arXiv subjects

M. D. Jones

Publications and source records attributed to M. D. Jones.

At least 19 recordsLinked to original sources

arXiv2025

Deviations from the Porter-Thomas Distribution due to Nonstatistical $γ$ Decay below the $^{150}$Nd Neutron Separation Threshold

We introduce a new method for the study of fluctuations of partial transition widths based on nuclear resonance fluorescence experiments with quasimonochromatic linearly polarized photon beams below particle separation thresholds. It is based on the average branching of decays of $J=1$ states of an even-even nucleus to the $2^+_1$ state in comparison to the ground state. Between 5 and 7 MeV, a constant average branching ratio for $γ$ decays from $1^-$ states of 0.490(16) is observed for the nuclide $^{150}$Nd. Assuming $χ^2$-distributed partial transition widths, this average branching ratio is related to a degree of freedom of $ν= 1.93(12)$, rejecting the validity of the Porter-Thomas distribution, requiring $ν=1$. The observed deviation can be explained by nonstatistical effects in the $γ$-decay behavior with contributions in the range of 9.4(10)% up to 94(10)%.

nucl-ex↗

arXiv2022

Model-independent determination of the dipole response of $^{66}$Zn using quasi-monoenergetic and linearly-polarized photon beams

[Background] Photon strength functions are an important ingredient in calculations relevant for the nucleosynthesis of heavy elements. The relation to the photoabsorption cross section allows to experimentally constrain photon strength functions by investigating the photo-response of atomic nuclei. [Purpose] We determine the photoresponse of $^{66}$Zn in the energy region of 5.6 MeV to 9.9 MeV and analyze the contribution of the "elastic" decay channel back to the ground state. In addition, for the elastic channel electric and magnetic dipole transitions were separated. [Methods] Nuclear resonance fluorescence experiments were performed using a linearly-polarized quasi-monoenergetic photon beam at the High Intensity $γ$-ray Source. Photon beam energies from 5.6 to 9.9 MeV with an energy spread of about 3% were selected in steps of 200-300 keV. Two High Purity Germanium detectors were used for the subsequent $γ$-ray spectroscopy. [Results] Full photoabsorption cross sections are extracted from the data making use of the monoenergetic character of the photon beam. For the ground-state decay channel, the average contribution of electric and magnetic dipole strengths is disentangled. The average branching ratio back to the ground state is determined as well. [Conclusions] The new results indicate lower cross sections when compared to the values extracted from a former experiment using bremsstrahlung on $^{66}$Zn. In the latter, the average branching ratio to the ground state is estimated from statistical-model calculations in order to analyze the data. Corresponding estimates from statistical-model calculations underestimate this branching ratio compared to the values extracted from the present analysis, which would partly explain the high cross sections determined from the bremsstrahlung data.

nucl-ex↗

arXiv2022

The Core of $^{25}$F studied by the $^{25}$F(-1p)$^{24}$O reaction

The $^{25}$F($5/2^+) (-1p) ^{24}$O reaction was studied at the NSCL using the S800 spectrometer. The experimental spectroscopic factor for the ground-state to ground-state transition indicates a substantial depletion of the proton $d_{5/2}$ strength compared to shell-model expectations. Our result supports the findings reported by Tang \textit{et al.}, from their study of the $(p,2p)$ reaction at RIBF. The overlap between the $^{25}$F and $^{24}$O ground-states is considerably less than anticipated if $^{24}$O acted as a robust and rigid doubly-magic core in $^{25}$F. We interpret the results within the framework of the Particle-Vibration Coupling (PVC) of a $d_{5/2}$ proton coupled to a quadrupole phonon of an effective core. This approach provides a good description of the experimental data by requiring an effective $^{24}$O* core with a phonon energy of $\hbarω_2$= 3.2 MeV, and a $B(E2) ~ 2.7$ W.u., softer and more collective than a bare $^{24}$O. Both the Nilsson deformed mean field and the PVC models appear to capture the properties of the effective core of $^{25}$F, suggesting that the additional proton tends to polarize the free, doubly magic $^{24}$O in such a way that it becomes either slightly deformed or a quadrupole vibrator.

