resistivity, $ρ(T)=ρ^{sf}_0+AT^2$. Using experimental data from archetypal heavy-fermion systems, we identify three robust empirical correlations: $\ln(\frac{T_c}θ) \propto A^{-1/2}$, $A \propto (ρ^{sf}_0)^2$, and $\ln(\frac{T_c}θ) \propto \big(ρ^{sf}_0\big)^{-1}$ ($θ$ is a characteristic temperature scale). Absent in conventional FL superconductors, these relationships indicate that QC fluctuations not only mediate inelastic scattering and Cooper pairing, but also generate an effective elastic channel responsible for $ρ^{sf}_0$. We explicitly calculate $ρ^{sf}_0$ on the high-pressure side of the quantum critical point (QCP) and introduce a characteristic length scale, $\ell \sim \big(ρ^{sf}_0\big)^{-1}$, that captures the spatial extent of fluctuation-induced scattering. Within this regime, and within the Migdal--Eliashberg framework combined with Boltzmann transport theory, we derive analytic expressions for $T_c(\ell)$ and $A(\ell)$, together with their interrelations, which are consistent with the observed empirical trends. These findings highlight the quantum-critical FL regime in HFSs as an intrinsically correlated phase, governed by fluctuations and marked by unconventional transport and pairing mechanisms.

cond-mat.str-el

Pressure-induced hole delocalization in the strongly correlated quasicubic charge-transfer perovskite $LaBa_2Fe_3O_{8+δ}$d

Analysis of the thermal and baric evolution of resistance in $LaBa_2Fe_3O_{8+δ}$ enabled the construction of its pressure-temperature (P-T) phase diagram, which prominently displays a critical boundary, $P^{MIT}_c(T)$, marking the transition from localized to hole-type extended states. The relatively low critical pressures [$P^{MIT}_c(T) \approx 3$-8 GPa] suggest that, as $P \rightarrow P_c$ in this narrow-gap, strongly correlated charge-transfer system, both the hybridization strength and the charge-transfer character are progressively enhanced - ultimately leading to the emergence of metallicity. Emphasizing the electronic nature of this transition, pressure-dependent structural analyses at room temperature reveal no associated structural phase transition at $P^{MIT}_c(T)$; the system retains a (weakly tetragonally distorted) quasicubic perovskite structure with Murnaghan-type compressibility up to 30\,GPa. The emergence of hole delocalization and metallic conduction, coupled with suppressed antiferromagnetism, suggests proximity to quantum criticality.

cond-mat.str-el

Investigation of role of antisite disorder in the pristine cage compound FeGa$_3$

The role of controlled disorder in the strong correlated narrow gap semiconductor candidate FeGa$_3$ has been investigated. Polycrystalline samples were synthesized by the combination of arc-melting furnace and successive annealing processes. Deviations of the occupation number of Fe and Ga sites from those expected in the pristine compound were quantified with X-ray analysis. Besides that, electrical transport and magnetization measurements reveal that hierarchy in Fe and Ga site disorder tunes the ground state of FeGa$_3$ from paramagnetic semiconducting to a magnetic metal. These findings are discussed within the framework of Anderson metal-insulator transitions and spin fluctuations.

cond-mat.mtrl-sci

Controlling spontaneous emission in inertial and dissipative nematic liquid crystals: the role of critical phenomena

We develop a rigorous, field-theoretical approach to the study of spontaneous emission in inertial and dissipative nematic liquid crystals, disclosing an alternative application of the massive Stueckelberg gauge theory to describe critical phenomena in these systems. This approach allows one not only to unveil the role of phase transitions in the spontaneous emission in liquid crystals but also to make quantitative predictions for quantum emission in realistic nematics of current scientific and technological interest in the field of metamaterials. Specifically, we predict that one can switch on and off quantum emission in liquid crystals by varying the temperature in the vicinities of the crystalline-to-nematic phase transition, for both the inertial and dissipative cases. We also predict from first principles the value of the critical exponent that characterizes such a transition, which we show not only to be independent of the inertial or dissipative dynamics, but also to be in good agreement with experiments. We determine the orientation of the dipole moment of the emitter relative to the nematic director that inhibits spontaneous emission, paving the way to achieve directionality of the emitted radiation, a result that could be applied in tuneable photonic devices such as metasurfaces and tuneable light sources.

cond-mat.mes-hall

Defect-engineered, universal kinematic correlations between superconductivity and Fermi liquid transport

