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M. Buchhold

Publications and source records attributed to M. Buchhold.

17 recordsLinked to original sources

Frustration-Free Control and Absorbing-State Transport in Entangled State Preparation

We study frustration-free control, a measurement-feedback protocol for quantum state preparation that extends the concept of frustration-free Hamiltonians to stochastic dynamics. The protocol drives many-body systems into highly entangled target states, common dark states of all measurement projectors, through minimal local unitary corrections that realize an absorbing-state dynamics without post-selection. We show that relaxation to the target state is governed by emergent transport of nonlocal charges, such as singlet excitations in SU$(2)$-symmetric dynamics. While measurement-feedback annihilates compatible charge configurations, both measurement and scrambling unitaries induce charge transport and thus determine the convergence time. Mapping a baseline model of SU$(N)$ SWAP measurements with local corrections to a solvable absorbing random walk yields a runtime scaling $t \sim L^z$ with transport exponent $z=2$. Simulations of Motzkin and Fredkin chains reveal subdiffusive scaling $z \ge \tfrac{8}{3}$, confirming the transport picture and suggesting strategies for controlled entangled-state preparation and charge-transport probing in monitored quantum dynamics.

quant-ph

A coherent phonon-induced hidden quadrupolar ordered state in Ca$_2$RuO$_4$

Ultrafast laser excitation provides a means to transiently realize long-range ordered electronic states of matter that are hidden in thermal equilibrium. Recently, this approach has unveiled a variety of thermally inaccessible ordered states in strongly correlated materials, including charge density wave, ferroelectric, magnetic, and intertwined charge-orbital ordered states. However, more exotic hidden states exhibiting higher multipolar ordering remain elusive owing to the challenge of directly manipulating and detecting them with light. Here we demonstrate a method to induce a dynamical transition from a thermally allowed to a thermally forbidden spin-orbit entangled quadrupolar ordered state in Ca$_2$RuO$_4$ by coherently exciting a phonon that is strongly coupled to the order parameter. Combining probe photon energy-resolved coherent phonon spectroscopy measurements with model Hamiltonian calculations, we show that the dynamical transition is manifested through anomalies in the temperature, pump excitation fluence, and probe photon energy dependence of the strongly coupled phonon. With this procedure, we introduce a general pathway to uncover hidden multipolar ordered states and to control their re-orientation on ultrashort timescales.

cond-mat.str-el

Entanglement phases, localization and multifractality of monitored free fermions in two dimensions

We investigate the entanglement structure and wave function characteristics of continuously monitored free fermions with U$(1)$-symmetry in two spatial dimensions (2D). By deriving the exact fermion replica-quantum master equation, we line out two approaches: (i) a nonlinear sigma model analogous to disordered free fermions, resulting in an SU$(R)$-symmetric field theory of symmetry class AIII in (2+1) space-time dimensions, or (ii) for bipartite lattices, third quantization leading to a non-Hermitian SU$(2R)$-symmetric Hubbard model. Using exact numerical simulations, we explore the phenomenology of the entanglement transition in 2D monitored fermions, examining entanglement entropy and wave function inverse participation ratio. At weak monitoring, we observe characteristic $L\log L$ entanglement growth and multifractal dimension $D_q=2$, resembling a metallic Fermi liquid. Under strong monitoring, wave functions localize and the entanglement saturates towards an area law. Between these regimes, we identify a high-symmetry point exhibiting both entanglement growth indicative of emergent conformal invariance and maximal multifractal behavior. While this multifractal behavior aligns with the nonlinear sigma model of the Anderson transition, the emergent conformal invariance is an unexpected feature not typically associated with Anderson localization. These discoveries add a new dimension to the study of 2D monitored fermions and underscore the need to further explore the connection between non-unitary quantum dynamics in $D$ dimensions and quantum statistical mechanics in $D+1$ dimensions.

cond-mat.str-el

Revealing measurement-induced phase transitions by pre-selection

Pushing forward the understanding of general non-unitary dynamics in controlled quantum platforms has been fueled by the recent discovery of measurement-induced phases and phase transitions. So far, these transitions remained largely elusive, since they are masked in standard quantum mechanical observables due to the randomness of measurement outcomes. Here, we establish a general scheme -- pre-selection -- to make them observable: The outcome randomness is broken explicitly by steering the system towards a representative state, which corresponds to one out of exponentially many possible measurement outcomes. Remarkably, this steering can be chosen so gently that the basic properties of the underlying measurement-induced transition, such as entanglement structure and critical exponents, are not modified. Pre-selection introduces a unique dark or absorbing state with macroscopic order, replacing the maximally mixed stationary state of the unconditioned measurement trajectory ensemble. This creates a link of measurement-induced phase transitions to new forms of quantum absorbing state transitions, which can be detected by standard means via a local order parameter. This insight further enables a quantum simulation strategy, determining the underlying universality class in state-of-the-art quantum platforms without measurement readout.

