arXiv subjects

M. D. Lumsden

Publications and source records attributed to M. D. Lumsden.

At least 73 records · Page 4Linked to original sources

arXiv2010

Doping Dependence of Spin Dynamics in Electron-Doped Ba(Fe1-xCox)2As2

The spin dynamics in single crystal, electron-doped Ba(Fe1-xCox)2As2 has been investigated by inelastic neutron scattering over the full range from undoped to the overdoped regime. We observe damped magnetic fluctuations in the normal state of the optimally doped compound (x=0.06) that share a remarkable similarity with those in the paramagnetic state of the parent compound (x=0). In the overdoped superconducting compound (x=0.14), magnetic excitations show a gap-like behavior, possibly related to a topological change in the hole Fermi surface (Lifshitz transition), while the imaginary part of the spin susceptibility prominently resembles that of the overdoped cuprates. For the heavily overdoped, non-superconducting compound (x=0.24) the magnetic scattering disappears, which could be attributed to the absence of a hole Fermi-surface pocket observed by photoemission.

cond-mat.supr-con↗

arXiv2010

Inelastic neutron scattering study on the resonance mode in an optimally doped superconductor LaFeAsO$_{0.92}$F$_{0.08}$

An optimally doped iron-based superconductor LaFeAsO$_{0.92}$F$_{0.08}$ with $T_c = 29$ K has been studied by inelastic powder neutron scattering. The magnetic excitation at $Q=1.15$ Å$^{-1}$ is enhanced below $T_c$, leading to a peak at $E_{res}\sim13$ meV as the resonance mode, in addition to the formation of a gap at low energy below the crossover energy $Δ_{c}\sim10 meV$. The peak energy at $Q=1.15$ Å$^{-1}$ corresponds to $5.2 k_B T_c$ in good agreement with the other values of resonance mode observed in the various iron-based superconductors, even in the high-$T_c$ cuprates. Although the phonon density of states has a peak at the same energy as the resonance mode in the present superconductor, the $Q$-dependence is consistent with the resonance being of predominately magnetic origin.

cond-mat.supr-con↗

arXiv2010

Magnetism in Fe-based superconductors

In this review, we present a summary of experimental studies of magnetism in Fe-based superconductors. The doping dependent phase diagram shows strong similarities to the generic phase diagram of the cuprates. Parent compounds exhibit magnetic order together with a structural phase transition both of which are progressively suppressed with doping allowing superconductivity to emerge. The stripe-like spin arrangement of Fe moments in the magnetically ordered state shows the identical in-plane structure for the RFeAsO (R=rare earth) and AFe2As2 (A=Sr, Ca, Ba, Eu and K) parent compounds, notably different than the spin configuration of the cuprates. Interestingly, Fe1+yTe orders with a different spin order despite very similar Fermi surface topology. Studies of the spin dynamics in the parent compounds shows that the interactions are best characterized as anisotropic three-dimensional (3D) interactions. Despite the room temperature tetragonal structure, analysis of the low temperature spin waves under the assumption of a Heisenberg Hamiltonian indicates strong in-plane anisotropy with a significant next-near neighbor interaction. In the superconducting state, a resonance, localized in both wavevector and energy is observed in the spin excitation spectrum as in the cuprates. This resonance is observed at a wavevector compatible with a Fermi surface nesting instability independent of the magnetic ordering of the relevant parent compound. The resonance energy (Er) scales with superconducting transition temperature (TC) as Er ~4.9 kBTC consistent with the canonical value of ~5 kBTC observed in the cuprates. Moreover, the relationship between the resonance energy and the superconducting gap, Δ, is similar to that observed in many unconventional superconductors (Er/2Δ~ 0.64).

cond-mat.supr-con↗

arXiv2010

Neutron scattering and scaling behavior in URu2Zn20 and YbFe2Zn20

The dynamic susceptibility chi"(deltaE), measured by inelastic neutron scattering measurements, shows a broad peak centered at Emax = 16.5 meV for the cubic actinide compound URu2Zn20 and 7 meV at the (1/2, 1/2, 1/2) zone boundary for the rare earth counterpart compound YbFe2Zn20. For URu2Zn20, the low temperature susceptibility and magnetic specific heat coefficient gamma = Cmag/T take the values chi = 0.011 emu/mole and gamma = 190 mJ/mole-K2 at T = 2 K. These values are roughly three times smaller, and Emax is three times larger, than recently reported for the related compound UCo2Zn20, so that chi and gamma scale inversely with the characteristic energy for spin fluctuations, Tsf = Emax/kB. While chi(T), Cmag(T), and Emax of the 4f compound YbFe2Zn20 are very well described by the Kondo impurity model, we show that the model works poorly for URu2Zn20 and UCo2Zn20, suggesting that the scaling behavior of the actinide compounds arises from spin fluctuations of itinerant 5f electrons.

