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M. Kowal

Publications and source records attributed to M. Kowal.

At least 19 recordsLinked to original sources

From Superfluid Coherence to High-$K$ Fragment Channels at Nuclear Scission

The origin of fission-fragment spin remains unresolved. For $^{236}$U fission, we combine deformation-dependent finite-temperature pairing with a multidimensional scission-spectrum analysis. Near the pairing-quenching boundary, pair breaking exposes near-Fermi high-$\Omega$ intruder orbitals and opens high-$K$ channels. The resulting maximum spectroscopic capacities range from a few to more than a dozen units of $\hbar$. Rapid neck rupture acts as a non-adiabatic projection freeze-out, where pairing serves as a dynamical gate: its critical attenuation does not generate angular momentum but allows existing high-$K$ projections to be retained diabatically as local fragment-$K$ components while total angular momentum remains conserved.

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A Question of Shape: New Mechanism Governing Superheavy Nuclei Survival

We demonstrate that hot superheavy nuclei do not retain spherical shapes, as traditionally assumed, but instead equilibrate in deformed, often oblate or triaxial, configurations at finite excitation energy. This behavior arises from a mechanism analogous to the Jahn-Teller effect: spherical systems exhibit high single-particle degeneracy near the Fermi surface, causing their shell corrections to damp out significantly faster with temperature than those of deformed shapes. Using a finite-temperature framework, we reveal a thermally induced inversion of the potential-energy landscape in the Z = 118-120 region, where deformed minima become energetically favored at U = 30-50 MeV. This shape inversion fundamentally alters the competition between neutron evaporation and fission. We derive a deformation-dependent correction to the survival probability, revealing a systematic bias in estimates based on spherical ground-state properties. Our results identify a finite-temperature structural effect that calls for a revision of current models of superheavy-nucleus synthesis and decay.

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Comparative Study of Langevin and Random Walk Models for Nuclear Fission in the Overdamped Regime

We present a comparative study of Langevin dynamics and a Metropolis random walk model applied to thermal neutron-induced fission of $^{229}$Th, $^{235}$U, $^{239}$Pu, $^{245}$Cm, $^{249}$Cf, and $^{255}$Fm. Both methods are implemented within an identical four-dimensional Fourier-over-Spheroid framework, using potential energy surfaces derived from the macroscopic-microscopic model. We show that the Metropolis walk corresponds to the overdamped limit of the Langevin equations and confirm this correspondence numerically by Langevin calculations performed in the strongly damped regime and with quantum corrections to the random force switched off. Under these conditions, the two approaches produce essentially identical mass distributions for the lighter actinides. Systematic deviations develop for the heavier actinides, where the Langevin dynamics yields a non-negligible symmetric fission component absent in the random walk results. We trace this difference to the kinematic structure of the Metropolis sampling and to the residual inertial dynamics retained in the Langevin framework. A parallel comparison of Langevin calculations with and without the quantum-corrected effective temperature $T^*$ isolates the contribution of zero-point fluctuations and suggests that their standard phenomenological treatment may overestimate their impact in certain cases. Both approaches qualitatively reproduce the asymmetric peak positions and their systematic evolution across the actinide chain, while a common quantitative limitation -- the narrowness of the predicted distributions -- points to the role of higher-dimensional deformation modes not included in the present parametrization.

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Survival of Pairing Correlations and Shell Effects at Scission in Finite-Temperature Nuclear Fission: Implications for Odd-Even Staggering

We investigate the finite-temperature evolution of microscopic free-energy corrections in nuclear fission, focusing on pairing and shell effects near scission. The analysis is based on a finite-temperature BCS treatment combined with the Strutinsky method and is performed for representative deformation points along the fission path. Both pairing and shell contributions exhibit regular thermal attenuation, but their deformation dependencies differ substantially. In particular, pairing remains strongly deformation-dependent in the scission region, and its free-energy contribution differs markedly between the constant and surface-dependent pairing-strength prescriptions. The shell correction near scission is also significant at low temperature and is progressively suppressed with increasing excitation energy. These results support the interpretation of odd-even staggering in fragment charge yields as a manifestation of pairing correlations surviving into the strongly deformed pre-scission configuration. They also show that pairing and shell effects should be treated separately in finite-temperature dynamical calculations, with distinct deformation- and temperature-dependent attenuation laws.

