arXiv subjects

M. F. Doty

Publications and source records attributed to M. F. Doty.

16 recordsLinked to original sources

arXiv2026

Dynamical decoupling of a quantum dot spin in a micropillar cavity for spin-multiphoton entanglement

Graph states of mutually entangled photons are key resources for quantum computation and communication and can be generated by leveraging the entanglement between a single resident spin and emitted photons from a charged semiconductor quantum dot (QD). This approach is intrinsically limited by the decoherence of the spin. We study how to mitigate this decoherence with dynamical decoupling of an electron spin in the weak transverse magnetic field regime using spin echo and Carr-Purcell-Meiboom-Gill (CPMG) techniques. Application of these techniques allows us to extend the coherence time of a spin by more than two orders of magnitude, extracting a $T_2^{CPMG}$ of $298\pm53$ ns. We further demonstrate that this technique is compatible with the generation of a spin-photon-photon entangled state at a high rate enabled by a micropillar cavity, with a 20% improvement in simulated state fidelity when using dynamical decoupling. These results pave the way for generating larger and more complex entangled states with QDs.

quant-ph↗

arXiv2025

The impact of hole $g$-factor anisotropy on spin-photon entanglement generation with InGaAs quantum dots

Self-assembled InGaAs/GaAs quantum dots (QDs) are of particular importance for the deterministic generation of spin-photon entanglement. One promising scheme relies on the Larmor precession of a spin in a transverse magnetic field, which is governed by the in-plane $g$-factors of the electron and valence band heavy-hole. We probe the origin of heavy-hole $g$-factor anisotropy with respect to the in-plane magnetic field direction and uncover how it impacts the entanglement generated between the spin and the photon polarization. First, using polarization-resolved photoluminescence measurements on a single QD, we determine that the impact of valence-band mixing dominates over effects due to a confinement-renormalized cubic Luttinger $q$ parameter. From this, we construct a comprehensive hole $g$-tensor model. We then use this model to simulate the concurrence and fidelity of spin-photon entanglement generation with anisotropic hole $g$-factors, which can be tuned via magnetic field angle and excitation polarization. The results demonstrate that post-growth control of the hole $g$-factor can be used to improve spin-photon cluster state generation.

cond-mat.mes-hall↗

arXiv2025

Deterministic and reconfigurable graph state generation with a single solid-state quantum emitter

Measurement-based quantum computing offers a promising route towards scalable, universal photonic quantum computation. This approach relies on the deterministic and efficient generation of photonic graph states in which many photons are mutually entangled with various topologies. Recently, deterministic sources of graph states have been demonstrated with quantum emitters in both the optical and microwave domains. In this work, we demonstrate deterministic and reconfigurable graph state generation with optical solid-state integrated quantum emitters. Specifically, we use a single semiconductor quantum dot in a cavity to generate caterpillar graph states, the most general type of graph state that can be produced with a single emitter. By using fast detuned optical pulses, we achieve full control over the spin state, enabling us to vary the entanglement topology at will. We perform quantum state tomography of two successive photons, measuring Bell state fidelities up to 0.80$\pm$0.04 and concurrences up to 0.69$\pm$0.09, while maintaining high photon indistinguishability. This simple optical scheme, compatible with commercially available quantum dot-based single photon sources, brings us a step closer to fault-tolerant quantum computing with spins and photons.

quant-ph↗

arXiv2024

Hybridized magnonic materials for THz frequency applications

The capability of magnons to hybridize and strongly couple with diverse excitations offers a promising avenue for realizing and controlling emergent properties that hold significant potential for applications in devices, circuits, and information processing. In this letter, we present recent theoretical and experimental developments in magnon-based hybrid systems, focusing on the combination of magnon excitation in an antiferromagnet with other excitations, namely plasmons in a topological insulator, phonons in a 2D AFM, and photons. The existence of THz frequency magnons, plasmons, and phonons makes magnon-based hybrid systems particularly appealing for high-operating-speed devices. In this context, we explore several directions to advance magnon hybrid systems, including strong coupling between a surface plasmon and magnon polariton in a TI/AFM bilayer, a giant spin Nernst effect induced by magnon phonon coupling in 2D AFMs, and control of magnon-photon coupling using spin torque.

cond-mat.mtrl-sci↗

arXiv2023

Giant spin Nernst effect in a two-dimensional antiferromagnet due to magnetoelastic coupling-induced gaps and interband transitions between magnon-like bands

