arXiv subjects

M. Esmann

Publications and source records attributed to M. Esmann.

14 recordsLinked to original sources

arXiv2024

Interference of ultrahigh frequency acoustic phonons from distant quasi-continuous sources

The generation of propagating acoustic waves is essential for telecommunication applications, quantum technologies, and sensing. Up to now, the electrical generation has been at the core of most implementations, but is technologically limited to a few gigahertz. Overcoming this frequency limit holds the prospect of faster modulators, quantum acoustics at higher working temperatures, nanoacoustic sensing from smaller volumes. Alternatively, the optical excitation of acoustic resonators has unlocked frequencies up to 1 THz, but in most cases, the acoustic energy cannot be efficiently extracted from the resonator into a propagating wave. Here, we demonstrate a quasi-continuous and coherent source of 20 GHz acoustic phonons, based on a ridge waveguide, structured in the vertical direction as a high-Q acousto-optic resonator. The high frequency phonons propagate up to 20 $\mu$m away from the source, with a decay rate of $\sim$1.14 dB/$\mu$m. We demonstrate the coherence between acoustic phonons generated from two distant sources through spatio-temporal interference. This concept could be scaled up to a larger number of sources, which enable a new generation of optically programmed, reconfigurable nanoacoustic devices and applications.

cond-mat.mes-hall↗

arXiv2022

Probing Gigahertz Coherent Acoustic Phonons in TiO$_{2}$ Mesoporous Thin Films

Ultrahigh-frequency acoustic-phonon resonators usually require atomically flat interfaces to avoid phonon scattering and dephasing, leading to expensive fabrication processes, such as molecular beam epitaxy. In contrast, mesoporous thin films are based on inexpensive wet chemical fabrication techniques. Here, we report mesoporous titanium dioxide-based acoustic resonators with resonances up to 90 GHz, and quality factors from 3 to 7. Numerical simulations show a good agreement with the picosecond ultrasonics experiments. We also numerically study the effect of changes in the speed of sound on the performance of the resonator. This change could be induced by liquid infiltration into the mesopores. Our findings constitute the first step towards the engineering of building blocks based on mesoporous thin films for reconfigurable optoacoustic sensors.

cond-mat.mes-hall↗

arXiv2021

Three-dimensional electrical control of the excitonic fine structure for a quantum dot in a cavity

The excitonic fine structure plays a key role for the quantum light generated by semiconductor quantum dots, both for entangled photon pairs and single photons. Controlling the excitonic fine structure has been demonstrated using electric, magnetic, or strain fields, but not for quantum dots in optical cavities, a key requirement to obtain high source efficiency and near-unity photon indistinguishability. Here, we demonstrate the control of the fine structure splitting for quantum dots embedded in micropillar cavities. We propose a scheme based on remote electrical contacts connected to the pillar cavity through narrow ridges. Numerical simulations show that such a geometry allows for a three-dimensional control of the electrical field. We experimentally demonstrate tuning and reproducible canceling of the fine structure, a crucial step for the reproducibility of quantum light source technology.

quant-ph↗

arXiv2020

Fiber-based angular filtering for high-resolution Brillouin spectroscopy in the 20-300 GHz frequency range

Brillouin spectroscopy emerges as a promising non-invasive tool for nanoscale imaging and sensing. One-dimensional semiconductor superlattice structures are eminently used for selectively enhancing the generation or detection of phonons at few GHz. While commercially available Brillouin spectrometers provide high-resolution spectra, they consist of complex experimental techniques and are not suitable for semiconductor cavities operating at a wide range of optical wavelengths. We develop a pragmatic experimental approach for conventional Brillouin spectroscopy integrating a widely tunable excitation-source. Our setup combines a fibered-based angular filtering and a spectral filtering based on a single etalon and a double grating spectrometer. This configuration allows probing confined acoustic phonon modes in the 20-300 GHz frequency range with excellent laser rejection and high spectral resolution. Remarkably, our scheme based on the excitation and collection of the enhanced Brillouin scattering signals through the optical cavity, allows for better angular filtering for low phonon frequency. It can be implemented for the study of cavity optomechanics and stimulated Brillouin scattering over broadband optical and acoustic frequency ranges.

physics.optics↗

arXiv2020

Fiber-integrated microcavities for efficient generation of coherent acoustic phonons

