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M. Horio

Publications and source records attributed to M. Horio.

46 records · Page 3Linked to original sources

Magnetic anisotropy of $L1_0$-ordered FePt thin films studied by Fe and Pt $L_{2,3}$-edges x-ray magnetic circular dichroism

The strong perpendicular magnetic anisotropy of $L{\rm1_0}$-ordered FePt has been the subject of extensive studies for a long time. However, it is not known which element, Fe or Pt, mainly contributes to the magnetic anisotropy energy (MAE). We have investigated the anisotropy of the orbital magnetic moments of Fe 3$d$ and Pt 5$d$ electrons in $L{\rm1_0}$-ordered FePt thin films by Fe and Pt $L_{2,3}$-edge x-ray magnetic circular dichroism (XMCD) measurements for samples with various degrees of long-range chemical order $S$. Fe $L_{2,3}$-edge XMCD showed that the orbital magnetic moment was larger when the magnetic field was applied perpendicular to the film than parallel to it, and that the anisotropy of the orbital magnetic moment increased with $S$. Pt $L_{2,3}$-edge XMCD also showed that the orbital magnetic moment was smaller when the magnetic field was applied perpendicular to the film than parallel to it, opposite to the Fe $L_{2,3}$-edge XMCD results although the anisotropy of the orbital magnetic moment increases with $S$ like the Fe edge. These results are qualitatively consistent with the first-principles calculation by Solovyev ${\it et\ al.}$ [Phys. Rev. B $\bf{52}$, 13419 (1995).], which also predicts the dominant contributions of Pt 5$d$ to the magnetic anisotropy energy rather than Fe 3$d$ due to the strong spin-orbit coupling and the small spin splitting of the Pt 5$d$ bands in $L{\rm1_0}$-ordered FePt.

cond-mat.mtrl-sci↗

Unusual nodal behaviors of the superconducting gap in the iron-based superconductor Ba(Fe$_{0.65}$Ru$_{0.35}$)$_2$As$_2$: Effects of spin-orbit coupling

We have investigated the superconducting gap of optimally doped Ba(Fe$_{0.65}$Ru$_{0.35}$)$_2$As$_2$ by angle-resolved photoemission spectroscopy (APRES) using bulk-sensitive 7 eV laser and synchrotron radiation. It was found that the gap is isotropic in the $k_x$-$k_y$ plane both on the electron and hole Fermi surfaces (FSs). The gap magnitudes of two resolved hole FSs show similar $k_z$ dependences and decrease as $k_z$ approaches $\sim$ 2$π$/$c$ (i.e., around the Z point) unlike the other Fe-based superconductors reported so far, where the superconducting gap of only one hole FS shows a strong $k_z$ dependence. This unique gap structure can be understood in the scenario that the $d_{z^2}$ orbital character is mixed into both hole FSs due to the finite spin-orbit coupling between almost degenerate FSs and is reproduced by calculations within the random phase approximation including the spin-orbit coupling.

cond-mat.supr-con↗

Fermi Surfaces and $p$-$d$ Hybridization in the Diluted Magnetic Semiconductor Ba$_{1-x}$K$_{x}$(Zn$_{1-y}$Mn$_{y}$)$_{2}$As$_{2}$ Studied by Soft X-ray Angle Resolved Photoemission Spectroscopy