Identifying universal scaling relations between two or more variables in a complex system plays a pivotal role in understanding various phenomena in different branches of science. Examples include the allometric scaling among food webs in biology, the scaling relationship between fluid flow and fracture stiffness in geophysics, and the gap-to-$T_c$ ratio, between energy gap, $Δ$, and critical transition temperature, $T_c$, hallmarks of superconductivity. Kinematics, in turn, is the branch of physics that governs the motion of bodies by imposing constraints correlating their masses, momenta, and energy; it is an essential ingredient for the analysis of high-energy quarkonium production, galaxy formation, as well as the $ρ_\circ+AT^2$ contribution to the normal state resistivity in a Fermi liquid (FL), $ρ_\circ$ being a measure of disorder and $A$ the hallmark of FL. Here, we report on the identification of a novel, universal kinematic scaling relation between $T_c(ρ_\circ)$ and $A(ρ_\circ)$ found in a plethora of defect-bearing conventional and non-conventional superconductors within their FL regime. We traced back this relation to the triggering and stabilization of an electron-electron scattering channel within a very specific, yet common, type of amorphized regions, ubiquitous in all such superconductors. Our theoretical treatment consisted of, first, analyzing the construct of a distorted lattice as a mimic of the kinematic aftermath of the formation of such amorphized regions. Then we applied standard many body techniques to derive expressions for $T_c(ρ_\circ)$, $A(ρ_\circ)$, and their correlations. Our results are in agreement with experiments and provide a solid theoretical foundation for reconciling superconductivity with FL transport in these systems.

cond-mat.supr-con

Unconventional superconductivity as a synchronization problem in nuclear oscillator networks

We formulate the problem of unconventional $d-$wave superconductivity, with phase fluctuations, pseudogap phenomenon, and local Cooper pairs, in terms of a synchronization problem in random, quantum dissipative, elasto-nuclear oscillator networks. The nodes of the network correspond to {\it localized, collective quadrupolar vibrations} of nuclei-like, elastic inhomogeneities embedded in a dissipative medium. Electrons interacting with such vibrations form local Cooper pairs, with a superfluid $d-$wave pseudogap $Δ_{PG}$, due to an effective, short range attractive interaction of $d_{x^2-y^2}$ character. Phase coherent, bulk superconductivity, with a $d-$wave gap $Δ$, is stabilized when the oscillator network is asymptotically entangled in a nearly decoherence-free environment. Phase coherence will in turn be destroyed, at $T_c$, when the thermal noise becomes comparable to the coupling between oscillators, the superfluid density $K$. The $2Δ/k_B T_c$ ratio is a function of Kuramoto's order parameter, $r=\sqrt{1-K_c/K}$, for the loss of synchronization at $K_c$, and is much larger than the nonuniversal $2Δ_{PG}/k_B T^*$ ratio, where $T^*$ is the temperature at which $Δ_{PG}$ is completely destroyed by thermal fluctuations. We discuss our findings in connection to the available data for various unconventionally high-temperature superconductors.

cond-mat.supr-con

Controlling spontaneous emission via electronic correlations in transparent metals

We study the spontaneous emission of agglomerates of two-level quantum emitters embedded in a correlated transparent metal. The characteristic emission energy corresponds to the splitting between ground and excited states of a neutral, nonmagnetic molecular impurity (F color center), while correlations are due to the existence of narrow bands in the metal. This is the case of transition metal oxides with an ABO3 Perovskite structure, such as SrVO3 and CaVO3, where oxygen vacancies are responsible for the emission of visible light, while the correlated metallic nature arises from the partial filling of a band with mostly d-orbital character. For these systems we put forward an interdisciplinary, tunable mechanism to control light emission governed by electronic correlations. We show that not only there exists a critical value for the correlation strength above which the metal becomes transparent in the visible, but also that strong correlations can lead to a remarkable enhancement of the light-matter coupling. By unveiling the role of electronic correlations in spontaneous emission, our findings set the basis for the design of controllable, solid-state, single-photon sources in correlated transparent metals.

cond-mat.str-el

Nonradiative emission and absorption rates of quantum emitters embedded in metallic systems: microscopic description and their determination from electronic transport

We investigate nonradiative emission and absorption rates of two-level quantum emitters embedded in a metal at low temperatures. We obtain the expressions for both nonradiative transition rates and identify a unique, experimentally accessible way to obtain the nonradiative decay rates via electronic transport in the host metallic system. Our findings not only provide a microscopic description of nonradiative decay channels in metals, but they also allows one to identify and differentiate them from other decay channels, which is crucial to understand and control light-matter interactions at the nanoscale.

