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M. Janoschek

Publications and source records attributed to M. Janoschek.

At least 55 records · Page 3Linked to original sources
arXiv2016

Comments on 'Phonon and magnetic structure in δ-plutonium from density-functional theory' by P. Söderlind et al

In their recent paper [Söderlind, P. et al., Sci. Rep. 5, 15958 (2015)], Söderlind et al. discuss two subjects from a theoretical point of view: the phonon spectra and the possible magnetic structure of δ-plutonium (Pu). Here, we comment on the second subject. Söderlind et al. compare the Pu magnetic form factor F(Q) calculated via density functional theory (DFT) with measurements of F(Q) by neutron spectroscopy [Janoschek, M. et al., Sci. Adv. 1, e1500188 (2015)]. In particular, this comparison does not consider a number of experimental facts established in the neutron spectroscopy study.

cond-mat.str-el↗
arXiv2015

Band structure of helimagnons in MnSi resolved by inelastic neutron scattering

A magnetic helix realizes a one-dimensional magnetic crystal with a period given by the pitch length $λ_h$. Its spin-wave excitations -- the helimagnons -- experience Bragg scattering off this periodicity leading to gaps in the spectrum that inhibit their propagation along the pitch direction. Using high-resolution inelastic neutron scattering the resulting band structure of helimagnons was resolved by preparing a single crystal of MnSi in a single magnetic-helix domain. At least five helimagnon bands could be identified that cover the crossover from flat bands at low energies with helimagnons basically localized along the pitch direction to dispersing bands at higher energies. In the low-energy limit, we find the helimagnon spectrum to be determined by a universal, parameter-free theory. Taking into account corrections to this low-energy theory, quantitative agreement is obtained in the entire energy range studied with the help of a single fitting parameter.

cond-mat.str-el↗
arXiv2015

The Valence-Fluctuating Ground State of Plutonium

A central issue in material science is to obtain understanding of the electronic correlations that control complex materials. Such electronic correlations frequently arise due to the competition of localized and itinerant electronic degrees of freedom. While the respective limits of well-localized or entirely itinerant ground states are well-understood, the intermediate regime that controls the functional properties of complex materials continues to challenge theoretical understanding. We have used neutron spectroscopy to investigate plutonium, which is a prototypical material at the brink between bonding and non-bonding configurations. Our study reveals that the ground state of plutonium is governed by valence fluctuations, that is, a quantum-mechanical superposition of localized and itinerant electronic configurations as recently predicted by dynamical mean field theory. Our results not only resolve the long-standing controversy between experiment and theory on plutonium's magnetism, but also suggest an improved understanding of the effects of such electronic dichotomy in complex materials.

cond-mat.str-el↗
arXiv2015

Electrodynamics of the antiferromagnetic phase in URu$_2$Si$_2$

We present data on the optical conductivity of URu$_{2-x}$(Fe,Os)$_{x}$Si$_{2}$. While the parent material URu$_2$Si$_2$ enters the enigmatic hidden order phase below 17.5 K, an antiferromagnetic phase is induced by the substitution of Fe or Os onto the Ru sites. We find that both the HO and the AFM phases exhibit an identical gap structure that is characterized by a loss of conductivity below the gap energy with spectral weight transferred to a narrow frequency region just above the gap, the typical optical signature of a density wave. The AFM phase is marked by strong increases in both transition temperature and the energy of the gap associated with the transition. In the normal phase just above the transition the optical scattering rate varies as $ω^2$. We find that in both the HO and the AFM phases, our data are consistent with elastic resonant scattering of a Fermi liquid. This indicates that the appearance of a coherent state is a necessary condition for either ordered phase to emerge. Our measurements favor models in which the HO and the AFM phases are driven by the common physics of a nesting-induced density-wave-gap.

cond-mat.str-el↗
arXiv2015

Magnetic structure of the antiferromagnetic Kondo lattice compounds CeRhAl4Si2 and CeIrAl4Si2

