arXiv subjects

M. Bowry

Publications and source records attributed to M. Bowry.

At least 37 records · Page 2Linked to original sources

arXiv2020

Structure of high-lying levels populated in the $^{96}$Y $\rightarrow ^{96}$Zr $β$ decay

The nature of $J^π=1^-$ levels of $^{96}$Zr below the $β$-decay $Q_β$ value of $^{96}$Y has been investigated in high-resolution $γ$-ray spectroscopy following the $β$ decay as well as in a campaign of inelastic photon scattering experiments. Branching ratios extracted from $β$ decay allow the absolute $E1$ excitation strength to be determined for levels populated in both reactions. The combined data represents a comprehensive approach to the wavefunction of $1^-$ levels below the $Q_β$ value, which are investigated in the theoretical approach of the Quasiparticle Phonon Model. This study clarifies the nuclear structure properties associated with the enhanced population of high-lying levels in the $^{96}$Y$_{gs}$ $β$ decay, one of the three most important contributors to the high-energy reactor antineutrino spectrum.

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arXiv2020

Two-neutron knockout as a probe of the composition of states in $^{22}$Mg, $^{23}$Al, and $^{24}$Si

Simpson and Tostevin proposed that the width and shape of exclusive parallel momentum distributions of the A-2 residue in direct two-nucleon knockout reactions carry a measurable sensitivity to the nucleon single-particle configurations and their couplings within the wave functions of exotic nuclei. We report here on the first benchmarks and use of this new spectroscopic tool. Exclusive parallel momentum distributions for states in the neutron-deficient nuclei $^{22}$Mg, $^{23}$Al, and $^{24}$Si populated in such direct two-neutron removal reactions were extracted and compared to predictions combining eikonal reaction theory and shell-model calculations. For the well-known $^{22}$Mg and $^{23}$Al nuclei, measurements and calculations were found to agree, supporting the dependence of the parallel momentum distribution width on the angular momentum composition of the shell-model two-neutron amplitudes. In $^{24}$Si, a level at 3439(9) keV, of relevance for the important $^{23}$Al(p,$γ$)$^{24}$Si astrophysical reaction rate, was confirmed to be the $2^+_2$ state, while the $4^+_1$ state, expected to be strongly populated in two-neutron knockout, was not observed. This puzzle is resolved by theoretical considerations of the Thomas-Ehrman shift, which also suggest that a previously reported 3471-keV state in $^{24}$Si is in fact the ($0^+_2$) level with one of the largest experimental mirror-energy shifts ever observed.

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arXiv2020

Evolution of Octupole Deformation in Radium Nuclei from Coulomb Excitation of Radioactive $^{222}$Ra and $^{228}$Ra Beams

There is sparse direct experimental evidence that atomic nuclei can exhibit stable pear shapes arising from strong octupole correlations. In order to investigate the nature of octupole collectivity in radium isotopes, electric octupole ($E3$) matrix elements have been determined for transitions in $^{222,228}$Ra nuclei using the method of sub-barrier, multi-step Coulomb excitation. Beams of the radioactive radium isotopes were provided by the HIE-ISOLDE facility at CERN. The observed pattern of $E$3 matrix elements for different nuclear transitions is explained by describing $^{222}$Ra as pear-shaped with stable octupole deformation, while $^{228}$Ra behaves like an octupole vibrator.

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arXiv2019

First direct measurement of the intrinsic dipole moment in pear-shaped thorium isotopes

It is now well established that atomic nuclei composed of certain combinations of protons and neutrons can adopt reflection-asymmetric, or octupole-deformed, shapes at low excitation energy. These nuclei show promise in the search for a permanent atomic electric dipole moment, the existence of which has implications for physics beyond the Standard Model. Theoretical studies have suggested that certain isotopes of thorium may have the largest octupole deformation. However, due to experimental challenges, the extent of the octupole collectivity in the low-energy states in these thorium nuclei has not yet been demonstrated. This paper reports measurements of the lifetimes of low-energy states in 228Th (Z = 90) undertaken using the mirror symmetric centroid difference method, which is a direct electronic fast-timing technique. Lifetime measurements of the low-lying Jp = 1- and 3- states, which are the first for a thorium isotope, have allowed the B(E1) rates and the intrinsic dipole moment to be determined. The results are in agreement with those of previous theoretical calculations allowing the extent of the octupole deformation of 228Th to be estimated. This study indicates that the nuclei 229Th and 229Pa (Z = 91) may be good candidates for the search for a permanent atomic electric dipole moment.