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Sensitivity of Isotopic Fission Yields in Actinides to the Macroscopic Liquid-Drop Model: LSD vs ISOLDA

The impact of the macroscopic liquid-drop prescription on isotope-resolved fission-fragment yields in the actinide region is assessed by comparing two alternative parameterizations: the Lublin--Strasbourg Drop (LSD) model and the ISOscalar Liquid Drop Approximation (ISOLDA). The two prescriptions differ primarily in the treatment of isospin dependence in the volume and surface terms; in ISOLDA, an explicit dependence on the isospin square $T(T+1)$, where $T=|N-Z|/2$, is introduced in both coefficients. Using an identical set of fragment-yield observables and the same experimental reference (fission of $^{250}$Cf$^*$ at low and high energies), the propagation of the macroscopic-energy choice into the predicted yields is quantified in terms of (i) the location of the most probable post-neutron isotopes along elemental chains, (ii) the widths and asymmetries of the isotopic distributions, and (iii) the population of neighboring nuclides on the distribution tails. A comparable description of the gross properties of the isotopic yield pattern is obtained with both prescriptions, particularly for light and intermediate fragments, where peak positions and near-maximum curvatures are reproduced similarly. The most discriminating differences are found for heavy-fragment chains, for which the ridge location and isotopic centroids are rendered more sensitive to macroscopic isospin terms. Overall, a closer average agreement with the evaluated data is obtained with LSD, while the LSD--ISOLDA spread is shown to provide a practical estimate of the macroscopic-model uncertainty in isotope-resolved yields.

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Isotope-Resolved Ba and Xe Yields in Actinide Fission and Correlated Heavy--Light Fragment Systematics

Isotope-resolved post-neutron fission yields in the Ba and Xe chains are calculated and benchmarked against evaluated reference data, with emphasis on element-resolved isotopic chains $Y(N_f)$ at fixed fragment charge $Z$ and on the consistency of heavy--light fragment correlations. Calculations are performed within a four-dimensional (4D) Langevin framework employing Fourier-over-Spheroid shape parametrization. The benchmark covers spontaneous fission of selected Cm and Cf isotopes (including $^{244,246}$Cm and $^{250}$Cf) as well as neutron-induced fission at thermal and 14-MeV energies for representative actinides in the Th--Pu region (including $^{229}$Th, $^{235}$U, $^{239}$Pu, and $^{249}$Cf). The dominant neutron-number maxima are reproduced for a large fraction of the isotopic chains considered, indicating that the mean charge partition and the average neutron content of the main fission channels are described consistently. A systematic residual discrepancy is observed in the isotopic widths: the calculated yields often fall off too rapidly on the distribution tails, producing distributions that are narrower than the evaluated data, most notably for heavy-fragment chains.

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Static Fission Properties of Even-Even Actinides within the Warsaw Macroscopic-Microscopic Model Using Fourier-over-Spheroid Parameterization

A systematic study of fission barrier heights and static properties of even-even actinide nuclei from Th to Cf has been performed within the Warsaw macroscopic-microscopic model using the five-dimensional Fourier-over-Spheroid (FoS) shape parameterization. The use of a large deformation grid, containing about $1.3\times10^{8}$ points for each nucleus, allows for a refined and numerically complete exploration of the potential energy landscape without dividing the configuration space into subregions or applying interpolation. Barrier heights, extracted via the Immersion Water Flow method, show good agreement with empirical evaluations (including the new IAEA RIPL-4 dataset) with mean deviations below 1 MeV. Special attention is given to the long-debated third, hyperdeformed minimum. For Th isotopes, a shallow but distinct third well appears, whereas it's absent in heavier actinides (U, Pu).

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Paths to Superheavy Nuclei

This document summarizes the discussions and outcomes of the Facility for Rare Isotope Beams Theory Alliance (FRIB-TA) topical program "The path to Superheavy Isotopes" held in June 2024 at FRIB. Its content is non-exhaustive, reflecting topics chosen and discussed by the participants. The program aimed to assess the current status of theory in superheavy nuclei (SHN) research and identify necessary theoretical developments to guide experimental programs and determine fruitful production mechanisms. This report details the intersection of SHN research with other fields, provides an overview of production mechanisms and theoretical models, discusses future needs in theory and experiment, explores other potential avenues for SHN synthesis, and highlights the importance of building a strong theory community in this area.

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Candidates for three-quasiparticle $K$-isomers in even-odd Fm-Cn nuclei

Following our study of possible $K$-isomers in odd-even Md-Rg nuclei, here we continue with searching for three-quasiparticle 1$\nu$2$\pi$ and 3$\nu$ isomer candidates in even-odd Fm - Cn nuclei. We use the same approach to calculate energies of different nuclear configurations using a microscopic-macroscopic model with the Woods-Saxon potential. We used two versions of pairing: quasi-particle BCS method and particle number projection formalism. The optimal deformations for both ground states and high-$K$ configurations are determined through a four-dimensional energy minimization process. We point out the most promising candidates for high-$K$ isomers and compare them, where possible, with existing experimental data.

