arXiv subjects

M. L. Liu

Publications and source records attributed to M. L. Liu.

17 recordsLinked to original sources

arXiv2025

A high-lying isomer in ^{92}Zr with lifetime modulated by the atomic charge states: a proposed approach for a nuclear gamma-ray laser

The nuclides ^{92}Zr are produced and transported by using a radioactive beam line to a lowbackground detection station. After a flight time of about 1.14 μs, the ions are implanted into a carbon foil, and four γ rays deexciting the 8+ state in ^{92}Zr are observed in coincidence with the implantation signals within a few nanoseconds. We conjecture that there exists an isomer located slightly above the 8^{+} state in ^{92}Zr. The isomeric lifetime in highly charged states is extended significantly due to the blocking of internal conversion decay channels, enabling its survival over the transportation. During the slowing-down process in the carbon foil, the ^{92}Zr ions capture electron and evolve toward neutral atoms, and consequently the lifetime is restored to a normal short value. Such a high-lying isomer depopulated by a low-energy transition may provide unique opportunity to develop nuclear γ laser.

nucl-ex↗

arXiv2021

Probing the nature of the conjectured low-spin wobbling bands in atomic nuclei

Precession is a unique motion in which the orientation of the rotational axis of a rotating body is not fixed but moving, and it generally exists in the Universe from giant stars through tiny atomic nuclei. In principle, the precession of an atomic nuclide can be approximately described as wobbling motion, arising from the coupling of a rotation and a harmonic vibration. Recently, a number of wobbling bands were reported at low spin, which violate the wobbling approximation that can be valid only at high spin. Here we explore the nature of the reported low-spin wobbling bands. Via a new experiment, we demonstrate that one such band in $^{187}$Au is generated by dominant single-particle excitation rather than by the excitation of a wobbling phonon. We point out that the imperfect research paradigm used previously would lead to unreliable identification of low-spin wobbling bands. Consequently, new experimental approaches should be developed to distinguish among the different excitation mechanisms that can give rise to the observed low-spin bands in odd-even nuclei.

nucl-th↗

arXiv2021

New $α$-Emitting Isotope $^{214}$U and Abnormal Enhancement of $α$-Particle Clustering in Lightest Uranium Isotopes

A new $α$-emitting isotope $^{214}$U, produced by fusion-evaporation reaction $^{182}$W($^{36}$Ar, 4n)$^{214}$U, was identified by employing the gas-filled recoil separator SHANS and recoil-$α$ correlation technique. More precise $α$-decay properties of even-even nuclei $^{216,218}$U were also measured in reactions of $^{40}$Ar, $^{40}$Ca with $^{180, 182, 184}$W targets. By combining the experimental data, improved $α$-decay reduced widths $δ^2$ for the even-even Po--Pu nuclei in the vicinity of magic neutron number $N=126$ were deduced. Their systematic trends are discussed in terms of $N_{p}N_{n}$ scheme in order to study the influence of proton-neutron interaction on $α$ decay in this region of nuclei. It is strikingly found that the reduced widths of $^{214,216}$U are significantly enhanced by a factor of two as compared with the $N_{p}N_{n}$ systematics for the $84 \leq Z \leq 90$ and $N<126$ even-even nuclei. The abnormal enhancement is interpreted by the strong monopole interaction between the valence protons and neutrons occupying the $π1f_{7/2}$ and $ν1f_{5/2}$ spin-orbit partner orbits, which is supported by a large-scale shell model calculation.

nucl-ex↗

arXiv2019

Fusion reactions in the $^9$Be + $^{197}$Au system above the Coulomb barrier

The cross sections of complete fusion and incomplete fusion for the $ ^{9} $Be + $ ^{197} $Au system, at energies not too much above the Coulomb barrier, were measured for the first time. The online activation followed by offline $γ$-ray spectroscopy method was used for the derivation of the cross sections. A slightly higher value of ICF/TF ratio has been observed, compared to other systems reported in the literature with $ ^{9} $Be beam. The experimental data were compared with coupled channel calculations without taking into account the coupling of the breakup channel, and experimental data of other reaction systems with weakly bound projectiles. A complete fusion suppression of about 40\% was found for the $ ^{9} $Be + $ ^{197} $Au system, at energies above the barrier, whereas the total fusion cross sections are in agreement with the calculations.

