arXiv subjects

M. Benjamin Jungfleisch

Publications and source records attributed to M. Benjamin Jungfleisch.

At least 19 recordsLinked to original sources

arXiv2026

Nanoscale Dipolar Fields in Artificial Spin Ice Probed by Scanning NV Magnetometry

We investigate dipolar coupling fields in two square-lattice artificial spin ice (ASI) systems with different lattice constants using scanning probe microscopy based on a single nitrogen-vacancy (NV) center in diamond. This technique offers unprecedented spatial resolution, operates under ambient condition, and provides quantitative stray field measurements, making it uniquely suited for studying nanoscale magnetic textures. Our approach combines fluorescence quenching imaging and continuous-wave optically detected magnetic resonance (cODMR). A comparison of the two ASI samples, which differ in their lattice constants of 1000 nm and 910 nm respectively, reveals differences in the appearance of ice-rule violations - deviations from the lowest energy configuration in ASI vertices. We attribute these variations to varying coupling strengths dictated by the lattice constant. From the cODMR data, we extract both axial and transverse components of the local magnetic field relative to the NV axis. Micromagnetic modeling of these measurements allows for an iterative determination of the external magnetic field orientation, the detection of subtle magnetization tilts induced by weak external fields (well below the nanomagnets' switching threshold), and an estimation of the effective saturation magnetization, thereby accounting for deviations in nanomagnet dimensions. These findings provide crucial insights into the tunable magnetic interactions in ASI, paving the way for the design of advanced magnonic and spintronic devices.

cond-mat.mes-hall↗

arXiv2026

Perpendicular magnetic anisotropy tuning of macrospin-to-vortex transitions in Co-based artificial spin-vortex ice

We investigate the macrospin-to-vortex (MS-to-V) transition in Co-based artificial spin-vortex ice (ASVI) in the presence of perpendicular magnetic anisotropy (PMA) by spin-wave spectroscopy. Detailed micromagnetic simulations using mumax3 reveal that the PMA modifies the magnetic energy landscape and facilitates vortex formation, suggesting that PMA can enhance the transition probability. To seek experimental validation of this hypothesis, we prepared Ti (3 nm)/Co (10 nm)/Ti (3 nm)/Pt (2 nm) (TCT) and Ti (3 nm)/Co (10 nm)/Pt (2 nm) (TCP) multilayer stacks. Vibrating sample magnetometry measurements confirm that the TCP film exhibits a larger PMA than the TCT film. Using these stacks, we then investigate the MS-to-V transition probability in ASVIs and found that TCP ASVIs exhibit a higher transition probability than TCT ASVIs, in agreement with the simulation prediction. These findings identify PMA as an effective design parameter for controlling vortex formation in ASVIs and provide a promising route toward task-dependent tuning of fading-memory properties for physical reservoir computing based on artificial spin lattices.

cond-mat.mtrl-sci↗

arXiv2026

Shaping non-reciprocal caustic spin-wave beams

A caustic is a mathematical concept describing the beam formation when the beam envelope is reflected or refracted by a manifold. While caustics are common in a wide range of physical systems, caustics typically exhibit a reciprocal wave propagation and are challenging to control. Here, we utilize the highly anisotropic dispersion and inherent non-reciprocity of a magnonic system to shape non-reciprocal emission of caustic-like spin wave beams in an extended 200 nm thick yttrium iron garnet (YIG) film from a nano-constricted rf waveguide. We introduce a near-field diffraction model to study spin-wave beamforming in homogeneous in-plane magnetized thin films, and reveal the propagation of non-reciprocal spin-wave beams directly emitted from the nanoconstriction by spatially resolved micro-focused Brillouin light spectroscopy (BLS). The experimental results agree well with both micromagnetic simulation, and the near-field diffraction model. The proposed method can be readily implemented to study spin-wave interference at the sub-micron scale, which is central to the development of wave-based computing applications and magnonic devices.