cond-mat.dis-nn

Monitored Open Fermion Dynamics: Exploring the Interplay of Measurement, Decoherence, and Free Hamiltonian Evolution

The interplay of unitary evolution and local measurements in many-body systems gives rise to a stochastic state evolution and to measurement-induced phase transitions in the pure state entanglement. In realistic settings, however, this dynamics may be spoiled by decoherence, e.g., dephasing, due to coupling to an environment or measurement imperfections. We investigate the impact of dephasing and the inevitable evolution into a non-Gaussian, mixed state, on the dynamics of monitored fermions. We approach it from three complementary perspectives: (i) the exact solution of the conditional master equation for small systems, (ii) quantum trajectory simulations of Gaussian states for large systems, and (iii) a renormalization group analysis of a bosonic replica field theory. For weak dephasing, constant monitoring preserves a weakly mixed state, which displays a robust measurement-induced phase transition between a critical and a pinned phase, as in the decoherence-free case. At strong dephasing, we observe the emergence of a new scale describing an effective temperature, which is accompanied with an increased mixedness of the fermion density matrix. Remarkably, observables such as density-density correlation functions or the subsystem parity still display scale invariant behavior even in this strongly mixed phase. We interpret this as a signature of gapless, classical diffusion, which is stabilized by the balanced interplay of Hamiltonian dynamics, measurements, and decoherence.

cond-mat.stat-mech

Dynamics of measured many-body quantum chaotic systems

We consider the dynamics of continuously measured many-body chaotic quantum systems. Focusing on the observable of state purification, we analytically describe the limits of strong and weak measurement rate, where in the latter case monitoring up to time scales exponentially long in the numbers of particles is required. We complement the analysis of the limiting regimes with the construction of an effective replica theory providing information on the stability and the symmetries of the respective phases. The analytical results are tested by comparison to exact numerical simulations for a measured SYK model.

cond-mat.dis-nn

Decoupling of static and dynamic criticality in a driven Mott insulator

Dynamically driven interacting quantum many-body systems have the potential to exhibit properties that defy the laws of equilibrium statistical mechanics. A widely studied model is the impulsively driven antiferromagnetic Mott insulator, which is predicted to realize exotic transient phenomena including dynamical phase transitions into thermally forbidden states and highly non-thermal magnon distributions. However such far-from-equilibrium regimes, where conventional time-dependent Ginzburg-Landau descriptions fail, are experimentally challenging to prepare and to probe especially in solid state systems. Here we use a combination of time-resolved second harmonic optical polarimetry and coherent magnon spectroscopy to interrogate $n$-type photo-doping induced ultrafast magnetic order parameter dynamics in the Mott insulator Sr$_2$IrO$_4$. We uncover an unusual far-from-equilibrium critical regime in which the divergences of the magnetic correlation length and relaxation time are decoupled. This violation of conventional thermal critical behavior arises from the interplay of photo-doping and non-thermal magnon population induced demagnetization effects. Our findings, embodied in a non-equilibrium "phase diagram", provide a blueprint for engineering the out-of-equilibrium properties of quantum matter, with potential applications to terahertz spintronics technologies.

cond-mat.str-el

Effective Theory for the Measurement-Induced Phase Transition of Dirac Fermions

A wave function exposed to measurements undergoes pure state dynamics, with deterministic unitary and probabilistic measurement induced state updates, defining a quantum trajectory. For many-particle systems, the competition of these different elements of dynamics can give rise to a scenario similar to quantum phase transitions. To access it despite the randomness of single quantum trajectories, we construct an $n$-replica Keldysh field theory for the ensemble average of the $n$-th moment of the trajectory projector. A key finding is that this field theory decouples into one set of degrees of freedom that heats up indefinitely, while $n-1$ others can be cast into the form of pure state evolutions generated by an effective non-Hermitian Hamiltonian. This decoupling is exact for free theories, and useful for interacting ones. In particular, we study locally measured Dirac fermions in $(1+1)$ dimensions, which can be bosonized to a monitored interacting Luttinger liquid at long wavelengths. For this model, the non-Hermitian Hamiltonian corresponds to a quantum Sine-Gordon model with complex coefficients. A renormalization group analysis reveals a gapless critical phase with logarithmic entanglement entropy growth, and a gapped area law phase, separated by a Berezinskii-Kosterlitz-Thouless transition. The physical picture emerging here is a pinning of the trajectory wave function into eigenstates of the measurement operators upon increasing the monitoring rate.

