arXiv subjects

M. De Giorgi

Publications and source records attributed to M. De Giorgi.

16 recordsLinked to original sources

arXiv2022

Strongly enhanced light-matter coupling of a monolayer WS2 from a bound state in the continuum

Optical bound states in the continuum (BIC) allow to totally prevent a photonic mode from radiating into free space along a given spatial direction. Polariton excitations derived from the strong radiation-matter interaction of a BIC with an excitonic resonance inherit an ultralong radiative lifetime and significant nonlinearities due to their hybrid nature. However, maximizing the light-matter interaction in these structures remains challenging, especially with 2D semiconductors, thus preventing the observation of room temperature nonlinearities of BIC polaritons. Here we show a strong light-matter interaction enhancement at room temperature by coupling monolayer WS2 excitons to a BIC, while optimizing for the electric field strength at the monolayer position through Bloch surface wave confinement. By acting on the grating geometry, the coupling with the active material is maximized in an open and flexible architecture, allowing to achieve a 100 meV photonic bandgap with the BIC in a local energy minimum and a record 70 meV Rabi splitting. Our novel architecture provides large room temperature optical nonlinearities, thus paving the way to tunable BIC-based polariton devices with topologically-protected robustness to fabrication imperfections.

physics.optics↗

arXiv2022

Rydberg polaritons in ReS2 crystals

Rhenium disulfide (ReS2) belongs to group-VII transition metal dichalcogenide (TMDs) with attractive properties such as exceptionally high refractive index and significant oscillator strength, large in-plane birefringence, and good chemical stability. Unlike most other TMDs, the peculiar optical properties of ReS2 persist from bulk to the monolayer, making this material potentially suitable for applications in optical devices. In this work, we demonstrate with unprecedented clarity the strong coupling between cavity modes and excited states, which results in a strong polariton interaction, showing the interest of such materials as a solid-state counterpart of Rydberg atomic systems. Moreover, we definitively clarify the nature of important spectral features, shedding light on some controversial aspects or incomplete interpretations and demonstrating that their origin is due to the interesting combination of the very high refractive index and the large oscillator strength expressed by these TMDs.

physics.optics↗

arXiv2022

Onset of vortex clustering and inverse energy cascade in dissipative quantum fluids

Turbulent phenomena are among the most striking effects that both classical and quantum fluids can exhibit. While classical turbulence is ubiquitous in nature, the observation of quantum turbulence requires the precise manipulation of quantum fluids such as superfluid helium or atomic Bose-Einstein condensates. In this work we demonstrate the turbulent dynamics of a 2D quantum fluid of exciton-polaritons, hybrid light-matter quasiparticles, both by measuring the kinetic energy spectrum and showing the onset of vortex clustering. We demonstrate that the formation of clusters of quantum vortices is triggered by the increase of the incompressible kinetic energy per vortex, showing the tendency of the vortex-gas towards highly excited configurations despite the dissipative nature of our system. These results lay the basis for the investigations of quantum turbulence in two-dimensional fluids of light.

cond-mat.quant-gas↗

arXiv2022

Polariton Bose-Einstein condensate from a Bound State in the Continuum

Optical bound states in the continuum (BIC) are peculiar topological states that, when realized in a planar photonic crystal lattice, are symmetry-protected from radiating in the far field despite lying within the light cone, i.e., in the energy-momentum dispersion region for which radiation can propagate out of the lattice plane. These BICs possess an invariant topological charge given by the winding number of the polarization vectors, similarly to vortices in quantum fluids, such as superfluid helium and atomic Bose-Einstein condensates. In spite of several reports of optical BICs in patterned dielectric slabs with evidence of lasing, their potential as topologically protected states with theoretically infinite lifetime has not been fully exploited, yet. Here we show Bose-Einstein condensation of polaritons, hybrid light-matter excitations, occuring in a BIC thanks to its peculiar non-radiative nature. The combination of the ultra-long BIC lifetime and the tight confinement of the waveguide geometry allow to achieve an extremely low threshold density for condensation, which is not reached in the dispersion minimum but at a saddle point in reciprocal space. By bridging bosonic condensation and symmetry-protected radiation eigenmodes, we unveil new ways of imparting topological properties onto macroscopic quantum states with unexplored dispersion features. Such an observation may open a route towards energy-efficient polariton condensation in cost-effective integrated devices, ultimately suited for the development of hybrid light-matter optical circuits