nucl-ex↗

arXiv2020

Search for the $1/2^+$ intruder state in $^{35}$P

The excitation energy of deformed intruder states (specifically the 2p2h bandhead) as a function of proton number $Z$ along $N=20$ is of interest both in terms of better understanding the evolution of nuclear structure between spherical $^{40}$Ca and the Island of Inversion nuclei, and for benchmarking theoretical descriptions in this region. At the center of the $N=20$ Island of Inversion, the npnh (where n=2,4,6) neutron excitations across a diminished $N=20$ gap result in deformed and collective ground states, as observed in $^{32}$Mg. In heavier isotones, npnh excitations do not dominate in the ground states, but are present in the relatively low-lying level schemes. With the aim of identifying the expected 2p2h$\otimes\mathrm{s}_{1/2^+}$ state in $^{35}$P, the only $N=20$ isotone for which the neutron 2p2h excitation bandhead has not yet been identified, the $^{36}$S(d,$^3$He)$^{35}$P reaction has been revisited in inverse kinematics with the HELical Orbit Spectrometer (HELIOS) at the Argonne Tandem Linac Accelerator System (ATLAS). While a candidate state has not been located, an upper limit for the transfer reaction cross-section to populate such a configuration within a 2.5 to 3.6\,MeV energy range, provides a stringent constraint on the wavefunction compositions in both $^{36}$S and $^{35}$P.

nucl-ex↗

arXiv2018

Architecture of the data aggregation and streaming system for the European Spallation Source neutron instrument suite

The European Spallation Source (ESS) will provide long neutron pulses for experiments on a suite of different instruments. Most of these will perform neutron data acquisition in event mode, i.e. each detected neutron will be characterised by one absolute timestamp and pixel identifier pair. Slow controls metadata from EPICS, such as sample environment measurements and motor positions, will also be timestamped at their source, so that all data and metadata are streamed as a list of events instead of histograms. A flexible data aggregation and streaming system is being developed combining both open source third-party software and in-house development. This is to be used at ESS and other neutron scattering facilities like ISIS and SINQ, replacing legacy solutions by a shared software collection maintained by a cross-facility effort. The architecture of the Apache Kafka-based system, its metadata forwarding and NeXus file writing components are presented, along with test results demonstrating their integration and the scalability in terms of performance.

physics.ins-det↗

arXiv2018

Understanding the Low-Energy Enhancement of the $γ$-ray Strength Function of $^{56}$Fe

A model-independent technique was used to determine the $γ$-ray Strength Function ($γ$SF) of $^{56}$Fe down to $γ$-ray energies less than 1 MeV for the first time with GRETINA using the $(p,p')$ reaction at 16 MeV. No difference was observed in the energy dependence of the $γ$SF built on $2^{+}$ and $4^{+}$ final states, supporting the Brink hypothesis. In addition, angular distribution and polarization measurements were performed. The angular distributions are consistent with dipole radiation. The polarization results show a small bias towards magnetic character in the region of the enhancement.

nucl-ex↗

arXiv2017

Search for excited states in $^{25}$O

Theoretical calculations suggest the presence of low-lying excited states in $^{25}$O. Previous experimental searches by means of proton knockout on $^{26}$F produced no evidence for such excitations. We search for excited states in $^{25}$O using the ${ {}^{24}\text{O} (d,p) {}^{25}\text{O} }$ reaction. The theoretical analysis of excited states in unbound $^{25,27}$O is based on the configuration interaction approach that accounts for couplings to the scattering continuum. We use invariant-mass spectroscopy to measure neutron-unbound states in $^{25}$O. For the theoretical approach, we use the complex-energy Gamow Shell Model and Density Matrix Renormalization Group method with a finite-range two-body interaction optimized to the bound states and resonances of $^{23-26}$O, assuming a core of $^{22}$O. We predict energies, decay widths, and asymptotic normalization coefficients. Our calculations in a large $spdf$ space predict several low-lying excited states in $^{25}$O of positive and negative parity, and we obtain an experimental limit on the relative cross section of a possible ${ {J}^π = {1/2}^{+} }$ state with respect to the ground-state of $^{25}$O at $σ_{1/2+}/σ_{g.s.} = 0.25_{-0.25}^{+1.0}$. We also discuss how the observation of negative parity states in $^{25}$O could guide the search for the low-lying negative parity states in $^{27}$O. Previous experiments based on the proton knockout of $^{26}$F suffered from the low cross sections for the population of excited states in $^{25}$O because of low spectroscopic factors. In this respect, neutron transfer reactions carry more promise.

nucl-ex↗

arXiv2017

Structure of 29F in the Rotation-aligned Coupling Scheme of the Particle-Rotor Model

Recent results from RIKEN/RIBF on the low-lying level structure of 29F are interpreted within the Particle-Rotor Model. We show that the experimental data can be understood in the Rotation-aligned Coupling Scheme, with the 5/2+ ground state as the bandhead of a decoupled band. In this picture, the energy of the observed 1/2+1 state correlates strongly with the rotational energy of the core and provides an estimate of the 2+ energy in 28O. Our analysis suggest a moderate deformation, epsilon_2 ~ 0.17, and places the 2+ in 28O at ~ 2.4 MeV.