cond-mat.stat-mech

Continuous Gaussian Measurements of the Free Boson CFT: A model for Exactly Solvable and Detectable Measurement-Induced Dynamics

Hybrid evolution protocols, composed of unitary dynamics and repeated, weak or projective measurements, give rise to new, intriguing quantum phenomena, including entanglement phase transitions and unconventional conformal invariance. Defying the complications imposed by the non-linear and stochastic nature of the measurement process, we introduce a scenario of measurement-induced many body evolution, which possesses an exact analytical solution: bosonic Gaussian measurements. The evolution features a competition between the continuous observation of linear boson operators and a free Hamiltonian, and it is characterized by a unique and exactly solvable covariance matrix. Within this framework, we then consider an elementary model for quantum criticality, the free boson conformal field theory, and investigate in which way criticality is modified under measurements. Depending on the measurement protocol, we distinguish three fundamental scenarios (a) enriched quantum criticality, characterized by a logarithmic entanglement growth with a floating prefactor, or the loss of criticality, indicated by an entanglement growth with either (b) an area-law or (c) a volume-law. For each scenario, we discuss the impact of imperfect measurements, which reduce the purity of the wavefunction and are equivalent to Markovian decoherence, and present a set of observables, e.g., real-space correlations, the relaxation time, and the entanglement structure, to classify the measurement-induced dynamics for both pure and mixed states. Finally, we present an experimental tomography scheme, which grants access to the density operator of the system by using the continuous measurement record only.

cond-mat.stat-mech

Signatures of ultrafast reversal of excitonic order in Ta$_2$NiSe$_5$

In the presence of electron-phonon coupling, an excitonic insulator harbors two degenerate ground states described by an Ising-type order parameter. Starting from a microscopic Hamiltonian, we derive the equations of motion for the Ising order parameter in the phonon coupled excitonic insulator Ta$_2$NiSe$_5$ and show that it can be controllably reversed on ultrashort timescales using appropriate laser pulse sequences. Using a combination of theory and time-resolved optical reflectivity measurements, we report evidence of such order parameter reversal in Ta$_2$NiSe$_5$ based on the anomalous behavior of its coherently excited order-parameter-coupled phonons. Our work expands the field of ultrafast order parameter control beyond spin and charge ordered materials.

cond-mat.str-el

Hydrodynamic stabilization of self-organized criticality in a driven Rydberg gas

Signatures of self-organized criticality (SOC) have recently been observed in an ultracold atomic gas under continuous laser excitation to strongly-interacting Rydberg states [S. Helmrich et al., Nature, 577, 481--486 (2020)]. This creates a unique possibility to study this intriguing dynamical phenomenon, e.g., to probe its robustness and universality, under controlled experimental conditions. Here we examine the self-organizing dynamics of a driven ultracold gas and identify an unanticipated feedback mechanism, which is especially important for systems coupled to thermal baths. It sustains an extended critical region in the trap center for a notably long time via hydrodynamic transport of particles from the flanks of the cloud toward the center. This compensates the avalanche-induced atom loss and leads to a characteristic flat-top density profile, providing an additional experimental signature for SOC and minimizing effects of inhomogeneity on the SOC features.

cond-mat.quant-gas

Epidemic growth and Griffiths effects on an emergent network of excited atoms

Whether it be physical, biological or social processes, complex systems exhibit dynamics that are exceedingly difficult to understand or predict from underlying principles. Here we report a striking correspondence between the collective excitation dynamics of a laser driven ultracold gas of Rydberg atoms and the spreading of diseases, which in turn opens up a highly controllable experimental platform for studying non-equilibrium dynamics on complex networks. We find that the competition between facilitated excitation and spontaneous decay results in a fast growth of the number of excitations that follows a characteristic sub-exponential time dependence which is empirically observed as a key feature of real epidemics. Based on this we develop a quantitative microscopic susceptible-infected-susceptible (SIS) model which links the growth and final excitation density to the dynamics of an emergent heterogeneous network and rare active region effects associated to an extended Griffiths phase. This provides physical insights into the nature of non-equilibrium criticality in driven many-body systems and the mechanisms leading to non-universal power-laws in the dynamics of complex systems.

