arXiv subjects

M. Busso

Publications and source records attributed to M. Busso.

At least 19 recordsLinked to original sources

arXiv2026

Energy-differential measurement of the $^{\mathrm{nat}}$C(n,p) and $^{\mathrm{nat}}$C(n,d) reactions at the n_TOF facility at CERN

Energy-differential cross section of the $^{\mathrm{nat}}$C(n,p) and $^{\mathrm{nat}}$C(n,d) reactions was measured at the neutron time of flight facility n_TOF at CERN. The measurement was performed in the first experimental area (EAR1; flight path of 182.5 m). Two position-sensitive $\Delta E$-$E$ silicon telescopes were used. Two naturally occurring carbon isotopes, $^{12}$C and $^{13}$C, contribute to the reactions on natural carbon, with the (n,p) reaction threshold at 13.7 MeV and the (n,d) threshold at 14.9 MeV (determined by the $^{12}$C isotope for both reactions). This paper provides the details of the analysis leading to the final results published previously as a Letter. The cross section results are reported up to 25 MeV. During the data analysis the population of the excited states in the daughter nuclei $^{11}$B, $^{12}$B, $^{13}$B had to be considered, requiring the adoption of the branching ratios and angular distributions of the emitted particles from an external source of information. TALYS-2.0 calculations were used as the main source and an in-depth analysis of the model-related uncertainties was performed. The n_TOF results are largely inconsistent with the major evaluation libraries. On the other hand, an unexpected agreement is found with TALYS-2.0 calculations. Specifically, the obtained cross section for the (n,p) reaction is significantly higher than in the available evaluations, fully supporting the earlier finding from an integral measurement at n_TOF.

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arXiv2025

Measurement of the $^\text{nat}$C(n,p) and $^\text{nat}$C(n,d) reactions from n_TOF at CERN

The energy dependence of the cross section of the (n,p) and (n,d) reactions on $^\text{nat}$C has been studied for the first time at the n_TOF facility at CERN, from the particle detection threshold up to 25 MeV. The measurement was performed with two telescopes made of position-sensitive silicon $\Delta E$-$E$ detectors, covering the angular range from 20{\deg} to 140{\deg}. A detector efficiency has been determined by means of Monte Carlo simulations of the experimental setup. Various assumptions on the angular distributions and branching ratios of the excited levels of the residual $^{11}$B, $^{12}$B, $^{13}$B nuclei were considered. In particular, theoretical calculations based on the TALYS-2.0 code were used and the systematic uncertainties in the analysis results were determined from the variations in these distributions. The n_TOF data on the (n,p) and (n,d) reaction on carbon are characterized by a higher accuracy and wider energy range than currently available in literature. A comparison with current evaluations from different libraries reveals a rather significant disagreement with the n_TOF results, while a remarkable agreement is observed with the prediction of TALYS-2.0 for this light element.

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arXiv2024

Measurement and analysis of the $^{246}$Cm and $^{248}$Cm neutron capture cross-sections at the EAR2 of the n TOF facility

The $^{246}$Cm(n,$\gamma$) and $^{248}$Cm(n,$\gamma$) cross-sections have been measured at the Experimental Area 2 (EAR2) of the n_TOF facility at CERN with three C$_6$D$_6$ detectors. This measurement is part of a collective effort to improve the capture cross-section data for Minor Actinides (MAs), which are required to estimate the production and transmutation rates of these isotopes in light water reactors and innovative reactor systems. In particular, the neutron capture in $^{246}$Cm and $^{248}$Cm open the path for the formation of other Cm isotopes and heavier elements such as Bk and Cf and the knowledge of (n,$\gamma$) cross-sections of these Cm isotopes plays an important role in the transport, transmutation and storage of the spent nuclear fuel. The reactions $^{246}$Cm(n,$\gamma$) and $^{248}$Cm(n,$\gamma$) have been the two first capture measurements analyzed at n_TOF EAR2. Until this experiment and two recent measurements performed at J-PARC, there was only one set of data of the capture cross-sections of $^{246}$Cm and $^{248}$Cm, that was obtained in 1969 in an underground nuclear explosion experiment. In the measurement at n_TOF a total of 13 resonances of $^{246}$Cm between 4 and 400 eV and 5 of $^{248}$Cm between 7 and 100 eV have been identified and fitted. The radiative kernels obtained for $^{246}$Cm are compatible with JENDL-5, but some of them are not with JENDL-4, which has been adopted by JEFF-3.3 and ENDF/B-VIII.0. The radiative kernels obtained for the first three $^{248}$Cm resonances are compatible with JENDL-5, however, the other two are not compatible with any other evaluation and are 20% and 60% larger than JENDL-5.

