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M. G. Cabezas

Publications and source records attributed to M. G. Cabezas.

8 recordsLinked to original sources

Bubble bursting in a sessile droplet

We analyzed experimentally and numerically the bursting of a bubble within a sessile droplet. Our experiments show that both sessile droplet curvature and confinement enhance the energy focusing. In the low-viscosity regime, this effect results in thinner, faster Worthington jets. In the high-viscosity regime, droplets are ejected for values of the Laplace number (the Reynolds number based on the visco-capillary velocity) smaller than the threshold for a bubble in an infinite liquid bath. This is probably the major result of the present work. Numerical simulations show the critical role of the additional pressure gradient arising from the curvature of the sessile droplet interface. The resulting force drives the liquid towards the bottom of the cavity, compressing it and accelerating jet formation. In the low-viscosity limit, the bottom of the cavity becomes smoother before jet ejection. This effect resembles the energy-focusing enhancement that occurs in an infinite liquid bath at the critical Laplace number, where short-wavelength waves are damped by viscosity.

physics.flu-dyn↗

Effect of surfactant kinetics on the wetting following the drop impact onto rough surfaces

We experimentally analyze the effect of a surfactant on wetting following drop impact on rough surfaces, paying special attention to the role of dynamic surface tension. To this end, we compare the results obtained with Triton X-100, SDS, and Surfynol 465. For concentrations below the critical micelle concentration $c_{\textin{cmc}}$, the evolution of the coverage area is nearly identical for all three surfactants, suggesting that the surfactant concentration is too low to significantly influence droplet spreading. In contrast, pronounced differences emerge due to the distinct dynamic surface tensions of the surfactants at $c/c_{\textin{cmc}}=2$. The evolution of the coverage area during spreading is nearly the same for pure water droplets and those containing Surfynol 465, indicating that surfactant depletion is negligible during the rapid spreading stage. As the Weber number increases, droplet spreading becomes progressively less sensitive to surface tension, thereby reducing the influence of surfactant adsorption kinetics. Nevertheless, Surfynol 465 produces larger coverage areas than Triton X-100 and SDS. The final coverage area is governed by the quasi-static recession of the triple contact line, which is controlled by the receding contact angle. Surfynol 465 consistently yields substantially larger final coverage areas across the range of surface roughness considered in this study.

physics.flu-dyn↗

Critical bubble bursting in real water. Effect of surface-active contaminants

We study the bursting of a bubble on a liquid free surface under critical conditions, i.e., those leading to the minimum (maximum) size (velocity) of the first-emitted jet droplet. Our experiments show that a tiny amount of surfactant considerably increases (decreases) the droplet radius (velocity). The volume of the first-emitted droplet increases by a factor of 20 for a concentration that produces an insignificant reduction in the bubble surface tension. The total liquid volume ejected by the bubble increases with the surfactant concentration. Surfactant accumulates at the bubble base due to cavity bottom shrinkage and surfactant convection. The resulting reduction in surface tension narrows the region of free surface reversal. Despite this effect, the size of the emitted droplet increases due to the Marangoni stress acting on the jet surface. Marangoni stress slows down the interface of the liquid jet, delaying the detachment of the droplet. More liquid flows into the droplet, increasing the mass and energy transfer to the resulting spray. A significant increase in the droplet size is also observed with a weak surfactant. This indicates that natural water contamination can substantially alter the bursting of bubbles under critical conditions. Our results may explain the size of the particles emitted by bubble bursting in seawater.

physics.flu-dyn↗

Global linear stability of the bubble rising in the presence of a soluble surfactant