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Entropies, level-density parameters, and fission probabilities along the triaxially- and axially-symmetric fission paths in $^{296}$Lv

We employ a statistical approach to investigate the influence of axial asymmetry on the nuclear level density and entropy along the fission pathways of a superheavy nucleus, explicitly focusing on the $^{296}$Lv isotope. These pathways are determined within multidimensional deformation spaces. Our analysis reveals a significant impact of triaxiality on entropy. Additionally, suppressing shell effects can alter the fission scenario depending on the available excitation energy. We derive the deformation-dependent level density parameter, which plays a crucial role in estimating the survival probability of a superheavy nucleus. Furthermore, we utilize a set of master equations to obtain the time-dependent fission probabilities and calculate the ratio of decay probabilities for both axial and triaxial paths.

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Candidates for three-quasiparticle $K$-isomers in odd-even Md-Rg nuclei

We performed a search for three-quasiparticle high-$K$ isomer candidates in odd-even Md - Rg nuclei by considering the lowest lying 1$π$2$ν$ and 3$π$ excitations. Our approach involves calculating the energies of different nuclear configurations using a microscopic-macroscopic model with the Woods-Saxon potential. We explore three pairing scenarios: blocking, quasi-particle BCS method, and particle number projection formalism. The optimal deformations for both ground-states and high-$K$ configurations are determined through a four-dimensional energy minimization process. By analyzing the obtained excitation energies, we discuss the most promising candidates for high-$K$ isomers and compare them, where possible, with existing experimental data. We also discuss a possible isomer $α$-decay hindrance using calculated $Q_α$-hindrances.

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Multi-step particle emission probabilities in superheavy nuclei at moderate excitation energies

The probabilities of $xn$-, $pxn$-, and $αxn$-evaporation channels in excited superheavy nuclei were evaluated using the Monte Carlo method. The calculations utilized microscopically determined nuclear level densities and were compared with results obtained from the phenomenological Jackson formula. Effective temperatures derived from the microscopic approach were incorporated into the Jackson formula for different evaporation channels at low and moderate excitation energies. Additionally, an analytical formula was introduced to estimate the average kinetic energy of emitted particles in multi-step processes.

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The Fusion-by-Diffusion model as a tool to calculate cross sections for the production of superheavy nuclei

This article summarizes recent progress in our understanding of the reaction mechanisms leading to the formation of superheavy nuclei in cold and hot fusion reactions. Calculations are done within the Fusion-by-Diffusion (FBD) model using the new nuclear data tables by Jachimowicz et al. [At. Data Nucl. Data Tables 138, 101393 (2021)]. The synthesis reaction is treated in a standard way as a three-step process (i.e., capture, fusion, and survival). Each reaction step is analyzed separately. Model calculations are compared with selected experimental data on capture, fissionlike and fusion cross sections, fusion probabilities, and evaporation residue excitation functions. The role of the angular momentum in the fusion step is discussed in detail. A set of fusion excitation functions with corresponding fusion probabilities is provided for cold and hot synthesis reactions.

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First observation of high-$K$ isomeric states in $^{249}$Md and $^{251}$Md

Decay spectroscopy of the odd-proton nuclei $^{249}$Md and $^{251}$Md has been performed. High-$K$ isomeric states were identified for the first time in these two nuclei through the measurement of their electromagnetic decay. An isomeric state with a half-life of $2.8(5)$ ms and an excitation energy $\geq 910$ keV was found in $^{249}$Md. In $^{251}$Md, an isomeric state with a half-life of $1.4(3)$ s and an excitation energy $\geq 844$ keV was found. Similarly to the neighbouring $^{255}$Lr, these two isomeric states are interpreted as 3 quasi-particle high-$K$ states and compared to new theoretical calculations. Excited nuclear configurations were calculated within two scenarios: via blocking nuclear states located in proximity to the Fermi surface or/and using the quasiparticle Bardeen-Cooper-Schrieffer method. Relevant states were selected on the basis of the microscopic-macroscopic model with a deformed Woods-Saxon potential. The most probable candidates for the configurations of $K$-isomeric states in Md nuclei are proposed.

