arXiv subjects

M. Barbui

Publications and source records attributed to M. Barbui.

At least 19 recordsLinked to original sources

arXiv2025

Quantifying alpha clustering in the ground states of 16-O and 20-Ne

Understanding the role of multi-nucleon correlations in the structure of light nuclei is at the forefront of modern nuclear science. In this letter, we present a quantitative benchmark study of alpha-cluster correlations in the ground states of 16-O and 20-Ne. Experimental data provide direct evidence that the wave functions of the ground states of 16-O and 20-Ne are dominated by alpha-cluster correlations, in agreement with the predictions of sophisticated nuclear structure models. We also provide a new model-independent constraint for the alpha asymptotic normalization coefficient of the 16-O ground state and discuss the implications of these findings on the 12-C(alpha,gamma)16-O reaction, which is of critical importance for nuclear astrophysics.

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arXiv2025

Potential absence of observed $\pi^2$ linear-chain structures in $^{14}$O via $^{10}$C($\alpha,\alpha$) resonant scattering

Background: The preference for light nuclear systems to coagulate into $\alpha$-particle clusters has been well-studied. The possibility of a linear chain configuration of $\alpha$-particles would allow for a new way to study this phenomenon. Purpose: A rotational band of states in $^{14}$C has been claimed showing a $\pi^2$ linear chain structure. The mirror system, $^{14}$O, has been studied here to examine how this linear chain structure is affected by replacing the valence neutrons with protons. Method: A beam of $^{10}$C was incident into a chamber filled with He:CO$_2$ gas with the tracks recorded inside the TexAT Time Projection Chamber and the recoil $\alpha$-particles detected by a silicon detector array to measure the $^{10}\mathrm{C}(\alpha,\alpha)$ cross section. Results: The experimental cross section was compared with previous studies and fit using R-Matrix theory with the previously-observed $^{14}$O states being transformed to the $^{14}$C using mirror symmetry. The measured cross section does not replicate the claimed states, with the predicted cross section exceeding that observed at several energies and angles. Conclusion: A series of possibilities are highlighted with the most likely being that the originally-seen $^{14}$C states did not constitute a $\pi^2$ rotational band with a potentially incorrect spin assignment due to the limitations of the angular correlation method with non-zero spin particles. The work highlights the difficulties in measuring broad resonances corresponding to a linear chain state in a high level density.

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arXiv2024

Cluster structure of 3$\alpha$+p states in $^{13}$N

Background: Cluster states in $^{13}$N are extremely difficult to measure due to the unavailability of $^{9}$B+$\alpha$ elastic scattering data. Purpose: Using $\beta$-delayed charged-particle spectroscopy of $^{13}$O, clustered states in $^{13}$N can be populated and measured in the 3$\alpha$+p decay channel. Method: One-at-a-time implantation/decay of $^{13}$O was performed with the Texas Active Target Time Projection Chamber (TexAT TPC). 149 $\beta 3\alpha p$ decay events were observed and the excitation function in $^{13}$N reconstructed. Results: Four previously unknown $\alpha$-decaying excited states were observed in $^{13}$N at an excitation energy of 11.3 MeV, 12.4 MeV, 13.1 MeV and 13.7 MeV decaying via the 3$\alpha$+p channel. Conclusion: These states are seen to have a [$^{9}\mathrm{B}(\mathrm{g.s}) \bigotimes \alpha$/ $p+^{12}\mathrm{C}(0_{2}^{+})$], [$^{9}\mathrm{B}(\frac{1}{2}^{+}) \bigotimes \alpha$], [$^{9}\mathrm{B}(\frac{5}{2}^{+}) \bigotimes \alpha$] and [$^{9}\mathrm{B}(\frac{5}{2}^{+}) \bigotimes \alpha$] structure respectively. A previously-seen state at 11.8 MeV was also determined to have a [$p+^{12}\mathrm{C}(\mathrm{g.s.})$/ $p+^{12}\mathrm{C}(0_{2}^{+})$] structure. The overall magnitude of the clustering is not able to be extracted however due to the lack of a total width measurement. Clustered states in $^{13}$N (with unknown magnitude) seem to persist from the addition of a proton to the highly $\alpha$-clustered $^{12}$C. Evidence of the $\frac{1}{2}^{+}$ state in $^{9}$B was also seen to be populated by decays from $^{13}$N$^{\star}$.