cond-mat.str-el↗

arXiv2010

Dispersion of the superconducting spin resonance in underdoped and antiferromagnetic Ba(Fe1-xCox)2As2

Inelastic neutron scattering measurements have been performed on underdoped Ba(Fe1-xCox)2As2 (x = 4.7%) where superconductivity and long-range antiferromagnetic (AFM) order coexist. The broad magnetic spectrum found in the normal state develops into a magnetic resonance feature below TC that has appreciable dispersion along c-axis with a bandwidth of 3-4 meV. This is in contrast to the optimally doped x = 8.0% composition, with no long-range AFM order, where the resonance exhibits a much weaker dispersion [see Lumsden et al. Phys. Rev. Lett. 102, 107005 (2009)]. The results suggest that the resonance dispersion arises from interlayer spin correlations present in the AFM ordered state.

cond-mat.supr-con↗

arXiv2009

Unusual Relationship between Magnetism and Superconductivity in FeTe$_{0.5}$Se$_{0.5}$

We use neutron scattering, to study magnetic excitations in crystals near the ideal superconducting composition of FeTe$_{0.5}$Se$_{0.5}$. Two types of excitations are found, a resonance at (0.5, 0.5, 0) and incommensurate fluctuations on either side of this position. We show that the two sets of magnetic excitations behave differently with doping, with the resonance being fixed in position while the incommensurate excitations move as the doping is changed. These unusual results show that a common behavior of the low energy magnetic excitations is not necessary for pairing in these materials.

cond-mat.supr-con↗

arXiv2009

Evolution of spin excitations into the superconducting state in FeTe1-xSex

The nature of the superconducting state in the recently discovered Fe-based superconductors1-3 is the subject of intense scrutiny. Neutron scattering investigations have already elucidated a strong correlation between magnetism and superconductivity in the form of a spin resonance in the magnetic excitation spectrum4-7. A central unanswered question concerns the nature of the normal state spin fluctuations which may be responsible for the pairing mechanism. Here we show inelastic neutron scattering measurements of Fe1.04Te0.73Se0.27, not superconducting in bulk, and FeTe0.51Se0.49, a bulk superconductor. These measurements demonstrate that the spin fluctuation spectrum is dominated by two-dimensional incommensurate excitations near the (1/2,1/2) (square lattice (pi,0)) wavevector, the wavevector of interest in other Fe-based superconductors, that extend to energies at least as high as 300 meV. Most importantly, the spin excitations in Fe1+yTe1-xSex exhibit four-fold symmetry about the (1,0) (square lattice (pi,pi)) wavevector and are described by the identical wavevector as the normal state spin excitations in the high-TC cuprates8-12 demonstrating a commonality between the magnetism in these classes of materials which perhaps extends to a common origin for superconductivity.

cond-mat.supr-con↗

arXiv2009

Spin Excitations in BaFe1.84Co0.16As2 Superconductor Observed by Inelastic Neutron Scattering

Superconductivity appears to compete against the spin-density-wave in Fe pnictides. However, optimally cobalt doped samples show a quasi-two-dimensional spin excitation centered at the (0.5, 0.5, L) wavevector, "the spin resonance peak", that is strongly tied to the onset of superconductivity. By inelastic neutron scattering on single crystals we show the similarities and differences of the spin excitations in BaFe1.84Co0.16As2, with respect to the spin excitations in the high-temperature superconducting cuprates. As in the cuprates the resonance occurs as an enhancement to a part of the spin excitation spectrum which extends to higher energy transfer and higher temperature. However, unlike in the cuprates, the resonance peak in this compound is asymmetric in energy.

cond-mat.supr-con↗

arXiv2009

Neutron scattering patterns show Superconductivity in FeTe0.5Se0.5 likely results from itinerant electron fluctuations