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arXiv2019

Direct observation of proton emission in 11Be

The elusive $β^-\text{p}^+$ decay was observed in $^{11}$Be by directly measuring the emitted protons and their energy distribution for the first time with the prototype Active Target Time Projection Chamber (pAT-TPC) in an experiment performed at ISAC-TRIUMF. The measured $β^-\text{p}^+$ branching ratio is orders of magnitude larger than any previous theoretical model predicted. This can be explained by the presence of a narrow resonance in $^{11}$B above the proton separation energy.

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arXiv2019

Shape coexistence in the neutron-deficient lead region: A systematic study of lifetimes in the even-even $^{188-200}$Hg with GRIFFIN

Lifetimes of $2^+_1$ and $4^+_1$ states, as well as some negative-parity and non-yrast states, in $^{188-200}$Hg were measured using $γ-γ$ electronic fast timing techniques with the LaBr$_3$(Ce) detector array of the GRIFFIN spectrometer. The excited states were populated in the $ε/β^+$-decay of $J^π=7^+/2^-$ $^{188-200}$Tl produced at the TRIUMF-ISAC facility. The deduced B(E2) values are compared to different interacting boson model predictions. The precision achieved in this work over previous ones allows for a meaningful comparison with the different theoretical models of these transitional Hg isotopes, which confirms the onset of state mixing in $^{190}$Hg.

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arXiv2019

Spectroscopy and lifetime measurements near the proton drip line: $^{26,27,28}$P

We report on the observation of excited states in the neutron-deficient phosphorus isotopes $^{26,27,28}$P via in-beam gamma-ray spectroscopy with both high-efficiency and high-resolution detector arrays. In $^{26}$P, a previously-unobserved level has been identified at 244(3) keV, two new measurements of the astrophysically-important 3/2$^+$ resonance in $^{27}$P have been performed, gamma decays have been assigned to the proton-unbound levels at 2216 keV and 2483 keV in $^{28}$P, and the gamma-ray lineshape method has been used to make the first determination of the lifetimes of the two lowest-lying excited states in $^{28}$P. The expected Thomas-Ehrman shifts were calculated and applied to levels in the mirror nuclei. The resulting level energies from this procedure were then compared with the energies of known states in $^{26,27,28}$P.

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arXiv2019

Isospin symmetry in $B(E2)$ values: Coulomb excitation study of ${}^{21}$Mg

The $T_z$~=~$-\frac{3}{2}$ nucleus ${}^{21}$Mg has been studied by Coulomb excitation on ${}^{196}$Pt and ${}^{110}$Pd targets. A 205.6(1)-keV $γ$-ray transition resulting from the Coulomb excitation of the $\frac{5}{2}^+$ ground state to the first excited $\frac{1}{2}^+$ state in ${}^{21}$Mg was observed for the first time. Coulomb excitation cross-section measurements with both targets and a measurement of the half-life of the $\frac{1}{2}^+$ state yield an adopted value of $B(E2;\frac{5}{2}^+\rightarrow\frac{1}{2}^+)$~=~13.3(4)~W.u. A new excited state at 1672(1)~keV with tentative $\frac{9}{2}^+$ assignment was also identified in ${}^{21}$Mg. This work demonstrates large difference of the $B(E2;\frac{5}{2}^+\rightarrow\frac{1}{2}^+)$ values between $T$~=~$\frac{3}{2}$, $A$~=~21 mirror nuclei. The difference is investigated in the shell-model framework employing both isospin conserving and breaking USD interactions and using modern \textsl{ab initio} nuclear structure calculations, which have recently become applicable in the $sd$ shell.

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arXiv2019

$β$ and $β$-delayed neutron decay of the $N=82$ nucleus $^{131}_{~49}$In$_{82}$

The half-lives of three $β$ decaying states of $^{131}_{~49}$In$_{82}$ have been measured with the GRIFFIN $γ$-ray spectrometer at the TRIUMF-ISAC facility to be $T_{1/2}(1/2^-)=328(15)$~ms, $T_{1/2}(9/2^+)=265(8)$~ms, and $T_{1/2}(21/2^+)=323(55)$~ms, respectively. The first observation of $γ$-rays following the $βn$ decay of $^{131}$In into $^{130}$Sn is reported. The $β$-delayed neutron emission probability is determined to be $P_{1n} = 12(7)\%$ for the $21/2^+$ state and $2.3(3)\%$ from the combined $1/2^-$ and $9/2^+$ states of $^{131}_{~49}$In$_{82}$ observed in this experiment. A significant expansion of the decay scheme of $^{131}$In, including 17 new excited states and 34 new $γ$-ray transitions in $^{131}_{~50}$Sn$_{81}$ is also reported. This leads to large changes in the deduced $β$ branching ratios to some of the low-lying states of $^{131}$Sn compared to previous work with implications for the strength of the first-forbidden $β$ transitions in the vicinity of doubly-magic $^{132}_{~50}$Sn$_{82}$.