We analyze theoretically the origin of the spin Nernst and thermal Hall effects in FePS3 as a realization of two-dimensional antiferromagnet (2D AFM). We find that a strong magnetoelastic coupling, hybridizing magnetic excitation (magnon) and elastic excitation (phonon), combined with time-reversal-symmetry-breaking, results in a Berry curvature hotspots in the region of anticrossing between the two distinct hybridized bands. Furthermore, large spin Berry curvature emerges due to interband transitions between two magnon-like bands, where a small energy gap is induced by magnetoelastic coupling between such bands that are energetically distant from anticrossing of hybridized bands. These nonzero Berry curvatures generate topological transverse transport (i.e., the thermal Hall effect) of hybrid excitations, dubbed magnon-polaron, as well as of spin (i.e., the spin Nernst effect) carried by them, in response to applied longitudinal temperature gradient. We investigate the dependence of the spin Nernst and thermal Hall conductivities on the applied magnetic field and temperature, unveiling very large spin Nernst conductivity even at zero magnetic field. Our results suggest FePS3 AFM, which is already available in 2D form experimentally, as a promising platform to explore the topological transport of the magnon-polaron quasiparticles at THz frequencies.

cond-mat.mes-hall↗

arXiv2023

A Brillouin light scattering study of the spin-wave magnetic field dependence in a magnetic hybrid system made of an artificial spin-ice structure and a film underlayer

We present a combined Brillouin light scattering and micromagnetic simulation investigation of the magnetic-field dependent spin-wave spectra in a hybrid structure made of permalloy (NiFe) artificial spin-ice (ASI) systems, composed of stadium-shaped nanoislands, deposited on the top of an unpatterned permalloy film with a nonmagnetic spacer layer. The thermal spin-wave spectra were recorded by Brillouin light scattering (BLS) as a function of the magnetic field applied along the symmetry direction of the ASI sample. Magneto-optic Kerr effect magnetometry was used to measure the hysteresis loops in the same orientation as the BLS measurements. The frequency and intensity of several spin-wave modes detected by BLS were measured as a function of the applied magnetic field. Micromagnetic simulations enabled us to identify the modes in terms of their frequency and spatial symmetry and to extract information about the existence and strength of the dynamic coupling, relevant only to a few modes of a given hybrid system. Using this approach, we suggest a way to understand if dynamic coupling between ASI and film modes is present or not, with interesting implications for the development of future three-dimensional magnonic applications and devices.

cond-mat.mtrl-sci↗

arXiv2014

Ultrafast voltage-tunable detectors for Terahertz radiation operating above 100K

Collective vibrations of proteins, rotations of small molecules, excitations of high-temperature superconductors, and electronic transitions in semiconductor nanostructures occur with characteristic frequencies between 1 and 10 THz. Applications to medicine, communications, security and other fields are emerging. However, mapping the coldest parts of the universe has been the largest driver for developing THz detectors. The result is a family of exquisitely-sensitive detectors requiring sub-4K temperatures. For earthbound THz science and technology, sensitivity remains important but many applications require high speed and operating temperatures. Room-temperature Schottky diodes enable some of these applications. Here we demonstrate a new type of detector in which THz radiation excites a collective oscillation of ~25,000 electrons between two gates in a microscopic four terminal transistor. The energy dissipates into other modes of the electron gas, warming it and changing the source-drain resistance. The detector shows amplifier-limited rise times near 1 ns and has detected THz laser radiation at temperatures up to 120K. The frequency of the collective oscillation tunes with small gate voltages. The first-generation tunable antenna-coupled intersubband Terahertz (TACIT) detectors tune between 1.5 and 2 THz with voltages <2V.

cond-mat.mes-hall↗

arXiv2011

Spectroscopic signatures of many-body interactions and delocalized states in self-assembled lateral quantum dot molecules

Lateral quantum dot molecules consist of at least two closely-spaced InGaAs quantum dots arranged such that the axis connecting the quantum dots is perpendicular to the growth direction. These quantum dot complexes are called molecules because the small spacing between the quantum dots is expected to lead to the formation of molecular-like delocalized states. We present optical spectroscopy of ensembles and individual lateral quantum dot molecules as a function of electric fields applied along the growth direction. The results allow us to characterize the energy level structure of lateral quantum dot molecules and the spectral signatures of both charging and many-body interactions. We present experimental evidence for the existence of molecular-like delocalized states for electrons in the first excited energy shell.

cond-mat.mes-hall↗

arXiv2009

Hole Spin Mixing in InAs Quantum Dot Molecules

Holes confined in single InAs quantum dots have recently emerged as a promising system for the storage or manipulation of quantum information. These holes are often assumed to have only heavy-hole character and further assumed to have no mixing between orthogonal heavy hole spin projections (in the absence of a transverse magnetic field). The same assumption has been applied to InAs quantum dot molecules formed by two stacked InAs quantum dots that are coupled by coherent tunneling of the hole between the two dots. We present experimental evidence of the existence of a hole spin mixing term obtained with magneto-photoluminescence spectroscopy on such InAs quantum dot molecules. We use a Luttinger spinor model to explain the physical origin of this hole spin mixing term: misalignment of the dots along the stacking direction breaks the angular symmetry and allows mixing through the light-hole component of the spinor. We discuss how this novel spin mixing mechanism may offer new spin manipulation opportunities that are unique to holes.