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arXiv2023

Radiative decay branching ratio of the Hoyle state

Background: The triple-alpha process is a vital reaction in nuclear astrophysics, characterized by two consecutive reactions [$2\alpha\leftrightarrows{^{8}\rm{Be}}(\alpha,\gamma){^{12}\rm{C}}$] that drive carbon formation. The second reaction occurs through the Hoyle state, a 7.65 MeV excited state in ${^{12}\rm{C}}$ with $J^{\pi}=0^{+}$. The rate of the process depends on the radiative width, which can be determined by measuring the branching ratio for electromagnetic decay. Recent measurements by Kib\'edi et al. conflicted with the adopted value and resulted in a significant increase of nearly 50\% in this branching ratio, directly affecting the triple-alpha reaction. Purpose: This work aims to utilize charged-particle spectroscopy with magnetic selection as a means to accurately measure the total radiative branching ratio ($\Gamma_{\rm{rad}}/\Gamma$) of the Hoyle state in $^{12}{\rm C}$. Methods: The Hoyle state in $^{12}{\rm C}$ was populated via $^{12}\rm{C}(\alpha, \alpha')^{12}\rm{C^{*}}$ inelastic scattering. The scattered $\alpha$ particles were detected using a $\Delta$E-E telescope, while the recoiled $^{12}{\rm C}$ ions were identified in a magnetic spectrometer. Results: A radiative branching ratio value of $\Gamma_{\rm{rad}}/\Gamma\times10^{4}=4.0\pm0.3({\rm stat.})\pm0.16({\rm syst.})$ was obtained. Conclusions: The radiative branching ratio for the Hoyle state obtained in this work is in agreement with the original adopted value. Our result suggests that the proton-$\gamma$-$\gamma$ spectroscopy result reported by Kib\'edi et al. may be excluded.

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arXiv2023

First observation of the $\beta$3$\alpha$p decay of $^{13}\mathrm{O}$ via $\beta$-delayed charged-particle spectroscopy

Background: The $\beta$-delayed proton-decay of $^{13}\mathrm{O}$ has previously been studied, but the direct observation of $\beta$-delayed $\alpha$+$\alpha$+$\alpha$+p decay has not been reported. Purpose: Observing rare 3$\alpha$+p events from the decay of excited states in $^{13}\mathrm{N}^{\star}$ allows for a sensitive probe of exotic highly-clustered configurations in $^{13}$N. Method: To measure the low-energy products following $\beta$-delayed 3$\alpha$p-decay, the TexAT Time Projection Chamber was employed using the one-at-a-time $\beta$-delayed charged-particle spectroscopy technique at the Cyclotron Institute, Texas A&M University. Results: A total of $1.9 \times 10^{5}$ $^{13}\mathrm{O}$ implantations were made inside the TexAT Time Projection Chamber. 149 3$\alpha$+p events were observed yielding a $\beta$-delayed 3$\alpha+p$ branching ratio of 0.078(6)%. Conclusion: Four previously unknown $\alpha$-decaying states were observed, one with a strong $^{9}\mathrm{B(g.s)}+\alpha$ characteristic at 11.3 MeV, one with a $^{9}\mathrm{B}(\frac{1}{2}^{+})+\alpha$ nature at 12.4 MeV, and another two that are dominated by $^{9}\mathrm{B}({\frac{5}{2}}^{+})+\alpha$ at 13.1 and 13.7 MeV. Population of the $\frac{1}{2}^{+}$ state in $^{9}\mathrm{B}$ has been unambiguously seen, cementing the predicted existence of the mirror-state based on the states observed in $^{9}\mathrm{Be}$.