Coherent phonon generation by optical pump-probe experiments has enabled the study of acoustic properties at the nanoscale in planar heterostructures, plasmonic resonators, micropillars and nanowires. Focalizing both pump and probe on the same spot of the sample is a critical part of pump-probe experiments. This is particularly relevant in the case of small objects. The main practical challenges for the actual implementation of this technique are: stability of the spatio-temporal overlap, reproducibility of the focalization and optical mode matching conditions. In this work, we solve these three challenges for the case of planar and micropillar optophononic cavities. We integrate the studied samples to single mode fibers lifting the need for focusing optics to excite and detect coherent acoustic phonons. The resulting excellent reflectivity contrast of at least 66% achieved in our samples allows us to observe stable coherent phonon signals over at least a full day and signals at extremely low excitation powers of 1uW. The monolithic sample structure is transportable and could provide a means to perform reproducible plug-and-play experiments.

physics.optics↗

arXiv2020

Topological optical and phononic interface mode by simultaneous band inversion

Interface modes have been widely explored in the field of electronics, optics, acoustics and nanophononics. One strategy to generate them is band inversion in one-dimensional superlattices. Most realizations of this type of topological states have so far been explored for a single kind of excitation. Despite its potential in the manipulation and engineering of interactions, platforms for the simultaneous topological confinement of multiple excitations remain an open challenge. GaAs/AlAs heterostructures exhibit enhanced optomechanical interactions due to the intrinsic colocalization of light and sound. In this work, we designed, fabricated, and experimentally studied a multilayered structure based on GaAs/AlAs. Due to the simultaneously inverted band structures for light and phonons, colocalized interface modes for both 1.34 eV photons and 18 GHz phonons appear. We experimentally validated the concept by optical reflectivity and coherent phonon generation and detection. Furthermore, we theoretically analyzed the performance of different topological designs presenting colocalized states in time-domain Brillouin scattering and deduce engineering rules. Potential future applications include the engineering of robust optomechanical resonators, compatible with the incorporation of active media such as quantum wells and quantum dots.

cond-mat.mes-hall↗

arXiv2020

Mesoporous Thin-Films for Acoustic Devices in the Gigahertz Range

The coherent manipulation of acoustic waves on the nanoscale usually requires multilayers with thicknesses and interface roughness defined down to the atomic monolayer. This results in expensive devices with predetermined functionality. Nanoscale mesoporous materials present high surface-to-volume ratio and tailorable mesopores, which allow the incorporation of chemical functionalization to nanoacoustics. However, the presence of pores with sizes comparable to the acoustic wavelength is intuitively perceived as a major roadblock in nanoacoustics. Here we present multilayered nanoacoustic resonators based on mesoporous SiO$_2$ thin-films showing acoustic resonances in the 5-100 GHz range. We characterize the acoustic response of the system using coherent phonon generation experiments. Despite resonance wavelengths comparable to the pore size, we observe for the first time unexpectedly well-defined acoustic resonances with Q-factors around 10. Our results open the path to a promising platform for nanoacoustic sensing and reconfigurable acoustic nanodevices based on soft, inexpensive fabrication methods.

physics.app-ph↗

arXiv2019

Sequential generation of linear cluster states from a single photon emitter

Light states composed of multiple entangled photons - such as cluster states - are essential for developing and scaling-up quantum computing networks. Photonic cluster states with discrete variables can be obtained from single-photon sources and entangling gates, but so far this has only been done with probabilistic sources constrained to intrinsically-low efficiencies, and an increasing hardware overhead. Here, we report the resource-efficient generation of polarization-encoded, individually-addressable, photons in linear cluster states occupying a single spatial mode. We employ a single entangling-gate in a fiber loop configuration to sequentially entangle an ever-growing stream of photons originating from the currently most efficient single-photon source technology - a semiconductor quantum dot. With this apparatus, we demonstrate the generation of linear cluster states up to four photons in a single-mode fiber. The reported architecture can be programmed to generate linear-cluster states of any number of photons with record scaling ratios, potentially enabling practical implementation of photonic quantum computing schemes.

quant-ph↗

arXiv2019

Phonon engineering with superlattices: generalized nanomechanical potentials

Earlier implementations to simulate coherent wave propagation in one-dimensional potentials using acoustic phonons with gigahertz-terahertz frequencies were based on coupled nanoacoustic resonators. Here, we generalize the concept of adiabatic tuning of periodic superlattices for the implementation of effective one-dimensional potentials giving access to cases that cannot be realized by previously reported phonon engineering approaches, in particular the acoustic simulation of electrons and holes in a quantum well or a double well potential. In addition, the resulting structures are much more compact and hence experimentally feasible. We demonstrate that potential landscapes can be tailored with great versatility in these multilayered devices, apply this general method to the cases of parabolic, Morse and double-well potentials and study the resulting stationary phonon modes. The phonon cavities and potentials presented in this work could be probed by all-optical techniques like pump-probe coherent phonon generation and Brillouin scattering.