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arXiv2018

The GRIFFIN Facility for Decay-Spectroscopy Studies at TRIUMF-ISAC

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new high-efficiency $γ$-ray spectrometer designed for use in decay spectroscopy experiments with low-energy radioactive ion beams provided by TRIUMF's Isotope Separator and Accelerator (ISAC-I) facility. GRIFFIN is composed of sixteen Compton-suppressed large-volume clover-type high-purity germanium (HPGe) $γ$-ray detectors combined with a suite of ancillary detection systems and coupled to a custom digital data acquisition system. The infrastructure and detectors of the spectrometer as well as the performance characteristics and the analysis techniques applied to the experimental data are described.

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arXiv2017

Spectroscopy of $^{54}$Ti and the systematic behavior of low energy octupole states in Ca and Ti isotopes

Excited states of the $N=32$ nucleus $^{54}$Ti have been studied, via both inverse-kinematics proton scattering and one-neutron knockout from $^{55}$Ti by a liquid hydrogen target, using the GRETINA $γ$-ray tracking array. Inelastic proton-scattering cross sections and deformation lengths have been determined. A low-lying octupole state has been tentatively identified in $^{54}$Ti for the first time. A comparison of $(p,p')$ results on low-energy octupole states in the neutron-rich Ca and Ti isotopes with the results of Random Phase Approximation calculations demonstrates that the observed systematic behavior of these states is unexpected.

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arXiv2017

The GRIFFIN Data Acquisition System

Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei, GRIFFIN, is a new experimental facility for radioactive decay studies at the TRIUMF-ISAC laboratory. This article describes the details of the custom designed GRIFFIN digital data acquisition system. The features of the system that will enable high-precision half-life and branching ratio measurements with levels of uncertainty better than 0.05% are described. The system has demonstrated the ability to effectively collect signals from High-purity germanium crystals at counting rates up to 50kHz while maintaining good energy resolution, detection efficiency and spectral quality.

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arXiv2017

High-Precision Half-life Measurement for the Superallowed Fermi $β^+$ Emitter $^{22}$Mg

A high-precision half-life measurement for the superallowed Fermi $β^+$ emitter $^{22}$Mg was performed at the TRIUMF-ISAC facility using a 4$π$ proportional gas counter. The result of $T_{1/2} = 3.87400 \pm 0.00079$ s is a factor of 3 more precise than the previously adopted world average and resolves a discrepancy between the two previously published $^{22}$Mg half-life measurements.

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arXiv2017

Spectroscopy of $^{50}$Sc and ab initio calculations of $B(M3)$ strengths

The GRIFFIN spectrometer at TRIUMF-ISAC has been used to study excited states and transitions in $^{50}$Sc following the $β$-decay of $^{50}$Ca. Branching ratios were determined from the measured $γ$-ray intensities, and angular correlations of $γ$ rays have been used to firmly assign the spins of excited states. The presence of an isomeric state that decays by an $M3$ transition with a $B(M3)$ strength of 13.6(7)\,W.u. has been confirmed. We compare with the first {\it ab initio} calculations of $B(M3$) strengths in light and medium-mass nuclei from the valence-space in-medium similarity renormalization group approach, using consistently derived effective Hamiltonians and $M3$ operator. The experimental data are well reproduced for isoscalar $M3$ transitions when using bare $g$-factors, but the strength of isovector $M3$ transitions are found to be underestimated by an order of magnitude.

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arXiv2017

Testing microscopically derived descriptions of nuclear collectivity: Coulomb excitation of 22Mg

Many-body nuclear theory utilizing microscopic or chiral potentials has developed to the point that collectivity might be dealt with in an {\it ab initio} framework without the use of effective charges; for example with the proper evolution of operators, or alternatively, through the use of an appropriate and manageable subset of particle-hole excitations. We present a precise determination of $E2$ strength in $^{22}$Mg and its mirror $^{22}$Ne by Coulomb excitation, allowing for rigorous comparisons with theory. No-core symplectic shell-model calculations were performed and agree with the new $B(E2)$ values while in-medium similarity-renormalization-group calculations consistently underpredict the absolute strength, with the missing strength found to have both isoscalar and isovector components.