nucl-ex↗

arXiv2017

Analysis of Spectroscopic Factors in 11Be and 12Be in the Nilsson Strong Coupling Limit

Spectroscopic factors in 10Be, 11Be and 12Be, extracted from (d,p), one neutron knockout, and (p,d) reactions are interpreted within the rotational model. Assuming that the ground state and first excited state of 11Be can be associated with the 1/2[220] and 1/2[101] Nilsson levels, the strong coupling limit gives simple expressions that relate the amplitudes of these wavefunctions (in the spherical basis) with the measured cross-sections and derived spectroscopic factors. We obtain good agreement with both the measured magnetic moment of the ground state in 11Be and the reaction data.

nucl-th↗

arXiv2015

Two-Neutron Sequential Decay of $^{24}$O

A two-neutron unbound excited state of $^{24}$O was populated through a (d,d') reaction at 83.4 MeV/nucleon. A state at $E = 715 \pm 110$ (stat) $\pm 45 $ (sys) keV with a width of $Γ< 2$ MeV was observed above the two-neutron separation energy placing it at 7.65 $\pm$ 0.2 MeV with respect to the ground state. Three-body correlations for the decay of $^{24}$O $\rightarrow$ $^{22}$O + $2n$ show clear evidence for a sequential decay through an intermediate state in $^{23}$O. Neither a di-neutron nor phase-space model for the three-body breakup were able to describe these correlations.

nucl-ex↗

arXiv2015

Population of 13Be in a Nucleon Exchange Reaction

The neutron-unbound nucleus 13Be was populated with a nucleon-exchange reaction from a 71 MeV/u secondary 13B beam. The decay energy spectrum was reconstructed using invariant mass spectroscopy based on 12Be fragments in coincidence with neutrons. The data could be described with an s-wave resonance at E = 0.73(9) MeV with a width of Gamma = 1.98(34) MeV and a d-wave resonance at E = 2.56(13) MeV with a width of Gamma = 2.29(73) MeV. The observed spectral shape is consistent with previous one-proton removal reaction measurements from 14B.

nucl-ex↗

arXiv2015

Search for unbound 15Be states in the 3n+12Be channel

15Be is expected to have low-lying 3/2+ and 5/2+ states. A first search did not observe the 3/2+ [A. Spyrou et al., Phys. Rev. C 84, 044309 (2011)], however, a resonance in 15Be was populated in a second attempt and determined to be unbound with respect to 14Be by 1.8(1) MeV with a tentative spin-parity assignment of 5/2+ [J. Snyder et al., Phys. Rev. C 88, 031303(R) (2013)]. Search for the predicted 15Be 3/2+ state in the three-neutron decay channel. A two-proton removal reaction from a 55 MeV/u 17C beam was used to populate neutron-unbound states in 15Be. The two-, three-, and four-body decay energies of the 12Be + neutron(s) detected in coincidence were reconstructed using invariant mass spectroscopy. Monte Carlo simulations were performed to extract the resonance and decay properties from the observed spectra. The low-energy regions of the decay energy spectra can be described with the first excited unbound state of 14Be (E_x=1.54 MeV, E_r=0.28 MeV). Including a state in 15Be that decays through the first excited 14Be state slightly improves the fit at higher energies though the cross section is small. A 15Be component is not needed to describe the data. If the 3/2+ state in 15Be is populated, the decay by three-neutron emission through 14Be is weak, less than or equal to 11% up to 4 MeV. In the best fit, 15Be is unbound with respect to 12Be by 1.4 MeV (unbound with respect to $14Be by 2.66 MeV) with a strength of 7%.

nucl-ex↗

arXiv2013

Fermi surface topology and de Hass-van Alphen orbits in PuIn$_{\rm 3}$ and PuSn$_{\rm 3}$ compounds

Since the recent discovery of plutonium-based superconductors such as PuCoIn$_{\rm 5}$, systematic studies of the electronic properties for plutonium compounds are providing insight into the itinerancy-localization crossover of Pu 5$f$ electrons. We are particularly interested in understanding the Fermi surface properties of PuIn$_{3}$ compound, which serves as the building block for the PuCoIn$_{\rm 5}$ superconductor. Motivated by the first observation of quantum oscillation and renewed interest in the de-Hass van-Alphen (dHvA) measurements on PuIn$_{\rm 3}$, we study the Fermi surface (FS) topology and the band dispersion in both paramagnetic and antiferromagnetic state of PuIn$_{\rm 3}$, based on density functional theory with generalized gradient approximation. We compare the results with its isostructural paramagnetic compound PuSn$_{\rm 3}$. We show the detailed Fermi surfaces of compounds PuIn$_{\rm 3}$ and PuSn$_{\rm 3}$ and conclude that the FS topology of an antiferromagnetic PuIn$_3$ agrees better with dHvA measurements. In addition, we show the magnetization of the antiferromagnetic order can alter the angle dependence and values of the effective mass for the dHvA orbits. We point out the accurate determination of the magnetic order orientation with respect to the crystal orientation is crucial to advance the understanding of the electronic structures of the PuIn$_{\rm 3}$ compound.

