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M. D. Shattuck

Publications and source records attributed to M. D. Shattuck.

At least 19 recordsLinked to original sources

Local and global measures of the shear moduli of jammed disk packings

Strain-controlled isotropic compression gives rise to jammed packings of repulsive, frictionless disks with either positive or negative global shear moduli. We carry out computational studies to understand the contributions of the negative shear moduli to the mechanical response of jammed disk packings. We first decompose the ensemble-averaged, global shear modulus as $\langle G\rangle = (1-{\cal F}_-) \langle G_+ \rangle + {\cal F}_- \langle G_-\rangle$, where ${\cal F}_-$ is the fraction of jammed packings with negative shear moduli and $\langle G_+\rangle$ and $\langle G_-\rangle$ are the average values from packings with positive and negative moduli, respectively. We show that $\langle G_+\rangle$ and $\langle|G_-|\rangle$ obey different power-law scaling relations above and below $pN^2 \sim 1$. We then calculate analytically that ${\cal P}(G)$ is a Gamma distribution in the $pN^2 \ll 1$ limit. As $pN^2$ increases, the skewness of ${\cal P}(G)$ decreases and ${\cal P}(G)$ becomes a skew-normal distribution with negative skewness in the $pN^2 \gg 1$ limit. We also partition jammed disk packings into subsystems using Delanunay triangulation of the disk centers to calculate local shear moduli. We show that the local shear moduli defined from groups of adjacent triangles can be negative even when $G > 0$. The spatial correlation function of local shear moduli $C({\vec r})$ displays weak correlations for $pn_{\rm sub}^2 < 10^{-2}$, where $n_{\rm sub}$ is the number of particles within each subsystem. However, $C({\vec r})$ begins to develop long-ranged spatial correlations with four-fold angular symmetry for $pn_{\rm sub}^2 \gtrsim 10^{-2}$.

cond-mat.soft

Hopper flows of deformable particles

Numerous experimental and computational studies show that continuous hopper flows of granular materials obey the Beverloo equation that relates the volume flow rate $Q$ and the orifice width $w$: $Q \sim (w/σ_{\rm avg}-k)^β$, where $σ_{\rm avg}$ is the average particle diameter, $kσ_{\rm avg}$ is an offset where $Q\sim 0$, the power-law scaling exponent $β=d-1/2$, and $d$ is the spatial dimension. Recent studies of hopper flows of deformable particles in different background fluids suggest that the particle stiffness and dissipation mechanism can also strongly affect the power-law scaling exponent $β$. We carry out computational studies of hopper flows of deformable particles with both kinetic friction and background fluid dissipation in two and three dimensions. We show that the exponent $β$ varies continuously with the ratio of the viscous drag to the kinetic friction coefficient, $λ=ζ/μ$. $β= d-1/2$ in the $λ\rightarrow 0$ limit and $d-3/2$ in the $λ\rightarrow \infty$ limit, with a midpoint $λ_c$ that depends on the hopper opening angle $θ_w$. We also characterize the spatial structure of the flows and associate changes in spatial structure of the hopper flows to changes in the exponent $β$. The offset $k$ increases with particle stiffness until $k \sim k_{\rm max}$ in the hard-particle limit, where $k_{\rm max} \sim 3.5$ is larger for $λ\rightarrow \infty$ compared to that for $λ\rightarrow 0$. Finally, we show that the simulations of hopper flows of deformable particles in the $λ\rightarrow \infty$ limit recapitulate the experimental results for quasi-2D hopper flows of oil droplets in water.

cond-mat.soft

Mechanical response of packings of non-spherical particles: A case study of 2D packings of circulo-lines

