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M. Herzog

Publications and source records attributed to M. Herzog.

15 recordsLinked to original sources
arXiv2026

Ultrafast Dissipative Localization of Electronic Energy in AuPt Superlattices

Controlling the spatial distribution of absorbed optical energy is central to nanoscale photothermal chemistry, plasmonics, and ultrafast materials control. Here, we show that a metallic AuPt superlattice concentrates electronic energy in Pt within a few hundred femtoseconds, regardless of the initial energy distribution between the two constituents. Ultrafast X-ray diffraction follows this energy redistribution through the amplitude of a coherent 570 GHz superlattice phonon driven by the stress imbalance at the AuPt interfaces. Despite the nearly homogeneous absorption at 400 nm, the observed lattice motion is identical to that produced by 800 nm excitation, which is absorbed predominantly in Pt. This dissipation driven localization of energy arises from the large electronic heat capacity of Pt and rapid electronic transport through the superlattice, providing a route to femtosecond control of nanoscale energy distributions.

cond-mat.mtrl-sci↗
arXiv2024

Transport of Intensity Phase Retrieval in the Presence of Intensity Variations and Unknown Boundary Conditions

The so-called Transport of Intensity Equation (TIE) phase retrieval technique is widely applied in light, x-ray and electron optics to reconstruct, e.g., refractive indices, electric and magnetic fields in solids. Here, we present a largely improved TIE reconstruction algorithm, which properly considers intensity variations as well as unknown boundary conditions in a finite difference implementation of the Transport of Intensity partial differential equation. That largely removes reconstruction artifacts encountered in state-of-the-art Poisson solvers of the TIE, and hence significantly increases the applicability of the technique.

cond-mat.mtrl-sci↗
arXiv2022

Phonon-dominated energy transport in purely metallic heterostructures

We use ultrafast x-ray diffraction to quantify the transport of energy in laser-excited nanoscale Au/Ni bilayers. Electron transport and efficient electron-phonon coupling in Ni convert the laser-deposited energy in the conduction electrons within a few picoseconds into a strong non-equilibrium between hot Ni and cold Au phonons at the bilayer interface. Modeling of the subsequent equilibration dynamics within various two-temperature models confirms that for ultrathin Au films the thermal transport is dominated by phonons instead of conduction electrons because of the weak electron-phonon coupling in Au.

cond-mat.mes-hall↗
arXiv2021

Another criterion for solvability of finite groups

Let G be a finite group. Denote by ψ(G) the sum ψ(G)=\sum_{x\in G}|x| where |x| denotes the order of the element x, and by o(G) the quotient o(G)=\frac{ψ(G)}{|G|}. Confirming a conjecture posed by E.I. Khukhro, A. Moreto and M. Zarrin, we prove that if o(G)< o(A_5), then G is solvable.

math.GR↗
arXiv2020

Mapping the unoccupied state dispersions in Ta$_2$NiSe$_5$ with resonant inelastic x-ray scattering

The transition metal chalcogenide Ta$_2$NiSe$_5$ undergoes a second-order phase transition at $T_c=328$ K involving a small lattice distortion. Below $T_c$, a band gap at the center of its Brillouin zone increases up to about 0.35 eV. In this work, we study the electronic structure of Ta$_2$NiSe$_5$ in its low-temperature semiconducting phase, using resonant inelastic x-ray scattering (RIXS) at the Ni $L_3$-edge. In addition to a weak fluorescence response, we observe a collection of intense Raman-like peaks that we attribute to electron-hole excitations. Using density functional theory calculations of its electronic band structure, we identify the main Raman-like peaks as interband transitions between valence and conduction bands. By performing angle-dependent RIXS measurements, we uncover the dispersion of these electron-hole excitations that allows us to extract the low-energy boundary of the electron-hole continuum. From the dispersion of the valence band measured by angle-resolved photoemission spectroscopy, we derive the effective mass of the lowest unoccupied conduction band.

