arXiv subjects

M. Eisterer

Publications and source records attributed to M. Eisterer.

At least 19 recordsLinked to original sources

arXiv2024

Universal degradation of high-temperature superconductors due to impurity scattering: predicting the performance loss in fusion magnets

Predicting the change of performance of superconductors under neutron radiation is indispensable for designing compact fusion devices. The favorable enhancement of the critical current caused by flux pinning is separated from the degrading effect of increased scattering of the charge carriers to derive a degradation function from the expected change of the superfluid density (reducing to Homes law in the dirty limit) and the observed increase in flux creep. The degradation turned out to be a universal function of disorder, not depending on the particular tape nor the particle radiation: thermal and/or fast neutrons, as well as 1.2 MeV protons. The universal behavior enables the analysis of changes in flux pinning corrected by the adverse enhancement of scattering. A more reliable prediction of the performance change of coated conductors in a fusion reactor based on proxies for neutrons is anticipated.

cond-mat.supr-con↗

arXiv2019

Coexisting spin resonance and long-range magnetic order of Eu in EuRbFe$_4$As$_4$

Magnetic excitations and magnetic structure of EuRbFe$_4$As$_4$ were investigated by inelastic neutron scattering (INS), neutron diffraction, and random phase approximation (RPA) calculations. Below the superconducting transition temperature $T_\text{c}=36.5$~K, the INS spectra exhibit the neutron spin resonances at $Q_\text{res}=1.27(2)$~$\textÅ^{-1}$ and $1.79(3)$~$\textÅ^{-1}$. They correspond to the $\mathbf{Q}=(0.5,0.5,1)$ and $(0.5,0.5,3)$ nesting wave vectors, showing three dimensional nature of the band structure. The characteristic energy of the neutron spin resonance is $E_\text{res}=17.7(3)$~meV corresponding to $5.7(1)k_\text{B}T_\text{c}$. Observation of the neutron spin resonance mode and our RPA calculations in conjunction with the recent optical conductivity measurements are indicative of the $s_\pm$ superconducting pairing symmetry in EuRbFe$_4$As$_4$. In addition to the neutron spin resonance mode, upon decreasing temperature below the magnetic transition temperature $T_\text{N}=15$~K, the spin wave excitation originating in the long-range magnetic order of the Eu sublattice was observed in the low-energy inelastic channel. Single-crystal neutron diffraction measurements demonstrate that the magnetic propagation vector of the Eu sublattice is $\mathbf{k}=(0, 0, 0.25)$, representing the three-dimensional antiferromagnetic order. Linear spin wave calculations assuming the obtained magnetic structure with the intra- and inter-plane nearest neighbor exchange couplings of $J_1/k_\text{B}=-1.31$~K and $J_c/k_\text{B}=0.08$~K can reproduce quantitatively the observed spin wave excitation. Our results show that superconductivity and long-range magnetic order of Eu coexist in EuRbFe$_4$As$_4$ whereas the coupling between them is rather weak.

cond-mat.supr-con↗

arXiv2017

Peculiarities of the electronic transport in half-metallic Co-based Heusler alloys

Electrical, magnetic and galvanomagnetic properties of half-metallic Heusler alloys of Co$_2$YZ (Y = Ti, V, Cr, Mn, Fe, Ni, and Z = Al, Si, Ga, Ge, In, Sn, Sb) were studied in the temperature range 4.2--900 K and in magnetic fields of up to 100 kOe. It was found that varying Y in affects strongly the electric resistivity and its temperature dependence $ρ(T)$, while this effect is not observed upon changing Z. When Y is varied, extrema (maximum or minimum) are observed in $ρ(T)$ near the Curie temperature $T_C$. At $T < T_C$, the $ρ(T)$ behavior can be ascribed to a change in electronic energy spectrum near the Fermi level. The coefficients of the normal and anomalous Hall effect were determined. It was shown that the latter coefficient, $R_S$, is related to the residual resistivity $ρ_0$ by a power law $R_S \sim ρ_0^k/M_S$ with $M_S$ the spontaneous magnetization. The exponent $k$ was found to be 1.8 for Co$_2$FeZ alloys, which is typical for asymmetric scattering mechanisms, and 2.9 for Co$_2$YAl alloys, which indicates an additional contribution to the anomalous Hall effect. The temperature dependence of resistivity at low temperatures is analyzed and discussed in the framework of the two-magnon scattering theory.

cond-mat.mtrl-sci↗

arXiv2016

Assessing composition gradients in multifilamentary superconductors by means of magnetometry methods