cond-mat.mes-hall

Magnetic quantum phase transitions of the antiferromagnetic J_{1}-J_{2} Heisenberg model

We obtain the complete phase diagram of the antiferromagnetic $J_{1}$-$J_{2}$ model, $0\leq α= J_2/J1 \leq 1$, within the framework of the $O(N)$ nonlinear sigma model. We find two magnetically ordered phases, one with N\' eel order, for $α\leq 0.4$, and another with collinear order, for $α\geq 0.6$, separated by a nonmagnetic region, for $0.4\leq α\leq 0.6$, where a gapped spin liquid is found. The transition at $α=0.4$ is of the second order while the one at $α=0.6$ is of the first order and the spin gaps cross at $α=0.5$. Our results are exact at $N\rightarrow\infty$ and agree with numerical results from different methods.

cond-mat.str-el

Skyrmions in a Doped Antiferromagnet

Magnetization and magnetoresistance have been measured in insulating antiferromagnetic La_{2}Cu_{0.97}Li_{0.03}O_{4} over a wide range of temperatures, magnetic fields, and field orientations. The magnetoresistance step associated with a weak ferromagnetic transition exhibits a striking nonmonotonic temperature dependence, consistent with the presence of skyrmions.

cond-mat.str-el

Hybridization driven quantum critical behavior in weakly-itinerant ferromagnets

We investigate the unusual magnetic properties of nearly-critical, weakly-itinerant ferromagnets with general formula UTX, where T=Rh,Co and X=Ge,Si. As a unique feature about these systems, we show that changes in the V_{df} hybridization control their proximity to a ferromagnetic instability, and determine the evolution of: the ground state magnetization, M_0, the Curie Temperature, T_C, the density of states at the Fermi level, N(E_F), the T^2 resistivity coefficient, A, and the specific heat coefficient, γ. The universal aspect of our findings comes from the dependence on only two parameters: the T_d bandwidth, W_d, and the distance between T_d and U_f band centers, C_{T_d}-C_{U_f}.

cond-mat.str-el

Magnetic and Quasiparticle Excitation Spectra of an Itinerant $J_1-J_2$ Model for Iron Pnictide Superconductors

We calculate the magnetic and quasiparticle excitation spectra of an itinerant $J_1-J_2$ model for iron pnictides. In addition to an acoustic spin-wave branch, the magnetic spectrum has a second, optical branch, resulting from the coupled four-sublattice magnetic structure. The spin-wave velocity has also a planar directional anisotropy, due to the collinear/striped antiferromagnetism. Within the magnetically ordered phase, the quasiparticle spectrum is composed of two Dirac cones, resulting from the folding of the magnetic Brillouin zone. We discuss the relevance of our findings to the understanding of both neutron scattering and photoemission spectroscopy results for SrFe$_{2}$As$_{2}$.

cond-mat.str-el

Strong correlations and the anisotropy of acceptor states in insulating La(2-x)Sr(x)CuO(4)

We use the Green's function formalism to discuss the role of strong correlations to the spatial structure of acceptor states doped into a two-dimensional Mott-Hubbard antiferromagnetic insulator. When the scattering between doped carriers, at the nesting wave vector ${\bf Q}=(π,π)$, is strong enough to produce a momentum dependent scattering rate, $Γ_{\bf k}$, the corresponding acceptor states become spatially anisotropic. As an example, we calculate the spatial structure of an acceptor state bound to an attractive two-dimensional Dirac delta potential, for a simple form of $Γ_{\bf k}$. We then discuss the role of such spatial anisotropy for the understanding of an apparent discrepancy between low temperature transport data and photoemission spectra in lightly doped La(2-x)Sr(x)CuO(4).

cond-mat.str-el

AC and DC Conductivity Anisotropies in Lightly Doped La(2-x)Sr(x)CuO(4)

The AC and DC conductivity anisotropies in the low temperature orthorhombic phase of lightly doped La(2-x)Sr(x)CuO(4) are ascribed to the rotational symmetry broken, localized impurity states resulting from the trapping of doped holes by Sr ions. The two lowest-energy p-wave-like states are split by orthorhombicity and partially filled with holes. This leaves a unique imprint in AC conductivity, which shows two distinct infrared continuum absorption energies. Furthermore, the existence of two independent channels for hopping conductivity, associated to the two orthorhombic directions, explains quantitatively the observed low temperature anisotropies in DC conductivity.

