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M. Chavez-Cervantes

Publications and source records attributed to M. Chavez-Cervantes.

5 recordsLinked to original sources

The Ultrafast Superconducting Diode Effect

Nonreciprocal transport is generally observed in superconductors in which time reversal and inversion symmetries are simultaneously broken. This effect, which may become one of the backbones for future superconducting electronics, arises because of asymmetric vortex transport in a magnetic field. However, vortex transport is also intrinsically dissipative and limited in speed. Here, we report on the discovery of ultrafast non-reciprocal transport in centrosymmetric superconductors. For NbN films biased with a quasi-DC supercurrent, picosecond current pulses with the same sign as the bias experience resistive impedance, whereas pulses of opposite polarity encounter an inductive response. Strikingly, the effect is at least three orders of magnitude faster than in conventional superconducting diodes, limited only by ultrafast current-induced depairing. We demonstrate rectification of a 100 GHz signal, with dissipation levels of a few fJ per cycle. We foresee potential for superconducting logic elements, operating at THz bit rates with aJ energy dissipation per operation.

cond-mat.supr-con

Probing picosecond depairing currents in type-II superconductors

Accessing the intrinsic critical current density (Jc*) in type II superconductors has significant fundamental and technological potential, both as a probe of the microscopic superconducting properties and as a means to increase current limits in high magnetic field devices and in electrical power systems. Yet, the experimental critical current density in type II superconductors (Jc), when measured with DC currents, is generally lower than the intrinsic limit, mostly due to vortex motion and self-heating. Here, we show that ultrafast picosecond electrical pulses, which interact with the material on timescales over which vortices are inertially immobile, carry supercurrents up to the intrinsic depairing limit Jc* >> Jc. We probe picosecond critical currents in NbN and YBa2Cu3O7 (YBCO), as representative s-wave and d-wave superconductors, respectively. In NbN, we find a sharp onset of the picosecond depairing at a current density as large as Jc*=2.2 Jc, a limit that is well described by microscopic dynamics based on BCS theory. In contrast, YBCO exhibits a gradual suppression of superconductivity as a function of the picosecond current, reflecting its d-wave symmetry. These results offer a powerful new probe of superconductors beyond the reach of conventional transport measurements. The ability to reach the depairing current may also lead to robust new platforms for superconducting electronics.

cond-mat.supr-con

Nonlinear transport in a photo-induced superconductor

Optically driven quantum materials exhibit a variety of non-equilibrium functional phenomena [1-11], which are potentially associated with unique transport properties. However, these transient electrical responses have remained largely unexplored, primarily because of the challenges associated with integrating quantum materials into ultrafast electrical devices. Here, thin films of K3C60 grown by Molecular Beam Epitaxy were connected by coplanar terahertz waveguides to a series of photo-conductive switches. This geometry enabled ultrafast transport measurements at high current densities, providing new information on the photo-induced phase created in the high temperature metal by mid-infrared excitation [12-16]. Nonlinearities in the current-voltage charactersitics of the transient state validate the assignment of transient superconductivity, and point to an inhomogeneous phase in which superconducting regions of the sample are connected by resistive weak links [17-23]. This work opens up the possibility of systematic transport measurements in driven quantum materials, both to probe their properties and to integrate them into ultrafast optoelectronic platforms.

cond-mat.supr-con

Microscopic understanding of ultrafast charge transfer in van-der-Waals heterostructures

Van-der-Waals heterostructures show many intriguing phenomena including ultrafast charge separation following strong excitonic absorption in the visible spectral range. However, despite the enormous potential for future applications in the field of optoelectronics, the underlying microscopic mechanism remains controversial. Here we use time- and angle-resolved photoemission spectroscopy combined with microscopic many-particle theory to reveal the relevant microscopic charge transfer channels in epitaxial WS$_2$/graphene heterostructures. We find that the timescale for efficient ultrafast charge separation in the material is determined by direct tunneling at those points in the Brillouin zone where WS$_2$ and graphene bands cross, while the lifetime of the charge separated transient state is set by defect-assisted tunneling through localized sulphur vacanices. The subtle interplay of intrinsic and defect-related charge transfer channels revealed in the present work can be exploited for the design of highly efficient light harvesting and detecting devices.

cond-mat.mes-hall

Angle-resolved photoemission spectroscopy with 9-eV photon-energy pulses generated in a gas-filled hollow-core photonic crystal fiber

A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few μJ energy generate vacuum ultraviolet (VUV) radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi2Se3 with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promises time-resolved ARPES measurements at repetition rates of hundreds of kHz or even MHz, with photon energies that cover the first Brillouin zone of most materials.

physics.optics