The electronic structure of the new diluted magnetic semiconductor Ba$_{1-x}$K$_{x}$(Zn$_{1-y}$Mn$_{y}$)$_{2}$As$_{2}$ ($x=0.30$, $y=0.15$) in single crystal form has been investigated by angle-resolved photoemission spectroscopy (ARPES). %High density of states of nondispersive bands composed of the Zn $3d$ orbitals are observed with ultraviolet incident light. Measurements with soft x-rays clarify the host valence-band electronic structure primarily composed of the As $4p$ states. Two hole pockets around the $Γ$ point, a hole corrugated cylinder surrounding the $Γ$ and Z points, and an electron pocket around the Z point are observed, and explain the metallic transport of Ba$_{1-x}$K$_{x}$(Zn$_{1-y}$Mn$_{y}$)$_{2}$As$_{2}$. This is contrasted with Ga$_{1-x}$Mn$_{x}$As (GaMnAs), where it is located above the As $4p$ valence-band maximum (VBM) and no Fermi surfaces have been clearly identified. Resonance soft x-ray ARPES measurements reveal a nondispersive (Kondo resonance-like) Mn $3d$ impurity band near the Fermi level, as in the case of GaMnAs. However, the impurity band is located well below the VBM, unlike the impurity band in GaMnAs, which is located around and above the VBM. We conclude that, while the strong hybridization between the Mn $3d$ and the As $4p$ orbitals plays an important role in creating the impurity band and inducing high temperature ferromagnetism in both systems, the metallic transport may predominantly occur in the host valence band in Ba$_{1-x}$K$_{x}$(Zn$_{1-y}$Mn$_{y}$)$_{2}$As$_{2}$ and in the impurity band in GaMnAs.

cond-mat.mtrl-sci↗

Se content $x$ dependence of electron correlation strength in Fe$_{1+y}$Te$_{1-x}$Se$_{x}$

The iron chalcogenide Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ on the Te-rich side is known to exhibit the strongest electron correlations among the Fe-based superconductors, and is non-superconducting for $x$ < 0.1. In order to understand the origin of such behaviors, we have performed ARPES studies of Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ ($x$ = 0, 0.1, 0.2, and 0.4). The obtained mass renormalization factors for different energy bands are qualitatively consistent with DFT + DMFT calculations. Our results provide evidence for strong orbital dependence of mass renormalization, and systematic data which help us to resolve inconsistencies with other experimental data. The unusually strong orbital dependence of mass renormalization in Te-rich Fe$_{1+y}$Te$_{1-x}$Se$_{x}$ arises from the dominant contribution to the Fermi surface of the $d_{xy}$ band, which is the most strongly correlated and may contribute to the suppression of superconductivity.

cond-mat.supr-con↗

In-plane electronic anisotropy in the antiferromagnetic-orthorhombic phase of isovalent-substituted Ba(Fe$_{1-x}$Ru$_x$)$_2$As$_2$

We have studied the anisotropy in the in-plane resistivity and the electronic structure of isovalent Ru-substituted BaFe$_2$As$_2$ in the antiferromagnetic-orthorhombic phase using well-annealed crystals. The anisotropy in the residual resistivity component increases in proportional to the Ru dopant concentration, as in the case of Co-doped compounds. On the other hand, both the residual resistivity and the resistivity anisotropy induced by isovalent Ru substitution is found to be one order of magnitude smaller than those induced by heterovalent Co substitution. Combined with angle-resolved photoemission spectroscopy results, which show almost the same anisotropic band structure both for the parent and Ru-substituted compounds, we confirm the scenario that the anisotropy in the residual resistivity arises from anisotropic impurity scattering in the magneto-structurally ordered phase rather than directly from the anisotropic band structure of that phase.

cond-mat.supr-con↗

Suppression of the antiferromagnetic pseudogap in the electron-doped high-temperature superconductor by "protect annealing"

In the hole-doped cuprates, a small amount of carriers suppresses antiferromagnetism and induces superconductivity. In the electron-doped cuprates, on the other hand, superconductivity appears only in a narrow range of high electron concentration ($\sim$ doped Ce content) after reduction annealing, and strong antiferromagnetic (AFM) correlation persists in the superconducting phase. Recently, Pr$_{1.3-x}$La$_{0.7}$Ce$_{x}$CuO$_{4}$ (PLCCO) bulk single crystals annealed by a "protect annealing" method showed a high $T_c$ of $\sim$ 27 K for small Ce content down to $x \sim 0.05$. By angle-resolved photoemission spectroscopy (ARPES) measurements of PLCCO crystals, we observed a sharp quasi-particle peak on the entire Fermi surface without signature of an AFM pseudogap unlike all the previous work, indicating a dramatic reduction of AFM correlation length and/or of magnetic moments. The superconducting state was found to extend over a wide electron concentration range. The present ARPES results fundamentally change the long-standing picture on the electronic structure in the electron-doped regime.