cond-mat.mtrl-sci↗

arXiv2008

Antibonding ground states in semiconductor artificial molecules

The spin-orbit interaction is a crucial element of many semiconductor spintronic technologies. Here we report the first experimental observation, by magneto-optical spectroscopy, of a remarkable consequence of the spin-orbit interaction for holes confined in the molecular states of coupled quantum dots. As the thickness of the barrier separating two coupled quantum dots is increased, the molecular ground state changes character from a bonding orbital to an antibonding orbital. This result is counterintuitive, and antibonding molecular ground states are never observed in natural diatomic molecules. We explain the origin of the reversal using a four band k.p model that has been validated by numerical calculations that account for strain. The discovery of antibonding molecular ground states provides new opportunities for the design of artificially structured materials with complex molecular properties that cannot be achieved in natural systems.

cond-mat.mtrl-sci↗

arXiv2007

Photoluminescence Spectroscopy of the Molecular Biexciton in Vertically Stacked Quantum Dot Pairs

We present photoluminescence studies of the molecular neutral biexciton-exciton spectra of individual vertically stacked InAs/GaAs quantum dot pairs. We tune either the hole or the electron levels of the two dots into tunneling resonances. The spectra are described well within a few-level, few-particle molecular model. Their properties can be modified broadly by an electric field and by structural design, which makes them highly attractive for controlling nonlinear optical properties.

cond-mat.other↗

arXiv2007

Spin Fine Structure in Optically Excited Quantum Dot Molecules

The interaction between spins in coupled quantum dots is revealed in distinct fine structure patterns in the measured optical spectra of InAs/GaAs double quantum dot molecules containing zero, one, or two excess holes. The fine structure is explained well in terms of a uniquely molecular interplay of spin exchange interactions, Pauli exclusion and orbital tunneling. This knowledge is critical for converting quantum dot molecule tunneling into a means of optically coupling not just orbitals, but spins.

cond-mat.other↗

arXiv2006

Engineering electron and hole tunneling with asymmetric InAs quantum dot molecules

Most self-assembled quantum dot molecules are intrinsically asymmetric with inequivalent dots resulting from imperfect control of crystal growth. We have grown vertically-aligned pairs of InAs/GaAs quantum dots by molecular beam epitaxy, introducing intentional asymmetry that limits the influence of intrinsic growth fluctuations and allows selective tunneling of electrons or holes. We present a systemic investigation of tunneling energies over a wide range of interdot barrier thickness. The concepts discussed here provide an important tool for the systematic design and characterization of more complicated quantum dot nanostructures.

cond-mat.mtrl-sci↗

arXiv2006

Electrically tunable g-factors in quantum dot molecular spin states

We present a magneto-photoluminescence study of individual vertically stacked InAs/GaAs quantum dot pairs separated by thin tunnel barriers. As an applied electric field tunes the relative energies of the two dots, we observe a strong resonant increase or decrease in the g-factors of different spin states that have molecular wavefunctions distributed over both quantum dots. We propose a phenomenological model for the change in g-factor based on resonant changes in the amplitude of the wavefunction in the barrier due to the formation of bonding and antibonding orbitals.

cond-mat.mtrl-sci↗

arXiv2005

Polarized fine structure in the excitation spectrum of a negatively charged quantum dot

We report polarized photoluminescence excitation spectroscopy of the negative trion in single charge tunable InAs/GaAs quantum dots. The spectrum exhibits a p-shell resonance with polarized fine structure arising from the direct excitation of the electron spin triplet states. The energy splitting arises from the axially symmetric electron-hole exchange interaction. The magnitude and sign of the polarization are understood from the spin character of the triplet states and a small amount of quantum dot asymmetry, which mixes the wavefunctions through asymmetric e-e and e-h exchange interactions.

cond-mat.other↗

arXiv2005

Verification of polarization selection rules and implementation of selective coherent manipulations of hydrogenic transitions in n-GaAs

Electrons bound to shallow donors in GaAs have orbital energy levels analogous to those of the hydrogen atom. The polarization selection rules for optical transitions between the states analogous to the 1s and 2p states of hydrogen in a magnetic field are verified using Terahertz (THz) radiation from the UCSB Free Electron Laser. A polarization-selective coherent manipulation of the quantum states is demonstrated and the relevance to quantum information processing schemes is discussed.

quant-ph↗