physics.optics↗

arXiv2021

Ultrafast, low-energy, all-optical switch in polariton waveguides

The requirement for optical-electrical-optical conversion of signals in optical technologies is often one of the majors bottleneck in terms of speed and energy consumption. The use of dressed photons (also called polaritons), that allows for intrinsic sizable interactions, could significantly improve the performances of optical integrated elements such as switches or optical gates. In this work we demonstrate the ultrafast switch of a laser coupled into a polaritonic waveguide triggered by an optical pulse resonant with the same dispersion but at a lower energy. Our experiments show two effects capable to interrupt the transmission of the laser in two different time ranges: a sub-picosecond time range due to the optical Stark effect, and a picosecond range governed by the creation of a charge reservoir. In the latter regime we found that at certain power of excitation the activation of dark states allows for a long persistence of the switching much beyond the bright exciton lifetime.

physics.optics↗

arXiv2019

Chromodynamics of photons in an artificial non-Abelian magnetic Yang-Mills field

Artificial gauge fields, simulating real phenomenologies that unfold in a vast variety of systems, offer extraordinary possibilities to study extreme physical effects in many different environments, from high energy physics to quantum mechanics and cosmology. They are also at the heart of topological physics. Here, exploiting a strongly anisotropic material under strong coupling regime, we experimentally synthesize a Yang-Mills non-Abelian gauge field acting on an exciton-polariton quantum flow like a magnetic field. We observe experimentally the corresponding curved trajectories and spin precession. This motion follows chromodynamics equations which normally describe the quarks strong interactions and their color. Our work therefore opens exciting perspectives of simulating quark-gluon dynamics using highly flexible photonic simulators. It makes of sub-atomic physics a potential new playground to apply topological physics concepts.

cond-mat.mes-hall↗

arXiv2019

Polaritonic neuromorphic computing outperforms linear classifiers

Machine learning software applications are nowadays ubiquitous in many fields of science and society for their outstanding capability of solving computationally vast problems like the recognition of patterns and regularities in big datasets. One of the main goals of research is the realization of a physical neural network able to perform data processing in a much faster and energy-efficient way than the state-of-the-art technology. Here we show that lattices of exciton-polariton condensates accomplish neuromorphic computing using fast optical nonlinearities and with lower error rate than any previous hardware implementation. We demonstrate that our neural network significantly increases the recognition efficiency compared to the linear classification algorithms on one of the most widely used benchmarks, the MNIST problem, showing a concrete advantage from the integration of optical systems in reservoir computing architectures.

cs.ET↗

arXiv2019

Direct measurement of the quantum geometric tensor in a two-dimensional continuous medium

Topological Physics relies on the specific structure of the eigenstates of Hamiltonians. Their geometry is encoded in the quantum geometric tensor containing both the celebrated Berry curvature, crucial for topological matter, and the quantum metric. The latter is at the heart of a growing number of physical phenomena such as superfluidity in flat bands, orbital magnetic susceptibility, exciton Lamb shift, and non-adiabatic corrections to the anomalous Hall effect. Here, we report the first direct measurement of both Berry curvature and quantum metric in a two-dimensional continuous medium. The studied platform is a planar microcavity of extremely high finesse, in the strong coupling regime. It hosts mixed exciton-photon modes (exciton-polaritons) subject to photonic spin-orbit-coupling which makes emerge Dirac cones and exciton Zeeman splitting breaking time-reversal symmetry. The monopolar and half-skyrmion pseudospin textures are measured by polarisation-resolved photoluminescence. The associated quantum geometry of the bands is straightforwardly extracted from these measurements. Our results unveil the intrinsic chirality of photonic modes which is at the basis of topological photonics. This technique can be extended to measure Bloch band geometries in artificial lattices. The use of exciton-polaritons (interacting photons) opens wide perspectives for future studies of quantum fluid physics in topological systems.