We present two magnetometry-based methods suitable for assessing gradients in the critical temperature and hence the composition of multifilamentary superconductors: AC magnetometry and Scanning Hall Probe Microscopy. The novelty of the former technique lies in the iterative evaluation procedure we developed, whereas the strength of the latter is the direct visualization of the temperature dependent penetration of a magnetic field into the superconductor. Using the example of a PIT Nb3Sn wire, we demonstrate the application of these techniques, and compare the respective results to each other and to EDX measurements of the Sn distribution within the sub-elements of the wire.

cond-mat.supr-con↗

arXiv2015

Performance Boost in Industrial Multifilamentary Nb3Sn Wires due to Radiation Induced Pinning Centers

We report non-Cu critical current densities of 4.09 * 10^9 A/m^2 at 12 T and 2.27 * 10^9 A/m^2 at 15 T obtained from transport measurements on a Ti-alloyed RRP Nb3Sn wire after irradiation to a fast neutron fluence of 8.9 * 10^21 m^-2. These values are to our knowledge unprecedented in multifilamentary Nb3Sn, and they correspond to a Jc enhancement of approximately 60% relative to the unirradiated state. Our magnetometry data obtained on short wire samples irradiated to fast neutron fluences of up to 2.5 * 10^22 m^-2 indicate the possibility of an even better performance, whereas earlier irradiation studies on bronze-processed Nb3Sn wires with a Sn content further from stoichiometry attested a decline of the critical current density at such high fluences. We show that radiation induced point-pinning centers rather than an increase of the upper critical field are responsible for this Jc enhancement, and argue that these results call for further research on pinning landscape engineering.

cond-mat.supr-con↗

arXiv2014

One-dimensional pinning behavior in Co-doped BaFe2As2 thin films

Angle-resolved transport measurements revealed that planar defects dominate flux pinning in the investigated Co-doped BaFe2As2 thin film. For any given field and temperature, the critical current depends only on the angle between the crystallographic c-axis and the applied magnetic field but not on the angle between the current and the field. The critical current is therefore limited only by the in-plane component of the Lorentz force but independent of the out-of-plane component, which is entirely balanced by the pinning force exerted by the planar defects. This one-dimensional pinning behavior shows similarities and differences to intrinsic pinning in layered superconductors.

cond-mat.supr-con↗

arXiv2013

Effects of Neutron Irradiation on Pinning Force Scaling in State-of-the-Art Nb3Sn Wires

We present an extensive irradiation study involving five state-of-the-art Nb3Sn wires which were subjected to sequential neutron irradiation up to a fast neutron fluence of 1.6 * 10^22 m^-2 (E > 0.1 MeV). The volume pinning force of short wire samples was assessed in the temperature range from 4.2 to 15 K in applied fields of up to 7 T by means of SQUID magnetometry in the unirradiated state and after each irradiation step. Pinning force scaling computations revealed that the exponents in the pinning force function differ significantly from those expected for pure grain boundary pinning, and that fast neutron irradiation causes a substantial change in the functional dependence of the volume pinning force. A model is presented, which describes the pinning force function of irradiated wires using a two-component ansatz involving a point-pinning contribution stemming from radiation induced pinning centers. The dependence of this point-pinning contribution on fast neutron fluence appears to be a universal function for all examined wire types.

cond-mat.supr-con↗

arXiv2013

Critical current anisotropy in Nd-1111 single crystals and the infuence of neutron irradiation

We report on angle-resolved magnetization measurements on NdFeAsO$_{0.65}$F$_{0.35}$ (Nd-1111) single crystals. The field dependence of the critical current density, $J_c$, is non-monotonous in these crystals at all orientations and temperatures due to the fishtail effect, which strongly influences the angular dependence of $J_c$. The currents decrease as the field is tilted from the crystallographic c-axis at low fields, but increase at high fields. A peak occurs in the angular dependence of $J_c$ at intermediate fields. The critical currents are significantly enhanced after irradiation with fast neutrons and the fishtail disappears. The different current anisotropies at low and high fields, however, persist. We discuss the data in the framework of the anisotropic scaling approach and propose a transition from dominant pinning by large defects of low density at low fields to pinning by small defects of high density at high fields in the pristine crystal. Strong pinning dominates at all fields after the irradiation, and the angular dependence of $J_c$ can be described by anisotropic scaling only after an appropriate extension to this pinning regime.

cond-mat.supr-con↗

arXiv2013

Stress dependence of the critical currents in neutron irradiated (RE)BCO coated conductors