We study the stability of the bubble rising in the presence of a soluble surfactant numerically and experimentally. For the surfactant concentration considered, the Marangoni stress almost immobilizes the interface. However, the non-zero surface velocity is crucial to understanding the surfactant behavior. The global linear stability analysis predicts the transition to an oblique path above the threshold of the Galilei number (the bubble radius). This transition is followed by the coexistence of stationary and oscillatory instabilities as the Galieli number increases. These predictions agree with the experimental observations without any fitting parameters. The bubble deformation, hydrostatic pressure variation, and perturbed viscous stress are evaluated. The velocity field perturbation causes a destabilizing vortex in the rear of the bubble. The perturbed viscous stress produces a torque opposing this vortex. The torque significantly decreases above the critical Galilei number, which may constitute the origin of instability. The linear stability analysis and the experiments were conducted for Surfynol, which can be regarded as a fast surfactant. Our experiments show the considerable differences between the rising of bubbles in the presence of this surfactant and a regular one.

physics.flu-dyn↗

Stability analysis of the flow in a coflowing device

We analyze the stability of the coflow configuration. The experiments and the global stability analysis show that the emitted jet always destabilizes before the tapering conical meniscus. This implies that the parameter conditions at which polydisperse dripping arises cannot be determined from the linear stability analysis of the steady jetting mode. Transient simulations show that the linear superposition of decaying eigenmodes triggered by an initial perturbation can lead to the jet breakup. The breakup process significantly depends on the initial perturbation. These results question the validity of the linear stability analysis as applied to the coflowing and other similar configurations.

physics.flu-dyn↗

A novel microfluidic method to produce monodisperse micrometer bubbles

We present a novel microfluidic method to produce quasi-monodisperse bubbles with diameters from tens to very few microns. A gaseous rivulet flows over the shallow groove printed on a T-junction exit channel. The triple contact line delimiting the rivulet is pinned to the groove edges. The rivulet breaks up into bubbles much smaller than the exit channel. When operating under adequate conditions, the flow transitions toward a singular mode where the rivulet remains quasi-static and emits bubbles smaller than the groove width. This allows the production of bubbles with diameters in the 3-5 $μ$m range, which is preferable for relevant therapeutical applications.

physics.flu-dyn↗

Transient bubble rising in the presence of a surfactant at very low concentrations

We study the formation of the dynamic adsorption layer when a bubble is released in a tank containing water with a tiny amount of surfactant. The influence of the sorption kinetic constants is examined by comparing the experiments with Sodium Dodecyl Sulfate (SDS) and Triton X-100. The experiments allowed us to determine the parameter conditions that lead to a stable bubble rising and to validate the simulation. A simple scaling analysis and the simulation show that the formation of the dynamic adsorption layer can be split into three phases characterized by disparate time scales. The mechanisms controlling those phases are surfactant convection, adsorption-desorption, and diffusion. The amount of surfactant adsorbed onto the interface increases monotonously throughout the three phases. The experiments and the simulation show that the rising velocity reaches a maximum at times of the order of $k_d^{-1}$ ($k_d$ is the desorption constant) when the dynamic adsorption layer is practically formed. This occurs even when only traces of surfactant are present in the liquid. The non-monotonous behavior of the maximum surfactant surface concentration is explained in terms of the reverse flow in the rear of the bubble right after the bubble release. This work contributes to the understanding of the complex interplay between hydrodynamics and surfactant transport and kinetics over bubble rising.

physics.flu-dyn↗

Global stability analysis of axisymmetric liquid-liquid flow focusing

We analyze both numerically and experimentally the stability of the steady jetting tip streaming produced by focusing a liquid stream with another liquid current when they coflow through the orifice of an axisymmetric nozzle. We calculate the global eigenmodes characterizing the response of this configuration to small-amplitude perturbations. In this way, the critical conditions leading to the instability of the steady jetting tip streaming are determined. The unstable perturbations are classified according to their oscillatory character and to the region where they are originated (convective and absolute instability). We derive and explain in terms of the velocity field a simple scaling law to predict the diameter of the emitted jet. The numerical stability limits are compared with experimental results finding reasonable agreement. The experiments confirm the existence of the two instability mechanisms predicted by the global stability analysis.

physics.flu-dyn↗