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arXiv2022

Measurement of the $^{14}$N(n,p)$^{14}$C cross section at the CERN n_TOF facility from sub-thermal energy to 800 keV

Background: The $^{14}$N(n,p)$^{14}$C reaction is of interest in neutron capture therapy, where nitrogen-related dose is the main component due to low-energy neutrons, and in astrophysics, where 14N acts as a neutron poison in the s-process. Several discrepancies remain between the existing data obtained in partial energy ranges: thermal energy, keV region and resonance region. Purpose: Measuring the 14N(n,p)14C cross section from thermal to the resonance region in a single measurement for the first time, including characterization of the first resonances, and providing calculations of Maxwellian averaged cross sections (MACS). Method: Time-of-flight technique. Experimental Area 2 (EAR-2) of the neutron time-of-flight (n_TOF) facility at CERN. $^{10}$B(n,${\alpha}$)$^7$Li and $^{235}$U(n,f) reactions as references. Two detection systems running simultaneously, one on-beam and another off-beam. Description of the resonances with the R-matrix code sammy. Results: The cross section has been measured from sub-thermal energy to 800 keV resolving the two first resonances (at 492.7 and 644 keV). A thermal cross-section (1.809$\pm$0.045 b) lower than the two most recent measurements by slightly more than one standard deviation, but in line with the ENDF/B-VIII.0 and JEFF-3.3 evaluations has been obtained. A 1/v energy dependence of the cross section has been confirmed up to tens of keV neutron energy. The low energy tail of the first resonance at 492.7 keV is lower than suggested by evaluated values, while the overall resonance strength agrees with evaluations. Conclusions: Our measurement has allowed to determine the $^{14}$N(n,p) cross-section over a wide energy range for the first time. We have obtained cross-sections with high accuracy (2.5 %) from sub-thermal energy to 800 keV and used these data to calculate the MACS for kT = 5 to kT = 100 keV.

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arXiv2021

Theoretical estimate of the half-life for the radioactive $^{134}$Cs and $^{135}$Cs in astrophysical scenarios

We analyze the $^{134}_{55}$Cs$\rightarrow^{134}_{56}$Ba and $^{135}_{55}$Cs$\rightarrow^{135}_{56}$Ba $\beta^-$ decays, which are crucial production channels for Ba isotopes in Asymptotic Giant Branch (AGB) stars. We reckon, from relativistic quantum mechanis, the effects of multichannel scattering onto weak decays, including nuclear and electronic excited states (ES) populated above $\simeq$ 10 keV, for both parent and daughter nuclei. We find increases in the half-lives for $T>10^8$ K (by more than a factor 3 for $^{134}$Cs) as compared to previous works based on systematics. We also discuss our method in view of these previous calculations. An important impact on half-lives comes from nuclear ES decays, while including electronic temperatures yields further increases of about 20\% at energies 10-30 keV, typical of AGB stars of moderate mass ($M \lesssim 8~M_{\odot}$). Despite properly considering these effects, the new rates remain sensitively lower than the TY values, implying longer half-lives at least above 8-9 keV. Our rate predictions are in substantial accord with recent results based on the shell model, and strongly modify branching ratios along the $s$-process path previously adopted. With our new rate, nucleosynthesis models well account for the isotopic admixtures of Ba in presolar SiC grains and in the Sun.