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Diffusion as a possible mechanism controlling the production of superheavy nuclei in cold fusion reactions

The fusion probability for the production of superheavy nuclei in cold fusion reactions was investigated and compared with recent experimental results for $^{48}$Ca, $^{50}$Ti, and $^{54}$Cr incident on a $^{208}$Pb target. Calculations were performed within the fusion-by-diffusion model (FbD) using new nuclear data tables by Jachimowicz et al. It is shown that the experimental data could be well explained within the framework of the FbD model. The saturation of the fusion probability at bombarding energies above the interaction barrier is reproduced. It emerges naturally from the physical effect of the suppression of contributions of higher partial waves in fusion reactions and is related to the critical angular momentum. The role of the difference in values of the rotational energies in the fusion saddle point and contact (sticking) configuration of the projectile-target system is discussed.

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Energy dependent ratios of level-density parameters in superheavy nuclei

The nuclear level densities and level-density parameters in fissioning nuclei at their saddle points of fission barriers - $a_{f}$, as well as those for neutron - $a_{n}$, proton - $a_{p}$ , and $α$-particle - $a_α$ emission residues at the ground states are calculated for isotopic chains of superheavy nuclei with $Z$=112-120. The calculations are performed with the superfluid formalism using the single-particle energies obtained from the diagonalization of the deformed Woods-Saxon potential. Spectra were generated at global minima of the adiabatic potential energy surfaces, found by the multidimensional minimization method, and at the proper saddle points, found by the "immersion water flow" technique on multidimensional energy grids, with allowed the reflection and axial symmetry breaking. The influence of shell effects on the energy dependence of the ratios of level-density parameters corresponding to residues of the considered decay modes to those of neutron emission is studied. We have shown that, in contrast to the $a_{f}/a_{n}$ ratio, the $a_{p}/a_{n}$ and $a_α/a_{n}$ ratios do not show characteristic maxima depending on the excitation energy of the compound nucleus being formed. In the case of alpha decay, we identified the collective enhancement caused by cluster degrees of freedom to play quite an important role. The energetic course of the variability of the level density parameters before reaching the asymptotic value, not taken into account so far, will be of great importance for the estimation of the probabilities of de-excitation cascades via light particles emission in competition with splitting and thus for the determination of the survival probabilities and finally for the total production cross-sections of superheavy nuclei in channels with their (light particles) participation.

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The decline rate of the production cross-section of superheavy nuclei with $Z=114-117$ at high excitation energies

The production cross sections of superheavy nuclei with charge numbers $114-117$ are predicted in the $(5-9)n$-evaporation channels of the $^{48}$Ca-induced complete fusion reactions for future experiments. The estimates of synthesis capabilities are based on a uniform and consistent set of input nuclear data provided by the multidimensional macroscopic-microscopic approach. The contributions of various factors to the final production cross section are discussed. As shown, the specific interplay between survival and fusion probabilities unexpectedly leads to a relatively slow decline of the total cross-sections with increasing excitation energy. This effect is supported by a favorable arrangement of fission barriers protecting the compound nucleus against splitting concerning energetic thresholds for the emission of successive neutrons. In particular, the probabilities of the formation of superheavy nuclei in the $5n$-, $6n$-, and in some cases even in $7n$-evaporation channels are still promising. This may offer a new opportunity for the future synthesis of unknown neutron-deficient superheavy isotopes.

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Properties of heaviest nuclei with $98\leq Z \leq 126$ and $134 \leq N \leq 192$

We systematically determine ground-state and saddle-point shapes and masses for 1305 heavy and superheavy nuclei with $Z=98-126$ and $N=134-192$, including odd-$A$ and odd-odd systems. From these, we derive static fission barrier heights, one- and two-nucleon separation energies, and $Q_α$ values for g.s. to g.s transitions. Our study is performed within the microscopic-macroscopic method with the deformed Woods-Saxon single-particle potential and the Yukawa-plus-exponential macroscopic energy taken as the smooth part. We use parameters of the model that were fitted previously to masses of even-even heavy nuclei. For systems with odd numbers of protons, neutrons, or both, we use a standard BCS method with blocking. Ground-state shapes and energies are found by the minimization over seven axially-symmetric deformations. A search for saddle-points was performed by using the "imaginary water flow" method in three consecutive stages, using five- (for nonaxial shapes) and seven-dimensional (for reflection-asymmetric shapes) deformation spaces. The results are collected in two main tables. Calculated ground-state mass excess, nucleon separation- and $Q_α$ energies, total, macroscopic(normalized to the macroscopic energy at the spherical shape) and shell corrections energies, and deformations are given for each nucleus in \mbox{Table 1}. \mbox{Table 2} contains calculated properties of the saddle-point configurations and the fission barrier heights. In \mbox{Tables 3-7}, are given calculated ground-state, inner and outer saddle-point and superdeformed secondary minima characteristics for 75 actinide nuclei, from Ac to Cf, for which experimental estimates of fission barrier heights are known. These results are an additional test of our model.

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