We investigate the mechanical response of jammed packings of circulo-lines, interacting via purely repulsive, linear spring forces, as a function of pressure $P$ during athermal, quasistatic isotropic compression. Prior work has shown that the ensemble-averaged shear modulus for jammed disk packings scales as a power-law, $\langle G(P) \rangle \sim P^β$, with $β\sim 0.5$, over a wide range of pressure. For packings of circulo-lines, we also find robust power-law scaling of $\langle G(P)\rangle$ over the same range of pressure for aspect ratios ${\cal R} \gtrsim 1.2$. However, the power-law scaling exponent $β\sim 0.8$-$0.9$ is much larger than that for jammed disk packings. To understand the origin of this behavior, we decompose $\langle G\rangle$ into separate contributions from geometrical families, $G_f$, and from changes in the interparticle contact network, $G_r$, such that $\langle G \rangle = \langle G_f\rangle + \langle G_r \rangle$. We show that the shear modulus for low-pressure geometrical families for jammed packings of circulo-lines can both increase {\it and} decrease with pressure, whereas the shear modulus for low-pressure geometrical families for jammed disk packings only decreases with pressure. For this reason, the geometrical family contribution $\langle G_f \rangle$ is much larger for jammed packings of circulo-lines than for jammed disk packings at finite pressure, causing the increase in the power-law scaling exponent.

cond-mat.soft

Contact network changes in ordered and disordered disk packings

We investigate the mechanical response of packings of purely repulsive, frictionless disks to quasistatic deformations. The deformations include simple shear strain at constant packing fraction and at constant pressure, "polydispersity" strain (in which we change the particle size distribution) at constant packing fraction and at constant pressure, and isotropic compression. For each deformation, we show that there are two classes of changes in the interparticle contact networks: jump changes and point changes. Jump changes occur when a contact network becomes mechanically unstable, particles "rearrange", and the potential energy (when the strain is applied at constant packing fraction) or enthalpy (when the strain is applied at constant pressure) and all derivatives are discontinuous. During point changes, a single contact is either added to or removed from the contact network. For repulsive linear spring interactions, second- and higher-order derivatives of the potential energy/enthalpy are discontinuous at a point change, while for Hertzian interactions, third- and higher-order derivatives of the potential energy/enthalpy are discontinuous. We illustrate the importance of point changes by studying the transition from a hexagonal crystal to a disordered crystal induced by applying polydispersity strain. During this transition, the system only undergoes point changes, with no jump changes. We emphasize that one must understand point changes, as well as jump changes, to predict the mechanical properties of jammed packings.

cond-mat.soft

Comparison of Shear and Compression Jammed Packings of Frictional Disks

We compare the structural and mechanical properties of mechanically stable (MS) packings of frictional disks in two spatial dimensions (2D) generated with isotropic compression and simple shear protocols from discrete element modeling (DEM) simulations. We find that the average contact number and packing fraction at jamming onset are similar (with relative deviations $< 0.5\%$) for MS packings generated via compression and shear. In contrast, the average stress anisotropy $\langle {\hat Σ}_{xy} \rangle = 0$ for MS packings generated via isotropic compression, whereas $\langle {\hat Σ}_{xy} \rangle >0$ for MS packings generated via simple shear. To investigate the difference in the stress state of MS packings, we develop packing-generation protocols to first unjam the MS packings, remove the frictional contacts, and then rejam them. Using these protocols, we are able to obtain rejammed packings with nearly identical particle positions and stress anisotropy distributions compared to the original jammed packings. However, we find that when we directly compare the original jammed packings and rejammed ones, there are finite stress anisotropy deviations $Δ{\hat Σ}_{xy}$. The deviations are smaller than the stress anisotropy fluctuations obtained by enumerating the force solutions within the null space of the contact networks generated via the DEM simulations. These results emphasize that even though the compression and shear jamming protocols generate packings with the same contact networks, there can be residual differences in the normal and tangential forces at each contact, and thus differences in the stress anisotropy.

