arXiv subjects

M. D. Fraser

Publications and source records attributed to M. D. Fraser.

13 recordsLinked to original sources

arXiv2019

Direct measurement of polariton-polariton interaction strength in the Thomas-Fermi regime of exciton-polariton condensation

Bosonic condensates of exciton polaritons (light-matter quasiparticles in a semiconductor) provide a solid-state platform for studies of non-equilibrium quantum systems with a spontaneous macroscopic coherence. These driven, dissipative condensates typically coexist and interact with an incoherent reservoir, which undermines measurements of key parameters of the condensate. Here, we overcome this limitation by creating a high-density exciton-polariton condensate in an optically-induced "box" trap. In this so-called Thomas-Fermi regime, the condensate is fully separated from the reservoir and its behaviour is dominated by interparticle interactions. We use this regime to directly measure the polariton-polariton interaction strength, and reduce the existing uncertainty in its value from four orders of magnitude to within three times the theoretical prediction. The Thomas-Fermi regime has previously been demonstrated only in ultracold atomic gases in thermal equilibrium. In a non-equilibrium exciton-polariton system, this regime offers a novel opportunity to study interaction-driven effects unmasked by an incoherent reservoir.

cond-mat.quant-gas↗

arXiv2017

Spontaneous condensation of exciton polaritons in the single-shot regime

Bose-Einstein condensate of exciton polaritons in a semiconductor microcavity is a macroscopically populated coherent quantum state subject to concurrent pumping and decay. Debates about the fundamental nature of the condensed phase in this open quantum system still persist. Here, we gain a new insight into the spontaneous condensation process by imaging long-lifetime exciton polaritons in a high-quality inorganic microcavity in the single-shot optical excitation regime, without averaging over multiple condensate realisations. In this highly non-stationary regime, a condensate is strongly influenced by the `hot' incoherent reservoir, and reservoir depletion is critical for the transition to the ground energy and momentum state. Condensates formed by more photonic exciton polaritons exhibit dramatic reservoir-induced density filamentation and shot-to-shot fluctuations. In contrast, condensates of more excitonic quasiparticles display smooth density and are second-order coherent. Our observations show that the single-shot measurements offer a unique opportunity to study formation of macroscopic phase coherence during a quantum phase transition in a solid state system.

cond-mat.quant-gas↗

arXiv2015

Exciton-Polariton Trapping and Potential Landscape Engineering

Exciton-polaritons in semiconductor microcavities have advanced to become a model system for studying dynamical Bose-Einstein condensation, macroscopic coherence, many-body effects, nonclassical states of light and matter, and possibly quantum phase transitions in a solid state. Being low mass bosons, these light-matter quasiparticles can condense at comparably high temperatures up to 300K, while preserving fundamental properties such as coherence in space and time domain even when they are out of equilibrium with the environment. Although the presence of an in-plane polariton confinement potential is not strictly necessary in order to observe condensation of polaritons, engineering the polariton confinement is a key to controlling, shaping and directing the flow of polaritons. Prototype polariton-based optoelectronic devices rely on ultrafast photon-like velocities and strong nonlinearities, as well as on tailored confinement. Nanotechnology provides several pathways to achieving such a confinement, and the specific features and advantages of the different techniques are discussed in this paper. As hybrid exciton-photon quasiparticles, polaritons can be trapped via their excitonic as well as their photonic component, which leads to a wide choice of highly complementary techniques. Here we highlight the almost free choice of trapping geometries and depths of confinement that provides a powerful tool for control and manipulation of polariton systems both in semi-classical and quantum domain. Furthermore, the possibility to observe effects of polariton blockade, Mott insulator physics, and population of higher-order bands in sophisticated lattice potentials is discussed. The observation of such effects will signify the opportunity for the realization of novel polaritonic non-classical light sources and quantum simulators.

cond-mat.quant-gas↗

arXiv2015

Observation of non-Hermitian degeneracies in a chaotic exciton-polariton billiard

Exciton-polaritons are hybrid light-matter quasiparticles formed by strongly interacting photons and excitons (electron-hole pairs) in semiconductor microcavities. They have emerged as a robust solid-state platform for next-generation optoelectronic applications as well as fundamental studies of quantum many-body physics. Importantly, exciton-polaritons are a profoundly open (i.e., non-Hermitian) quantum system: it requires constant pumping of energy and continuously decays releasing coherent radiation. Thus, the exciton-polaritons always exist in a balanced potential landscape of gain and loss. However, the inherent non-Hermitian nature of this potential has so far been largely ignored in exciton-polariton physics. Here we demonstrate that non-Hermiticity dramatically modifies the structure of modes and spectral degeneracies in exciton-polariton systems, and, therefore, will affect their quantum transport, localisation, and dynamical properties. Using a spatially-structured optical pump, we create a chaotic exciton-polariton billiard. Eigenmodes of this billiard exhibit multiple non-Hermitian spectral degeneracies -- exceptional points. These are known to cause remarkable wave phenomena, such as unidirectional transport, anomalous lasing/absorption, and chiral modes. By varying parameters of the billiard, we observe crossing and anti-crossing of energy levels and reveal the nontrivial topological modal structure exclusive to non-Hermitian systems. We also observe the mode switching and topological Berry phase for a parameter loop encircling the exceptional point. Our findings pave the way for studies of non-Hermitian quantum dynamics of exciton-polaritons, which can lead to novel functionalities of polariton-based devices.

