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M. Ducloy

Publications and source records attributed to M. Ducloy.

10 recordsLinked to original sources

Selective reflection Casimir-Polder spectroscopy in vapor cells: the influence of the thermal velocity distribution

Selective reflection is a high-resolution spectroscopic method that allows the probing of atomic and molecular gases in the near field of dielectric cell windows. It is a sensitive technique for measuring interactions between excited atoms and surfaces, thus providing a unique tool to probe resonant effects in Casimir-Polder physics. The theoretical modelling of selective reflection spectra has thus far employed the infinite Doppler approximation which assumes that the Doppler shift dominates over the atom-surface interactions as well as the homogeneous transition linewidth. Here we extend the theoretical treatment of selective reflection spectra to include the effects of finite Doppler width. This allows us to analyse the regime of very large Casimir-Polder interactions, relevant for Rydberg atom spectroscopy, and revisit previous analyses of experiments with low-lying excited states. Further, this will aid in determining the signatures of quantum friction in vapor cell spectroscopy.

quant-ph

Casimir-Polder effect with thermally excited surfaces

We take a closer look at the fundamental Casimir-Polder interaction between quantum particles and dispersive dielectric surfaces with surface polariton or plasmon resonances. Linear response theory shows that in the near field, van der Waals, regime the free energy shift of a particle contains a thermal component that depends exclusively on the population/excitation of the evanescent surface polariton/plasmon modes. Our work makes evident the link between particle surface interaction and near field thermal emission and demonstrates how this can be used to engineer Casimir-Polder forces. We also examine how the exotic effects of surface waves are washed out as the distance from the surface increases. In the case of molecules or excited state atoms, far field approximations result in a classical dipole-dipole interaction which depends on the surface reflectivity and the mean number of photons at the frequency of the atomic/molecular transition. Finally we present numerical results for the CP interaction between Cs atoms and various dielectric surfaces with a single polariton resonance and discuss the implications of temperature and retardation effects for specific spectroscopic experiments.

physics.atom-ph

Anisotropic Atom-Surface Interactions in the Casimir-Polder Regime

The distance-dependence of the anisotropic atom-wall interaction is studied. The central result is the 1/z^6 quadrupolar anisotropy decay in the retarded Casimir-Polder regime. Analysis of the transition region between non-retarded van der Waals regime (in 1/z^3) and Casimir-Polder regime shows that the anisotropy cross-over occurs at very short distances from the surface, on the order of 0.03 Lambda, where Lambda is the atom characteristic wavelength. Possible experimental verifications of this distance dependence are discussed.

physics.atom-ph

Atom reflection echoes and surface matter waves in atom meta-optics

Evanescent matter-waves produced by an atom wave packet incident onto a repulsive barrier edge can be back-refracted and reconstructed by the application of negative-index "comoving" potential pulses. One shows that those collapses and revivals of evanescent matter waves give rise to surface matter waves and should be observable via atom reflection echoes issued from the barrier interface. This property, together with the property of inducing negative refraction, makes such potentials the matter-wave counterpart of negative-index materials in light optics.

quant-ph

Negative-index media for matter-wave optics

We consider the extension of optical meta-materials to matter waves. We show that the generic property of pulsed comoving magnetic fields allows us to fashion the wave-number dependence of the atomic phase shift. It can be used to produce a transient negative group velocity of an atomic wave packet, which results into a negative refraction of the matter wave. Application to slow metastable argon atoms Ar*(3P2) shows that the device is able to operate either as an efficient beam splitter or an atomic meta-lens. Implications of "meta-media" in atom optics are considered.

quant-ph

Detecting of photons in optical fields of complicated spatial structure

We show that a photon detector, sensitive to the gradients of electromagnetic fields, or to magnetic fields, should be a useful tool to characterize the quantum properties of spatially-dependent optical fields. We discuss the excitation of an atom on a magnetic dipole or electric quadrupole transitions with the spiral photons of a Laguerre-Gauss (LG) or Bessel beams. We show that these beams are not true hollow beams, due to the presence of magnetic fields and gradients of electric fields on beam axis. This approach paves the way to an analysis at the quantum level of the spatial structure and angular momentum properties of singular light beams.

quant-ph

Detection of Spiral photons in Quantum Optics

We show that a new type of photon detector, sensitive to the gradients of electromagnetic fields, should be a useful tool to characterize the quantum properties of spatially-dependent optical fields. As a simple detector of such a kind, we propose using magnetic dipole or electric quadrupole transitions in atoms or molecules and apply it to the detection of spiral photons in Laguerre-Gauss (LG) beams. We show that LG beams are not true hollow beams, due to the presence of magnetic fields and gradients of electric fields on beam axis. This approach paves the way to an analysis at the quantum level of the spatial structure and angular momentum properties of singular light beams.

quant-ph

Saturation effects in the sub-Doppler spectroscopy of Cesium vapor confined in an Extremely Thin Cell

Saturation effects affecting absorption and fluorescence spectra of an atomic vapor confined in an Extremely Thin Cell (cell thickness $L < 1 μm$) are investigated experimentally and theoretically. The study is performed on the $D_{2}$ line ($λ~= ~852 nm)$ of $Cs$ and concentrates on the two situations $L = λ/2$ and $L =λ$, the most contrasted ones with respect to the length dependence of the coherent Dicke narrowing. For $L = λ/2$, the Dicke-narrowed absorption profile simply broadens and saturates in amplitude when increasing the light intensity, while for $L =λ$, sub-Doppler dips of reduced absorption at line-center appear on the broad absorption profile. For a fluorescence detection at $L =λ$, saturation induces narrow dips, but only for hyperfine components undergoing a population loss through optical pumping. These experimental results are interpreted with the help of the various existing models, and are compared with numerical calculations based upon a two-level modelling that considers both a closed and an open system.

physics.class-ph

Quadrupole transitions near interface: general theory and application to atom inside a planar cavity

Quadrupole radiation of an atom in an arbitrary environment is investigated within classical as well as quantum electrodynamical approaches. Analytical expressions for decay rates are obtained in terms of Green function of Maxwell equations. The equivalence of both approaches is shown. General expressions are applied to analyze the quadrupole decay rate of an atom placed between two half spaces with arbitrary dielectric constant. It is shown that in the case when the atom is close to the surface, the total decay rate is inversely proportional to the fifth power of distance between an atom and a plane interface.

physics.optics

Spontaneous emission rate of an excited atom placed near a nanofiber

The spontaneous decay rates of an excited atom placed near a dielectric cylinder are investigated. A special attention is paid to the case when the cylinder radius is small in comparison with radiation wavelength (nanofiber or photonic wire). In this case, the analytical expressions of the transition rates for different orientations of dipole are derived. It is shown that the main contribution to decay rates is due to quasistatic interaction of atom dipole momentum with nanofiber and the contributions of guided modes are exponentially small. On the contrary, in the case when the radius of fiber is only slightly less than radiation wavelength, the influence of guided modes can be substantial. The results obtained are compared with the case of dielectric nanospheroid and ideally conducting wire.

physics.atom-ph