arXiv subjects

M. D. Lukin

Publications and source records attributed to M. D. Lukin.

At least 37 records · Page 2Linked to original sources

arXiv2015

Phonon-Induced Population Dynamics and Intersystem Crossing in Nitrogen-Vacancy Centers

We report direct measurement of population dynamics in the excited state manifold of a nitrogen-vacancy (NV) center in diamond. We quantify the phonon-induced mixing rate and demonstrate that it can be completely suppressed at low temperatures. Further, we measure the intersystem crossing (ISC) rate for different excited states and develop a theoretical model that unifies the phonon-induced mixing and ISC mechanisms. We find that our model is in excellent agreement with experiment and that it can be used to predict unknown elements of the NV center's electronic structure. We discuss the model's implications for enhancing the NV center's performance as a room-temperature sensor.

quant-ph↗

arXiv2015

Heralded quantum gates with integrated error detection in optical cavities

We propose and analyze heralded quantum gates between qubits in optical cavities. They employ an auxiliary qubit to report if a successful gate occurred. In this manner, the errors, which would have corrupted a deterministic gate, are converted into a non-unity probability of success: once successful the gate has a much higher fidelity than a similar deterministic gate. Specifically, we describe that a heralded , near-deterministic controlled phase gate (CZ-gate) with the conditional error arbitrarily close to zero and the success probability that approaches unity as the cooperativity of the system, C, becomes large. Furthermore, we describe an extension to near-deterministic N- qubit Toffoli gate with a favorable error scaling. These gates can be directly employed in quantum repeater networks to facilitate near-ideal entanglement swapping, thus greatly speeding up the entanglement distribution.

quant-ph↗

arXiv2014

Quasi Many-body Localization in Translation Invariant Systems

It is typically assumed that disorder is essential to realize Anderson localization. Recently, a number of proposals have suggested that an interacting, translation invariant system can also exhibit localization. We examine these claims in the context of a one-dimensional spin ladder. At intermediate time scales, we find slow growth of entanglement entropy consistent with the phenomenology of many-body localization. However, at longer times, all finite wavelength spin polarizations decay in a finite time, independent of system size. We identify a single length scale which parametrically controls both the eventual spin transport times and the divergence of the susceptibility to spin glass ordering. We dub this long pre-thermal dynamical behavior, intermediate between full localization and diffusion, quasi-many body localization.

cond-mat.dis-nn↗

arXiv2014

Efficient readout of a single spin state in diamond via spin-to-charge conversion

Efficient readout of individual electronic spins associated with atom-like impurities in the solid state is essential for applications in quantum information processing and quantum metrology. We demonstrate a new method for efficient spin readout of nitrogen-vacancy (NV) centers in diamond. The method is based on conversion of the electronic spin state of the NV to a charge state distribution, followed by single-shot readout of the charge state. Conversion is achieved through a spin-dependent photoionization process in diamond at room temperature. Using NVs in nanofabricated diamond beams, we demonstrate that the resulting spin readout noise is within a factor of three of the spin projection noise level. Applications of this technique for nanoscale magnetic sensing are discussed.

quant-ph↗

arXiv2014

Efficient fiber-optical interface for nanophotonic devices

We demonstrate a method for efficient coupling of guided light from a single mode optical fiber to nanophotonic devices. Our approach makes use of single-sided conical tapered optical fibers that are evanescently coupled over the last ~10 um to a nanophotonic waveguide. By means of adiabatic mode transfer using a properly chosen taper, single-mode fiber-waveguide coupling efficiencies as high as 97(1)% are achieved. Efficient coupling is obtained for a wide range of device geometries which are either singly-clamped on a chip or attached to the fiber, demonstrating a promising approach for integrated nanophotonic circuits, quantum optical and nanoscale sensing applications.

physics.optics↗

arXiv2014

Single-photon nonlinear optics with graphene plasmons

We show that it is possible to realize significant nonlinear optical interactions at the few photon level in graphene nanostructures. Our approach takes advantage of the electric field enhancement associated with the strong confinement of graphene plasmons and the large intrinsic nonlinearity of graphene. Such a system could provide a powerful platform for quantum nonlinear optical control of light. As an example, we consider an integrated optical device that exploits this large nonlinearity to realize a single photon switch.