cond-mat.str-el↗
arXiv2019

Full spatiotemporal control of laser-excited periodic surface deformations

We demonstrate full control of acoustic and thermal periodic deformations at solid surfaces down to sub-nanosecond time scales and few-micrometer length scales via independent variation of the temporal and spatial phase of two optical transient grating (TG) excitations. For this purpose, we introduce an experimental setup that exerts control of the spatial phase of subsequent time-delayed TG excitations depending on their polarization state. Specific exemplary coherent control cases are discussed theoretically and corresponding experimental data are presented in which time-resolved x-ray reflectivity measures the spatiotemporal surface distortion of nanolayered heterostructures. Finally, we discuss examples where the application of our method may enable the control of functional material properties via tailored spatiotemporal strain fields.

physics.app-ph↗
arXiv2018

Tracking picosecond strain pulses in heterostructures that exhibit giant magnetostriction

We combine ultrafast X-ray diffraction (UXRD) and time-resolved Magneto-Optical Kerr Effect (MOKE) measurements to monitor the strain pulses in laser-excited TbFe2/Nb heterostructures. Spatial separation of the Nb detection layer from the laser excitation region allows for a background free characterization of the laser-generated strain pulses. We clearly observe symmetric bipolar strain pulses when the excited TbFe2 surface terminates the sample and a decomposition of the strain wavepacket into an asymmetric bipolar and a unipolar pulse, when a SiO2 glass capping layer covers the excited TbFe2 layer. The inverse magnetostriction of the temporally separated unipolar strain pulses in this sample leads to a MOKE signal that linearly depends on the strain pulse amplitude measured through UXRD. Linear chain model simulations accurately predict the timing and shape of UXRD and MOKE signals that are caused by the strain reflections from multiple interfaces in the heterostructure.

physics.app-ph↗
arXiv2018

Ultrafast negative thermal expansion driven by spin-disorder

We measure the transient strain profile in a nanoscale multilayer system composed of Yttrium, Holmium and Niobium after laser excitation using ultrafast X-ray diffraction. The strain propagation through each layer is determined by transient changes of the material-specific Bragg angles. We experimentally derive the exponentially decreasing stress profile driving the strain wave and show that it closely matches the optical penetration depth. Below the Neel temperature of Ho, the optical excitation triggers negative thermal expansion, which is induced by a quasi-instantaneous contractive stress, and a second contractive stress contribution rising on a 12 ps timescale. These two timescales have recently been measured for the spin-disordering in Ho [Rettig et al, PRL 116, 257202 (2016)]. As a consequence we observe an unconventional bipolar strain pulse with an inverted sign travelling through the heterostructure.

cond-mat.mtrl-sci↗
arXiv2018

Layer specific observation of slow thermal equilibration in ultrathin metallic nanostructures by femtosecond x-ray diffraction

Ultrafast heat transport in nanoscale metal multilayers is of great interest in the context of optically-induced demagnetization, remagnetization and switching. We investigate the structural response and the energy flow in the ultrathin double-layer system Gold (Au) on ferromagnetic Nickel (Ni) by ultrafast x-ray diffraction (UXRD). The penetration depth of light exceeds the bilayer thickness, preventing unambiguous layer-specific information from optical probes. Even though the excitation pulse is incident from the Au side, we observe a very rapid heating of the Ni lattice, whereas the Au lattice initially remains cold; the subsequent heat transfer from Ni to the Au lattice is found to be two orders of magnitude slower than predicted by the conventional heat equation and much slower than electron-phonon coupling times in Au. Both observations are independent of the excitation wavelength, although for the same fluence 400nm light excites electrons in Au ten times more than 800nm light. Simple model calculations show that the different specific heat of electrons in Ni and Au as well as the different electron-phonon coupling rapidly force the majority of thermal energy into the Ni lattice. Our results show that femtosecond UXRD provides an experimental account of heat transport over single digit nanometer distances as the thermal framework for ultrafast spin dynamics.