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arXiv2021

Magnetic-buoyancy-induced mixing in AGB Stars: fluorine nucleosynthesis at different metallicities

Asymptotic giant branch (AGB) stars are considered to be among the most significant contributors to the fluorine budget in our Galaxy. While at close-to-solar metallicity observations and theory agree, at lower metallicities stellar models overestimate the fluorine production with respect to heavy elements. We present ${}^{19}$F nucleosynthesis results for a set of AGB models with different masses and metallicities in which magnetic buoyancy acts as the driving process for the formation of the ${}^{13}$C neutron source (the so-called ${}^{13}$C pocket). We find that ${}^{19}$F is mainly produced as a result of nucleosynthesis involving secondary ${}^{14}$N during convective thermal pulses, with a negligible contribution from the ${}^{14}$N present in the ${}^{13}$C pocket region. A large ${}^{19}$F production is thus prevented, resulting in lower fluorine surface abundances. As a consequence, AGB stellar models with magnetic-buoyancy-induced mixing at the base of the convective envelope well agree with available fluorine spectroscopic measurements at both low and close-to-solar metallicity.

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arXiv2020

Imaging neutron capture cross sections: i-TED proof-of-concept and future prospects based on Machine-Learning techniques

i-TED is an innovative detection system which exploits Compton imaging techniques to achieve a superior signal-to-background ratio in ($n,\gamma$) cross-section measurements using time-of-flight technique. This work presents the first experimental validation of the i-TED apparatus for high-resolution time-of-flight experiments and demonstrates for the first time the concept proposed for background rejection. To this aim both $^{197}$Au($n,\gamma$) and $^{56}$Fe($n, \gamma$) reactions were measured at CERN n\_TOF using an i-TED demonstrator based on only three position-sensitive detectors. Two \cds detectors were also used to benchmark the performance of i-TED. The i-TED prototype built for this study shows a factor of $\sim$3 higher detection sensitivity than state-of-the-art \cds detectors in the $\sim$10~keV neutron energy range of astrophysical interest. This paper explores also the perspectives of further enhancement in performance attainable with the final i-TED array consisting of twenty position-sensitive detectors and new analysis methodologies based on Machine-Learning techniques.

physics.ins-det↗

arXiv2019

Review and new concepts for neutron-capture measurements of astrophysical interest

The idea of slow-neutron capture nucleosynthesis formulated in 1957 triggered a tremendous experimental effort in different laboratories worldwide to measure the relevant nuclear physics input quantities, namely ($n,\gamma$) cross sections over the stellar temperature range (from few eV up to several hundred keV) for most of the isotopes involved from Fe up to Bi. A brief historical review focused on total energy detectors will be presented to illustrate how, advances in instrumentation have led, over the years, to the assessment and discovery of many new aspects of $s$-process nucleosynthesis and to the progressive refinement of theoretical models of stellar evolution. A summary will be presented on current efforts to develop new detection concepts, such as the Total-Energy Detector with $\gamma$-ray imaging capability (i-TED). The latter is based on the simultaneous combination of Compton imaging with neutron time-of-flight (TOF) techniques, in order to achieve a superior level of sensitivity and selectivity in the measurement of stellar neutron capture rates.

physics.ins-det↗

arXiv2019

The effects of a revised $^7$Be e$^-$-capture rate on solar neutrino fluxes

The electron-capture rate on $^7$Be is the main production channel for $^7$Li in several astrophysical environments. Theoretical evaluations have to account for not only the nuclear interaction, but also the processes in the plasma where $^7$Be ions and electrons interact. In the past decades several estimates were presented, pointing out that the theoretical uncertainty in the rate is in general of few percents. In the framework of fundamental solar physics, we consider here a recent evaluation for the $^7$Be+e$^-$ rate, not used up to now in the estimate of neutrino fluxes. We analysed the effects of the new assumptions on Standard Solar Models (SSMs) and compared the results obtained by adopting the revised $^7$Be+e$^-$ rate to those obtained by the one reported in a widely used compilation of reaction rates (ADE11). We found that new SSMs yield a maximum difference in the efficiency of the $^7$Be channel of about -4\% with respect to what is obtained with the previously adopted rate. This fact affects the production of neutrinos from $^8$B, increasing the relative flux up to a maximum of 2.7\%. Negligible variations are found for the physical and chemical properties of the computed solar models. The agreement with the SNO measurements of the neutral current component of the $^8$B neutrino flux is improved.