The application of HTS coated conductors in future fusion or accelerator magnets is currently of increasing interest. High Lorentz forces and therefore high hoop stresses act on the conductors in large coils. The conductor is furthermore exposed to neutron radiation in fusion or accelerator magnets. The expected neutron fluence over the desired lifetime of such magnets can be simulated by irradiation experiments in a fission reactor. The coated conductors were characterized in the pristine state and after irradiation to the ITER design fluence. The sensitivity of the critical currents to applied stress was measured in liquid nitrogen. The cold part of the set-up was positioned between a rotatable split coil electro-magnet for assessing the Ic-anisotropy up to 1.4T under maximum Lorentz force configuration. The Ic-sensitivity to applied stress changed significantly in the GdBCO/IBADconductors after irradiation, whereas nearly no change was observed in the YBCO/RABiTS-conductor. Furthermore, Ic and Tc were strongly reduced in the GdBCO/IBAD-sample after irradiation. The angular dependence of Ic changed for both samples in different ways after the irradiation, but no change in the angular dependence was observed upon applying stress. The high neutron capture cross-section of Gd and the resulting strong reduction of Tc seem to be responsible for the different stress dependence of Ic in irradiated Gd-123 coated conductors.

cond-mat.supr-con↗

arXiv2011

Rotating sample magnetometer for cryogenic temperatures and high magnetic fields

We report on the design and implementation of a rotating sample magnetometer (RSM) operating in the variable temperature insert of a cryostat equipped with a high-field magnet. The limited space and the cryogenic temperatures impose the most critical design parameters: the small bore size of the magnet requires a very compact pick-up coil system and the low temperatures demand a very careful design of the bearings. Despite these difficulties the RSM achieves excellent resolution at high magnetic field sweep rates, exceeding that of a typical vibrating sample magnetometer by about a factor of ten. In addition the gas-flow cryostat and the high-field superconducting magnet provide a temperature and magnetic field range unprecedented for this type of magnetometer.

cond-mat.supr-con↗

arXiv2011

Anisotropic critical currents in FeSe0.5Te0.5 films and the influence of neutron irradiation

We report on measurements of the superconducting properties of FeSe05Te05 thin films grown on lanthanum aluminate. The films have high transition temperatures (above 19 K) and sharp resistive transitions in fields up to 15 T. The temperature dependence of the upper critical field and the irreversibility lines are steep and anisotropic, as recently reported for single crystals. The critical current densities, assessed by magnetization measurements in a vector VSM, were found to be well above 10^9 Am-2 at low temperatures. In all samples, the critical current as a function of field orientation has a maximum, when the field is oriented parallel to the film surface. The maximum indicates the presence of correlated pinning centers. A minimum occurs in three films, when the field is applied perpendicular to the film plane. In the forth film, instead, a local maximum caused by c-axis correlated pinning centers was found at this orientation. The irradiation of two films with fast neutrons did not change the properties drastically, where a maximum enhancement of the critical current by a factor of two was found.

cond-mat.supr-con↗

arXiv2011

Magnetic measurement of the critical current anisotropy in coated conductors

We determine the critical current anisotropy at maximum Lorentz force from hysteresis loops in a vibrating sample magnetometer. To eliminate the signal of spurious variable Lorentz force currents it is sufficient to cut the sample to a specific length, which is calculated from the position dependent sensitivity of the instrument. The procedure increases the resolution of the measurement and the results compare well to transport data on the same sample. As the electric field in magnetisation measurements is lower than in transport experiments the anisotropy at high currents (low temperatures and fields) can be measured without the need of making current contacts or any special sample preparation.

cond-mat.supr-con↗

arXiv2010

Effects of high pressure on the physical properties of MgB2

The synthesis of MgB2-based materials under high pressure gave the possibility to suppress the evaporation of magnesium and to obtain near theoretically dense nanograined structures with high superconducting, thermal conducting, and mechanical characteristics: critical current densities of 1.8-1.0 \cdot 106 A/cm2 in the self field and 103 A/cm2 in a magnetic field of 8 T at 20 K, 5-3 \cdot 105 A/cm2 in self field at 30 K, the corresponding critical fields being HC2 = 15 T at 22 K and irreversible fields Hirr =13 T at 20 K, and Hirr =3.5 T at 30 K, thermal conduction of 53+/-2 W/(m \cdot κ), the Vickers hardness Hv=10.12+/-0.2 GPa under a load of 148.8 N and the fracture toughness K1C = 7.6+/-2.0 MPa m0.5 under the same load, the Young modulus E=213 GPa. Estimation of quenching current and AC losses allowed the conclusion that highpressure-prepared materials are promising for application in transformer-type fault current limiters working at 20-30 K.

