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M. L. Avila

Publications and source records attributed to M. L. Avila.

At least 19 recordsLinked to original sources

Detailed Study of the $^{59}$Cu(p,$α)^{56}$Ni Reaction and Constraints on Its Astrophysical Reaction Rate

The $^{59}$Cu$(p,α)^{56}$Ni reaction plays an important role in explosive astrophysical scenarios such as Type I X-ray bursts and the $νp$-process in neutrino-driven winds following a core-collapse supernova, where it regulates the flow of nucleosynthesis through the NiCu cycle and the synthesis of heavier nuclei. We present a direct measurement of the $^{59}\mathrm{Cu}(p,α)^{56}\mathrm{Ni}$ excitation function from 2.43--5.88~MeV in the center-of-mass frame, performed in inverse kinematics with the high-efficiency MUSIC active-target detector at FRIB. The angle- and energy-integrated cross sections extend direct measurements to lower energies than previously reported and remove the angular-integration model dependence of earlier work. To extrapolate the rate to astrophysical energies, we constrain the statistical-model description through a systematic optimization of the DEM-3 $α$-optical model potential geometry, and quantify the model-selection uncertainty with a Bayesian model averaging analysis over 96 TALYS combinations. The resulting stellar rate carries a temperature-dependent uncertainty factor of 1.26--1.63 over $T_9 = 0.2$--10 and is systematically lower than the REACLIB evaluation, remaining below the competing $(p,γ)$ rate for $T_9 \lesssim 3.94$. These results substantially weaken the inferred NiCu cycle strength and establish the $^{59}$Cu$(p,γ)^{60}$Zn rate as the dominant remaining uncertainty.

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Direct Measurement of the $^{59}$Cu$(p,α)^{56}$Ni Excitation Function to Constrain the Ni--Cu Cycle Strength and Its Impact on Explosive Nucleosynthesis

A new direct measurement of the 59Cu(p,a)56Ni excitation function from 2.43-5.88 MeV in the center-of-mass was performed in inverse kinematics using the high-efficiency MUSIC active-target detector at FRIB. This reaction plays a critical role in constraining the strength of the NiCu cycle in different explosive astrophysical scenarios such as Type I X-ray bursts and the nu-p process in neutrino-driven winds after a core-collapse supernova. The newly derived stellar rate is systematically lower than previous estimates, suppressing NiCu cycle recycling in X-ray bursts to below 3% and enhancing nu-p process efficiency throughout the relevant temperature range, potentially extending its effective operation to temperatures as high as T9 = 3.94 (+0.99/-0.85).

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Implications for Type Ia Supernova Nucleosynthesis from an Experimentally Constrained $^{16}$O$(p,α)^{13}$N Reaction Rate

The $^{16}$O$(p,α)^{13}$N reaction plays a key role in shaping the $α$-particle abundance during explosive oxygen burning in Type Ia supernovae. By enhancing $α$-production, this reaction directly affects the calcium-to-sulphur (Ca/S) and argon-to-sulphur (Ar/S) ratios, which serves as a tracer of progenitor metallicity. However, recent work suggests that the rate must be enhanced by a factor of up to seven over the standard value to explain observed Ca/S ratios across a range of progenitor metallicities. To explore this impact, available experimental cross-section data for the $^{16}$O$(p,α)^{13}$N reaction have been compiled and critically evaluated. Significant discrepancies are identified in the low-energy region ($E_{\mathrm{cm}}$ = 5.7--7.0 MeV), primarily due to limitations of the activation method. To resolve this, the first direct measurement at astrophysical energies has been performed using the MUSIC active-target detector. The new $^{16}$O$(p,α)^{13}$N thermonuclear reaction rate is found to be approximately 1.5 times higher than the REACLIB rate in the temperature range T = 3--4 GK, with more constrained uncertainties that resolve the previously large spread among existing data. The suggested factor of seven enhancement is excluded and these results indicate that this reaction alone cannot fully explain the variation in the Ca/S and Ar/S ratios observed across different progenitor metallicities. Therefore, future work should focus on reducing the uncertainties in other key oxygen-burning reactions, particularly $^{16}$O+$^{16}$O and $^{12}$C+$^{16}$O. Further reducing the constraints on the $^{16}$O$(p,α)^{13}$N rate is also needed to fully determine to whether a nuclear physics solution to this discrepancy is possible.