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arXiv2017

Total Absorption Spectroscopy Study of the Beta Decay of $^{86}$Br and $^{91}$Rb

The beta decays of $^{86}$Br and $^{91}$Rb have been studied using the total absorption spectroscopy technique. The radioactive nuclei were produced at the IGISOL facility in Jyväskylä and further purified using the JYFLTRAP. $^{86}$Br and $^{91}$Rb are considered to be major contributors to the decay heat in reactors. In addition $^{91}$Rb was used as a normalization point in direct measurements of mean gamma energies released in the beta decay of fission products by Rudstam {\it et al.} assuming that this decay was well known from high-resolution measurements. Our results show that both decays were suffering from the {\it Pandemonium} effect and that the results of Rudstam {\it et al.} should be renormalized. The relative impact of the studied decays in the prediction of the decay heat and antineutrino spectrum from reactors has been evaluated.

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arXiv2017

$β$-decay half-lives and $β$-delayed neutron emission probabilities for several isotopes of Au, Hg, Tl, Pb and Bi, beyond N=126

$Background:$ Previous measurements of $β$-delayed neutron emitters comprise around 230 nuclei, spanning from the $^{8}$He up to $^{150}$La. Apart from $^{210}$Tl, with a minuscule branching ratio of 0.007\%, no other neutron emitter is measured yet beyond $A=150$. Therefore new data are needed, particularly in the heavy mass region around N=126, in order to guide theoretical models and to understand the formation of the third r-process peak at $A\sim195$. $Purpose:$ To measure both, $β$-decay half-lives and neutron branching ratios of several neutron-rich Au, Hg, Tl, Pb and Bi isotopes beyond $N=126$. $Method:$ Ions of interest are produced by fragmentation of a $^{238}$U beam, selected and identified via the GSI-FRS fragment separator. A stack of segmented silicon detectors (SIMBA) is used to measure ion-implants and $β$-decays. An array of 30 $^3$He tubes embedded in a polyethylene matrix (BELEN) is used to detect neutrons with high efficiency and selectivity. A self-triggered digital system is employed to acquire data and to enable time-correlations. The latter are analyzed with an analytical model and results for the half-lives and neutron-branching ratios are derived using the binned Maximum-Likelihood method. $Results:$ Twenty new $β$-decay half-lives are reported for $^{204-206}$Au, $^{208-211}$Hg,$^{211-216}$Tl,$^{215-218}$Pb and $^{218-220}$Bi, nine of them for the first time. Neutron emission probabilities are reported for $^{210,211}$Hg and $^{211-216}$Tl. $Conclusions:$ The new $β$-decay half-lives are in good agreement with previous measurements in this region. The measured neutron emission probabilities are comparable or smaller than values predicted by global models like RHB+RQRPA.

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arXiv2016

Total Absorption Gamma-Ray Spectroscopy of 87Br, 88Br and 94Rb Beta-Delayed Neutron Emitters

We investigate the decay of 87Br, 88Br and 94Rb using total absorption gamma-ray spectroscopy. These important fission products are beta-delayed neutron emitters. Our data show considerable gamma-intensity, so far unobserved in high-resolution gamma-ray spectroscopy, from states at high excitation energy. We also find significant differences with the beta intensity that can be deduced from existing measurements of the beta spectrum. We evaluate the impact of the present data on reactor decay heat using summation calculations. Although the effect is relatively small it helps to reduce the discrepancy between calculations and integral measurements of the photon component for 235U fission at cooling times in the range 1 to 100 s. We also use summation calculations to evaluate the impact of present data on reactor antineutrino spectra. We find a significant effect at antineutrino energies in the range of 5 to 9 MeV. In addition, we observe an unexpected strong probability for gamma emission from neutron unbound states populated in the daughter nucleus. The gamma branching is compared to Hauser-Feshbach calculations which allow one to explain the large value for bromine isotopes as due to nuclear structure. However the branching for 94Rb, although much smaller, hints of the need to increase the radiative width by one order-of-magnitude. This leads to a similar increase in the calculated (n,gamma) cross section for this very neutron-rich nucleus with a potential impact on r-process abundance calculations.

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