nucl-ex↗

arXiv2019

Fine structure in the $α$ decay of $^{223}$U

Fine structure in the $α$ decay of $^{223}$U was observed in the fusion-evaporation reaction $^{187}$Re($^{40}$Ar, p3n) by using fast digital pulse processing technique. Two $α$-decay branches of $^{223}$U feeding the ground state and 244 keV excited state of $^{219}$Th were identified by establishing the decay chain $^{223}$U $\xrightarrow{α_{1}}$ $^{219}$Th $\xrightarrow{α_{2}}$ $^{215}$Ra $\xrightarrow{α_{3}}$ $^{211}$Rn. The $α$-particle energy for the ground-state to ground-state transition of $^{223}$U was determined to be 8993(17) keV, 213 keV higher than the previous value, the half-life was updated to be 62$^{+14}_{-10}$ $μ$s. Evolution of nuclear structure for $N$ = 131 even-$Z$ isotones from Po to U was discussed in the frameworks of nuclear mass and reduced $α$-decay width, a weakening octupole deformation in the ground state of $^{223}$U relative to its lighter isotones $^{219}$Ra and $^{221}$Th was suggested.

nucl-ex↗

arXiv2019

Experimentally well-constrained masses of $^{27}$P and $^{27}$S: Implications for studies of explosive binary systems

The mass of $^{27}$P was predicted to impact the X-ray burst (XRB) model predictions of burst light curves and the composition of the burst ashes. To address the uncertainties and inconsistencies in the reported $^{27}$P masses in literature, a wealth of information has been extracted from the $β$-decay spectroscopy of the drip-line nucleus $^{27}$S. We determine the most precise mass excess of $^{27}$P to date to be $-659(9)$~keV, which is 63~keV (2.3$σ$) higher than the AME2016 recommended value of $-722(26)$~keV. The experimentally unknown mass excess of $^{27}$S was estimated to be 17030(400)~keV in AME2016, and we constrain this mass to be 17678(77)~keV based on the measured $β$-delayed two-proton energy. In the temperature region of $(0.06-0.3)$~GK, the $^{26}$Si$(p,γ)^{27}$P reaction rate determined in this work is significantly lower than the rate recommended in the reaction rate libraries, up to two orders of magnitude around 0.1~GK. The impact of these newly determined masses and well-constrained rate on the modeling of the explosive astrophysical scenarios has been explored by hydrodynamic nova and post-processing XRB models. No substantial change was found in the nova contribution to the synthesis of galactic $^{26}$Al or in the XRB energy generation rate, but we found that the calculated abundances of $^{26}$Al and $^{26}$Si at the last stage of XRB are increased by a factor of 2.4. We also conclude that $^{27}$S is not a significant waiting point in the rapid proton capture process.

nucl-ex↗

arXiv2019

Simultaneous measurement of beta-delayed proton and gamma emission of $^{26}$P for $^{25}$Al($p,γ$)$^{26}$Si reaction rate

$β$ decay of $^{26}$P was used to populate the astrophysically important $E_x=$5929.4(8) keV $J^π=3{^+}$ state of $^{26}$Si. Both $β$-delayed proton at 418(8) keV and gamma ray at 1742(2) keV emitted from this state were measured simultaneously for the first time with corresponding absolute intensities of 11.1(12)\% and 0.59(44)\%, respectively. Besides, shell model calculations with weakly bound effects were performed to investigate the decay properties of other resonant states and a spin-parity of $4^+$ rather than $0^+$ was favored for the $E_x=$5945.9(40) keV state. Combining the experimental results and theoretical calculations, $^{25}$Al($p,γ$)$^{26}$Si reaction rate in explosive hydrogen burning environments was calculated and compared with previous studies.

nucl-ex↗

arXiv2019

Chirality of $^{135}$Nd reexamined: Evidence for multiple chiral doublet bands

One new pair of positive-parity chiral doublet bands have been identified in the odd-$A$ nucleus $^{135}$Nd which together with the previously reported negative-parity chiral doublet bands constitute a third case of multiple chiral doublet (M$χ$D) bands in the $A\approx130$ mass region. The properties of the M$χ$D bands are well reproduced by constrained covariant density functional theory and particle rotor model calculations. The newly observed M$χ$D bands in $^{135}$Nd represents an important milestone in supporting the existence of M$χ$D in nuclei.

nucl-ex↗

arXiv2019

Masses of ground and isomeric states of $^{101}$In and configuration-dependent shell evolution in odd-$A$ indium isotopes