cond-mat.mes-hall↗

arXiv2018

Brillouin Scattering in Hybrid Optophononic Bragg Micropillar Resonators at 300 GHz

We introduce a monolithic Brillouin generator based on a semiconductor micropillar cavity embedding a high frequency nanoacoustic resonator operating in the hundreds of GHz range. The concept of two nested resonators allows an independent design of the ultrahigh frequency Brillouin spectrum and of the optical device. We develop an optical free-space technique to characterize spontaneous Brillouin scattering in this monolithic device and propose a measurement protocol that maximizes the Brillouin generation efficiency in the presence of optically induced thermal effects. The compact and versatile Brillouin generator studied here could be readily integrated into fibered and on-chip architectures.

physics.optics↗

arXiv2018

Coherent generation and detection of acoustic phonons in topological nanocavities

Inspired by concepts developed for fermionic systems in the framework of condensed matter physics, topology and topological states are recently being explored also in bosonic systems. The possibility of engineering systems with unidirectional wave propagation and protected against disorder is at the heart of this growing interest. Topogical acoustic effects have been observed in a variety of systems, most of them based on kHz-MHz sound waves, with typical wavelength of the order of the centimeter. Recently, some of these concepts have been successfully transferred to acoustic phonons in nanoscaled multilayered systems. The reported demonstration of confined topological phononic modes was based on Raman scattering spectroscopy, yet the resolution did not suffice to determine lifetimes and to identify other acoustic modes in the system. Here, we use time-resolved pump-probe measurements using an asynchronous optical sampling (ASOPS) technique to overcome these resolution limitations. By means of one-dimensional GaAs/AlAs distributed Bragg reflectors (DBRs) as building blocks, we engineer high frequency ($\sim$ 200 GHz) topological acoustic interface states. We are able to clearly distinguish confined topological states from stationary band edge modes. The detection scheme reflects the symmetry of the modes directly through the selection rules, evidencing the topological nature of the measured confined state. These experiments enable a new tool in the study of the more complex topology-driven phonon dynamics such as phonon nonlinearities and optomechanical systems with simultaneous confinement of light and sound.

cond-mat.mes-hall↗

arXiv2018

Topological acoustics in coupled nanocavity arrays

The Su-Schrieffer-Heeger (SSH) model is likely the simplest one-dimensional concept to study non-trivial topological phases and topological excitations. Originally developed to explain the electric conductivity of polyacetylene, it has become a platform for the study of topological effects in electronics, photonics and ultra-cold atomic systems. Here, we propose an experimentally feasible implementation of the SSH model based on coupled one-dimensional acoustic nanoresonators working in the GHz-THz range. In this simulator it is possible to implement different signs in the nearest neighbor interaction terms, showing full tunability of all parameters in the SSH model. Based on this concept we construct topological transition points generating nanophononic edge and interface states and propose an easy scheme to experimentally probe their spatial complex amplitude distribution directly by well-established optical pump-probe techniques.

cond-mat.mes-hall↗

arXiv2017

Nanomechanical resonators based on adiabatic periodicity-breaking in a superlattice

We propose a novel acoustic cavity design where we confine a mechanical mode by adiabatically changing the acoustic properties of a GaAs/AlAs superlattice. By means of high resolution Raman scattering measurements, we experimentally demonstrate the presence of a confined acoustic mode at a resonance frequency around 350 GHz. We observe an excellent agreement between the experimental data and numerical simulations based on a photoelastic model. We demonstrate that the spatial profile of the confined mode can be tuned by changing the magnitude of the adiabatic deformation, leading to strong variations of its mechanical quality factor and Raman scattering cross section. The reported alternative confinement method could lead to the development of a novel generation of nanophononic and optomechanical systems.

cond-mat.mes-hall↗

arXiv2017

Optomechanical properties of GaAs/AlAs micropillar resonators operating in the 18 GHz range

Recent experiments demonstrated that GaAs-AlAs based micropillar cavities are promising systems for quantum optomechanics, allowing the simultaneous three-dimensional confinement of near-infrared photons and acoustic phonons in the 18-100 GHz range. Here, we investigate through numerical simulations the optomechanical properties of this new platform. We evidence how the Poisson's ratio and semiconductor-vacuum boundary conditions lead to very distinct features in the mechanical and optical three dimensional confinement. We find a strong dependence of the mechanical quality factor and strain distribution on the micropillar radius, in great contrast to what is predicted and observed in the optical domain. The derived optomechanical coupling constants g_0 reach ultra-large values in the 10^6 rad/s range.

cond-mat.mes-hall↗