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M. I. Marqués

Publications and source records attributed to M. I. Marqués.

2 recordsLinked to original sources

Strong collective currents of gold nanoparticles in an optical vortex lattice

Self-organized collective behaviour of active units is inspiring new designs of artificial swarms of micron-sized objects. However, active control at the nanoscale remains elusive. We have accurately solved the collective optofluidic dynamics of gold plasmonic 50 nm-radius nanoparticles moving in aqueous solution under a nonconservative optical vortex lattice. Above a critical field intensity and concentration, the interplay between optical forces, thermal fluctuations and hydrodynamic pairing leads to a spontaneous transition towards synchronised motion exhibiting a rich assortment of collective dynamics. The critical phenomenon creates strong unidirectional currents of nanoparticles, reaching speeds of centimeters per second along the diagonals of the lattice.

cond-mat.mes-hall↗

Effect of long range spatial correlations on the lifetime statistics of an emitter in a two-dimensional disordered lattice

The effect of spatial correlations on the Purcell effect in a bidimensional dispersion of resonant nanoparticles is analyzed. We perform extensive calculations on the fluorescence decay rate of a point emitter embedded in a system of nanoparticles statistically distributed according to a simple 2D lattice-gas model near the critical point. For short-range correlations (high temperature thermalization) the Purcell factors present a long-tailed statistic which evolves towards a bimodal distribution when approaching the critical point where the spatial correlation length diverges. Our results suggest long-range correlations as a possible origin of the large fluctuations of experimental decay rates in disordered metal films.

physics.optics↗