cond-mat.mes-hall↗

arXiv2026

Deeply nonlinear magnon-photon hybrid excitation

We investigate the microwave-power dependence of magnon-photon coupling in a yttrium iron garnet-sphere/split-ring-resonator hybrid system at room temperature and demonstrate that nonlinear spin-wave interactions suppress the coupling through power-induced dissipation of magnetostatic modes. At low microwave power, the modes exhibit pronounced level repulsion, evidencing strong coupling to the microwave field. As the power increases, however, magnon linewidth broadening progressively weakens the coupling and ultimately suppresses it entirely below a threshold external magnetic field. We show that this behavior originates from Suhl's first-order instability: magnetostatic modes, which couple to the resonator, parametrically excites two counter-propagating magnons at half its frequency, causing modes below the threshold external magnetic field to vanish. In contrast, magnon modes above the threshold field remain robust even at high power, as the instability criterion is not satisfied in that regime. These results reveal a well-defined nonlinear boundary for magnon-photon coupled systems and highlight a favorable regime for exploiting nonlinear magnonics for frequency conversion, switching, and other functional magnonic devices.

cond-mat.mes-hall↗

arXiv2026

Broken intrinsic symmetry induced magnon-magnon coupling in synthetic ferrimagnets

Synthetic antiferromagnets offer rich magnon energy spectra in which optical and acoustic magnon branches can hybridize. Here, we demonstrate a broken intrinsic symmetry induced coupling of acoustic and optical magnons in a synthetic ferrimagnet consisting of two dissimilar antiferromagnetically interacting ferromagnetic metals. Two distinct magnon modes hybridize at degeneracy points, as indicated by an avoided level-crossing. The avoided level-crossing gap depends on the interlayer exchange interaction between the magnetic layers, which can be controlled by adjusting the non-magnetic interlayer thickness. A large avoided level crossing gap of 3.9 GHz is revealed, exceeding the coupling strength that is typically found in other magnonic hybrid systems based on a coupling of magnons with photons or magnons with phonons.

cond-mat.mtrl-sci↗

arXiv2025

Perspective: Magnon-magnon coupling in hybrid magnonics

The internal coupling of magnetic excitations (magnons) with themselves has created a new research sub-field in hybrid magnonics, i.e., magnon-magnon coupling, which focuses on materials discovery and engineering for probing and controlling magnons in a coherent manner. This is enabled by, one, the abundant mechanisms of introducing magnetic interactions, with examples of exchange coupling, dipolar coupling, RKKY coupling, and DMI coupling, and two, the vast knowledge of how to control magnon band structure, including field and wavelength dependences of frequencies, for determining the degeneracy of magnon modes with different symmetries. In particular, we discuss how magnon-magnon coupling is implemented in various materials systems, with examples of magnetic bilayers, synthetic antiferromagnets, nanomagnetic arrays, layered van der Waals magnets, and (DMI SOT materials) in magnetic multilayers. We then introduce new concept of applications for these hybrid magnonic materials systems, with examples of frequency up/down conversion and magnon-exciton coupling, and discuss what properties are desired for achieving those applications.

cond-mat.mtrl-sci↗

arXiv2025

Magnon-Magnon Interaction Induced by Dynamic Coupling in a Hybrid Magnonic Crystal

We report a combined experimental and numerical investigation of spin-wave dynamics in a hybrid magnonic crystal consisting of a CoFeB artificial spin ice (ASI) of stadium-shaped nanoelements patterned atop a continuous NiFe film, separated by a 5 nm Al2O3 spacer. Using Brillouin light scattering spectroscopy, we probe the frequency dependence of thermal spin waves as functions of applied magnetic field and wavevector, revealing the decisive role of interlayer dipolar coupling in the magnetization dynamics. Micromagnetic simulations complement the experiments, showing a strong interplay between ASI edge modes and backward volume modes in the NiFe film. The contrast in saturation magnetization between CoFeB and NiFe enhances this coupling, leading to a pronounced hybridization manifested as a triplet of peaks in the spectra - predicted by simulations and observed experimentally. This magnon-magnon coupling persists over a wide magnetic field range, shaping both the spin-wave dispersion and frequency-field response throughout the hysteresis loop. Our findings establish how ASI geometry can selectively enhance specific spin-wave wavelengths in the underlying film, identifying them as preferential channels for magnonic signal transport and manipulation.

cond-mat.mtrl-sci↗

arXiv2025

Quantum geometric origins of the orbital degrees of freedom of hybrid bosonic quasiparticles in magnetic systems