cond-mat.mes-hall↗

arXiv2018

Two-Dimensional hybrid perovskites sustaining strong polariton interactions at room temperature

Polaritonic devices exploit the coherent coupling between excitonic and photonic degrees of freedom to perform highly nonlinear operations with low input powers. Most of the current results exploit excitons in epitaxially grown quantum wells and require low temperature operation, while viable alternatives have yet to be found at room temperature. Here we show that large single-crystal flakes of two-dimensional layered perovskite are able to sustain strong polariton nonlinearities at room temperature with no need to be embedded in an optical cavity. In particular, exciton-exciton interaction energies are measured to be remarkably similar to the ones known for inorganic quantum wells at cryogenic temperatures, and more than one order of magnitude larger than alternative room temperature polariton devices reported so far. Thanks to their easy fabrication, large dipolar oscillator strengths and strong nonlinearities, these materials hold great promises to realize actual polariton devices at room temperature.

physics.optics↗

arXiv2018

Tunable out-of-plane excitons in 2D single crystal perovskites

Hybrid organic-inorganic perovskites have emerged as very promising materials for photonic applications, thanks to the great synthetic versatility that allows to tune their optical properties. In the two-dimensional (2D) crystalline form, these materials behave as multiple quantum-well heterostructures with stable excitonic resonances up to room temperature. In this work strong light-matter coupling in 2D perovskite single-crystal flakes is observed, and the polarization-dependent exciton-polariton response is used to disclose new excitonic features. For the first time, an out-of-plane component of the excitons is observed, unexpected for such 2D systems and completely absent in other layered materials, such as transition-metal dichalcogenides. By comparing different hybrid perovskites with the same inorganic layer but different organic interlayers, it is shown how the nature of the organic ligands controllably affects the out-of-plane exciton-photon coupling. Such vertical dipole coupling is particularly sought in those systems, e.g. plasmonic nanocavities, in which the direction of the field is usually orthogonal to the material sheet. Organic interlayers are shown to affect also the strong birefringence associated to the layered structure, which is exploited in this work to completely rotate the linear polarization degree in only few microns of propagation, akin to what happens in metamaterials.

cond-mat.mes-hall↗

arXiv2018

Superluminal X-waves in a polariton quantum fluid

In this work we experimentally demonstrate for the first time spontaneous generation of two-dimensional exciton-polariton X-waves. X-waves belong to the family of localized packets, which are capable of sustaining their shape with no spreading even in the linear regime. This allows to keep the packet shape and size for very low densities and very long times compared, for instance, to soliton waves, which always necessitate a nonlinearity to compensate the diffusion. Here we exploit the polariton nonlinearity and unique structured dispersion, comprising both positive- and negative-mass curvatures, to trigger an asymmetric four wave mixing in the momentum space. This ultimately enables self-formation of a spatial X-wave front. By means of ultrafast imaging experiments we observe the early reshaping of the initial Gaussian packet into the X-pulse and its propagation even for vanishing small densities. This allows us to outline the crucial effects and parameters driving the phenomena and to tune the degree of peak superluminal propagation, which we found to be in a good agreement with numerical simulations.

cond-mat.other↗

arXiv2015

Vortex and half-vortex dynamics in a spinor quantum fluid of interacting polaritons