We have investigated the magnetic ground state of the antiferromagnetic Kondo-lattice compounds CeMAl$_{4}$Si$_{2}$ (M = Rh, Ir) using neutron powder diffraction. Although both of these compounds show two magnetic transitions $T_{N1}$ and $T_{N2}$ in the bulk properties measurements, evidence for magnetic long-range order was only found below the lower transition $T_{N2}$. Analysis of the diffraction profiles reveals a commensurate antiferromagnetic structure with a propagation vector $\mathbf{k}$= (0, 0, 1/2). The magnetic moment in the ordered state of CeRhAl$_{4}$Si$_{2}$ and CeIrAl$_{4}$Si$_{2}$ were determined to be 1.14(2) and 1.41(3) $μ_{B}$/Ce, respectively, and are parallel to the crystallographic $c$-axis in agreement with magnetic susceptibility measurements.

cond-mat.str-el↗
arXiv2014

Chemical pressure tuning of URu$_2$Si$_2$ via isoelectronic substitution of Ru with Fe

We have used specific heat and neutron diffraction measurements on single crystals of URu$_{2-x}$Fe$_x$Si$_2$ for Fe concentrations $x$ $\leq$ 0.7 to establish that chemical substitution of Ru with Fe acts as "chemical pressure" $P_{ch}$ as previously proposed by Kanchanavatee et al. [Phys. Rev. B {\bf 84}, 245122 (2011)] based on bulk measurements on polycrystalline samples. Notably, neutron diffraction reveals a sharp increase of the uranium magnetic moment at $x=0.1$, reminiscent of the behavior at the "hidden order" (HO) to large moment antiferromagnetic (LMAFM) phase transition observed at a pressure $P_x\approx$ 0.5-0.7~GPa in URu$_2$Si$_2$. Using the unit cell volume determined from our measurements and an isothermal compressibility $κ_{T} = 5.2 \times 10^{-3}$ GPa$^{-1}$ for URu$_2$Si$_2$, we determine the chemical pressure $P_{ch}$ in URu$_{2-x}$Fe$_x$Si$_2$ as a function of $x$. The resulting temperature $T$-chemical pressure $P_{ch}$ phase diagram for URu$_{2-x}$Fe$_x$Si$_2$ is in agreement with the established temperature $T$-external pressure $P$ phase diagram of URu$_2$Si$_2$.

cond-mat.str-el↗
arXiv2014

The magnitude of the magnetic exchange interaction in the heavy fermion antiferromagnet CeRhIn$_5$

We have used high-resolution neutron spectroscopy experiments to determine the complete spin wave spectrum of the heavy fermion antiferromagnet CeRhIn$_5$. The spin wave dispersion can be quantitatively reproduced with a simple $J_1$-$J_2$ model that also naturally explains the magnetic spin-spiral ground state of CeRhIn$_5$ and yields a dominant in-plane nearest-neighbor magnetic exchange constant $J_0$ = 0.74 meV. Our results pave the way to a quantitative understanding of the rich low-temperature phase diagram of the prominent Ce$T$In$_5$ ($T$ = Co, Rh, Ir) class of heavy fermion materials.

cond-mat.str-el↗
arXiv2014

Probing the superconductivity of PrPt4Ge12 through Ce substitution

We report measurements of electrical resistivity, magnetic susceptibility, specific heat, and thermoelectric power on the system Pr1-xCexPt4Ge12. Superconductivity is suppressed with increasing Ce concentration up to x = 0.5, above which there is no evidence for superconductivity down to 1.1 K. The Sommerfeld coefficient γ increases with increasing x from 48 mJ/mol K^2 up to 120 mJ/mol K^2 at x = 0.5, indicating an increase in strength of electronic correlations. The temperature dependence of the specific heat at low temperatures evolves from roughly T^3 for x = 0 to e^(-Δ/T) behavior for x = 0.05 and above, suggesting a crossover from a nodal to a nodeless superconducting energy gap or a transition from multiband to single-band superconductivity. Fermi-liquid behavior is observed throughout the series in low-temperature magnetization, specific heat, and electrical resistivity measurements.