The orbital degree of freedom has recently attracted significant attention due to the novel phenomena it enables in condensed matter systems. However, the interpretation of the orbital degree of freedom in bosonic quasiparticles remains conceptually ambiguous and the mechanisms governing the transfer of orbital angular moment (OAM) between distinct quasiparticles, such as magnons and phonons, are not yet fully understood. We investigate orbital dynamics in bosonic systems and identify two origins of OAM: (i) global rotational motion of the system, and (ii) the quantum geometry of wavefunctions. Focusing on the latter, we study strongly coupled magnon-phonon systems in two-dimensional antiferromagnets as a test case. We uncover finite OAM arising from quantum geometric effects via two mechanisms: (a) time-parity symmetry breaking, yielding intra band OAM, and (b) interband coupling, generating interband OAM. We propose that an electrical detection scheme based on the transverse voltage generated by hybrid magnon phonon modes can be used to experimentally probe the bosonic orbital degree of freedom. Our results establish a foundation for the emerging field of phonon orbitronics, providing both a conceptual bridge between phonon and magnon orbitronics and a tool for better understanding magnon-polarons. They also advance a unified framework for harnessing orbital degrees of freedom in bosonic systems and pave the way toward electrical control of magnetization and phononic transport.

cond-mat.mes-hall↗

arXiv2025

Direct Comparison of Static and Dynamic Measurements of Spin Generation in a Topological Insulator Thin Film

The competition between intrinsic spin-orbit physics, magnetic phenomena, and the quality of materials and interfaces governs the charge-to-spin conversion processes that are essential to the implementation of spintronic devices. Direct comparisons of spin parameters, which serve as metrics of device quality, obtained by different measurement techniques are scarce, leading to uncertainty regarding discrepancies and the reliability of the methods. Here, we directly compare the spin Hall coefficient ($θ_{SH}$) in molecular beam epitaxy grown films of $(Bi_{1-x}Sb_{x})_{2}Te_{3-y}Se_{y}$ (BSTS, x = 0.58, y = 1) at room temperature using two complementary techniques: a static method using non-local voltage (NLV) measurements in BSTS Hall bars with DC charge current, and a dynamic method using spin-torque ferromagnetic resonance (ST-FMR) measurement in $BSTS/Ni_{80}Fe_{20}$ heterostructures at GHz frequencies. We obtain comparable spin Hall coefficients in angular-dependent ST-FMR ($θ_{SH}$=$4.7\pm1.1$) and in NLV ($θ_{SH}$=$2.8\pm0.6$). The complex effects of ferromagnetic interfaces while determining spin Hall coefficients using static or dynamic techniques becomes evident by contrasting our results to literature.

cond-mat.mtrl-sci↗

arXiv2025

Spin pumping driven by magnon-polaritons in a ferromagnet-coplanar superconducting resonator hybrid system

We demonstrate spin pumping driven by a strongly coupled magnon-photon system using a ferromagnet-coplanar superconducting resonator hybrid system at 1.4 K. Electrical readout via the inverse spin-Hall effect reveals characteristic coupling features, including mode splitting and linewidth broadening, demonstrating the electrical detection of strongly coupled microwave photons and magnons. The magnon-photon coupling strength obtained by combined spin pumping and inverse spin-Hall effect measurements is compared to microwave transmission experiments. Furthermore, microwave power-dependent measurements reveal a decrease in the coupling strength with increasing microwave power alongside the onset of nonlinearities of the superconducting resonator above a critical microwave power threshold.

cond-mat.mes-hall↗

arXiv2025

Dynamic Fingerprint of Controlled Structural Disorder in Artificial Spin Lattices

Investigating the emergence of complexity in disordered interacting systems, central to fields like spin glass physics, remains challenging due to difficulties in systematic experimental tuning. We introduce a tunable artificial spin lattice platform to directly probe the connection between controlled structural disorder and collective spin-wave dynamics. By precisely varying positional and rotational randomness in Ni81Fe19 nanobar arrays from periodic to random, we map the evolution from discrete spectral modes to a complex, dense manifold. Crucially, we establish a quantitative correlation between information-theoretic measures of static disorder and the dynamic spectral complexity derived from the GHz spin-wave response. This correlation provides a dynamic fingerprint of an increasingly complex energy landscape resulting from tuned disorder. Furthermore, thermal probe via thermal Brillouin light scattering reveal significantly richer microstates diversity in disordered states than driven probe using broadband ferromagnetic resonance. Our work presents a unique experimental testbed for studying how the ingredients of glassy physics manifest in high-frequency dynamics, offering quantitative insights into the onset of complexity in interacting nanomagnet systems.