cond-mat.mes-hall↗
arXiv2013

Localized excited charge carriers generate ultrafast inhomogeneous strain in the multiferroic BiFeO$_3$

We apply ultrafast X-ray diffraction with femtosecond temporal resolution to monitor the lattice dynamics in a thin film of multiferroic BiFeO$_3$ after above-bandgap photoexcitation. The sound-velocity limited evolution of the observed lattice strains indicates a quasi-instantaneous photoinduced stress which decays on a nanosecond time scale. This stress exhibits an inhomogeneous spatial profile evidenced by the broadening of the Bragg peak. These new data require substantial modification of existing models of photogenerated stresses in BiFeO$_3$: the relevant excited charge carriers must remain localized to be consistent with the data.

cond-mat.mtrl-sci↗
arXiv2013

Combustion of a neutron star into a strange quark star: The neutrino signal

There are strong indications that the process of conversion of a neutron star into a strange quark star proceeds as a strong deflagration implying that in a few milliseconds almost the whole star is converted. Starting from the three-dimensional hydrodynamic simulations of the combustion process which provide the temperature profiles inside the newly born strange star, we calculate for the first time the neutrino signal that is to be expected if such a conversion process takes place. The neutrino emission is characterized by a luminosity and a duration that is typical for the signal expected from protoneutron stars and represents therefore a powerful source of neutrinos which could be possibly directly detected in case of events occurring close to our Galaxy. We discuss moreover possible connections between the birth of strange stars and explosive phenomena such as supernovae and gamma-ray-bursts.

astro-ph.HE↗
arXiv2013

Inverse problems in Additive Number Theory and in Non-Abelian Group Theory

The aim of this paper is threefold: a) Finding new direct and inverse results in the additive number theory concerning Minkowski sums of dilates. b) Finding a connection between the above results and some direct and inverse problems in the theory of Baumslag-Solitar (non-abelian) groups. c) Solving certain inverse problems in Baumslag-Solitar groups or monoids, assuming appropriate small doubling properties.

math.NT↗
arXiv2013

Following Strain-Induced Mosaicity Changes of Ferroelectric Thin Films by Ultrafast Reciprocal Space Mapping

We investigate coherent phonon propagation in a thin film of ferroelectric PbZr0.2Ti0.8O3 (PZT) by ultrafast x-ray diffraction (UXRD) experiments, which are analyzed as time-resolved reciprocal space mapping (RSM) in order to observe the in- and out-of-plane structural dynamics simultaneously. The mosaic structure of the PZT leads to a coupling of the excited out-of-plane expansion to in-plane lattice dynamics on a picosecond timescale, which is not observed for out-of-plane compression.

cond-mat.mtrl-sci↗
arXiv2012

On the brightness distribution of Type Ia supernovae from violent white dwarf mergers

We investigate the brightness distribution expected for thermonuclear explosions that might result from the ignition of a detonation during the violent merger of white dwarf (WD) binaries. Determining their brightness distribution is critical for evaluating whether such an explosion model could be responsible for a significant fraction of the observed population of SNe Ia. We argue that the brightness of an explosion realized via the violent merger model is determined by the mass of nickel 56 produced in the detonation of the primary WD. We use a set of sub-Chandrasekhar mass WD detonation models to derive a relationship between primary WD mass and expected peak bolometric brightness. We use this relationship to convert the masses of merging primary WDs from binary population models to a predicted distribution of explosion brightness. We find a striking similarity between the shape of our theoretical peak-magnitude distribution and that observed for SNe Ia: our model produces a brightness distribution that roughly covers the range and matches the shape of the one observed for SNe Ia. However, this agreement hinges on a particular phase of mass accretion during binary evolution: the primary WD gains ~0.15-0.35 Msun from a slightly-evolved helium star companion. We also find that with high probability, violent WD mergers involving the most massive primaries (which should produce bright SNe) have delay times <500 Myr (Abridged).

astro-ph.SR↗