astro-ph.SR↗

arXiv2018

On the Origin of the Early Solar System Radioactivities. Problems with the AGB and Massive Star Scenarios

Recent improvements in stellar models for intermediate-mass and massive stars are recalled, together with their expectations for the synthesis of radioactive nuclei of lifetime $\tau \lesssim 25$ Myr, in order to re-examine the origins of now extinct radioactivities, which were alive in the solar nebula. The Galactic inheritance broadly explains most of them, especially if $r$-process nuclei are produced by neutron star merging according to recent models. Instead, $^{26}$Al, $^{41}$Ca, $^{135}$Cs and possibly $^{60}$Fe require nucleosynthesis events close to the solar formation. We outline the persisting difficulties to account for these nuclei by Intermediate Mass Stars (2 $\lesssim $ M/M$_\odot \lesssim 7 - 8$). Models of their final stages now predict the ubiquitous formation of a $^{13}$C reservoir as a neutron capture source; hence, even in presence of $^{26}$Al production from Deep Mixing or Hot Bottom Burning, the ratio $^{26}$Al/$^{107}$Pd remains incompatible with measured data, with a large excess in $^{107}$Pd. This is shown for two recent approaches to Deep Mixing. Even a late contamination by a Massive Star meets problems. In fact, inhomogeneous addition of Supernova debris predicts non-measured excesses on stable isotopes. Revisions invoking specific low-mass supernovae and/or the sequential contamination of the pre-solar molecular cloud might be affected by similar problems, although our conclusions here are weakened by our schematic approach to the addition of SN ejecta. The limited parameter space remaining to be explored for solving this puzzle is discussed.

astro-ph.SR↗

arXiv2018

The $^{7}$Be($\boldsymbol{n,p}$)$^{7}$Li reaction and the Cosmological Lithium Problem: measurement of the cross section in a wide energy range at n_TOF (CERN)

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n\_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed.

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arXiv2018

The importance of the 13C(alpha,n)16O reaction in Asymptotic Giant Branch stars

Low mass Asymptotic Giant Branch stars are among the most important polluters of the interstellar medium. In their interiors, the main component (A>90) of the slow neutron capture process (the s-process) is synthesized, the most important neutron source being the 13C(alpha,n)16O reaction. In this paper we review its current experimental status discussing possible future synergies between some experiments currently focused on the determination of its rate. Moreover, in order to determine the level of precision needed to fully characterize this reaction, we present a theoretical sensitivity study, carried out with the FUNS evolutionary stellar code and the NEWTON post-process code. We modify the rate up to a factor of two with respect to a reference case. We find that variations of the 13C(alpha,n)16O rate do not appreciably affect s-process distributions for masses above 3 Msun at any metallicity. Apart from a few isotopes, in fact, the differences are always below 5%. The situation is completely different if some 13C burns in a convective environment: this occurs in FUNS models with M<3 Msun at solar-like metallicities. In this case, a change of the 13C(alpha,n)16O reaction rate leads to non-negligible variations of the elements Surface distribution (10% on average), with larger peaks for some elements (as rubidium) and for neutron-rich isotopes (as 86Kr and 96Zr). Larger variations are found in low-mass low-metallicity models, if protons are mixed and burnt at very high temperatures. In this case, the surface abundances of the heavier elements may vary by more than a factor 50.

astro-ph.SR↗

arXiv2018

The $^{7}$Be(n,p)$^{7}$Li reaction and the Cosmological Lithium Problem: measurement of the cross section in a wide energy range at n_TOF (CERN)