cond-mat.str-el

Negative Hopping Magnetoresistance and Dimensional Crossover in Lightly Doped Cuprate Superconductors

We show that, due to the weak ferromagnetism of La$_{2-x}$Sr$_x$CuO$_4$, an external magnetic field leads to a dimensional crossover 2D $\to$ 3D for the in-plane transport. The crossover results in an increase of the hole's localization length and hence in a dramatic negative magnetoresistance in the variable range hopping regime. This mechanism quantitatively explains puzzling experimental data on the negative magnetoresistance in the Néel phase of La$_{2-x}$Sr$_x$CuO$_4$.

cond-mat.str-el

Impurity susceptibility and the fate of spin-flop transitions in lightly-doped La(2)CuO(4)

We investigate the occurrence of a two-step spin-flop transition and spin reorientation when a longitudinal magnetic field is applied to lightly hole-doped La(2)CuO(4). We find that for large and strongly frustrating impurities, such as Sr in La(2-x)Sr(x)CuO(4), the huge enhancement of the longitudinal susceptibility suppresses the intermediate flop and the reorientation of spins is smooth and continuous. Contrary, for small and weakly frustrating impurities, such as O in La(2)CuO(4+y), a discontinuous spin reorientation (two-step spin-flop transition) takes place. Furthermore, we show that for La(2-x)Sr(x)CuO(4) the field dependence of the magnon gaps differs qualitatively from the La(2)CuO(4) case, a prediction to be verified with Raman spectroscopy or neutron scattering.

cond-mat.str-el

Competing impurities and reentrant magnetism in La(2-x)Sr(x)Cu(1-z)Zn(z)O(4) revisited. The role of the Dzyaloshinskii-Moriya and XY anisotropies

We study the order-from-disorder transition and reentrant magnetism in La(2-x)Sr(x)Cu(1-z)Zn(z)O(4) within the framework of a long-wavelength nonlinear sigma model that properly incorporates the Dzyaloshinskii-Moriya and XY anisotropies. Doping with nonmagnetic impurities, such as Zn, is considered according to classical percolation theory, whereas the effect of Sr, which introduces charge carriers into the CuO(2) planes, is described as a dipolar frustration of the antiferromagnetic order. We calculate several magnetic, thermodynamic, and spectral properties of the system, such as the antiferromagnetic order parameter, the Neel temperature, the spin-stiffness, and the anisotropy gaps, as well as their evolution with both Zn and Sr doping. We explain the nonmonotonic and reentrant behavior experimentally observed for T_N by Hucker et al. in Phys. Rev. B 59, R725 (1999), as resulting from the reduction, due to the nonmagnetic impurities, of the dipolar frustration induced by the charge carriers (order-from-disorder). Furthermore, we find a similar nonmonotonic and reentrant behavior for all the other observables studied. Most remarkably, our results show that while for x=2% and z=0 the Dzyaloshinskii-Moriya gap Δ_{DM}=0, for z=15% it is approximately Δ_{DM} = 7.5 cm^(-1). The later is larger than the lowest low-frequency cutoff for Raman spectroscopy (~ 5 cm^(-1)), and could thus be observed in one-magnon Raman scattering.

cond-mat.str-el

Field dependence of the magnetic spectrum in anisotropic and Dzyaloshinskii-Moriya antiferromagnets: I. Theory

We consider theoretically the effects of an applied uniform magnetic field on the magnetic spectrum of anisotropic two-dimensional and Dzyaloshinskii-Moriya layered quantum Heisenberg antiferromagnets. The first case is relevant for systems such as the two-dimensional square lattice antiferromagnet Sr(2)CuO(2)Cl(2), while the later is known to be relevant to the physics of the layered orthorhombic antiferromagnet La(2)CuO(4). We first establish the correspondence betwenn the low-energy spectrum obtained within the anisotropic non-linear sigma model and by means of the spin-wave approximation for a standard easy-axis antiferromagent. Then, we focus on the field-theory approach to calculate the magnetic field dependence of the magnon gaps and spectral intensities for magnetic fields applied along the three possible crystallographic directions. We discuss the various possible ground states and their evolution with temperature for the different field orientations, and the occurrence of spin-flop transitions for fields perpendicular to the layers (transverse fields) as well as for fields along the easy axis (longitudinal fields). Measurements of the one-magnon Raman spectrum in Sr(2)CuO(2)Cl(2) and La(2)CuO(4) and a comparison between the experimental results and the predictions of the present theory will be reported in part II of this research work [L. Benfatto et al., cond-mat/0602664].

cond-mat.str-el