cond-mat.quant-gas↗

arXiv2014

Spatial Coherence Properties of One-Dimensional Exciton-Polariton-Condensates

In this work, we combine a systematic experimental investigation of the power- and temperaturedependent evolution of the spatial coherence function, g(1) (r), in a one-dimensional excitonpolariton channel with a modern microscopic numerical theory based on a stochastic master equation approach. The spatial coherence function g(1) (r) is extracted via high-precision Michelson interferometry, which allows us to demonstrate that in the regime of non-resonant excitation, the dependence g(1) (r) reaches a saturation value with a plateau, determined by the intensity of pump and effective temperature of the crystal lattice. The theory, which was extended to allow for treating incoherent excitation in a stochastic frame, matches the experimental data with good qualitative and quantitative agreement. This allows us to verify the prediction that the decay of the off-diagonal long range order can be almost fully suppressed in one-dimensional condensate systems.

cond-mat.mes-hall↗

arXiv2013

Self-localization of polariton condensates in periodic potentials

We predict the existence of novel spatially localized states of exciton-polariton Bose-Einstein condensates in semiconductor microcavities with fabricated periodic in-plane potentials. Our theory shows that, under the condition of continuous off-resonant pumping and losses associated with polariton decay, localization is observed for a wide range of optical pump parameters due to effective potentials self-induced by the polariton flows in the spatially periodic system. We reveal that the self-localization of exciton-polaritons in the lattice may occur both in the gaps and bands of the single-particle linear spectrum, and is dominated by the effects of gain and dissipation rather than the applied potential, in sharp contrast to the conservative condensates of ultracold alkali atoms.

cond-mat.quant-gas↗

arXiv2012

Vortex-antivortex pair dynamics in an exciton-polariton condensate

The study of superfluid and Berezinskii-Kosterlitz-Thouless phases in exciton-polaritons requires an understanding of vortex dynamics in a dissipative unconfined condensate. In this article we study the motion of dynamic vortex-antivortex pairs and show that vortex pair stability defined as ordered motion as opposed to rapid separation or recombination is the result of balance between dissipative velocities in the condensate and interaction with thermal polaritons. The addition of a trapping potential is further shown to considerably enhance the lifetime of a single vortex pair in this system. These investigations have important consequences for interpretation of recent results and future investigations of two-dimensional superfluid phases in polariton condensates.

cond-mat.quant-gas↗

arXiv2006

Detecting the full polarisation state of terahertz transients

We have developed a detector which records the full polarisation state of a terahertz (THz) pulse propagating in free space. The three-electrode photoconductive receiver simultaneously records the electric field of an electromagnetic pulse in two orthogonal directions as a function of time. A prototype device fabricated on Fe+ ion implanted InP exhibited a cross polarised extinction ratio better than 390:1. The design and optimisation of this device are discussed along with its significance for the development of new forms of polarisation sensitive time domain spectroscopy, including THz circular dichroism spectroscopy.

cond-mat.other↗

arXiv2006

Simulation and optimization of arsenic-implanted THz emitters

We have used a three-dimensional pseudo-classical Monte Carlo simulation to investigate the effects of As+ ionimplantation on pulsed terahertz radiation emitters. Devices based on surface-field emitters and photoconductive switches have been modelled. Two implantations of As+ ions at 1.0 MeV and 2.4 MeV were found to produce a uniform distribution of vacancies over the volume of GaAs contributing to THz generation in these devices. We calculate that ionimplantation increases the THz bandwidth of the devices with the cost of decreasing the spectral intensity at lower THz frequencies.

cond-mat.other↗

arXiv2006

Polarisation-Sensitive THz Detectors

We have developed a detector of coherent terahertz (THz) radiation that can recover the full polarisation state of a THz transient. The device is three-contact photoconductive receiver, which is capable of recording two time-varying electric field components of a THz pulse simultaneously. Our receiver was fabricated on Fe+ implanted InP and showed a cross-polarised extinction ratio greater than 100:1. The detector will be useful for spectroscopy of birefringent and optically active materials.

cond-mat.other↗

arXiv2006

Photoconductive detection of arbitrary polarised terahertz pulses

To perform polarization sensitive THz-TDS, it is necessary to be able to measure two (preferably orthogonal) electric field components of a terahertz transient. We have developed a polarization sensitive detector by fabricating a three-contact photoconductive receiver.

cond-mat.other↗

arXiv2005

Polarisation-sensitive terahertz detection by multicontact photoconductive receivers

We have developed a terahertz radiation detector that measures both the amplitude and polarization of the electric field as a function of time. The device is a three-contact photoconductive receiver designed so that two orthogonal electric-field components of an arbitrary polarized electromagnetic wave may be detected simultaneously. The detector was fabricated on Fe+ ion-implanted InP. Polarization-sensitive detection is demonstrated with an extinction ratio better than 100:1. This type of device will have immediate application in studies of birefringent and optically active materials in the far-infrared region of the spectrum.

cond-mat.other↗

arXiv2005

Carrier dynamics in ion-implanted GaAs studied by simulation and observation of terahertz emission

We have studied terahertz (THz) emission from arsenic-ion implanted GaAs both experimentally and using a three-dimensional carrier dynamics simulation. A uniform density of vacancies was formed over the optical absorption depth of bulk GaAs samples by performing multi-energy implantations of arsenic ions (1 and 2.4MeV) and subsequent thermal annealing. In a series of THz emission experiments the frequency of peak THz power was found to increase significantly from 1.4 to 2.2THz when the ion implantation dose was increased from 10^13 to 10^16 cm-3. We used a semi-classical Monte-Carlo simulation of ultra-fast carrier dynamics to reproduce and explain these results. The effect of the ion-induced damage was included in the simulation by considering carrier scattering at neutral and charged impurities, as well as carrier trapping at defect sites. Higher vacancy concentrations and shorter carrier trapping times both contributed to shorter simulated THz pulses, the latter being more important over experimentally realistic parameter ranges.

cond-mat.mtrl-sci↗