We report on the measurement of the $^{7}$Be($n, p$)$^{7}$Li cross section from thermal to approximately 325 keV neutron energy, performed in the high-flux experimental area (EAR2) of the n_TOF facility at CERN. This reaction plays a key role in the lithium yield of the Big Bang Nucleosynthesis (BBN) for standard cosmology. The only two previous time-of-flight measurements performed on this reaction did not cover the energy window of interest for BBN, and showed a large discrepancy between each other. The measurement was performed with a Si-telescope, and a high-purity sample produced by implantation of a $^{7}$Be ion beam at the ISOLDE facility at CERN. While a significantly higher cross section is found at low-energy, relative to current evaluations, in the region of BBN interest the present results are consistent with the values inferred from the time-reversal $^{7}$Li($p, n$)$^{7}$Be reaction, thus yielding only a relatively minor improvement on the so-called Cosmological Lithium Problem (CLiP). The relevance of these results on the near-threshold neutron production in the p+$^{7}$Li reaction is also discussed.

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arXiv2017

s-Processing from MHD-induced mixing and isotopic abundances in presolar SiC grains

In the past years the observational evidence that s-process elements from Sr to Pb are produced by stars ascending the socalled Asymptotic Giant Branch (or AGB) could not be explained by self-consistent models, forcing researchers to extensive parameterizations. The crucial point is to understand how protons can be injected from the envelope into the He-rich layers, yielding the formation of 13C and then the activation of the 13C(a,n)16O reaction. Only recently, attempts to solve this problem started to consider quantitatively physically-based mixing mechanisms. Among them, MHD processes in the plasma were suggested to yield mass transport through magnetic buoyancy. In this framework, we compare results of nucleosynthesis models for Low Mass AGB Stars (M<=3Mo), developed from the MHD scenario, with the record of isotopic abundance ratios of s-elements in presolar SiC grains, which were shown to offer precise constraints on the 13C reservoir. We find that n-captures driven by magnetically-induced mixing can indeed account for the SiC data quite well and that this is due to the fact that our 13C distribution fulfils the above constraints rather accurately. We suggest that similar tests should be now performed using different physical models for mixing. Such comparisons would indeed improve decisively our understanding of the formation of the neutron source.

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arXiv2017

Science with e-ASTROGAM (A space mission for MeV-GeV gamma-ray astrophysics)

e-ASTROGAM (enhanced ASTROGAM) is a breakthrough Observatory space mission, with a detector composed by a Silicon tracker, a calorimeter, and an anticoincidence system, dedicated to the study of the non-thermal Universe in the photon energy range from 0.3 MeV to 3 GeV - the lower energy limit can be pushed to energies as low as 150 keV for the tracker, and to 30 keV for calorimetric detection. The mission is based on an advanced space-proven detector technology, with unprecedented sensitivity, angular and energy resolution, combined with polarimetric capability. Thanks to its performance in the MeV-GeV domain, substantially improving its predecessors, e-ASTROGAM will open a new window on the non-thermal Universe, making pioneering observations of the most powerful Galactic and extragalactic sources, elucidating the nature of their relativistic outflows and their effects on the surroundings. With a line sensitivity in the MeV energy range one to two orders of magnitude better than previous generation instruments, e-ASTROGAM will determine the origin of key isotopes fundamental for the understanding of supernova explosion and the chemical evolution of our Galaxy. The mission will provide unique data of significant interest to a broad astronomical community, complementary to powerful observatories such as LIGO-Virgo-GEO600-KAGRA, SKA, ALMA, E-ELT, TMT, LSST, JWST, Athena, CTA, IceCube, KM3NeT, and LISA.

astro-ph.HE↗

arXiv2015

$s$-Processing in AGB Stars Revisited. II. Enhanced $^{13}$C Production Through MHD-Induced Mixing

