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M. K. Lajer

Publications and source records attributed to M. K. Lajer.

2 recordsLinked to original sources

Observation of multipartite spin entanglement in a cuprate chain

Quantum materials are believed to host highly entangled states of matter, but probing and quantifying such entanglement has long remained experimentally elusive. Here, we use resonant inelastic X-ray scattering (RIXS) as a probe of multipartite spin entanglement. By projecting the RIXS cross section onto the appropriate spin excitation channel, we show that the Quantum Fisher Information can be extracted directly from the measured spin fluctuation spectrum. We detect at least 7-partite spin entanglement in the model one-dimensional cuprate Sr$_2$CuO$_3$, revealing one of the largest entanglement depths yet reported in a solid. The observed entanglement depth agrees with Hubbard-model expectations and persists to elevated temperatures. Our results establish RIXS as an experimental probe of many-body spin entanglement and provide a platform for extensions to charge and orbital sectors and nonequilibrium settings.

cond-mat.str-el

Layer Architecture Shapes Electronic, Magnetic, and Lattice Interactions in Ruddlesden-Popper Nickelates

The discovery of superconductivity in Ruddlesden-Popper nickelates has raised a central question: how does layer architecture shape the electronic, magnetic, and lattice interactions relevant to pairing? Here, we report a detailed comparative study of the two polymorphs of La3Ni2O7--the alternating monolayer-trilayer (LNO-1313) and bilayer (LNO-2222) structures--and the related trilayer compound La4Ni3O10, using both Ni L3- and O K-edge RIXS. We find that LNO-1313 and La4Ni3O10 share strikingly similar electronic, magnetic, and lattice excitations, whereas bilayer LNO-2222 exhibits distinct features. Compared to LNO-2222, LNO-1313 and La4Ni3O10 have weaker orbital polarization, enhanced 3d8L character, a reduced out-of-plane magnetic-exchange scale, and stronger EPC. Within an effective local-moment framework, an entangled-dimer scenario provides a natural description of the spin excitations generated by strong antiferromagnetic interlayer coupling. Its advantage over conventional spin-wave theory is clearest in bilayer LNO-2222, where the interlayer coupling dominates the intralayer interactions. These findings provide critical experimental constraints for future theoretical models for the low-energy physics relevant to superconductivity in these layered nickelates.

cond-mat.str-el