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M. J. Naughton

Publications and source records attributed to M. J. Naughton.

At least 19 recordsLinked to original sources

Transmission anomalies in 2D photonic crystals from the checkerboard family: From broken to hidden symmetries and plasmon "spoofing"

In a field representation, the main symmetry of the electromagnetic response of complementary metal film structures is described by the Babinet principle, expected to be obeyed by structures in vanishingly thin films of a perfect electric conductor. A softer transmittance Babinet principle (TBP) is not so restrictive. The goal of this work is to study how severely this broken symmetry affects the optical response of such structures. We consider two geometrically distinct series of planar complementary structures from the checkerboard family: regular and bowtie. The self-complementary structure of these series is very singular and breaks even the rigorous Babinet principle. We study complete simulated transmittance spectral maps (T-Maps) that accumulate the whole spectral response of an entire series of structures in a single plot. The ab initio T-Maps of these 2D photonic crystals were simulated for linearly polarized waves propagating perpendicular to the planar structures, made in a vanishingly thin film of a perfect electric conductor. While confirming the expected long wavelength validity of the TBP, we show that in the frequency range where diffraction effects dominate, the standard derivation of the TBP no longer applies, and with the help of our T-Maps, we demonstrate a total collapse of the TBP in the structures considered. This broken symmetry practically eliminates all but one transmission band on the hole side of the T-Maps, the remaining strong band being a "spoof" plasmon, free of multiple frequency replicas, an important feature for filter applications. By symmetry arguments and simulations, we discovered that the T-Maps for bowtie and doubled-period regular structures are identical. We discuss how this hidden symmetry can benefit applications by providing a convenient scaling, whereby simplified structures can deliver a tailored response.

physics.optics

Towards spectrally selective catastrophic response

We study the large amplitude response of classical molecules to electromagnetic radiation, showing the universality of the transition from the linear to nonlinear response and brakeup at sufficiently large amplitudes. A range of models, from the simple harmonic oscillator to the successful Peyrard-Bishop-Dauxois (PBD) type models of DNA, lead to characteristic universal behavior: formation of domains of dissociation in the driving force amplitude-frequency space, characterized by the presence of local boundary minima. We demonstrate, that by simply following the progression of the resonance maxima in this space, while gradually increasing intensity of the radiation one must necessarily arrive at one of these minima, i.e. a point where the ultra-high spectral selectivity is retained. We show that this universal property, applicable to other oscillatory system, is a consequence of the fact that these models belong to the fold catastrophe universality class of the catastrophe theory. This in turn implies that for most bio-structures, including DNA, a high spectral sensitivity near the onset of the denaturation processes can be expected. Such spectrally selective molecular denaturation could find important applications in biology and medicine.

physics.app-ph

The Effects of Geometry on a-Si:H Solar Cell Performance

We present a model for simulating performance of 3D nano -coaxial and -hemispherical thin film solar cells. The material system considered in these simulations is hydrogenated amorphous silicon (a-Si:H), with solar cells fabricated in an n-i-p stacking architecture. Simulations for the performance of the planar a-Si:H device are compared against simulations performed using SCAPS-1D and found to be in close agreement. Electrical and optical properties of devices are discussed for the respective geometries. Maximum power point efficiencies are plotted as a function of i-layer thickness for insight into optimizing spatial parameters. Simulation results show that while geometrical changes in the energy band diagram impact charge carrier collection, a-Si:H solar cell performance is most significantly impacted by light absorption properties associated with nanoscopic arrays of non-planar structures. We compare our simulations to results of fabricated nanocoaxial a-Si:H solar cells and infer the mechanisms of enhanced absorption observed experimentally in such solar cells.

cond-mat.mtrl-sci

Spectroscopic evidence for negative electronic compressibility in a quasi-three-dimensional spin-orbit correlated metal

Negative compressibility is a sign of thermodynamic instability of open or non-equilibrium systems. In quantum materials consisting of multiple mutually coupled subsystems, the compressibility of one subsystem can be negative if it is countered by positive compressibility of the others. Manifestations of this effect have so far been limited to low-dimensional dilute electron systems. Here we present evidence from angle-resolved photoemission spectroscopy (ARPES) for negative electronic compressibility (NEC) in the quasi-three-dimensional (3D) spin-orbit correlated metal (Sr1-xLax)3Ir2O7. Increased electron filling accompanies an anomalous decrease of the chemical potential, as indicated by the overall movement of the deep valence bands. Such anomaly, suggestive of NEC, is shown to be primarily driven by the lowering in energy of the conduction band as the correlated bandgap reduces. Our finding points to a distinct pathway towards an uncharted territory of NEC featuring bulk correlated metals with unique potential for applications in low-power nanoelectronics and novel metamaterials.