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First experimental determination of the $^{40}$Ar($n,2n$)$^{39}$Ar reaction cross section and $^{39}$Ar production in Earth's atmosphere

The cosmogenic $^{39}$Ar(t$_{1/2}$= 268 years) isotope of argon is used for geophysical dating and tracing owing to its appropriate half-life and chemical inertness as a noble gas; $^{39}$Ar serves also in nuclear weapon test monitoring. We measured for the first time the total cross section of the main $^{39}$Ar cosmogenic production reaction in the atmosphere, namely $^{40}$Ar$(n,2n)^{39}$Ar, using 14.8$\pm0.3$ MeV neutrons. The neutrons, produced by a deuterium-tritium generator, impinged on a stainless steel sphere filled with Ar gas highly enriched in the $^{40}$Ar isotope. The reaction yield was measured by atom counting of $^{39}$Ar with noble gas accelerator mass spectrometry and, independently, by decay counting relative to atmospheric argon. A total $^{40}$Ar$(n,2n)^{39}$Ar cross section of 610$\pm100$ mb was determined. This result serves as a benchmark for recent theoretical calculations and evaluations, found to reproduce well the experimental total cross section. We use these energy-dependent theoretical cross sections together with experimental spectra of cosmogenic neutrons at different altitudes to calculate the global average rate of neutron-induced $^{39}$Ar atmospheric production, resulting in $770\pm240$ $^{39}$Ar atoms/cm$^2$/day. The secular equilibrium between the $^{39}$Ar calculated production rate and radioactive decay rate leads to a partial isotopic abundance $^{39}$Ar/Ar$= (5.9\pm 1.8) \times 10^{-16}$, showing that $\approx$73% of atmospheric $^{39}$Ar is produced by cosmogenic neutrons. The $^{40}$Ar($n,2n$)$^{39}$Ar cross section at 14 MeV is also a key parameter for quantifying the anthropogenic contribution to atmospheric $^{39}$Ar produced during the thermonuclear tests of the 1960s. We estimate that anthropogenic $^{39}$Ar accounts for roughly 20% of the present atmospheric inventory.

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Quenching of single-particle strength inferred from nucleon-removal transfer reactions on $^{15}$C

The difference in the proton and neutron separation energies ($ΔS$) of the weakly bound $^{15}$C ground state is -19.86 MeV, an extreme value. Data from intermediate-energy heavy-ion induced (HI-induced) knockout reactions on nuclei spanning $-20\lesssimΔS\lesssim+20$ MeV, suggest that the degree to which single-particle strength is quenched, $R\mathrm{_{s}}$, has a negative correlation with $ΔS$, decreasing from unity around $-20$~MeV to around 0.2 at $+20$~MeV. For the $^{15}$C ground state ($R_s=0.96(4)$ in HI-induced knockout), contrasting results have recently been obtained via the neutron-adding transfer reaction, which reveal a value of $R_s=0.64(15)$, similar to the value observed at modest $ΔS$ and more extreme values of $ΔS$ with reaction probes other than HI knockout. In order to explore the any potential differences between $adding$ and $removing$ processes in transfer reactions at extreme $ΔS$, single-neutron removal transfer reactions on $^{15}$C were performed at 7.1MeV/u in inverse kinematics. The removal of a valence neutron in 2$s_{1/2}$ orbit using both ($p$,$d$) and ($d$,$t$) reactions shows consistent quenching factors and agrees with those from the neutron-adding reaction. The present results, which can be compared with neutron knockout reaction, suggest that correlations, represented by the quenching factor, show limited dependence on neutron-proton asymmetry under the most extreme asymmetry conditions so far achieved in transfer reactions.

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First measurement of 87Rb(α, xn) cross sections at weak r-process energies in supernova ν-driven ejecta to investigate elemental abundances in low-metallicity stars

Observed abundances of Z ~ 40 elements in metal-poor stars vary from star to star, indicating that the rapid and slow neutron capture processes may not contribute alone to the synthesis of elements beyond iron. The weak r-process was proposed to produce Z ~ 40 elements in a subset of old stars. Thought to occur in the ν-driven ejecta of a core-collapse supernova, (α, xn) reactions would drive the nuclear flow toward heavier masses at T = 2-5 GK. However, current comparisons between modelled and observed yields do not bring satisfactory insights into the stellar environment, mainly due to the uncertainties of the nuclear physics inputs where the dispersion in a given reaction rate often exceeds one order of magnitude. Involved rates are calculated with the statistical model where the choice of an α-optical-model potential (αOMP) leads to such a poor precision. The first experiment on 87Rb(α, xn) reactions at weak r-process energies is reported here. Total inclusive cross sections were assessed at Ec.m. = 8.1 - 13 MeV (3.7 - 7.6 GK) with the active target MUlti-Sampling Ionization Chamber (MUSIC). With a N = 50 seed nucleus, the measured values agree with statistical model estimates using the αOMP Atomki-V2. A re-evaluated reaction rate was incorporated into new nucleosynthesis calculations, focusing on ν-driven ejecta conditions known to be sensitive to this specific rate. These conditions were found to fail to reproduce the lighter-heavy element abundances in metal-poor stars.