cond-mat.mes-hall↗

arXiv2014

Preparation of Non-equilibrium Nuclear Spin States in Double Quantum Dots

We theoretically study the dynamic polarization of lattice nuclear spins in GaAs double quantum dots containing two electrons. In our prior work [Phys. Rev. Lett. 104, 226807 (2010)] we identified three regimes of long-term dynamics, including the build up of a large difference in the Overhauser fields across the dots, the saturation of the nuclear polarization process associated with formation of so-called "dark states," and the elimination of the difference field. In particular, when the dots are different sizes we found that the Overhauser field becomes larger in the smaller dot. Here we present a detailed theoretical analysis of these problems including a model of the polarization dynamics and the development of a new numerical method to efficiently simulate semiclassical central-spin problems. When nuclear spin noise is included, the results agree with our prior work indicating that large difference fields and dark states are stable configurations, while the elimination of the difference field is unstable; however, in the absence of noise we find all three steady states are achieved depending on parameters. These results are in good agreement with dynamic nuclear polarization experiments in double quantum dots.

cond-mat.mes-hall↗

arXiv2014

Nanoplasmonic Lattices for Ultracold atoms

We propose to use sub-wavelength confinement of light associated with the near field of plasmonic systems to create nanoscale optical lattices for ultracold atoms. Our approach combines the unique coherence properties of isolated atoms with the sub-wavelength manipulation and strong light-matter interaction associated with nano-plasmonic systems. It allows one to considerably increase the energy scales in the realization of Hubbard models and to engineer effective long-range interactions in coherent and dissipative many-body dynamics. Realistic imperfections and potential applications are discussed.

physics.atom-ph↗

arXiv2014

Nanophotonic quantum phase switch with a single atom

In analogy to transistors in classical electronic circuits, a quantum optical switch is an important element of quantum circuits and quantum networks. Operated at the fundamental limit where a single quantum of light or matter controls another field or material system, it may enable fascinating applications such as long-distance quantum communication, distributed quantum information processing and metrology, and the exploration of novel quantum states of matter. Here, by strongly coupling a photon to a single atom trapped in the near field of a nanoscale photonic crystal cavity, we realize a system where a single atom switches the phase of a photon, and a single photon modifies the atom's phase. We experimentally demonstrate an atom-induced optical phase shift that is nonlinear at the two-photon level, a photon number router that separates individual photons and photon pairs into different output modes, and a single-photon switch where a single "gate" photon controls the propagation of a subsequent probe field. These techniques pave the way towards integrated quantum nanophotonic networks involving multiple atomic nodes connected by guided light.

quant-ph↗

arXiv2014

Phase diagram and excitations of a Shiba molecule

We analyze the phase diagram associated with a pair of magnetic impurities trapped in a superconducting host. The natural interplay between Kondo screening, superconductivity and exchange interactions leads to a rich array of competing phases, whose transitions are characterized by discontinuous changes of the total spin. Our analysis is based on a combination of numerical renormalization group techniques as well as semi-classical analytics. In addition to the expected screened and unscreened phases, we observe a new molecular doublet phase where the impurity spins are only partially screened by a single extended quasiparticle. Direct signatures of the various Shiba molecule states can be observed via RF spectroscopy.

cond-mat.supr-con↗

arXiv2014

Interferometric probes of many-body localization

We propose a method for detecting many-body localization (MBL) in disordered spin systems. The method involves pulsed, coherent spin manipulations that probe the dephasing of a given spin due to its entanglement with a set of distant spins. It allows one to distinguish the MBL phase from a non-interacting localized phase and a delocalized phase. In particular, we show that for a properly chosen pulse sequence the MBL phase exhibits a characteristic power-law decay reflecting its slow growth of entanglement. We find that this power-law decay is robust with respect to thermal and disorder averaging, provide numerical simulations supporting our results, and discuss possible experimental realizations in solid-state and cold atom systems.

cond-mat.dis-nn↗

arXiv2014

Scattering resonances and bound states for strongly interacting Rydberg polaritons

We provide a theoretical framework describing slow-light polaritons interacting via atomic Rydberg states. We use a diagrammatic method to analytically derive the scattering properties of two polaritons. We identify parameter regimes where polariton-polariton interactions are repulsive. Furthermore, in the regime of attractive interactions, we identify multiple two-polariton bound states, calculate their dispersion, and study the resulting scattering resonances. Finally, the two-particle scattering properties allow us to derive the effective low-energy many-body Hamiltonian. This theoretical platform is applicable to ongoing experiments.

quant-ph↗

arXiv2013

All-optical sensing of a single-molecule electron spin

We demonstrate an all-optical method for magnetic sensing of individual molecules in ambient conditions at room temperature. Our approach is based on shallow nitrogen-vacancy (NV) centers near the surface of a diamond crystal, which we use to detect single paramagnetic molecules covalently attached to the diamond surface. The manipulation and readout of the NV centers is all-optical and provides a sensitive probe of the magnetic field fluctuations stemming from the dynamics of the electronic spins of the attached molecules. As a specific example, we demonstrate detection of a single paramagnetic molecule containing a gadolinium (Gd$^{3+}$) ion. We confirm single-molecule resolution using optical fluorescence and atomic force microscopy to co-localize one NV center and one Gd$^{3+}$-containing molecule. Possible applications include nanoscale and in vivo magnetic spectroscopy and imaging of individual molecules.