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arXiv2022

alpha-cluster structure of 18Ne

In this work we study alpha-clustering in 18Ne and compare it with what is known about clustering in the mirror nucleus 18O. The excitation function of 18Ne was measured in inverse kinematics from the resonant elastic scattering reaction of 14O on 4He in the excitation energy range from 8 to 17 MeV, using the active target TexAT. The analysis was performed using a multi-channel R-matrix approach. Detailed spectroscopic information is obtained from the R-matrix analysis: excitation energy of the states, spin and parity as well as partial alpha and total widths. This information is compared with theoretical models and previous data. Clustering structures appear to be robust and mostly isospin symmetric. A good correspondence was found between the levels in 18O and 18Ne. We carried out an extensive shell model analysis of the experimental data. This comparison suggests that strongly clustered states remain organized in relation to the corresponding reaction channel identified by the number of nodes in the relative alpha plus core wave function. The agreement between theory and experiment is very good and especially useful when it comes to understanding the clustering strength distribution. The comparison of the experimental data with theory shows that certain states, especially at high excitation energies, are significantly more clustered than predicted. This indicates that the structure of these states is collective and is aligned towards the corresponding alpha reaction channel.

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arXiv2020

Almost medium-free measurement of the Hoyle state direct-decay component with a TPC

Background: The structure of the Hoyle state, a highly $\alpha$-clustered state at 7.65 MeV in $^{12}\mathrm{C}$, has long been the subject of debate. Understanding if the system comprises of three weakly-interacting $\alpha$-particles in the 0s orbital, known as an $\alpha$-condensate state, is possible by studying the decay branches of the Hoyle state. Purpose: The direct decay of the Hoyle state into three $\alpha$-particles, rather than through the $^{8}\mathrm{Be}$ ground state, can be identified by studying the energy partition of the 3 $\alpha$-particles arising from the decay. This paper provides details on the break-up mechanism of the Hoyle stating using a new experimental technique. Method: By using beta-delayed charged-particle spectroscopy of $^{12}\mathrm{N}$ using the TexAT (Texas Active Target) TPC, a high-sensitivity measurement of the direct 3 $\alpha$ decay ratio can be performed without contributions from pile-up events. Results: A Bayesian approach to understanding the contribution of the direct components via a likelihood function shows that the direct component is $<0.043\%$ at the 95\% confidence level (C.L.). This value is in agreement with several other studies and here we can demonstrate that a small non-sequential component with a decay fraction of about $10^{-4}$ is most likely. Conclusion: The measurement of the non-sequential component of the Hoyle state decay is performed in an almost medium-free reaction for the first time. The derived upper-limit is in agreement with previous studies and demonstrates sensitivity to the absolute branching ratio. Further experimental studies would need to be combined with robust microscopic theoretical understanding of the decay dynamics to provide additional insight into the idea of the Hoyle state as an $\alpha$-condensate.

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arXiv2020

Evidence against the Efimov effect in $^{12}\mathrm{C}$ from spectroscopy and astrophysics

Background: The Efimov effect is a universal phenomenon in physics whereby three-body systems are stabilized via the interaction of an unbound two-body sub-systems. A hypothetical state in $^{12}\mathrm{C}$ at 7.458 MeV excitation energy, comprising of a loose structure of three $\alpha$-particles in mutual two-body resonance, has been suggested in the literature to correspond to an Efimov state in nuclear physics. The existence of such a state has not been demonstrated experimentally. Method: Using the combined data sets from two recent experiments, one with the TexAT TPC to measure $\alpha$-decay and the other with Gammasphere to measure $\gamma$-decay of states in $^{12}\mathrm{C}$ populated by $^{12}\mathrm{N}$ and $^{12}\mathrm{B}$ $\beta$-decay respectively, we achieve high sensitivity to states in close-proximity to the $\alpha$-threshold in $^{12}\mathrm{C}$. Results: No evidence of a state at 7.458 MeV is seen in either data set. Using a likelihood method, the 95\% C.L. $\gamma$-decay branching ratio is determined as a function of the $\beta$-decay feeding strength relative to the Hoyle state. In parallel, calculations of the triple-alpha reaction rate show the inclusion of the Efimov corresponds to a large increase in the reaction rate around $5 \times 10^{7}$ K. Conclusion: From decay spectroscopy - at the 95\% C.L., the Efimov state cannot exist at 7.458 MeV with any $\gamma$-decay branching ratio unless the $\beta$-strength is less than 0.7\% of the Hoyle state. This limit is evaluated for a range of different excitation energies and the results are not favorable for existence of the hypothetical Efimov state in $^{12}\mathrm{C}$. Furthermore, the triple-alpha reaction rate with the inclusion of a state between 7.43 and 7.53 MeV exceeds the rate required for stars to undergo the red giant phase.