cond-mat.str-el↗
arXiv2014

Critical spin-flip scattering at the helimagnetic transition of MnSi

We report spherical neutron polarimetry (SNP) and discuss the spin-flip scattering cross sections as well as the chiral fraction $η$ close to the helimagnetic transition in MnSi. For our study, we have developed a miniaturised SNP device that allows fast data collection when used in small angle scattering geometry with an area detector. Critical spin-flip scattering is found to be governed by chiral paramagnons that soften on a sphere in momentum space. Carefully accounting for the incoherent spin-flip background, we find that the resulting chiral fraction $η$ decreases gradually above the helimagnetic transition reflecting a strongly renormalised chiral correlation length with a temperature dependence in excellent quantitative agreement with the Brazovskii theory for a fluctuation-induced first order transition.

cond-mat.str-el↗
arXiv2013

Hybridization-Driven Orthorhombic Lattice Instability in URu2Si2

We have measured the elastic constant (C11-C12)/2 in URu2Si2 by means of high-frequency ultrasonic measurements in pulsed magnetic fields H || [001] up to 61.8 T in a wide temperature range from 1.5 to 116 K. We found a reduction of (C11-C12)/2 that appears only in the temperature and magnetic field region in which URu2Si2 exhibits a heavy-electron state and hidden-order. This change in (C11-C12)/2 appears to be a response of the 5f-electrons to an orthorhombic and volume conservative strain field ε_xx-ε_yy with Γ3-symmetry. This lattice instability is likely related to a symmetry-breaking band instability that arises due to the hybridization of the localized f electrons with the conduction electrons, and is probably linked to the hidden-order parameter of this compound.

cond-mat.str-el↗
arXiv2013

Nuclear magnetic resonance studies of pseudospin fluctuations in URu$_2$Si$_2$

We report $^{29}$Si NMR measurements in single crystals and aligned powders of URu$_2$Si$_2$ in the hidden order and paramagnetic phases. The spin-lattice-relaxation data reveal evidence of pseudospin fluctuations of U moments in the paramagnetic phase. We find evidence for partial suppression of the density of states below 30 K, and analyze the data in terms of a two component spin-fermion model. We propose that this behavior is a realization of a pseudogap between the hidden order transition $T_{HO}$ and 30 K. This behavior is then compared to other materials that demonstrate precursor fluctuations in a pseudogap regime above a ground state with long-range order.

cond-mat.str-el↗
arXiv2013

Yb Valence Change in (Ce,Yb)CoIn5 from spectroscopy and bulk properties

The electronic structure of (Ce,Yb)CoIn5 has been studied by a combination of photoemission, x-ray absorption and bulk property measurements. Previous findings of a Ce valence near 3+ for all x and of an Yb valence near 2.3+ for x>0.3 were confirmed. One new result of this study is that the Yb valence for x<0.2 increases rapidly with decreasing x from 2.3+ toward 3+, which correlates well with de Haas van Alphen results showing a change of Fermi surface around x=0.2. Another new result is the direct observation by angle resolved photoemission Fermi surface maps of about 50% cross sectional area reductions of the α- and β-sheets for x=1 compared to x=0, and a smaller, essentially proportionate, size change of the α-sheet for x=0.2. These changes are found to be in good general agreement with expectations from simple electron counting. The implications of these results for the unusual robustness of superconductivity and Kondo coherence with increasing x in this alloy system are discussed.

cond-mat.str-el↗
arXiv2013

Absence of a static in-plane magnetic moment in the "hidden-order" phase of URu$_2$Si$_2$