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Direct cross-section measurement of the weak r-process 88Sr(α,n)91Zr reaction in ν-driven winds of core collapse supernovae

About half of the heavy elements beyond iron are known to be produced by the rapid neutron capture process, known as r-process. However, the astrophysical site producing the r-process is still uncertain. Chemical abundances observed in several cosmic sites indicate that different mechanisms should be at play. For instance, the abundances around silver measured in a subset of metal-poor stars indicate the presence of a weak r-process. This process may be active in neutrino-driven winds of core collapse supernovae where ($α$,n) reactions dominate the synthesis of Z ~ 40 elements in the expelled materials. Scarcely measured, the rates of ($α$,n) reactions are determined from statistical Hauser-Feshbach calculations with $α$-optical-model potentials, which are still poorly constrained. The uncertainties of the ($α$,n) reaction rates therefore make a significant contribution to the uncertainties of the abundances determined from stellar modeling. In this work, the $^{88}$Sr($α$,n)$^{91}$Zr reaction which impacts the weak r-process abundances has been probed at astrophysics energy for the first time; directly measuring the total cross sections at astrophysical energies of 8.37 - 13.09 MeV in the center of mass (3.8 - 7.5 GK). Two measurements were performed at ATLAS with the electrically-segmented ionization chamber MUSIC, in inverse kinematics, while following the active target technique. The cross sections of this $α$-induced reaction on $^{88}$Sr, located at the shell closure N = 50, have been found to be lower than expected, by a factor of 3, despite recent statistical calculations validated by measurements on neighboring nuclei. This result encourages more experimental investigations of ($α$,n) reactions, at N = 50 and towards the neutron-rich side, to further test the predictive power and reliability of such calculations.

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Probing the quadrupole transition strength of 15C via deuteron inelastic scattering

Deuteron elastic scattering from 15C and inelastic scattering reactions to the first excited state of 15C were studied using a radioactive beam of 15C in inverse kinematics. The scattered deuterons were measured using HELIOS. The elastic scattering differential cross sections were analyzed using the optical model. A matter deformation length δd = 1.04(11) fm has been extracted from the differential cross sections of inelastic scattering to the first excited state. The ratio of neutron and proton matrix elements Mn/Mp = 3.6(4) has been determined from this quadrupole transition. Neutron effective charges and core-polarization parameters of 15C were determined and discussed. Results from ab-initio no-core configuration interaction calculations were also compared with the experimental observations. This result supports a moderate core decoupling effect of the valence neutron in 15C similarly to its isotone 17O, in line with the interpretation of other neutron-rich carbon isotopes.

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Study of the $^{22}$Mg waiting point relevant for x-ray burst nucleosynthesis via the $^{22}$Mg($α$,$p$)$^{25}$Al reaction

The $^{22}$Mg($α$,$p$)$^{25}$Al reaction rate has been identified as a major source of uncertainty for understanding the nucleosynthesis flow in Type-I x-ray bursts (XRBs). We report a direct measurement of the energy- and angle-integrated cross sections of this reaction in a 3.3-6.9 MeV center-of-mass energy range using the MUlti-Sampling Ionization Chamber (MUSIC). The new $^{22}$Mg($α$,$p$)$^{25}$Al reaction rate is a factor of $\sim$4 higher than the previous direct measurement of this reaction within temperatures relevant for XRBs, resulting in the $^{22}$Mg waiting point of x-ray burst nucleosynthesis flow to be significantly bypassed via the ($α,p$) reaction

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Study of the Isomeric State in $^{16}$N Using the $^{16}$N$^{g,m}$($d$,$^3$He) Reaction

The isomeric state of $^{16}$N was studied using the $^{16}$N$^{g,m}$($d$,$^3$He)~proton-removal reactions at \mbox{11.8~MeV/$u$} in inverse kinematics. The $^{16}$N beam, of which 24% was in the isomeric state, was produced using the ATLAS in-fight facility and delivered to the HELIOS spectrometer, which was used to analyze the $^{3}$He ions from the ($d$,$^{3}$He) reactions. The simultaneous measurement of reactions on both the ground and isomeric states, reduced the systematic uncertainties from the experiment and in the analysis. A direct and reliable comparison of the relative spectroscopic factors was made based on a Distorted-Wave Born Approximation approach. The experimental results suggest that the isomeric state of $^{16}$N is an excited neutron-halo state. The results can be understood through calculations using a Woods-Saxon potential model, which captures the effects of weak-binding.