physics.atom-ph

Signatures of Self-Organised Criticality in an Ultracold Atomic Gas

Self organisation provides an elegant explanation for how complex structures emerge and persist throughout nature. Surprisingly often, these structures exhibit remarkably similar scale-invariant properties. While this is sometimes captured by simple models that feature a critical point as an attractor for the dynamics, the connection to real-world systems is exceptionally hard to test quantitatively. Here we observe three key signatures of self-organised criticality in the dynamics of a driven-dissipative gas of ultracold atoms: (i) self-organisation to a stationary state that is largely independent of the initial conditions, (ii) scale-invariance of the final density characterised by a unique scaling function, and (iii) large fluctuations of the number of excited atoms (avalanches) obeying a characteristic power-law distribution. This establishes a well-controlled platform for investigating self-organisation phenomena and non-equilibrium criticality with unprecedented experimental access to the underlying microscopic details of the system.

cond-mat.quant-gas

Quantum dynamics in strongly driven random dipolar magnets

The random dipolar magnet LiHo$_x$Y$_{1-x}$F$_4$ enters a strongly frustrated regime for small Ho$^{3+}$ concentrations with $x<0.05$. In this regime, the magnetic moments of the Ho$^{3+}$ ions experience small quantum corrections to the common Ising approximation of LiHo$_x$Y$_{1-x}$F$_4$, which lead to a $Z_2$-symmetry breaking and small, degeneracy breaking energy shifts between different eigenstates. Here we show that destructive interference between two almost degenerate excitation pathways burns spectral holes in the magnetic susceptibility of strongly driven magnetic moments in LiHo$_x$Y$_{1-x}$F$_4$. Such spectral holes in the susceptibility, microscopically described in terms of Fano resonances, can already occur in setups of only two or three frustrated moments, for which the driven level scheme has the paradigmatic $Λ$-shape. For larger clusters of magnetic moments, the corresponding level schemes separate into almost isolated many-body $Λ$-schemes, in the sense that either the transition matrix elements between them are negligibly small or the energy difference of the transitions is strongly off-resonant to the drive. This enables the observation of Fano resonances, caused by many-body quantum corrections to the common Ising approximation also in the thermodynamic limit. We discuss its dependence on the driving strength and frequency as well as the crucial role that is played by lattice dissipation.

cond-mat.dis-nn

Keldysh Field Theory for Driven Open Quantum Systems

Recent experimental developments in diverse areas - ranging from cold atomic gases over light-driven semiconductors to microcavity arrays - move systems into the focus, which are located on the interface of quantum optics, many-body physics and statistical mechanics. They share in common that coherent and driven-dissipative quantum dynamics occur on an equal footing, creating genuine non-equilibrium scenarios without immediate counterpart in condensed matter. This concerns both their non-thermal flux equilibrium states, as well as their many-body time evolution. It is a challenge to theory to identify novel instances of universal emergent macroscopic phenomena, which are tied unambiguously and in an observable way to the microscopic drive conditions. In this review, we discuss some recent results in this direction. Moreover, we provide a systematic introduction to the open system Keldysh functional integral approach, which is the proper technical tool to accomplish a merger of quantum optics and many-body physics, and leverages the power of modern quantum field theory to driven open quantum systems.

cond-mat.quant-gas

Absorbing state phase transition with competing quantum and classical fluctuations

Stochastic processes with absorbing states feature remarkable examples of non-equilibrium universal phenomena. While a broad understanding has been progressively established in the classical regime, relatively little is known about the behavior of these non-equilibrium systems in the presence of quantum fluctuations. Here we theoretically address such a scenario in an open quantum spin model which in its classical limit undergoes a directed percolation phase transition. By mapping the problem to a non-equilibrium field theory, we show that the introduction of quantum fluctuations stemming from coherent, rather than statistical, spin-flips alters the nature of the transition such that it becomes first-order. In the intermediate regime, where classical and quantum dynamics compete on equal terms, we highlight the presence of a bicritical point with universal features different from the directed percolation class in low dimension. We finally propose how this physics could be explored within gases of interacting atoms excited to Rydberg states.

cond-mat.stat-mech

Creating exotic condensates via quantum-phase-revival dynamics in engineered lattice potentials

In the field of ultracold atoms in optical lattices a plethora of phenomena governed by the hopping energy $J$ and the interaction energy $U$ have been studied in recent years. However, the trapping potential typically present in these systems sets another energy scale and the effects of the corresponding time scale on the quantum dynamics have rarely been considered. Here we study the quantum collapse and revival of a lattice Bose-Einstein condensate (BEC) in an arbitrary spatial potential, focusing on the special case of harmonic confinement. Analyzing the time evolution of the single-particle density matrix, we show that the physics arising at the (temporally) recurrent quantum phase revivals is essentially captured by an effective single particle theory. This opens the possibility to prepare exotic non-equilibrium condensate states with a large degree of freedom by engineering the underlying spatial lattice potential.

cond-mat.quant-gas