cond-mat.str-el

Analytical Device-Physics Framework for Non-Planar Solar Cells

Non-planar solar-cell devices have been promoted as a means to enhance current collection in absorber materials with charge-transport limitations. This work presents an analytical framework for assessing the ultimate performance of non-planar solar-cells based on materials and geometry. Herein, the physics of the p-n junction is analyzed for low-injection conditions, when the junction can be considered spatially separable into quasi-neutral and space-charge regions. For the conventional planar solar cell architecture, previously established one-dimensional expressions governing charge carrier transport are recovered from the framework established herein. Space-charge region recombination statistics are compared for planar and non-planar geometries, showing variations in recombination current produced from the space-charge region. In addition, planar and non-planar solar cell performance are simulated, based on a semi-empirical expression for short-circuit current, detailing variations in charge carrier transport and efficiency as a function of geometry, thereby yielding insights into design criteria for solar cell architectures. For the conditions considered here, the expressions for generation rate and total current are shown to universally govern any solar cell geometry, while recombination within the space-charge region is shown to be directly dependent on the geometrical orientation of the p-n junction.

cond-mat.mtrl-sci

Direct-write, focused ion beam-deposited,7 K superconducting C-Ga-O nanowire

We have fabricated C-Ga-O nanowires by gallium focused ion beam-induced deposition from the carbon-based precursor phenanthrene. The electrical conductivity of the nanowires is weakly temperature dependent below 300 K, and indicates a transition to a superconducting state below Tc = 7 K. We have measured the temperature dependence of the upper critical field Hc2(T), and estimate a zero temperature critical field of 8.8 T. The Tc of this material is approximately 40% higher than that of any other direct write nanowire, such as those based on C-W-Ga, expanding the possibility of fabricating direct-write nanostructures that superconduct above liquid helium temperatures

cond-mat.mes-hall

Discretely guided electromagnetic effective medium

A material comprised of an array of subwavelength coaxial waveguides decomposes incident electromagnetic waves into spatially discrete wave components, propagates these components without frequency cut-off, and reassembles them on the far side of the material. The propagation of these wave components is fully controlled by the physical properties of the waveguides and their geometrical distribution in the array. This allows for an exceptional degree of control over the electromagnetic response of this effective medium, with numerous potential applications. With the development of nanoscale subwavelength coaxial waveguides, these applications (including metamaterial functionality) can be enabled in the visible frequency range.

cond-mat.mtrl-sci

Reply to Comment

Our experiments \cite{Wang05,Li05,Wang06} persuade us that the Meissner transition at $T_c$ in hole-doped cuprates is driven by the loss of long-range phase coherence caused by singular phase fluctuations, a scenario at odds with the mean-field (MF), Gaussian Ginzburg Landau (GGL) approach advocated by Cabo, Mosquiera and Vidal \cite{Cabo}.

cond-mat.supr-con

Magnetization, Nernst effect and vorticity in the cuprates

Nernst and magnetization experiments reveal the existence of a large region of the cuprate phase diagram above the $T_c$ curve in which vorticity and weak diamagnetism exist without phase coherence. We discuss the implication that the transition at $T_c$ is caused by the loss of long-range phase coherence caused by spontaneous vortex creation. Below $T_c$, these measurements provide an estimate of the depairing field $H_{c2}$ which is found to be very large (40-100 T depending on doping). We discuss the high-field Nernst and magnetization results, binding energy, and the phase diagram of hole-doped cuprates. Some new magnetization results on the vortex liquid in very underdoped LSCO in the limit $T\to 0$ are reported as well.

cond-mat.supr-con

Depairing field, onset temperature and the nature of the transition in cuprates

The depairing (upper critical) field $H_{c2}$ in hole-doped cuprates has been inferred from magnetization curves $M$-$H$ measured by torque magnetometry in fields $H$ up to 45 T. We discuss the implications of the results for the pair binding energy, the Nernst onset temperature, fluctuations and the nature of the Meissner transition at $T_c$.

cond-mat.supr-con

Field-enhanced diamagnetism in intense magnetic field in the pseudogap state of the cuprate $\rm Bi_2Sr_2CaCu_2O_{8+δ}

In hole-doped cuprates, Nernst experiments imply that the superconducting state is destroyed by spontaneous creation of vortices which destroy phase coherence. Using torque magnetometry on $\rm Bi_2Sr_2CaCu_2O_{8+δ}$, we uncover a field-enhanced diamagnetic signal $M$ above the transition temperature $T_c$ that increases with applied field to 32 Tesla and scales just like the Nernst signal. The magnetization results above $T_c$ distinguish $M$ from conventional amplitude fluctuations, and strongly support the vortex scenario for the loss of phase coherence at $T_c$.