cond-mat.soft

The response of jammed packings to thermal fluctuations

We focus on the response of mechanically stable (MS) packings of frictionless, bidisperse disks to thermal fluctuations, with the aim of quantifying how nonlinearities affect system properties at finite temperature. Packings of disks with purely repulsive contact interactions possess two main types of nonlinearities, one from the form of the interaction potential and one from the breaking (or forming) of interparticle contacts. To identify the temperature regime at which the contact-breaking nonlinearities begin to contribute, we first calculated the minimum temperatures $T_{cb}$ required to break a single contact in the MS packing for both single and multiple eigenmode perturbations of the $T=0$ MS packing. We then studied deviations in the constant volume specific heat $C_V$ and deviations of the average disk positions $Δr$ from their $T=0$ values in the temperature regime $T_{cb} < T < T_{r}$, where $T_r$ is the temperature beyond which the system samples the basin of a new MS packing. We find that the deviation in the specific heat per particle $Δ{\overline C}_V^0/{\overline C}_V^0$ relative to the zero temperature value ${\overline C}_V^0$ can grow rapidly above $T_{cb}$, however, the deviation $Δ{\overline C}_V^0/{\overline C}_V^0$ decreases as $N^{-1}$ with increasing system size. To characterize the relative strength of contact-breaking versus form nonlinearities, we measured the ratio of the average position deviations $Δr^{ss}/Δr^{ds}$ for single- and double-sided linear and nonlinear spring interactions. We find that $Δr^{ss}/Δr^{ds} > 100$ for linear spring interactions and is independent of system size.

cond-mat.soft

Protocol dependence of the jamming transition

We propose a theoretical framework for predicting the protocol dependence of the jamming transition for frictionless spherical particles that interact via purely repulsive contact forces. We study isostatic jammed disk packings obtained via two protocols: isotropic compression and simple shear. We show that for frictionless systems, all jammed packings can be obtained via either protocol. However, the probability to obtain a particular jammed packing depends on the packing-generation protocol. We predict the average shear strain required to induce jamming in initially unjammed packings from the measured probability to jam at packing fraction $ϕ$ from isotropic compression. We compare our predictions to results from numerical simulations of jamming and find quantitative agreement. We also show that the packing fraction range, over which strain-induced jamming occurs, tends to zero in the large system limit for frictionless packings with overdamped dynamics.

cond-mat.soft

Experiments demonstrate that the null space of the rigidity matrix determines grain motion during vibration-induced compaction

Using a previously developed experimental method to reduce friction in mechanically stable packings of disks, we find that frictional packings form tree-like structures of geometrical families that lie on reduced dimensional manifolds in configuration space. Each branch of the tree begins at a point in configuration space with an isostatic number of contacts and spreads out to sequentially higher dimensional manifolds as the number of contacts are reduced. We find that gravitational deposition of disks produces an initially under-coordinated packing stabilized by friction on a high-dimensional manifold. Using short vibration bursts to reduce friction, we compact the system through many stable configurations with increasing contact number and decreasing dimensionality until the system reaches an isostatic frictionless state. We find that this progression can be understood as the system moving through the null-space of the rigidity matrix defined by the interparticle contact network in the direction of the gravitational force. We suggest that this formalism can also be used to explain the evolution of frictional packings under other forcing conditions.

cond-mat.soft

On the origin of multi-component bulk metallic glasses: Atomic size mismatches and de-mixing

The critical cooling rate $\mathcal{R}_c$, below which liquids crystallize upon cooling, characterizes the glass-forming ability (GFA) of the system. While pure metals are typically poor glass formers with $\mathcal {R}_c>10^{12}\, {\rm K/s}$, specific multi-component alloys can form bulk metallic glasses (BMGs) even at cooling rates below $\mathcal {R}\sim 1\, {\rm K/s}$. Conventional wisdom asserts that metal alloys with three or more components are better glass formers (with smaller ${\cal R}_c$) than binary alloys. However, there is currently no theoretical framework that provides quantitative predictions for $\mathcal{R}_c$ for multi-component alloys. We perform simulations of ternary hard-sphere systems, which have been shown to be accurate models for the glass-forming ability of BMGs, to understand the roles of geometric frustration and demixing in determining $\mathcal {R}_c$. Specifically, we compress ternary hard sphere mixtures into jammed packings and measure the critical compression rate, below which the system crystallizes, as a function of the diameter ratios $σ_B/σ_A$ and $σ_C/σ_A$ and number fractions $x_A$, $x_B$, and $x_C$. We find two distinct regimes for the GFA in parameter space for ternary hard spheres. When the diameter ratios are close to $1$, such that the largest ($A$) and smallest ($C$) species are well-mixed, the GFA of ternary systems is no better than that of the optimal binary glass former. However, when $σ_C/σ_A \lesssim 0.8$ is below the demixing threshold for binary systems, adding a third component $B$ with $σ_C < σ_B < σ_A$ increases the GFA of the system by preventing demixing of $A$ and $C$. Analysis of the available data from experimental studies indicates that most ternary BMGs are below the binary demixing threshold with $σ_C/σ_A < 0.8$.