cond-mat.str-el↗

arXiv2010

Band Narrowing and Mott Localization in Iron Oxychalcogenides La2O2Fe2O(Se,S)2

Bad metal properties have motivated a description of the parent iron pnictides as correlated metals on the verge of Mott localization. What has been unclear is whether interactions can push these and related compounds to the Mott insulating side of the phase diagram. Here we consider the iron oxychalcogenides La2O2Fe2O(Se,S)2, which contain an Fe square lattice with an expanded unit cell. We show theoretically that they contain enhanced correlation effects through band narrowing compared to LaOFeAs, and we provide experimental evidence that they are Mott insulators with moderate charge gaps. We also discuss the magnetic properties in terms of a Heisenberg model with frustrating J1-J2-J2' exchange interactions on a "doubled" checkerboard lattice.

cond-mat.str-el↗

arXiv2010

KEKB Beam Collision Stability at the Picosecond Timing and Micron Position Resolution as observed with the Belle Detector

Using the Belle detector we study the characteristics of beam collisions at the KEKB 3.5 GeV $e^+$ on 8 GeV $e^-$ asymmetric energy collider. We investigate the collision timing {\tip} and its $z$-coordinate along the beam axis {\zip} as a function of the position of the colliding bunch in a beam train. The various {\tip} and {\zip} behaviors observed by Belle are attributed to beam loading effects in the radio frequency cavities that accelerate the beams with a beam abort gap. We report these results in detail and discuss the prospects for the SuperKEKB collider.

physics.ins-det↗

arXiv2008

Spin-Orbit Coupling in an f-electron Tight-Binding Model

We extend a tight-binding method to include the effects of spin-orbit coupling, and apply it to the study of the electronic properties of the actinide elements Th, U, and Pu. These tight-binding parameters are determined for the fcc crystal structure using the equivalent equilibrium volumes. In terms of the single particle energies and the electronic density of states, the overall quality of the tight-binding representation is excellent and of the same quality as without spin-orbit coupling. The values of the optimized tight-binding spin-orbit coupling parameters are comparable to those determined from purely atomic calculations.

cond-mat.mtrl-sci↗

arXiv2008

Many-body Electronic Structure of Metallic alpha-Uranium

We present results for the electronic structure of alpha uranium using a recently developed quasiparticle self-consistent GW method (QSGW). This is the first time that the f-orbital electron-electron interactions in an actinide has been treated by a first-principles method beyond the level of the generalized gradient approximation (GGA) to the local density approximation (LDA). We show that the QSGW approximation predicts an f-level shift upwards of about 0.5 eV with respect to the other metallic s-d states and that there is a significant f-band narrowing when compared to LDA band-structure results. Nonetheless, because of the overall low f-electron occupation number in uranium, ground-state properties and the occupied band structure around the Fermi energy is not significantly affected. The correlations predominate in the unoccupied part of the f states. This provides the first formal justification for the success of LDA and GGA calculations in describing the ground-state properties of this material.

cond-mat.str-el↗

arXiv2007

Spectral Properties of delta-Plutonium: Sensitivity to 5f Occupancy

By combining the local density approximation (LDA) with dynamical mean field theory (DMFT), we report a systematic analysis of the spectral properties of $δ$-plutonium with varying $5f$ occupancy. The LDA Hamiltonian is extracted from a tight-binding (TB) fit to full-potential linearized augmented plane-wave (FP-LAPW) calculations. The DMFT equations are solved by the exact quantum Monte Carlo (QMC) method and the Hubbard-I approximation. We have shown for the first time the strong sensitivity of the spectral properties to the $5f$ occupancy, which suggests using this occupancy as a fitting parameter in addition to the Hubbard $U$. By comparing with PES data, we conclude that the ``open shell'' $5f^{5}$ configuration gives the best agreement, resolving the controversy over $5f$ ``open shell'' versus ``close shell'' atomic configurations in $δ$-Pu.

cond-mat.str-el↗