Slow neutron captures are responsible for the production of about $50\%$ of elements heavier than iron, mainly, occurring during the asymptotic giant branch phase of low-mass stars ($1$ $\lesssim M$/M$_{\odot}$ $\lesssim$ $3$), where the main neutron source is the $^{13}$C($\alpha$,n)$^{16}$O reaction. This last is activated from locally-produced $^{13}$C, formed by partial mixing of hydrogen into the He-rich layers. We present here the first attempt at describing a physical mechanism for the formation of the $^{13}$C reservoir, studying the mass circulation induced by magnetic buoyancy and without adding new free parameters to those already involved in stellar modelling. Our approach represents the application, to the stellar layers relevant for $s$-processing, of recent exact, analytical 2D and 3D models for magneto-hydrodynamic processes at the base of convective envelopes in evolved stars in order to promote downflows of envelope material for mass conservation, during the occurrence of a dredge-up phenomenon. We find that the proton penetration is characterized by small concentrations, but extended over a large fractional mass of the He-layers, thus producing $^{13}$C reservoirs of several $10^{-3}$ M$_{\odot}$. The ensuing $^{13}$C-enriched zone has an almost flat profile, while only a limited production of $^{14}$N occurs. In order to verify the effects of our new findings we show how the abundances of the main $s$-component nuclei can be accounted for in solar proportions and how our large $^{13}$C-reservoir allows us to solve a few so far unexplained features in the abundance distribution of post-AGB objects.

astro-ph.SR↗

arXiv2014

A new solar fluorine abundance and a fluorine determination in the two open clusters M 67 and NGC 6404

We present a new determination of the solar fluorine abundance together with abundance measurements of fluorine in two Galactic open clusters. We analyzed a sunspot spectrum, observed by L. Wallace and W. Livingston with the FTS at the McMath/Pierce Solar Telescope situated on Kitt Peak and spectra of four giants in the old cluster M 67 ($\sim$4.5 Gyr) and three giants in the young cluster NGC 6404 ($\sim$0.5 Gyr), obtained with the CRIRES spectrograph at VLT. Fluorine was measured through synthesis of the available HF lines. We adopted the recent set of experimental molecular parameters of HF delivered by the HITRAN database, and found a new solar fluorine abundance of $A(F) = 4.40\pm 0.25$, in good agreement with the M 67 average fluorine abundance of $A(F) = 4.49\pm 0.20$. The new solar abundance is in a very good agreement with the meteoritic value. The used modern spectrosynthesis tools, the agreement with the meteoritic value and with the results in open cluster M67, known to be a solar analogue, make our solar determination very robust. At the same time, the fluorine measurement in the above-mentioned open clusters is the first step in the understanding of its evolution during the last $\sim$10 Gyr in the Galactic disk. In order to develop this project, a larger sample of open clusters is required, so that it would allow us to trace the evolution of fluorine as a function of time and, in turn, to better understand its origin.

astro-ph.SR↗

arXiv2014

MHD and deep mixing in evolved stars. 1. 2D and 3D analytical models for the AGB

The advection of thermonuclear ashes by magnetized domains emerging from near the H-shell was suggested to explain AGB star abundances. Here we verify this idea quantitatively through exact MHD models. Starting with a simple 2D geometry and in an inertia frame, we study plasma equilibria avoiding the complications of numerical simulations. We show that, below the convective envelope of an AGB star, variable magnetic fields induce a natural expansion, permitted by the almost ideal MHD conditions, in which the radial velocity grows as the second power of the radius. We then study the convective envelope, where the complexity of macro-turbulence allows only for a schematic analytical treatment. Here the radial velocity depends on the square root of the radius. We then verify the robustness of our results with 3D calculations for the velocity, showing that, for both the studied regions, the solution previously found can be seen as a planar section of a more complex behavior, in which anyway the average radial velocity retains the same dependency on radius found in 2D. As a final check, we compare our results to approximate descriptions of buoyant magnetic structures. For realistic boundary conditions the envelope crossing times are sufficient to disperse in the huge convective zone any material transported, suggesting magnetic advection as a promising mechanism for deep mixing. The mixing velocities are smaller than for convection, but larger than for diffusion and adequate to extra-mixing in red giants.

astro-ph.SR↗