cond-mat.mes-hall↗

arXiv2013

Phonon Cooling and Lasing with Nitrogen-Vacancy Centers in Diamond

We investigate the strain-induced coupling between a nitrogen-vacancy impurity and a resonant vibrational mode of a diamond nanoresonator. We show that under near-resonant laser excitation of the electronic states of the impurity, this coupling can modify the state of the resonator and either cool the resonator close to the vibrational ground state or drive it into a large amplitude coherent state. We derive a semi-classical model to describe both effects and evaluate the stationary state of the resonator mode under various driving conditions. In particular, we find that by exploiting resonant single and multi-phonon transitions between near-degenerate electronic states, the coupling to high-frequency vibrational modes can be significantly enhanced and dominate over the intrinsic mechanical dissipation. Our results show that a single nitrogen-vacancy impurity can provide a versatile tool to manipulate and probe individual phonon modes in nanoscale diamond structures.

cond-mat.mes-hall↗

arXiv2013

Nanometer scale quantum thermometry in a living cell

Sensitive probing of temperature variations on nanometer scales represents an outstanding challenge in many areas of modern science and technology. In particular, a thermometer capable of sub-degree temperature resolution as well as integration within a living system could provide a powerful new tool for many areas of biological research, including temperature-induced control of gene expression and cell-selective treatment of disease. Here, we demonstrate a new approach to nanoscale thermometry that utilizes coherent manipulation of the electronic spin associated with nitrogen-vacancy (NV) color centers in diamond. We show the ability to detect temperature variations down to 1.8 mK (sensitivity of 9 mK/sqrt(Hz)) in an ultra-pure bulk diamond sample. Using NV centers in diamond nanocrystals (nanodiamonds), we directly measure the local thermal environment at length scales down to 200 nm. Finally, by introducing both nanodiamonds and gold nanoparticles into a single human embryonic fibroblast, we demonstrate temperature-gradient control and mapping at the sub-cellular level, enabling unique potential applications in life sciences.

quant-ph↗

arXiv2013

Phonon-induced spin-spin interactions in diamond nanostructures: application to spin squeezing

We propose and analyze a novel mechanism for long-range spin-spin interactions in diamond nanostructures. The interactions between electronic spins, associated with nitrogen-vacancy centers in diamond, are mediated by their coupling via strain to the vibrational mode of a diamond mechanical nanoresonator. This coupling results in phonon-mediated effective spin-spin interactions that can be used to generate squeezed states of a spin ensemble. We show that spin dephasing and relaxation can be largely suppressed, allowing for substantial spin squeezing under realistic experimental conditions. Our approach has implications for spin-ensemble magnetometry, as well as phonon-mediated quantum information processing with spin qubits.

cond-mat.mes-hall↗

arXiv2012

Continuous mode cooling and phonon routers for phononic quantum networks

We study the implementation of quantum state transfer protocols in phonon networks, where in analogy to optical networks, quantum information is transmitted through propagating phonons in extended mechanical resonator arrays or phonon waveguides. We describe how the problem of a non-vanishing thermal occupation of the phononic quantum channel can be overcome by implementing optomechanical multi- and continuous mode cooling schemes to create a 'cold' frequency window for transmitting quantum states. In addition, we discuss the implementation of phonon circulators and switchable phonon routers, which rely on strong coherent optomechanical interactions only, and do not require strong magnetic fields or specific materials. Both techniques can be applied and adapted to various physical implementations, where phonons coupled to spin or charge based qubits are used for on-chip networking applications.

quant-ph↗

arXiv2012

Single-photon nonlinearities in two-mode optomechanics

We present a detailed theoretical analysis of a weakly driven multimode optomechanical system, in which two optical modes are strongly and near-resonantly coupled to a single mechanical mode via a three-wave mixing interaction. We calculate one- and two-time intensity correlations of the two optical fields and compare them to analogous correlations in atom-cavity systems. Nonclassical photon correlations arise when the optomechanical coupling $g$ exceeds the cavity decay rate $κ$, and we discuss signatures of one- and two-photon resonances as well as quantum interference. We also find a long-lived correlation that decays slowly with the mechanical decay rate $γ$, reflecting the heralded preparation of a single phonon state after detection of a photon. Our results provide insight into the quantum regime of multimode optomechanics, with potential applications for quantum information processing with photons and phonons.

quant-ph↗