The discovery of the Fe pnictide superconductors generated great interest as the structure consists of planes of a magnetic material quite similar to the cuprate superconductors. Fe(Te0.5Se0.5) is a particularly simple system whose planes are isostructural to the FeAs layers found in the originally discovered superconductors of this type. We report here neutron scattering measurements on this material that provide an understanding of the superconductivity. Since the information about the Fermi surface is available both from photoemission and band structure calculations for FeTe, FeSe and other related materials the neutron spectra can be used to see if the itinerant electron picture is valid. The results are consistent with a picture where there are both electron and hole Fermi surfaces that make exact (pi,pi) transitions possible. This would normally favor either a spin or charge density wave state. However, our measurements show the extent of the region where (pi,pi) transitions take place and demonstrate that there are a much larger number of transitions near pi,pi). The near (pi,pi) transitions are observed both above and below Tc and are expected to be strongly pairing. The superconductivity can be attributed to these excitations while the exactly (pi,pi) transitions produce the narrow resonance excitation that appears below Tc.

cond-mat.supr-con↗

arXiv2009

Static and Dynamic Magnetism in Underdoped Superconductor BaFe$_{1.92}$Co$_{0.08}$As$_2$

We report neutron scattering measurements on single crystals of BaFe$_{1.92}$Co$_{0.08}$As$_2$. The magnetic Bragg peak intensity is reduced by 6 % upon cooling through T$_C$. The spin dynamics exhibit a gap of 8 meV with anisotropic three-dimensional (3d) interactions. Below T$_C$ additional intensity appears at an energy of $\sim$4.5(0.5) meV similar to previous observations of a spin resonance in other Fe-based superconductors. No further gapping of the spin excitations is observed below T$_C$ for energies down to 2 meV. These observations suggest the redistribution of spectral weight from the magnetic Bragg position to a spin resonance demonstrating the direct competition between static magnetic order and superconductivity.

cond-mat.supr-con↗

arXiv2009

Two-dimensional resonant magnetic excitation in BaFe1.84Co0.16As2

Inelastic neutron scattering measurements on single crystals of superconducting BaFe1.84Co0.16As2 reveal a magnetic excitation located at wavevectors (1/2 1/2 L) in tetragonal notation. On cooling below TC, a clear resonance peak is observed at this wavevector with an energy of 8.6(0.5) meV, corresponding to 4.5(0.3) kBTC. This is in good agreement with the canonical value of 5 kBTC observed in the cuprates. The spectrum shows strong dispersion in the tetragonal plane but very weak dispersion along the c-axis, indicating that the magnetic fluctuations are two-dimensional in nature. This is in sharp contrast to the anisotropic three dimensional spin excitations seen in the undoped parent compounds.

cond-mat.supr-con↗

arXiv2008

Charge order in LuFe2O4: antiferroelectric ground state and coupling to magnetism

X-ray scattering by multiferroic LuFe2O4 is reported. Below 320 K, superstructure reflections indicate an incommensurate charge order with propagation close to (1/3,1/3,3/2). The corresponding charge configuration, also found by electronic structure calculations as most stable, contains polar Fe/O double-layers with antiferroelectric stacking. Diffuse scattering at 360 K, with (1/3,1/3,0) propagation, indicates ferroelectric short-range correlations between neighboring double-layers. The temperature dependence of the incommensuration indicates that charge order and magnetism are coupled.

cond-mat.str-el↗

arXiv2008

Phonon softening and anomalous mode near the $x_{c}=0.5$ quantum critical point in Ca$_{2-x}$Sr$_{x}$RuO$_4$

Inelastic neutron scattering is used to measure the temperature dependent phonon dispersion in Ca$_{2-x}$Sr$_{x}$RuO$_{4}$ ($x=0.4$, 0.6). The in-plane $Σ_{4}$ octahedral tilt mode softens significantly at the zone boundary of the high temperature tetragonal (HTT) \textit{I4}$_{\mathit{1}}$\textit{/acd} structure as the temperature approaches the transition to a low temperature orthorhombic (LTO) \textit{Pbca} phase. This behavior is similar to that in La$_2$CuO$_4$, but a new inelastic feature that is not found in the cuprate is present. An anomalous phonon mode is observed at energy transfers greater than the $Σ_{4}$ albeit with similar dispersion. This anomalous phonon mode never softens below $\sim 5$ meV, even for temperatures below the HTT-LTO transition. This mode is attributed to the presence of intrinsic structural disorder within the \textit{I4}$_{\mathit{1}}$\textit{/acd} tetragonal structure of the doped ruthenate.

cond-mat.str-el↗

arXiv2008

Anisotropic three-dimensional magnetism in CaFe2As2

Inelastic neutron scattering measurements on the low energy spin waves in CaFe2As2 show that the magnetic exchange interactions in the Fe layers are exceptionally large and similar to the cuprates. However, the exchange between layers is ~10% of the coupling in the layers and the magnetism is more appropriately categorized as anisotropic three-dimensional, in contrast to the two-dimensional cuprates. Band structure calculations of the spin dynamics and magnetic exchange interactions are in good agreement with the experimental data.