cond-mat.mes-hall↗

arXiv2025

Edge-prompted spin waves probed via magneto-optical effect in the infrared

Recent advances in magnonics highlight the need for employing spin wave characteristics as new state variables, which is to be detected and mapped out with high precision in all-onchip, small scale devices. Spin wave modes that are prompted by the sample edges in planar structures are of particular fundamental importance to the future design and characterization of magnonic device functionalities. In this work, we demonstrate an infrared light-based, magneto-optical technique that concurrently functions both as a spectroscopic and an imaging tool. The detected precessional phase contrast can be directly used to construct the map of the spin wave wavefront in the continuous wave regime of spin-wave propagation and in the stationary state, without needing any optical reference path. We experimentally detect the edge spin wave modes of a Y3Fe5O12 film sample, and study the evolution and interference from edge dominated modes to their bulk counterparts. Distinct wavevector groups and propagation characteristics are observed for the edge and bulk spin wave modes. Further, the magnon dispersion relation in the infrared is obtained by Fourier transforming the wavefronts measured in real space, which is a huge advantage to the wavevector-resolved Brillouin light scattering (BLS) technique, where the angle of incidence has to be varied, and is also much less cumbersome than the phase-resolved BLS. Our results demonstrate that the infrared optical strobe light can serve as a versatile platform for magneto-optical probing of magnetization dynamics, with potential implications in investigating hybrid magnonic systems.

cond-mat.mes-hall↗

arXiv2025

Artificial Spin Ice: A Tutorial on Design and Control of Geometry, Microstate, Magnon Dynamics & Neuromorphic Computing

Artificial spin ice, arrays of strongly interacting nanomagnets, are complex magnetic systems with many emergent properties, rich microstate spaces, intrinsic physical memory, high-frequency dynamics in the GHz range and compatibility with a broad range of measurement approaches. This tutorial article aims to provide the foundational knowledge needed to understand, design, develop, and improve the dynamic properties of artificial spin ice (ASI). Special emphasis is placed on introducing the theory of micromagnetics, which describes the complex dynamics within these systems, along with their design, fabrication methods, and standard measurement and control techniques. The article begins with a review of the historical background, introducing the underlying physical phenomena and interactions that govern artificial spin ice. We then explore standard experimental techniques used to prepare the microstate space of the nanomagnetic array and to characterize magnetization dynamics, both in artificial spin ice and more broadly in ferromagnetic materials. Finally, we introduce the basics of neuromorphic computing applied to the case of artificial spin ice systems with goal to help researchers new to the field grasp these exciting new developments.

cond-mat.mes-hall↗

arXiv2025

Observation of thermally activated coherent magnon-magnon coupling in a magnonic hybrid system

We experimentally demonstrate strong magnon-magnon coupling by thermal spin excitations in yttrium iron garnet/permalloy (YIG/Py) hybrid structures using microfocused Brillouin light scattering - an optical technique that enables the detection of zero-wavevector and higher-order wavevector spin waves in a broad frequency range. The thermally activated magnons in the bilayer lead to a hybrid excitation between magnon modes in the conductive Py layer with a wide wavevector range and the first perpendicular standing magnon modes in the insulating YIG layer, facilitated by strong interfacial exchange coupling. To further investigate this coupling, we compare the thermal magnon spectra with the results obtained from electrical excitation and detection methods, which primarily detect the uniform Py mode. The realization of coherent coupling between incoherent (thermal) magnons is important for advancing energy-efficient magnonic devices, particularly in classical as well as quantum spin-wave computing technologies.

cond-mat.mes-hall↗

arXiv2025

Deciphering the origin of spin current in spintronic terahertz emitters and its imprint on their electromagnetic radiation via time-dependent density functional theory

Spin current flowing between femtosecond laser pulse (fsLP)-driven ferromagnetic metal and adjacent normal metal (NM) hosting strong spin-orbit coupling is invariably invoked to explain terahertz (THz) radiation believed to be emitted solely by NM layer. Despite being such a central concept, the microscopic origin of interlayer spin current remains vague. Here, we employ recently developed [A. Kefayati {\em et al.}, Phys. Rev. Lett. {\bf 133}, 136704 (2024)] time-dependent density functional theory plus Jefimenko equations approach to extract spin current between Co and NM=Pt or NM=W layer where Co is driven by fsLP responsible for its demagnetization, i.e., shrinking of its magnetization vector, $M^y(t)/M^y(t=0)<1$. By comparing time dependence of spin current with those of other relevant quantities, we find that: ({\em i}) spin current is generated by demagnetization dynamics because it {\em follows} closely $dM^y/dt$, thus it is an example of quantum pumping phenomenon that cannot be captured by phenomenological notions (such as ``spin voltage'') and related semiclassical transport theories; ({\em ii}) time dependence of pumped spin current {\em does not follow} closely that of charge current emerging within NM layer via spin-to-charge conversion mechanisms; ({\em iii}) THz emission can be governed by {\em both} charge current (i.e., its time derivative entering the Jefimenko equations) within Co layer or NM layer, but in different times frames. We also unravel a special case of NM=W where spin-to-charge conversion by the inverse spin Hall effect and its contribution to THz emission is suppressed, despite large spin Hall angle of W, because of localization of excited electrons onto the outer unfilled $d$-orbitals of W.