cond-mat.mtrl-sci

Calculations of the Structure of Basin Volumes for Mechanically Stable Packings

There are a finite number of distinct mechanically stable (MS) packings in model granular systems composed of frictionless spherical grains. For typical packing-generation protocols employed in experimental and numerical studies, the probabilities with which the MS packings occur are highly nonuniform and depend strongly on parameters in the protocol. Despite intense work, it is extremely difficult to predict {\it a priori} the MS packing probabilities, or even which MS packings will be the most versus the least probable. We describe a novel computational method for calculating the MS packing probabilities by directly measuring the volume of the MS packing `basin of attraction', which we define as the collection of initial points in configuration space at {\it zero packing fraction} that map to a given MS packing by following a particular dynamics in the density landscape. We show that there is a small core region with volume $V^c_n$ surrounding each MS packing $n$ in configuration space in which all initial conditions map to a given MS packing. However, we find that the MS packing probabilities are very weakly correlated with core volumes. Instead, MS packing probabilities obtained using initially dilute configurations are determined by complex geometric features of the basin of attraction that are distant from the MS packing.

cond-mat.soft

Jammed particulate systems are inherently nonharmonic

Jammed particulate systems, such as granular media, colloids, and foams, interact via one-sided forces that are nonzero only when particles overlap. We find that systems with one-sided repulsive interactions possess no linear response regime in the large system limit ($N\rightarrow \infty$) for all pressures $p$ (or compressions $Δϕ$), and for all $N$ near jamming onset $p\rightarrow 0$. We perform simulations on 2D frictionless bidisperse mechanically stable disk packings over a range of packing fractions $Δϕ= ϕ-ϕ_J$ above jamming onset $ϕ_J$. We apply perturbations with amplitude $δ$ to the packings along each eigen-direction from the dynamical matrix and determine whether the response of the system evolving at constant energy remains in the original eigenmode of the perturbation. For $δ> δ_c$, which we calculate analytically, a single contact breaks and fluctuations abruptly spread to all harmonic modes. As $δ$ increases further all discrete harmonic modes disappear into a continuous frequency band. We find that $<δ_c >\sim Δϕ/N^λ$, where $1 > λ> 0.5$, and thus jammed particulate systems are inherently nonharmonic with no linear vibrational response regime as $N\rightarrow \infty$ over the full range of $Δϕ$, and as $Δϕ\rightarrow 0$ at any $N$.

cond-mat.soft

First-order phase transition and the equation of state in a 2D granular fluid

We present experimental evidence for a first-order freezing/melting phase transition in a nonequilibrium system -- an oscillated two-dimensional isobaric granular fluid. The steady-state transition occurs between a gas and a crystal and is characterized by a discontinuous change in both density and temperature. It is suppressed if the number of particles is incommensurate with the cell size, shows rate-dependent hysteresis, and obeys the Lindemann criterion for melting. Further, the measured equation of state both above and below the phase transition compares well with theory.

cond-mat.soft

Lattice Dynamics and Melting of a Nonequilibrium Pattern

We present a new description of nonequilibrium square patterns as a harmonically coupled crystal lattice. In a vertically oscillating granular layer, different transverse normal modes of the granular square-lattice pattern are observed for different driving frequencies ($f_d$) and accelerations. The amplitude of a mode can be further excited by either frequency modulation of $f_d$ or reduction of friction between the grains and the plate. When the mode amplitude becomes large, the lattice melts (disorders), in accord with the Lindemann criterion for melting in two-dimensions.