cond-mat.supr-con

Strongly nonlinear magnetization above $T_c$ in $\rm Bi_2Sr_2CaCu_2O_{8+δ}$

Using high-resolution magnetometry we have investigated in detail the magnetization $M$ above the critical temperature $T_c$ in $\rm Bi_2Sr_2CaCu_2O_{8+δ}$. In a broad range of temperature $T$ above $T_c$, we find that $M(T,H)$ is strongly non-linear in the field $H$. We show that as $T\to T_c$, the susceptibility $χ(T,H)$ diverges to very large values ($χ\to$ -1) if measured in weak $H$. In addition, $M(H)$ displays an anomalous non-analytic form $M\sim H^{1/δ}$ in weak fields with a strongly $T$-dependent exponent $δ(T)$. These features strongly support the proposal that, above $T_c$, the pair condensate survives to support significant London rigidity.

cond-mat.supr-con

Coexistence of Superconductivity and Antiferromagnetism Probed by Simultaneous NMR and Electrical Transport in (TMTSF)2PF6

We report simultaneous NMR and electrical transport experiments in the pressure range near the boundary of the antiferromagnetic spin density wave (SDW) insulator and the metal-lic/superconducting (SC) phase in (TMTSF)2PF6. Measurements indicate a tricritical point separat-ing a line of second order SDW/metal transitions from a line of first order SDW/metal(SC) transi-tions with coexistence of macroscopic regions of SDW and metal(SC) order, with little mutual in-teraction but strong hysteretic effects. NMR results quantify the fraction of each phase.

cond-mat.supr-con

Interference Effects Due to Commensurate Electron Trajectories and Topological Crossovers in (TMTSF)2ClO4

We report angle-dependent magnetoresistance measurements on (TMTSF)2ClO4 that provide strong support for a new macroscopic quantum phenomenon, the interference commensurate (IC) effect, in quasi-one dimensional metals. In addition to observing rich magnetoresistance oscillations, and fitting them with one-electron calculations, we observe a clear demarcation of field-dependent behavior at local resistance minima and maxima (versus field angle). Anticipated by a theoretical treatment of the IC effect in terms of Bragg reflections in the extended Brillouin zone, this behavior results from 1D-2D topological crossovers of electron wave functions as a function of field orientation.

cond-mat.str-el

Angular Magnetoresistance Oscillations in Organic Conductors

We demonstrate that electron wave functions change their dimensionality at some commensurate directions of a magnetic field in conductors with open [quasi-one-dimensional (Q1D)] sheets of Fermi surface. These 1D -> 2D dimensional crossovers lead to delocalization of wave functions and are responsible for angular magnetoresistance oscillations. As an example, we show that suggested theory is in qualitative and quantitative agreements with the recent experimental data obtained on (TMTSF)2ClO4 conductor.

cond-mat.supr-con

Magic Angle Effects and AMRO as Dimensional Crossovers

It is shown that interference effects between velocity and density of states, which occur as electrons move along open orbits in the extended Brillouin zone, result in a change of wave functions dimensionality at Magic Angle (MA) directions of a magnetic field. In a particular, we demonstrate that these 1D -> 2D dimensional crossovers result in the appearance of sharp minima in a resistivity component Rzz, perpendicular to conducting layers, which explains the main qualitative features of MA and Angular Magneto-Resistance Oscillations (AMRO) phenomena observed in low-dimensional conductors (TMTSF)2X, (DMET-TSeF)2X, and a-(BEDT-TTF)2MHg(SCN)4.

cond-mat.supr-con

Magnetic Determination of $H_{c2}$ under Accurate Alignment in (TMTSF)$_2$ClO$_4$

Cantilever magnetometry has been used to measure the upper critical magnetic field $H_{c2}$ of the quasi-one dimensional molecular organic superconductor (TMTSF)$_2$ClO$_4$. From simultaneous resistivity and torque magnetization experiments conducted under precise field alignment, $H_{c2}$ at low temperature is shown to reach 5T, nearly twice the Pauli paramagnetic limit imposed on spin singlet superconductors. These results constitute the first thermodynamic evidence for a large $H_{c2}$ in this system and provide support for spin triplet pairing in this unconventional superconductor

cond-mat.supr-con

Interference Commensurate Oscillations in Q1D Conductors

We suggest an analytical theory to describe angular magnetic oscillations recently discovered in quasi-one-dimensional conductor (TMTSF)2PF6 [see Phys. Rev. B, 57, 7423 (1998)] and define the positions of the oscillation minima. The origin of these oscillations is related to interference effects resulting from an interplay of quasi-periodic and periodic ("commensurate") electron trajectories in an inclined magnetic field. We reproduce via calculations existing experimental data and predict some novel effects.

cond-mat.supr-con