SearcharxivSearch

arXiv subjects

M. Ji

Publications and source records attributed to M. Ji.

6 recordsLinked to original sources

Lifetimes of excited states in P-, As- and Sb-

Radiative lifetimes of three elements of the nitrogen group have been experimentally investigated at the Double ElectroStatic Ion Ring Experiment (DESIREE) facility at Stockholm University. The experiments were performed through selective laser photodetachment of excited states of P$^-$, As$^-$ and Sb$^-$ ions stored in a cryogenic storage ring. The experimental results were compared with theoretically predicted lifetimes, yielding a mixture of very good agreements in some cases and large discrepancies in others. These results are part of our efforts to map out the lifetimes of all excited states in negative ions. This data can be used to benchmark atomic theories, in particularly with respect to the degree of electron correlation that is incorporated in various theoretical models.

physics.atom-ph

Lifetimes of excited states in Rh-

The radiative decay of excited states of the negative ion of rhodium, Rh$^-$, has been investigated experimentally and theoretically. The experiments were conducted at the Double ElectroStatic Ion Ring Experiment (DESIREE) facility at Stockholm University using selective photodetachment from a stored ion beam to monitor the time evolution of the excited state populations. The lifetimes of the Rh$^-$ $^3F_{3}$ and $^3F_{2}$ fine structure levels were measured to be 3.2(6)~s and 21(4)~s, respectively. An additional, previously unreported, higher-lying bound state of mixed $^1D_2+^3P_2+(4d^95s)^1D_2+^3F_2$ composition was observed and found to have a lifetime of 10.9(8)s. The binding energy of this state was determined to be in the interval $0.1584(2) $ eV $ < E_b < 0.2669(2)$ eV, using laser photodetachment threshold (LPT) spectroscopy. An autodetaching state with a lifetime of 480(10) microseconds was also observed. Theoretical calculations of the excited-state compositions, energies, and magnetic-dipole transition lifetimes were performed using the multiconfiguration Dirac-Hartree-Fock and relativistic configuration interaction methods. The calculated lifetimes of the $^3F_{3}$ and $^3F_{2}$ fine structure levels are in excellent agreement with the measured values. The present study should provide valuable insights into electron correlation effects in negative ions and forbidden radiative transitions.

physics.atom-ph

Precision measurements on Si-

High-precision measurements of the electron affinities (EA) of the three stable isotopes of silicon, $^{28}$Si, $^{29}$Si and $^{30}$Si, have been performed at the cryogenic electrostatic ion-beam storage ring DESIREE. The quantum states of the ions were manipulated using laser depletion, and the ions were photodetached by laser photodetachment threshold spectroscopy. These EA values are the first reported for $^{29}$Si$^-$ and $^{30}$Si$^-$ and provide a reduced uncertainty for $^{28}$Si$^-$. The resulting EAs are $EA(^{28}$Si$) = 1.38952201(17)$ eV, $EA(^{29}$Si$) = 1.38952172(12)$ eV and $EA(^{29}$Si$) = 1.38952078(12)$ eV, with the corresponding isotope shifts $IS(^{29-28}$Si$) = 0.29(16)$ micro eV and $IS(^{30-28}$Si$) = 1.23(16) $ micro eV. In addition to these measurements, the resolution and signal-to-background level was sufficient to reveal the hyperfine structure splitting in the $^{29}$Si$^-$ isotope, which we report to be $1.8(4) micro eV.

physics.atom-ph

Thermal and electromagnetic properties of Bi$_2$Sr$_2$CaCu$_2$O$_8$ intrinsic Josephson junction stacks studied via one-dimensional coupled sine-Gordon equations

We used one-dimensional coupled sine-Gordon equations combined with heat diffusion equations to numerically investigate the thermal and electromagnetic properties of a $300\,μ\mathrm{m}$ long intrinsic Josephson junction stack consisting of $N = 700$ junctions. The junctions in the stack are combined to $M$ segments where we assume that inside a segment all junctions behave identically. Most simulations are for $M = 20$. For not too high bath temperatures there is the appearence of a hot spot at high bias currents. In terms of electromagnetic properties, robust standing wave patterns appear in the current density and electric field distributions. These patterns come together with vortex/antivortex lines across the stack that correspond to $π$ kink states, discussed before in the literature for a homogeneous temperature distribution in the stack. We also discuss scaling of the thermal and electromagnetic properties with $M$, on the basis of simulations with $M$ between 10 and 350.

cond-mat.supr-con

Adaptive Genetic Algorithm for Crystal Structure Prediction

We present a genetic algorithm (GA) for structural search that combines the speed of structure exploration by classical potentials with the accuracy of density functional theory (DFT) calculations in an adaptive and iterative way. This strategy increases the efficiency of the DFT-based GA by several orders of magnitude. This gain allows considerable increase in size and complexity of systems that can be studied by first principles. The method's performance is illustrated by successful structure identifications of complex binary and ternary inter-metallic compounds with 36 and 54 atoms per cell, respectively. The discovery of a multi-TPa Mg-silicate phase with unit cell containing up to 56 atoms is also reported. Such phase is likely to be an essential component of terrestrial exoplanetary mantles.

cond-mat.mtrl-sci

Modeling the linewidth dependence of coherent terahertz emission from intrinsic Josephson junction stacks in the hot-spot regime

Recently it has been found that, when operated at large input power, the linewidth of terahertz radiation emitted from intrinsic Josephson junction stacks can be as narrow as some megahertz. In this high-bias regime a hot spot coexists with regions which are still superconducting. Surprisingly, the linewidth was found to decrease with increasing bath temperature. We present a simple model describing the dynamics of the stack in the presence of a hot spot by two parallel arrays of pointlike Josephson junctions and an additional shunt resistor in parallel. Heat diffusion is taken into account by thermally coupling all elements to a bath at temperature T_b. We present current-voltage characteristics of the coupled system and calculations of the linewidth of the radiation as a function of T_b. In the presence of a spatial gradient of the junction parameters critical current and resistance, the linewidth deceases with increasing T_b, similar to the experimental observation.

cond-mat.supr-con