cond-mat.supr-con↗

arXiv2008

Spin-lozenge thermodynamics and magnetic excitations in Na$_3$RuO$_4$

We report inelastic and elastic neutron scattering, magnetic susceptibility, and heat capacity measurements of polycrystalline sodium ruthenate (Na$_3$RuO$_4$). Previous work suggests this material consists of isolated tetramers of $S=3/2$ Ru$^{5+}$ ions in a so-called "lozenge" configuration. Using a Heisenberg antiferromagnet Hamiltonian, we analytically determine the energy eigenstates for general spin $S$. From this model, the neutron scattering cross-sections for excitations associated with spin-3/2 spin-tetramer configurations is determined. Comparison of magnetic susceptibility and inelastic neutron scattering results shows that the proposed "lozenge" model is not distinctly supported, but provides evidence that the system may be better described as a pair of non-interacting inequivalent dimers, \textit{i.e} double dimers. However, the existence of long-range magnetic order below $T_c \approx 28$ K immediately questions such a description. Although no evidence of the lozenge model is observed, future studies on single crystals may further clarify the appropriate magnetic Hamiltonian.

cond-mat.mtrl-sci↗

arXiv2008

Lattice and Magnetic structures of PrFeAsO, PrFeAsO0.85F0.15 and PrFeAsO0.85

We use powder neutron diffraction to study the spin and lattice structures of polycrystalline samples of nonsuperconducting PrFeAsO and superconducting PrFeAsO0.85F0.15 and PrFeAsO0.85. We find that PrFeAsO exhibits an abrupt structural phase transitions at 153 K, followed by static long range antiferromagnetic order at 127 K. Both the structural distortion and magnetic order are identical to other rare-earth oxypnictides. Electron-doping the system with either Fluorine or oxygen deficiency suppresses the structural distortion and static long range antiferromagnetic order, therefore placing these materials into the same class of FeAs-based superconductors.

cond-mat.supr-con↗

arXiv2008

Resonant Spin Excitation in the High Temperature Superconductor Ba0.6K0.4Fe2As2

The recent observations of superconductivity at temperatures up to 55K in compounds containing layers of iron arsenide have revealed a new class of high temperature superconductors that show striking similarities to the more familiar cuprates. In both series of compounds, the onset of superconductivity is associated with the suppression of magnetic order by doping holes and/or electrons into the band leading to theories in which magnetic fluctuations are either responsible for or strongly coupled to the superconducting order parameter. In the cuprates, theories of magnetic pairing have been invoked to explain the observation of a resonant magnetic excitation that scales in energy with the superconducting energy gap and is suppressed above the superconducting transition temperature, Tc. Such resonant excitations have been shown by inelastic neutron scattering to be a universal feature of the cuprate superconductors, and have even been observed in heavy fermion superconductors with much lower transition temperatures. In this paper, we show neutron scattering evidence of a resonant excitation in Ba0.6K0.4Fe2As2, which is a superconductor below 38K, at the momentum transfer associated with magnetic order in the undoped compound, BaFe2As2, and at an energy transfer that is consistent with scaling in other strongly correlated electron superconductors. As in the cuprates, the peak disappears at Tc providing the first experimental confirmation of a strong coupling of the magnetic fluctuation spectrum to the superconducting order parameter in the new iron arsenide superconductors.

cond-mat.supr-con↗

arXiv2008

Neutron diffraction in a model itinerant metal near a quantum critical point

Neutron diffraction measurements on single crystals of Cr1-xVx (x=0, 0.02, 0.037) show that the ordering moment and the Neel temperature are continuously suppressed as x approaches 0.037, a proposed Quantum Critical Point (QCP). The wave vector Q of the spin density wave (SDW) becomes more incommensurate as x increases in accordance with the two band model. At xc=0.037 we have found temperature dependent, resolution limited elastic scattering at 4 incommensurate wave vectors Q=(1+/-delta_1,2, 0, 0)*2pi/a, which correspond to 2 SDWs with Neel temperatures of 19 K and 300 K. Our neutron diffraction measurements indicate that the electronic structure of Cr is robust, and that tuning Cr to its QCP results not in the suppression of antiferromagnetism, but instead enables new spin ordering due to novel nesting of the Fermi surface of Cr.

cond-mat.str-el↗