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arXiv2020

Isotopic equilibrium constants for very low-density and low-temperature nuclear matter

Yields of equatorially emitted light isotopes, $1\le Z\le 14$, observed in ternary fission in the reaction $^{241}$Pu($n_{\rm th}$,f) are employed to determine apparent chemical equilibrium constants for low-temperature and low-density nuclear matter. The degree of liberation and role of medium modifications are probed through a comparison of experimentally derived reaction quotients with equilibrium constants calculated using a relativistic mean-field model employing a universal medium modification correction for the attractive $\sigma$ meson coupling. The results of these comparisons indicate that equilibrium is achieved for the lighter ternary fission isotopes. For the heavier isotopes experimental reaction quotients are well below calculated equilibrium constants. This is attributed to a dynamical limitation reflecting insufficient time for full equilibrium to develop. The role of medium effects leading to yield reductions is discussed as is the apparent enhancement of yields for $^8$He and other very neutron rich exotic nuclei.

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arXiv2019

Texas Active Target (TexAT) detector for experiments with rare isotope beams

The TexAT (Texas Active Target) detector is a new active-target time projection chamber (TPC) that was built at the Cyclotron Institute Texas A$\&$M University. The detector is designed to be of general use for nuclear structure and nuclear astrophysics experiments with rare isotope beams. TexAT combines a highly segmented Time Projection Chamber (TPC) with two layers of solid state detectors. It provides high efficiency and flexibility for experiments with low intensity exotic beams, allowing for the 3D track reconstruction of the incoming and outgoing particles involved in nuclear reactions and decays.

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arXiv2019

Structure of 9C through proton resonance scattering with Texas Active Target detector

Background: Level structure of the most neutron deficient nucleon-bound carbon isotope, 9C, is not well known. Definitive spin-parity assignments are only available for two excited states. No positive parity states have been conclusively identified so far and the location of the sd-shell in A=9 T=3/2 isospin quadruplet is not known. Purpose: We have studied the level structure of exotic nucleus 9C at excitation energies below 6.4 MeV. Methods: Excited states in 9C were populated in 8B+p resonance elastic scattering and excitation functions were measured using active target approach. Results: Two excited states in 9C were conclusively observed, and R-matrix analysis of the excitation functions was performed to make the spin-parity assignments. The first positive parity state in A=9 T=3/2 nuclear system, the 5/2+ resonance at 4.3 MeV, has been identified. Conclusions: The new 5/2+ state at 4.3 MeV in 9C is a single-particle L=0 broad resonance and it determines the energy of the 2s shell. The 2s shell in this exotic nucleus appears well within the region dominated by the p-shell states.

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arXiv2018

Dedicated $\Delta$E-E detector system for searching long lived heaviest nuclei deposited in scintillators

We present a dedicated experimental setup which is currently used to search for long lived super heavy elements (SHE) implanted in catcher scintillators which were irradiated by reaction products of $^{197}$Au (7.5 A.MeV) projectile and $^{232}$Th target collisions during our experiment performed at Cyclotrone Institute, Texas A$\&$M University in 2015. The built-in novel measuring apparatus consists of $\Delta$E-E detector pairs which are able to register $\alpha$ or spontaneous fission (SF) decays of heavy reaction products deposited in the scintillators. Their unique feature is that the examined scintillators are at the same time $\Delta$E part of each of $\Delta$E-E detector while E part is a silicon detector. Our apparatus is dedicated to search for SHEs which have a lifetime of a year till tens of years. Results of commissioning tests of our setup are presented.

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arXiv2018

A novel experimental setup for rare events selection and its potential application to super heavy elements search

The paper presents a novel instrumentation for rare events selection which was tested in our research of short lived super heavy elements production and detection. The instrumentation includes an active catcher multi elements system and dedicated electronics. The active catcher located in the forward hemisphere is composed of 63 scintillator detection modules. Reaction products of damped collisions between heavy ion projectiles and heavy target nuclei are implanted in the fast plastic scintillators of the active catcher modules. The acquisition system trigger delivered by logical branch of the electronics allows to record the reaction products which decay via the alpha particle emissions or spontaneous fission which take place between beam bursts. One microsecond wave form signal from FADCs contains information on heavy implanted nucleus as well as its decays.