We report first precision mass measurements of the $1/2^-$ isomeric and $9/2^+$ ground states of $^{101}$In. The determined isomeric excitation energy continues a smooth trend of odd-$A$ indium isotopes up to the immediate vicinity of $N=50$ magic number. This trend can be confirmed by dedicated shell model calculations only if the neutron configuration mixing is considered. We find that the single particle energies are different for different states of the same isotope. The presented configuration-dependent shell evolution, type II shell evolution, in odd-$A$ nuclei is discussed for the first time. Our results will facilitate future studies of single-particle neutron states.

nucl-ex↗

arXiv2019

Valence Neutron-Proton Orientation in Atomic Nuclei

It is shown that the renormalized nuclear deformations in different mass regions can be globally scaled by two probability partition factors of Boltzmann-like distribution, which are derived from the competing valence $np$ and like-nucleon interactions. The partition factors are simply related to the probabilities of anti-parallel and fully-aligned orientations of the angular momenta of the neutrons and protons in the valence $np$ pairs, responsible for spherical- and deformed-shape phases, respectively. The partition factors derived from the renormalized deformations are also present in the new scaling law for the energies of the first $2^+$ states. A striking concordance between the distributions of the renormalized deformations and of the newly introduced parameter for the energies of the first $2^+$ states over the extended mass region from Ge to Cf is achieved, giving strong support to the existence of two phases: anti-aligned and fully-aligned subsets of $np$ pairs.

nucl-th↗

arXiv2019

Diversity of shapes and rotations in the gamma-soft 130Ba nucleus: first observation of a t-band in the A=130 mass region

Several new bands have been identified in 130Ba, among which there is one with band-head spin 8+. Its properties are in agreement with the Fermi-aligned νh11/2^2 , 7/2+[523] \otimes 9/2-[514] Nilsson configuration. This is the first observation of a two-quasiparticle t-band in the A=130 mass region. The t-band is fed by a dipole band involving two additional h11/2 protons. The odd-spin partners of the proton and neutron S-bands and the ground-state band at high spins are also newly identified. The observed bands are discussed using several theoretical models, which strongly suggest the coexistence of prolate and oblate shapes polarized by rotation aligned two-proton and two-neutron configurations, as well as prolate collective rotations around axes with different orientations. With the new results, 130Ba presents one of the best and most complete sets of collective excitations that a gamma-soft nucleus can manifest at medium and high spins, revealing a diversity of shapes and rotations for the nuclei in the A = 130 mass region.

nucl-ex↗

arXiv2019

Beta-decay spectroscopy of $^{27}$S

Background: Beta-decay spectroscopy provides valuable nuclear physics input for thermonuclear reaction rates of astrophysical interest and stringent test for shell-model theories far from the stability line. Purpose: The available decay properties of proton drip-line nucleus $^{27}$S is insufficient to constrain the properties of the key resonance in $^{26}$Si$(p,γ)^{27}$P reaction rate and probe the possible isospin asymmetry. The decay scheme of $^{27}$S is complicated and far from being understood, which has motivated but also presented challenges for our experiment. Method: The $^{27}$S ions were implanted into a double-sided silicon strip detector array surrounded by the high-purity germanium detectors, where the $β$-delayed protons and $γ$ rays were measured simultaneously. Results: The improved spectroscopic properties including the precise half-life of $^{27}$S, the excitation energies, $β$-decay branching ratios, log~$ft$ values, and $B$(GT) values for the states of $^{27}$P populated in the $β$ decay of $^{27}$S were measured and compared to the $^{27}$Mg mirror states and the shell-model calculations. The present work has expanded greatly on the previously established decay scheme of $^{27}$S. Conclusions: The precise proton-separation energy of $^{27}$P, the energy and the ratio between $γ$ and proton partial widths of the $3/2^+$ resonance were obtained, thereby determining the $^{26}$Si$(p,γ)^{27}$P reaction rate based mainly on experimental constraints. The first evidence for the observation of a large isospin asymmetry for the mirror decays of $^{27}$S and $^{27}$Na is also provided. The experimental spectroscopic information can be reproduced by the shell-model calculation taking the weakly bound effect of the proton $1s_{1/2}$ orbit into account.

nucl-ex↗

arXiv2016

The decay characteristic of $^{22}$Si and its ground-state mass significantly affected by three-nucleon forces