nlin.PS

Phase Bubbles and Spatiotemporal Chaos in Granular Patterns

We use inelastic hard sphere molecular dynamics simulations and laboratory experiments to study patterns in vertically oscillated granular layers. The simulations and experiments reveal that {\em phase bubbles} spontaneously nucleate in the patterns when the container acceleration amplitude exceeds a critical value, about $7g$, where the pattern is approximately hexagonal, oscillating at one-fourth the driving frequency ($f/4$). A phase bubble is a localized region that oscillates with a phase opposite (differing by $π$) to that of the surrounding pattern; a localized phase shift is often called an ${\em arching}$ in studies of two-dimensional systems. The simulations show that the formation of phase bubbles is triggered by undulation at the bottom of the layer on a large length scale compared to the wavelength of the pattern. Once formed, a phase bubble shrinks as if it had a surface tension, and disappears in tens to hundreds of cycles. We find that there is an oscillatory momentum transfer across a kink, and this shrinking is caused by a net collisional momentum inward across the boundary enclosing the bubble. At increasing acceleration amplitudes, the patterns evolve into randomly moving labyrinthian kinks (spatiotemporal chaos). We observe in the simulations that $f/3$ and $f/6$ subharmonic patterns emerge as primary instabilities, but that they are unstable to the undulation of the layer. Our experiments confirm the existence of transient $f/3$ and $f/6$ patterns.

cond-mat.soft

Shocks in supersonic sand

We measure time-averaged velocity, density, and temperature fields for steady granular flow past a wedge and calculate a speed of granular pressure disturbances (sound speed) equal to 10% of the flow speed. The flow is supersonic, forming shocks nearly identical to those in a supersonic gas. Molecular dynamics simulations of Newton's laws and Monte Carlo simulations of the Boltzmann equation yield fields in quantitative agreement with experiment. A numerical solution of Navier-Stokes-like equations agrees with a molecular dynamics simulation for experimental conditions excluding wall friction.

cond-mat.soft

Velocity Distributions and Correlations in Homogeneously Heated Granular Media

We compare the steady state velocity distributions from our three-dimensional inelastic hard sphere molecular dynamics simulation for homogeneously heated granular media, with the predictions of a mean field-type Enskog-Boltzmann equation for inelastic hard spheres [van Noije & Ernst, Gran. Matt. {\bf 1}, 57 (1998)]. Although we find qualitative agreement for all values of density and inelasticity, the quantitative disagreement approaches $\sim 40%$ at high inelasticity or density. By contrast the predictions of the pseudo-Maxwell molecule model [Carrillo, Cercignani & Gamba, Phys. Rev. E, {\bf 62}, 7700 (2000)] are both qualitatively and quantitatively different from those of our simulation. We also measure short-range and long-range velocity correlations exhibiting non-zero correlations at contact before the collision, and being consistent with a slow algebraic decay over a decade in the unit of the diameter of the particle, proportional to $r^{-(1+α)}$, where $0.2 < α< 0.3$. The existence of these correlations imply the failure of the molecular chaos assumption and the mean field approximation, which is responsible for the quantitative disagreement of the inelastic hard sphere kinetic theory.

cond-mat.soft

Characterization of the Emergence of Order in an Oscillated Granular Layer

The formation of textured patterns has been predicted to occur in two stages. The first is an early time, domain-forming stage with dynamics characterized by a disorder function $\barδ(β) \sim t^{-σ_{E}}$, with $σ_{E} = {1/2}β$; this decay is universal. Coarsening of domains occurs in the second stage, in which $\barδ(β) \sim t^{-σ_{L}}$, where $σ_{L}$ is a nonlinear function of $β$ whose form is system and model dependent. Our experiments on a vertically oscillated granular layer are in accord with theory, yielding $σ_{E}\approx 0.5β$, and $σ_{L}$ a nonlinear function of $β$.

nlin.PS

Velocity Correlations in Driven Two-Dimensional Granular Media

Simulations of volumetrically forced granular media in two dimensions produce s tates with nearly homogeneous density. In these states, long-range velocity correlations with a characteristic vortex structure develop; given sufficient time, the correlations fill the entire simulated area. These velocity correlations reduce the rate and violence of collisions, so that pressure is smaller for driven inelastic particles than for undriven elastic particles in the same thermodynamic state. As the simulation box size increases, the effects of veloc ity correlations on the pressure are enhanced rather than reduced.

cond-mat.stat-mech