We have carried out a careful magnetic neutron scattering study of the heavy fermion compound \URuSi\ to probe the possible existence of a small magnetic moment parallel to tetragonal basal plane in the "hidden-order" phase. This small in-plane component of the magnetic moment on the uranium sites $S_\parallel$ has been postulated by two recent models (rank-5 superspin/hastatic order) aiming to explain the hidden-order phase, in addition to the well-known out-of-plane component $S_\perp ~ \approx~0.01-0.04 $μ_B$/U. In order to separate $S_\parallel$ and $S_\perp$ we take advantage of the condition that for magnetic neutron scattering only the components of the magnetic structure that are perpendicular to the scattering vector $Q$ contribute to the magnetic scattering. We find no evidence for an in-plane magnetic moment $S_\parallel$. Based on the statistics of our measurement, we establish that the upper experimental limit for the size of any possible in-plane component is $S^{\rm{max}}_\parallel ~ \leq~1\cdot 10^{-3} ~μ_B$/U.

cond-mat.str-el↗
arXiv2013

Ferromagnetic quantum critical point in UCo1-xFexGe

We have carried out a comprehensive study of the UCo1-xFexGe series across the entire range of compositions 0 <= x <= 1, and report the results of x-ray diffraction, magnetization, specific heat, and electrical resistivity to uncover the T-x phase diagram. Substitution of Fe into UCoGe initially results in an increase in the Curie temperature and a rapid destruction of the superconductivity. Near x = 0.22, the ferromagnetic transition is suppressed to zero temperature at an apparent ferromagnetic itinerant electron quantum critical point, where the temperature dependence of the electrical resistivity and specific heat in this region reveal non-Fermi liquid behavior.

cond-mat.str-el↗
arXiv2012

Non-Fermi liquid behavior with and without quantum criticality in Ce(1-x)Yb(x)CoIn(5)

One of the greatest challenges to Landau's Fermi liquid theory - the standard theory of metals - is presented by complex materials with strong electronic correlations. In these materials, non-Fermi liquid transport and thermodynamic properties are often explained by the presence of a continuous quantum phase transition which happens at a quantum critical point (QCP). A QCP can be revealed by applying pressure, magnetic field, or changing the chemical composition. In the heavy-fermion compound CeCoIn$_5$, the QCP is assumed to play a decisive role in defining the microscopic structure of both normal and superconducting states. However, the question of whether QCP must be present in the material's phase diagram to induce non-Fermi liquid behavior and trigger superconductivity remains open. Here we show that the full suppression of the field-induced QCP in CeCoIn$_5$ by doping with Yb has surprisingly little impact on both unconventional superconductivity and non-Fermi liquid behavior. This implies that the non-Fermi liquid metallic behavior could be a new state of matter in its own right rather then a consequence of the underlying quantum phase transition.

cond-mat.mtrl-sci↗
arXiv2011

Transport, magnetic, and thermal properties of non-centrosymmetric Yb2Co12P7

We report magnetization and specific heat measurements down to 2 K and electrical resistivity down to millikelvin temperatures on polycrystalline samples of the non-centrosymmetric compound Yb2Co12P7. In addition to the previously reported ferromagnetic ordering of the cobalt sub-lattice at T_C = 136 K we find a magnetic transition below T_M = 5 K that is likely associated with ordering of the Yb ions. The broad nature of the specific heat anomaly suggests disordered magnetism and possible short range correlations well above T_M.

cond-mat.str-el↗
arXiv2010

Helimagnon Bands as Universal Spin Excitations of Chiral Magnets

MnSi is a cubic compound with small magnetic anisotropy, which stabilizes a helimagnetic spin spiral that reduces to a ferromagnetic and antiferromagnetic state in the long- and short-wavelength limit, respectively. We report a comprehensive inelastic neutron scattering study of the collective magnetic excitations in the helimagnetic state of MnSi. In our study we observe a rich variety of seemingly anomalous excitation spectra, as measured in well over twenty different locations in reciprocal space. Using a model based on only three parameters, namely the measured pitch of the helix, the measured ferromagnetic spin wave stiffness and the amplitude of the signal, as the only free variable, we can simultaneously account for \textit{all} of the measured spectra in excellent quantitative agreement with experiment. Our study identifies the formation of intense, strongly coupled bands of helimagnons as a universal characteristic of systems with weak chiral interactions.

cond-mat.str-el↗