cond-mat.mes-hall↗

arXiv2025

Tunable magnon band topology and magnon orbital Nernst effect in noncollinear antiferromagnets

We theoretically investigate the intrinsic magnon orbital Nernst effect (ONE) in noncollinear antiferromagnets with Kagomé spin systems. Our analysis reveals that an externally applied magnetic field induces topological phase transitions in the magnonic system, characterized by the closing and reopening of the band gap between distinct magnon bands. These transitions enable tunable control of the magnon orbital Nernst effect with applied magnetic field, with a pronounced enhancement in magnon orbital Nernst conductivity near the phase transition points. This tunability presents a promising direction for experimental detection of the magnon ONE.

cond-mat.mtrl-sci↗

arXiv2024

Revisiting altermagnetism in RuO2: a study of laser-pulse induced charge dynamics by time-domain terahertz spectroscopy

Altermagnets are a recently discovered class of magnetic material with great potential for applications in the field of spintronics, owing to their non-relativistic spin-splitting and simultaneous antiferromagnetic order. One of the most studied candidates for altermagnetic materials is rutile structured RuO2. However, it has recently come under significant scrutiny as evidence emerged for its lack of any magnetic order. In this work, we study bilayers of epitaxial RuO2 and ferromagnetic permalloy (Fe19Ni81) by time-domain terahertz spectroscopy, probing for three possible mechanisms of laser-induced charge dynamics: the inverse spin Hall effect (ISHE), electrical anisotropic conductivity (EAC), and inverse altermagnetic spin-splitting effect (IASSE). We examine films of four common RuO2 layer orientations: (001), (100), (110), and (101). If RuO2 is altermagnetic, then the (100) and (101) oriented samples are expected to produce anisotropic emission from the IASSE, however, our results do not indicate the presence of IASSE for either as-deposited or field annealed samples. The THz emission from all samples is instead consistent with charge dynamics induced by only the relativistic ISHE and the non-relativistic and non-magnetic EAC, casting further doubt on the existence of altermagnetism in RuO2. In addition, we find that in the (101) oriented RuO2 sample, the combination of ISHE and EAC emission mechanisms produces THz emission which is tunable between linear and elliptical polarization by modulation of the external magnetic field.

cond-mat.mtrl-sci↗

arXiv2024

Charge and spin current pumping by ultrafast demagnetization dynamics

The surprising discovery of ultrafast demagnetization -- where electric field of femtosecond laser pulse couples to electrons of a ferromagnetic (FM) layer causing its magnetization vector {\em to shrink while not rotating}, is also assumed to be accompanied by generation of spin current in the direction orthogonal to electric field. However, understanding of the microscopic origin of such spin current and how efficiently it can be converted into charge current, as the putative source of THz radiation, is lacking despite nearly three decades of intense studies. Here we connect the standard pumping phenomena driven by microwave precession of magnetization vector replacing periodic time-dependence of magnetization precession with nonperiodic time-dependence of demagnetization, as obtained from experiments on ultrafast-light-driven Ni layer. Applying time-dependent nonequilibrium Green's functions, able to evolve such setup with arbitrary time dependence, reveals how demagnetization dynamics pumps both charge and spin currents in directions both parallel and orthogonal to electric field of laser pulse, even in the absence of spin-orbit coupling and thereby induced spin-to-charge conversion mechanisms. Although pumped currents follow $dM_z/dt$ in some setups, this becomes obscured when NM layers are disconnected and pumped currents start to reflect from FM boundaries (as is the case of experimental setups). Finally, we use the Jefimenko equations to compute electromagnetic radiation by charge current pumped in disconnected setup during demagnetization, or later during its slow recovery, unraveling that radiated electric field only in the former time interval exhibits features in 0.1--30 THz frequency range probed experimentally or explored for applications of spintronic THz emitters.

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