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First direct measurement of the $^{13}$N($α$,$p$)$^{16}$O reaction relevant for core-collapse supernovae nucleosynthesis

Understanding the explosion mechanism of a core-collapse supernova (CCSN) is important to accurately model CCSN scenarios for different progenitor stars using model-observation comparisons. The uncertainties of various nuclear reaction rates relevant for CCSN scenarios strongly affect the accuracy of these stellar models. Out of these reactions, the $^{13}$N($α$,$p$)$^{16}$O reaction has been found to affect various stages of a CCSN at varying temperatures. This work presents the first direct measurement of the $^{13}$N($α$,$p$)$^{16}$O reaction performed using a 34.6 MeV beam of radioactive $^{13}$N ions and the active-target detector MUSIC (MUlti-Sampling Ionization Chamber) at Argonne National Laboratory. The resulting total $^{13}$N($α$,$p$)$^{16}$O reaction cross sections from this measurement in the center-of-mass energy range of 3.26 - 6.02 MeV are presented and compared with calculations using the Hauser-Feshbach formalism. Uncertainties in the reaction rate have been dramatically reduced at CCSN temperatures.

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Cross sections of $α$-induced reactions slightly below doubly-magic $^{40}$Ca from the statistical model

New experimental data for the $^{38}$Ar($α$,n)$^{41}$Ca and $^{38}$Ar($α$,p)$^{41}$K reactions were used to find a best-fit set of parameters for statistical model calculations. The very good agreement between the experimental data and the best-fit calculation confirms the applicability of the statistical model for nuclei in the vicinity of the doubly-magic $^{40}$Ca despite of their relatively low level densities. The present study investigates the sensitivities and finds that the $α$-nucleus and the nucleon-nucleus potentials are the most important ingredients for the calculation of ($α$,n) and ($α$,p) reactions in the statistical model. Furthermore, the width fluctuation correction plays an essential role in the peculiar case of $^{38}$Ar. The best-fit parameters from $^{38}$Ar are applied to the mirror nucleus $^{38}$Ca and the neighboring $^{36}$Ar and $^{40}$Ar nuclei. For $^{38}$Ca this results in an astrophysical reaction rate of the $^{38}$Ca($α$,p)$^{41}$Sc reaction which has a flatter temperature dependence compared to all previous calculations. For $^{40}$Ar a better reproduction of $^{40}$Ar($α$,p)$^{43}$K data from literature is obtained. The disagreement between calculation and an early experimental data point for the $^{36}$Ar($α$,p)$^{39}$K reaction persists.

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Stellar $^{36,38}$Ar$(n,γ)^{37,39}$Ar reactions and their effect on light neutron-rich nuclide synthesis

The $^{36}$Ar$(n,γ)^{37}$Ar ($t_{1/2}$ = 35 d) and $^{38}$Ar$(n,γ)^{39}$Ar (269 y) reactions were studied for the first time with a quasi-Maxwellian ($kT \sim 47$ keV) neutron flux for Maxwellian Average Cross Section (MACS) measurements at stellar energies. Gas samples were irradiated at the high-intensity Soreq applied research accelerator facility-liquid-lithium target neutron source and the $^{37}$Ar/$^{36}$Ar and $^{39}$Ar/$^{38}$Ar ratios in the activated samples were determined by accelerator mass spectrometry at the ATLAS facility (Argonne National Laboratory). The $^{37}$Ar activity was also measured by low-level counting at the University of Bern. Experimental MACS of $^{36}$Ar and $^{38}$Ar, corrected to the standard 30 keV thermal energy, are 1.9(3) mb and 1.3(2) mb, respectively, differing from the theoretical and evaluated values published to date by up to an order of magnitude. The neutron capture cross sections of $^{36,38}$Ar are relevant to the stellar nucleosynthesis of light neutron-rich nuclides; the two experimental values are shown to affect the calculated mass fraction of nuclides in the region A=36-48 during the weak $s$-process. The new production cross sections have implications also for the use of $^{37}$Ar and $^{39}$Ar as environmental tracers in the atmosphere and hydrosphere.