Spinorial or multi-component Bose-Einstein condensates may sustain fractional quanta of circulation, vorticant topological excitations with half integer windings of phase and polarization. Matter-light quantum fluids, such as microcavity polaritons, represent a unique test bed for realising strongly interacting and out-of-equilibrium condensates. The direct access to the phase of their wavefunction enables us to pursue the quest of whether half vortices ---rather than full integer vortices--- are the fundamental topological excitations of a spinor polariton fluid. Here, we are able to directly generate by resonant pulsed excitations, a polariton fluid carrying either the half or full vortex states as initial condition, and to follow their coherent evolution using ultrafast holography. Surprisingly we observe a rich phenomenology that shows a stable evolution of a phase singularity in a single component as well as in the full vortex state, spiraling, splitting and branching of the initial cores under different regimes and the proliferation of many vortex anti-vortex pairs in self generated circular ripples. This allows us to devise the interplay of nonlinearity and sample disorder in shaping the fluid and driving the phase singularities dynamics

cond-mat.quant-gas↗

arXiv2015

Real-space collapse of a polariton condensate

Polaritons in microcavities are versatile quasi-2D bosonic particles with a high degree of coherence and strong nonlinearities, thanks to their hybrid light-matter character. In their condensed form, they display striking quantum hydrodynamic features analogous to atomic Bose-Einstein condensates, such as long-range order coherence, superfluidity and quantized vorticity. Their variegated dispersive and dissipative properties, however, set significant differences from their atomic counterpart. In this work, we report the unique phenomenology that is observed when a pulse of light impacts the polariton vacuum: the condensate that is instantaneously formed does not splash in real space but instead coheres into an enigmatic structure, featuring concentric rings and, most notably, a sharp and bright peak at the center. Using a state-of-the-art ultrafast imaging with 50 fs time steps, we are able to track the dynamics of the polariton mean-field wavefunction in both real and reciprocal space. The observation of the real-space collapse of the condensate into an extremely localized---resolution limited---peak is at odd with the repulsive interactions of polaritons and their positive effective mass. An unconventional mechanism is therefore at play to account for our observations. Our modeling suggests that self-trapping due to a local heating of the crystal lattice---that can be described as a collective polaron formed by a polariton condensate---could be involved. These observations hint at the fascinating fluid dynamics of polaritons in conditions of extreme intensities and ultrafast times.

cond-mat.quant-gas↗

arXiv2014

Ultrafast control of Rabi oscillations in a polariton condensate

We report the experimental observation and control of space and time-resolved light-matter Rabi oscillations in a microcavity. Our setup precision and the system coherence are so high that coherent control can be implemented with amplification or switching off of the oscillations and even erasing of the polariton density by optical pulses. The data is reproduced by a fundamental quantum optical model with excellent accuracy, providing new insights on the key components that rule the polariton dynamics.

cond-mat.quant-gas↗

arXiv2013

Control and ultrafast dynamics of a two-fluid polariton switch

We investigate the cross-interactions in a two-component polariton quantum fluid coherently driven by two independent pumping lasers tuned at different energies and momenta. We show that both the hysteresis cycles and the ON/OFF threshold of one polariton signal can be entirely controlled by a second polariton fluid. Furthermore, we study the ultrafast switching dynamics of a driven polariton state, demonstrating the ability to control the polariton population with an external laser pulse, in less than a few picoseconds.

cond-mat.mes-hall↗

arXiv2011

All-optical control of the quantum flow of a polariton superfluid

While photons in vacuum are massless particles that do not interact with each other, significant photon-photon interactions appear in suitable nonlinear media, leading to novel hydrodynamic behaviors typical of quantum fluids. Here we show the formation of vortex-antivortex pairs in a Bose-Einstein condensate of exciton-polaritons -a coherent gas of strongly dressed photons- flowing at supersonic speed against an artificial potential barrier created and controlled by a light beam in a planar semiconductor microcavity. The observed hydrodynamical phenomenology is in agreement with original theoretical predictions based on the Gross-Pitaevskii equation, recently generalized to the polariton context. However, in contrast to this theoretical work, we show how the initial position and the subsequent trajectory of the vortices crucially depend on the strength and size of the artificial barrier. Additionally, we demonstrate how a suitably tailored optical beam can be used to permanently trap and store the vortices that are hydrodynamically created in the wake of a natural defect. These observations are borne out by time-dependent theoretical simulations.

cond-mat.mes-hall↗