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arXiv2018

A nucleation model analysis of neck emission yields in 124Sn+112,124Sn reactions at 26 MeV/nucleon

A recent analysis of experimental ternary fission fragment yields using a nucleation moderated statistical equilibrium model reproduced observed yields with fairly good accuracy. In the present work, the same approach is applied to neck emission in peripheral and mid-peripheral 124Sn+112,124Sn collisions at 26A MeV. The model can reasonably reproduce the yields of lithium to silicon isotopes with realistic time and temperature values. A comparison is made between equilibrium constants derived from the present data and those previously obtained for ternary fission of 242Pu.

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arXiv2018

Searching for states analogous to the 12C Hoyle state in heavier nuclei using the thick target inverse kinematics technique

Identification of alpha cluster states analogous to the 12C Hoyle state in heavier alpha- conjugate nuclei can provide tests of the existence of alpha condensates in nuclei. Such states are predicted for 16O, 20Ne, 24Mg, 28Si etc. at excitation energies slightly above the multi-alpha particle decay threshold, but have not yet been experimentally identified. The Thick Target Inverse Kinematics (TTIK) technique can be used to study the breakup of excited self-conjugate nuclei into many alpha particles. The reaction 20Ne+{\alpha} was studied using a 20Ne beam at 12 MeV/nucleon from the K150 cyclotron at Texas A&M University. The TTIK method was used to study both single {\alpha}-particle emission and multiple {\alpha}-particle decays. Events with alpha multiplicity up to four were analyzed. The analysis of the three {\alpha} - particle emission data allowed the identification of the Hoyle state and other 12C excited states decaying into three alpha particles. The results are shown and compared with other data available in the literature. Although the statistics for events with alpha multiplicity four is low, the data show a structure at about 15.2 MeV that could indicate the existence in 16O of a state analogous to the 12C Hoyle state. This structure is confirmed by the re-analysis of alpha multiplicity four events from a previous experiment performed at 9.7 MeV/nucleon with a similar setup but lower granularity. Moreover, the reconstructed excitation energy of 24Mg for these events peaks at around 34 MeV, very close to the predicted excitation energy for an excited state analogous to the 12C Hoyle state in 24Mg.

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arXiv2018

An experimental survey of the production of alpha decaying heavy elements in the reactions of $^{238}$U +$^{232}$Th at 7.5-6.1 MeV/nucleon

The production of alpha particle decaying heavy nuclei in reactions of 7.5-6.1 MeV/nucleon $^{238}$U +$^{232}$Th has been explored using an in-beam detection array composed of YAP scintillators and gas ionization chamber-Si telescopes. Comparisons of alpha energies and half-lives for the observed products with those of the previously known isotopes and with theoretically predicted values indicate the observation of a number of previously unreported alpha emitters. Alpha particle decay energies reaching as high as 12 MeV are observed. Many of these are expected to be from decay of previously unseen relatively neutron rich products. While the contributions of isomeric states require further exploration and specific isotope identifications need to be made, the production of heavy isotopes with quite high atomic numbers is suggested by the data.

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arXiv2018

Evidence for high excitation energy resonances in the 7 alpha disassembly of $^{28}$Si

The excitation function for the 7 alpha de-excitation of $^{28}$Si nuclei excited to high excitation energies in the collisions of 35 MeV/nucleon $^{28}$Si with $^{12}$C reveals resonance structures that may indicate the population of high spin toroidal isomers such as those predicted by a number of recent theoretical calculations. This interpretation is supported by extended theoretical analyses.

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arXiv2016

Alpha Conjugate Neck Structures in the Collisions of 35 MeV/nucleon 40Ca with 40Ca

The de-excitation of alpha-conjugate nuclei produced in reactions of 35 MeV/nucleon 40Ca with 40Ca has been investigated. Particular emphasis is placed on examining the dynamics of collisions leading to projectile-like fragment exit channels. A general exploration of the reaction systematics reveals the binary dissipative character of the collisions and a hierarchy effect similar to that seen for heavier systems. Investigation of the subset of events characterized by a total alpha-conjugate mass (alpha particles plus alpha-conjugate fragments) equal to 40 and atomic number equal to 20 reveals a dominance of alpha-conjugate exit channels. The hierarchy effect for these channels leads to the production of alpha-clustered neck structures with potentially exotic geometries and properties.

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