The decay of the proton-rich nucleus $^{22}$Si was studied by a silicon array coupled with germanium clover detectors. Nine charged-particle groups are observed and most of them are recognized as $β$-delayed proton emission. A charged-particle group at 5600 keV is identified experimentally as $β$-delayed two-proton emission from the isobaric analog state of $^{22}$Al. Another charged-particle emission without any $β$ particle at the low energy less than 300 keV is observed. The half-life of $^{22}$Si is determined as 27.5 (18) ms. The experimental results of $β$-decay of $^{22}$Si are compared and in nice agreement with shell-model calculations. The mass excess of the ground state of $^{22}$Si deduced from the experimental data shows that three-nucleon (3N) forces with repulsive contributions have significant effects on nuclei near the proton drip line.

nucl-ex↗

arXiv2016

Isomerism in the "south-east" of $^{132}$Sn and a predicted neutron-decaying isomer in $^{129}$Pd

Excited states in neutron-rich nuclei located south-east of $^{132}$Sn are investigated by shell-model calculations. A new shell-model Hamiltonian is constructed for the present study. The proton-proton and neutron-neutron interactions of the Hamiltonian are obtained through the existing CD-Bonn $G$ matrix results, while the proton-neutron interaction across two major shells is derived from the monopole based universal interaction plus the M3Y spin-orbit force. The present Hamiltonian can reproduce well the experimental data available in this region, including one-neutron separation energies, level energies and the experimental $B(E2)$ values of isomers in $^{134,136,138}$Sn, $^{130}$Cd, and $^{128}$Pd. New isomers are predicted in this region, $e.g.$ in $^{135}$Sn, $^{131}$Cd, $^{129}$Pd, $^{132,134}$In and $^{130}$Ag, in which almost no excited states are known experimentally yet. In the odd-odd $^{132,134}$In and $^{130}$Ag, the predicted very long $E2$ life-times of the low-lying $5^{-}$ states are discussed, demanding more information on the related proton-neutron interaction. The low-lying states of $^{132}$In are discussed in connection with the recently observed $γ$ rays. The predicted $19/2^{-}$ isomer in $^{129}$Pd could decay by both electromagnetic transitions and neutron emission with comparable partial life-times, making it a good candidate for neutron radioactivity, a decay mode which is yet to be discovered.

nucl-th↗

arXiv2013

Identification of a $9/2^-$[505] isomer in the neutron-rich $^{193}$Os nucleus

The neutron rich nucleus $^{193}$Os was produced in the $^{192}$Os($^{7}$Li,$^{6}$Li)$^{193}$Os reaction. An isomeric state based on the $9/2^-$[505] nilsson orbital was identified in the present work. Half-life of the isomeric state was extracted and discussed in terms of the $K$ quantum number. Level scheme built on the isomeric state was proposed based on the experimental data.

nucl-ex↗

arXiv2010

Reexamination of reaction rates for a key stellar reaction of $^{14}$O($α$,p)$^{17}$F

The reaction rates of the key stellar reaction of $^{14}$O($α$,p)$^{17}$F have been reexamined. The previous conclusion, the 6.15-MeV state ($J^π$=1$^-$) dominating this reaction rate, has been overthrown by a careful reanalysis of the previous experimental data [J. Gómez del Campo {\it et al.}, Phys. Rev. Lett. {\bf 86}, 43 (2001)]. According to the present $R$-matrix analysis, the previous 1$^-$ assignment for the 6.15-MeV state is definitely wrong. Most probably, the 6.286-MeV state is the 1$^-$ state and the 6.15-MeV state is a 3$^-$ one, and hence the resonance at $E_x$=6.286 MeV ($J^π$=1$^-$) dominates the reaction rates in the temperature region of astrophysical interests. The newly calculated reaction rates for the $^{14}$O($α$,p)$^{17}$F reaction are quite different from the previous ones, for instance, it's only about 1/6 of the previous value around 0.4 GK, while it's about 2.4 times larger than the previous value around 2 GK. The astrophysical implications have been discussed based on the present conclusions.

astro-ph.SR↗

arXiv2001

Experimental NMR Realization of A Generalized Quantum Search Algorithm

A generalized quantum search algorithm, where phase inversions for the marked state and the prepared state are replaced by $π/2$ phase rotations, is realized in a 2-qubit NMR heteronuclear system. The quantum algorithm searches a marked state with a smaller step compared to standard Grover algorithm. Phase matching requirement in quantum searching is demonstrated by comparing it with another generalized algorithm where the two phase rotations are $π/2$ and $3π/2$ respectively. Pulse sequences which include non 90 degree pulses are given.

quant-ph↗