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Probing the single-particle character of rotational states in $^{19}$F using a short-lived isomeric beam

A beam containing a substantial component of both the $J^π=5^+$, $T_{1/2}=162$ ns isomeric state of $^{18}$F and its $1^+$, 109.77-min ground state has been utilized to study members of the ground-state rotational band in $^{19}$F through the neutron transfer reaction $(d$,$p)$ in inverse kinematics. The resulting spectroscopic strengths confirm the single-particle nature of the 13/2$^+$ band-terminating state. The agreement between shell-model calculations, using an interaction constructed within the $sd$ shell, and our experimental results reinforces the idea of a single-particle/collective duality in the descriptions of the structure of atomic nuclei.

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Study of $\boldsymbol{(α,p)}$ and $\boldsymbol{(α,n)}$ reactions with a Multi-Sampling Ionization Chamber

A large number of $(α,p)$ and $(α,n)$ reactions are known to play a fundamental role in nuclear astrophysics. This work presents a novel technique to study these reactions with the active target system MUSIC whose segmented anode allows the investigation of a large energy range of the excitation function with a single beam energy. In order to verify the method, we performed a direct measurements of the previously measured reactions $^{17}$O$(α,n)^{20}$Ne, $^{23}$Na$(α,p)^{26}$Mg, and $^{23}$Na$(α,n)^{26}$Al. These reactions were investigated in inverse kinematics using $^{4}$He gas in the detector to study the excitation function in the range of about 2 to 6 MeV in the center of mass. We found good agreement between the cross sections of the $^{17}$O$(α,n)^{20}$Ne reaction measured in this work and previous measurements. Furthermore we have successfully performed a simultaneous measurement of the $^{23}$Na$(α,p)^{26}$Mg and $^{23}$Na$(α,n)^{26}$Al reactions.

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Study of the astrophysically important $\boldsymbol{^{23}\mathrm{Na}(α,p)^{26}\mathrm{Mg}}$ and $\boldsymbol{^{23}\mathrm{Na}(α,n)^{26}\mathrm{Al}}$ reactions

The $^{23}$Na$(α,p)^{26}$Mg and $^{23}$Na$(α,n)^{26}$Al reactions are important for our understanding of the $^{26}$Al abundance in massive stars. The aim of this work is to report on a direct and simultaneous measurement of these astrophysically important reactions using an active target system. The reactions were investigated in inverse kinematics using $^{4}$He as the active target gas in the detector. We measured the excitation functions in the energy range of about 2 to 6 MeV in the center of mass. We have found that the cross sections of the $^{23}$Na$(α,p)^{26}$Mg and the $^{23}$Na$(α,n)^{26}$Al reactions are in good agreement with previous experiments, and with statistical model calculations.

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Independent measurement of the Hoyle state $β$ feeding from 12B using Gammasphere

Using an array of high-purity Compton-suppressed germanium detectors, we performed an independent measurement of the $β$-decay branching ratio from $^{12}\mathrm{B}$ to the second-excited (Hoyle) state in $^{12}\mathrm{C}$. Our result is $0.64(11)\%$, which is a factor $\sim 2$ smaller than the previously established literature value, but is in agreement with another recent measurement. This could indicate that the Hoyle state is more clustered than previously believed. The angular correlation of the Hoyle state $γ$ cascade has also been measured for the first time. It is consistent with theoretical predictions.

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New $α$ ANC measurement of the 1/2$^+$ state in $^{17}$O at 6.356 MeV, that dominates the $^{13}$C($α$,n)$^{16}$O reaction rate at temperatures relevant for the s-process

Background: Accurate knowledge of the $^{13}$C($α$,$n$)$^{16}$O reaction cross section is important for the understanding of the s-process in AGB stars, since it is considered to be the main source of neutrons. The sub-threshold 1/2$^+$ state at excitation energy of 6.356 MeV in $^{17}$O has a strong influence on the reaction cross section at energies relevant for astrophysics. Several experiments have been performed to determine the contribution of this state to the $^{13}$C($α,n)^{16}$O reaction rate. Nevertheless, significant discrepancies between different measurements remain. Purpose: The aim of this work is to investigate these discrepancies. Method: An 8 MeV $^{13}$C beam (below the Coulomb barrier) was used to study the $α$-transfer reaction $^6$Li($^{13}$C,$d$)$^{17}$O. Results: The squared Coulomb modified ANC of the 1/2$^+$ state in $^{17}$O measured in this work is $(\tilde C^{^{17}\text{O}(1/2+)}_{α-^{13}\text{C}})^2=3.6\pm0.7\hspace{0.2cm}\text{fm}^{-1}$. Conclusions: Discrepancy between the results of $α$-transfer experiments have been resolved. However, some discrepancy with the most recent measurement using the Trojan Horse method remains.

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