cond-mat.supr-con↗

Fate of $yz$/$zx$ orbital degeneracy and $xy$ Fermi surface in Ru substituted FeSe$_{1-x}$Te$_{x}$

We have investigated the impact of Ru substitution on the multi-band electronic structure of FeSe$_{1-x}$Te$_x$ by means of angle-resolved photoemission spectroscopy (ARPES). The ARPES results exhibit suppression of the $xy$ Fermi surface and the spectral broadening near the zone boundaries, which can be associated with the lattice disorder introduced by the Ru substitution. The degeneracy of the Fe 3$d$ $yz$/$zx$ bands at the zone center, which is broken in FeSe$_{1-x}$Te$_x$, is partly recovered with the Ru substitution, indicating coexistence of nematic and non-nematic electronic states.

cond-mat.supr-con↗

Spectromicroscopy of electronic phase separation in K$_x$Fe$_{2-y}$Se$_2$ superconductor

Structural phase separation in A$_x$Fe$_{2-y}$Se$_2$ system has been studied by different experimental techniques, however, it should be important to know how the electronic uniformity is influenced, on which length scale the electronic phases coexist, and what is their spatial distribution. Here, we have used novel scanning photoelectron microscopy (SPEM) to study the electronic phase separation in K$_x$Fe$_{2-y}$Se$_2$, providing a direct measurement of the topological spatial distribution of the different electronic phases. The SPEM results reveal a peculiar interconnected conducting filamentary phase that is embedded in the insulating texture. The filamentary structure with a particular topological geometry could be important for the high T$_c$ superconductivity in the presence of a phase with a large magnetic moment in A$_x$Fe$_{2-y}$Se$_2$ materials.

cond-mat.supr-con↗

Important Roles of Te 5p and Ir 5d Spin-orbit Interactions on the Multi-band Electronic Structure of Triangular Lattice Superconductor Ir1-xPtxTe2

We report an angle-resolved photoemission spectroscopy (ARPES) study on a triangular lattice superconductor Ir$_{1-x}$Pt$_{x}$Te$_2$ in which the Ir-Ir or Te-Te bond formation, the band Jahn-Teller effect, and the spin-orbit interaction are cooperating and competing with one another. The Fermi surfaces of the substituted system are qualitatively similar to the band structure calculations for the undistorted IrTe$_2$ with an upward chemical potential shift due to electron doping. A combination of the ARPES and the band structure calculations indicates that the Te $5p$ spin-orbit interaction removes the $p_x/p_y$ orbital degeneracy and induces $p_x \pm ip_y$ type spin-orbit coupling near the A point. The inner and outer Fermi surfaces are entangled by the Te $5p$ and Ir $5d$ spin-orbit interactions which may provide exotic superconductivity with singlet-triplet mixing.

cond-mat.supr-con↗

Electronic structure reconstruction by orbital symmetry breaking in IrTe2

We report an angle-resolved photoemission spectroscopy (ARPES) study on IrTe2 which exhibits an interesting lattice distortion below 270 K and becomes triangular lattice superconductors by suppressing the distortion via chemical substitution or intercalation. ARPES results at 300 K show multi-band Fermi surfaces with six-fold symmetry which are basically consistent with band structure calculations. At 20 K in the distorted phase, whereas the flower shape of the outermost Fermi surface does not change from that at 300 K, topology of the inner Fermi surfaces is strongly modified by the lattice distortion. The Fermi surface reconstruction by the distortion depends on the orbital character of the Fermi surfaces, suggesting importance of Ir 5d and/or Te 5p orbital symmetry breaking.

cond-mat.supr-con↗