cond-mat.supr-con↗

arXiv2010

Disorder effects and current percolation in FeAs based superconductors

We report the influence of atomic disorder introduced by sequential neutron irradiation on the basic superconducting properties, flux pinning and grain connectivity. Two different polycrystalline Sm-1111 samples (SmFeAsO_{1-x}F_x) and two Ba-122 single crystals (BaFe_{1.8}Co_{0.2}As_2) were investigated. The monotonous decrease of the transition temperature with neutron fluence degrades the upper critical field, at least in the investigated temperature region. Pinning on the other hand is largely improved, with a different optimal defect concentration (fluence) in the two materials. The analysis of the current flow in the polycrystalline samples reveals weak link behaviour in the majority of grain connections and the existence of stronger grain connections. The density of the latter seems to be close to the percolation threshold (i.e. the minimum fraction for a continuous current path). Both types of connections are sensitive to disorder and degrade upon neutron irradiation.

cond-mat.supr-con↗

arXiv2010

The influence of weak texture on the critical currents in polycrystalline MgB$_2$

The current transport in polycrystalline MgB$_2$ is strongly influenced by the intrinsic anisotropy of this superconductor. Untextured bulks and wires are macroscopically isotropic, but the grains retain their anisotropic properties and the field dependence of the critical currents is much stronger than in isotropic superconductors. Weakly or partially textured tapes are macroscopically anisotropic, but the anisotropy of the zero resistivity (or irreversibility) field is smaller than the intrinsic upper critical field anisotropy, $γ$. The \Jc-anisotropy is field and temperature dependent and can be much larger than $γ$. The most suitable parameter for the quantification of the macroscopic anisotropy is, therefore, the anisotropy of the zero resistivity field. It is difficult to distinguish between a higher degree of texture at a lower intrinsic anisotropy and a weaker texture at higher anisotropy and hardly possible based on the field dependence of the critical current anisotropy alone. The knowledge of the upper critical field is crucial and angular resolved measurements of either the critical currents or, better, the resistive in-field transitions are favorable for this purpose.

cond-mat.supr-con↗

arXiv2010

Thickness dependence of the critical current density in superconducting films: a geometrical approach

We analyze the influence of the magnetic field generated by the supercurrents (self-field) on the current density distribution by numerical simulations. The thickness of the superconducting film determines the self-field and consequently the critical current density at zero applied field. We find an equation, which derives the thickness dependence of the critical current density from its dependence on the magnetic induction. Solutions of the equation reproduce numerical simulations to great accuracy, thus enabling a quantification of the dependence of the self-field critical current density with increasing film thickness. This result is technologically relevant for the development of coated conductors with thicker superconducting layers.

cond-mat.supr-con↗

arXiv2009

Nanostructural Superconducting Materials for Fault Current Limiters and Cryogenic Electrical Machines

Materials of the Y-Ba-Cu-O (melt-textured YBa2Cu3O7-d-based materials or MT-YBCO) and Mg-B-O (MgB2-based materials) systems with high superconducting performance, which can be attained due to the formation of regularly distributed nanostructural defects and inhomogenities in their structure can be effectively used in cryogenic technique, in particular in fault current limiters and electrical machines (electromotors, generators, pumps for liquid gases, etc.). The developed processes of high-temperature (900-800 oC) oxygenation under elevated pressure (16 MPa) of MT-YBCO and high-pressure (2 GPa) synthesis of MgB2-based materials allowed us to attain high SC (critical current densities, upper critical fields, fields of irreversibility, trapped magnetic fields) and mechanical (hardness, fracture toughness, Young modulus) characteristics. It has been shown that the effect of materials properties improvement in the case of MT-YBCO was attained due to the formation of high twin density (20-22 micron-1), prevention of macrockracking and reduction (by a factor of 4.5) of microcrack density, and in the case of MgB2-based materials due to the formation of oxygen-enriched as compared to the matrix phase fine-dispersed Mg-B-O inhomogenities as well as inclusions of higher borides with near-MgB12 stoichiometry in the Mg-B-O matrix (with 15-37 nm average grain sizes). The possibility is shown to obtain the rather high Tc (37 K) and critical current densities in materials with MgB12 matrix (with 95 percent of shielding fraction as calculated from the resistant curve).

cond-mat.supr-con↗

arXiv2009

Inhomogeneity of Magnesium Diboride Structure and its Effect on Critical Current Density

The influence of the oxygen segregation into Mg-B-O inclusions (which are oxygen enriched as compared to the matrix material) and the formation of boron enriched phases (with near MgB12 composition) in MgB2 structure on pinning in magnesium diboride and the effect of SiC and Ti alloying on the formation of structural inhomogenities in MgB2 are discussed. A nanostructural material of near theoretical density (2.7 g/cm3) based on MgB2-SiC (10 wt. percents of 200-800 nm SiC was added), which is characterized by high jc (1000000 A/cm2 in 1 T - 100000 A/cm2 in 3.5 T at 20 K and 100000 A/cm2 at 35 K) has been synthesized at 2 GPa.

cond-mat.supr-con↗